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Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV Brabcová Kateřina Spurný František Jadrníčková Iva Department of Radiation Dosimetry, Nuclear Physics Institute, Academy of Sciences of the Czech Republic, Prague, [email protected]

Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

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Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV. Brabcová Kateřina Spurn ý F ranti šek Jadrníčková Iva Department o f Radiation Dosimetry, Nuclear Physics Institute, Academy of Sciences of the Czech Republic, Prague , [email protected]. content. - PowerPoint PPT Presentation

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Page 1: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

Brabcová Kateřina

Spurný František

Jadrníčková Iva

Department of Radiation Dosimetry, Nuclear Physics Institute, Academy of Sciences of the Czech Republic, Prague, [email protected]

Page 2: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

content

• briefly about neutron dosimetry

• track etched detectors (TED)

• conditions of our experiments

• results

• conclusion

Page 3: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

about neutron dosimetry

• indirectly ionizing radiation, energy transferred through the kinetic energy of secondary charged particles

• large spectrum of the secondary particles created in detector or around

• LET spectra should be known

Page 4: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experimental methods of LET spectrometry

• tissue-equivalent proportional counters, bubble detectors, nuclear emulsions,

• in case of long exposure, limitation in weight and dimension, presence of intense low LET radiation :

track etched based LET spectrometers

Page 5: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

TED generally• mostly polyallyldiglycolcarbonate C12H18O • evaluation by etching • measuring of track parameters

• calibration

B

T

V

VV

etch rate of damaged material

etch rate of unaffected material

)(VfLET

etch ratio

Page 6: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

• polyallyldiglycolcarbonate C12H18O Page, 0.5 mm (Page Moulgings Ltd, England)

Tastrak, 0.5 mm (Track Analysis Systems Ltd, Bristol)

• evaluation by etching 5 M NaOH at 70oC for 18 hours

• measuring of track parameters automatic optical image analyzer LUCIA G

• calibration

our TED

Page 7: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

calibration of TED

• heavy charged particle beams12C – 84Kr

LET from 7.5 to 600 keV/μm

• performed in cooperation withHIMAC (NIRS Chiba, Japan) in the frame of ICCHIBAN

programs – ICCHIBAN 2, 4, 6, and 8

NASA Space Radiation Laboratory (Brookhaven National Laboratory) in the frame of ICCHIBAN BNL

Nuclotron of the Laboratory of High Energies, JINR, Dubna

Page 8: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

• done at the Van de Graaff facility at the EC-JRC, Geel

• quasi mono-energetic neutron beams produced by protons and deuterons

• 7 different energies of neutron beams from 200 keV to 20 MeV

• reference values – neutron fluences and neutron spectra, ambient dose equivalent H*(10)

Page 9: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment iThemba

• done in iThemba laboratory, Cape Town

• quasi mono-energetic neutron beams produced by deuterons and Li targets

• 2 energies of neutron beams – 100 and 200 MeV

• reference values – neutron fluences and neutron spectra, ambient dose equivalent H*(10)

Page 10: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

Page - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

0.30

10 100 1000

LET [keV.μm-1]

LE

T*H

0.2 MeV

?

Page 11: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

Page - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

0.30

10 100 1000

LET [keV.μm-1]

LE

T*H 0.2 MeV

0.5 MeV

recoil protons up to 100 keV.μm-1

Page 12: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

Page - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

0.30

10 100 1000

LET [keV.μm-1]

LE

T*H

0.2 MeV

0.5 MeV

1 MeV

Page 13: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

Page - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

0.30

10 100 1000

LET [keV.μm-1]

LE

T*H

0.2 MeV

0.5 MeV

1 MeV

3.5 MeV

Page 14: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

Page - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

0.30

10 100 1000

LET [keV.μm-1]

LE

T*H

0.2 MeV

0.5 MeV

1 MeV

3.5 MeV

7 MeV

(n,x)X

Page 15: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

Page - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

0.30

10 100 1000

LET [keV.μm-1]

LE

T*H

0.2 MeV

0.5 MeV

1 MeV

3.5 MeV

7 MeV

16 MeV

Page 16: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

Page - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

0.30

10 100 1000

LET [keV.μm-1]

LE

T*H

0.2 MeV

0.5 MeV

1 MeV

3.5 MeV

7 MeV

16 MeV

20 MeV

Page 17: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

0.5 mm Tastrak - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

10 100 1000

LET [keV.μm-1]

LE

T*H

0.2 MeV

Page 18: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

0.5 mm Tastrak - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

10 100 1000

LET [keV.μm-1]

LE

T*H 0.2 MeV

0.5 MeV

recoil protons up to 100 keV.μm-1

Page 19: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

0.5 mm Tastrak - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

10 100 1000

LET [keV.μm-1]

LE

T*H

0.2 MeV

0.5 MeV

1 MeV

Page 20: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

0.5 mm Tastrak - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

10 100 1000

LET [keV.μm-1]

LE

T*H

0.2 MeV

0.5 MeV

1 MeV

3.5 MeV

Page 21: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

0.5 mm Tastrak - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

10 100 1000

LET [keV.μm-1]

LE

T*H

0.2 MeV

0.5 MeV

1 MeV

3.5 MeV

7 MeV

(n,x)X

Page 22: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

0.5 mm Tastrak - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

10 100 1000

LET [keV.μm-1]

LE

T*H

0.2 MeV

0.5 MeV

1 MeV

3.5 MeV

7 MeV

16 MeV

Page 23: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

experiment EC-JRC

0.5 mm Tastrak - LET distribution of H

0.00

0.05

0.10

0.15

0.20

0.25

10 100 1000

LET [keV.μm-1]

LE

T*H

0.2 MeV

0.5 MeV

1 MeV

3.5 MeV

7 MeV

16 MeV

20 MeV

Page 24: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

100 MeV

0

0.02

0.04

0.06

0.08

0.1

0.12

0.14

0.16

0.18

0.2

10 100 1000

LET [keV.μm-1]

LE

T*H

Page

0.5 mm Tastrak

experiment iThemba

Page 25: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

100 MeV and 200 MeV

0

0,02

0,04

0,06

0,08

0,1

0,12

0,14

0,16

0,18

0,2

10 100 1000

LET [keV.μm-1]

LE

T*H

Page 100 meV

Tastrak 100 MeV

Page 200 MeV

Tastrak 200 MeV

experiment iThemba

Page 26: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

dosimetric characteristic

HLET = ∫ (dN / dLET) . LET . Q(LET) . dLET

dose equivalent due to registered particles

dN/dLET – number of tracks N in a LET interval dLET

Q(LET) – ICRP 60 quality factor

H*(10)

ambient dose equivalent (reference value)

Page 27: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

response of detectors

0.1

1

10

0.1 1 10 100 1000

neutron energy in MeV

rati

o H

LE

T/H

*(1

0) Page

T0,5

Page 28: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

conclusion

• TED provides new information about neutron energy transfer to the matter

• dose equivalent of secondary particles is lower than ambient dose equivalent H*(10)

• intention of futher studiesexperiment with another neutron energies

deal with unexpected values of 200 keV and 7 MeV

Page 29: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

Acknowledgements• Part of study has been realised in the frame of

ESA DOBIES project. We are obliged to Filip Vanhavere (SCK MOL, Belgium) for the coordination of the project, and to ESA Prodex Office for financial assistance.

• Many of results presented in this contribution were obtained by using the results of ICCHIBAN research project using heavy Ions at HIMAC-NIRS, NSRL–BNL, nuclotron JINR Dubna. We are much obliged to the staff of all laboratories and, particularly, to organizers of the run, Y. Uchihori, N. Yasuda, J. Miller, E.R. Benton, A.G. Molokanov, and V.P. Bamblevski† for their help.

• Studies were also partially supported through the grant No. 202/04/0795 of the GA CR and the IRP AV0Z10480505.

Page 30: Track etch based LET spectrometry in beams of neutrons with energies from 0.2 to 200 MeV

Thank you!