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Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory [email protected]

Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory [email protected]

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Page 1: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

Shortening a laser pulse at the focus of a lens

Yuelin LiAccelerator Systems DivisionArgonne National [email protected]

Page 2: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

2CLEO 08, San Jose, May 4-9, 2008

Content Introduction

– Pulse lengthening at lens focus Fourier formulation of the problem

– Axial temporal history

– Pulse shortening due to GVDE and SPM

– Numerical simulation Experiment outlook Summary

Page 3: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

3CLEO 08, San Jose, May 4-9, 2008

Content Introduction

– Pulse lengthening at lens focus Fourier formulation of the problem

– Axial temporal history

– Pulse shortening due to GVD

– Numerical simulation Experiment outlook Summary

Page 4: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

4CLEO 08, San Jose, May 4-9, 2008

Pulse lengthening due to Group Velocity Delay

Z. Bor, Opt. Lett. 15, 119 (1989)

Page 5: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

5CLEO 08, San Jose, May 4-9, 2008

Content Introduction

– Pulse lengthening at lens focus Fourier formulation of the problem

– Axial temporal profile

– Pulse shortening due to GVD, with SPM

– Numerical simulation Experiment outlook Summary

Page 6: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

6CLEO 08, San Jose, May 4-9, 2008

Formula of the problem: Fourier optics

Full wave optics (Fresnel diffraction) adapted from Kempe et al. (JOSA B 9, 1158 (1992))

Group velocity dispersion and group velocity delay effect considered up to the second order

Page 7: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

7CLEO 08, San Jose, May 4-9, 2008

On axis formula

),()(2)( rrdrAU

2

22

exp

)1(2)(exp

2exp),(

TTjk

fn

rkkjr

f

kjdjkr al

al

U: field in frequency domain representation at the focus f : is the focal length r: ray location Kl, ka: wave vectors in the lens and air,n: refractive index in the lens. A(): input filed (homogeneous) in the frequency domain. , Lens transfer function

r

rdratu 2)(

Inverse Fourier transform

a=a(t)=F-1A() and =(r,t)=F-1(r,)

Field at focus, on axis

.2

11,,

)1(2)(

2

22

d

nd

d

dn

fn

rdrT

df

Page 8: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

8CLEO 08, San Jose, May 4-9, 2008

Pulse with no SPM

For a=a0exp(-2ln2t2/2), no SPM,

,)(tanexp)1(

)1(2ln2exp

1

12)( 1

22

2

4/120

jjTkt

rdratu

=4kT/2.

.2

11,,

)1(2)(

2

22

d

nd

d

dn

fn

rdrT

Chirping and broadening due to Group Velocity DIspersion (GVDI)

Relative delay between pulse slices due to Group Velocity DElay (GVDE)

GVDE and GVDI have both been studied.

Page 9: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

9CLEO 08, San Jose, May 4-9, 2008

Max phase modulation, over lens of thickness d:

.2ln4expexp2ln2exp)(

2

2

2

2

0

Tkt

jTkt

rdratu

2

2

2

2

0 2ln4expexp2ln2exp),(t

jt

atra

Pulse with SPM

Assume smaller bandwidth and d2/dn2=0,

=4kT/2.

.2

11,,

)1(2)(

2

22

d

nd

d

dn

fn

rdrT

Delay due to GVDE

Case not been studied.

Tkttr ),(

Interference due to GVDE

dakn 202

Page 10: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

10CLEO 08, San Jose, May 4-9, 2008

Pulse shortening at the focus

-2 -1 0 1 2

0.0

0.5

1.0

-2 -1 0 1 2

0

4

8

12

(a)

r (m

m)

(c)

|u|2 (

a.u

.)

t (ps)

(b)

-1

-0.5

0

0.5

1

(d)

t (ps)

Li and Crowell, Opt. Lett. 32, 92 (2007).

The real part of the complex field arriving at the focus as a function of time and radius for =T/d (a) and =1 (b), and the corresponding intensity of the integrated field (solid) and the input pulse (dashed) as a function of time for the same cases [(c) and (d)]. The FWHM of the pulse is shortened from 1 ps to 210 fs (c) and 200 fs (d), a reduction by a factor of 5. The calculation assumes an f=150 mm lens with R=12 mm and d=5 mm. The pulse wavelength is 0.249 nm with =15 at laser intensity of 5×1011 W/cm2.

Page 11: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

11CLEO 08, San Jose, May 4-9, 2008

Parameter f/i

0 20 40 600.0

0.5

1.0

0 20 40 600.0

0.5

1.0

(rad)

0

0.2

0.4

0.6

0.8

1.0

R

NAfn

R2

)1(2

2

dakn 202

Max GVDE to pulse duration ratio

Max phase modulation

=2

=3

Page 12: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

12CLEO 08, San Jose, May 4-9, 2008

Numerical simulation

-2 -1 0 1 2-0.6

-0.3

0.0

0.3

0.6

(a)

t (ps)

z (

mm

)

0

0.2

0.4

0.6

0.9

1.1

0

2

4

(b)

r (m

)

-2 -1 0 1 20

2

4

(c)

t (ps)

Li and Crowell, Opt. Lett. 32, 92 (2007).

On-axis laser pulse envelope as a function of the defocusing distance; the intensity as a function

of time and radius for a pulse without (b) and with the SPM effect (c).

Page 13: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

13CLEO 08, San Jose, May 4-9, 2008

Content Introduction

– Pulse lengthening at lens focus Fourier formulation of the problem

– Axial temporal history

– Pulse shortening due to GVD

– Numerical simulation Experiment outlook Summary

Page 14: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

14CLEO 08, San Jose, May 4-9, 2008

An envisaged experiment

C

AL

ZSL

SF

PP

D

ODL

Page 15: Shortening a laser pulse at the focus of a lens Yuelin Li Accelerator Systems Division Argonne National Laboratory ylli@aps.anl.gov

15CLEO 08, San Jose, May 4-9, 2008

Summary

Pulse shortening demonstrated in simulation, up to 5 time shortening observed

Potential for few cycle pulse generation with simpler setup