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A general model for the permeability of fibrous porous media based on fluid
flow simulations using the lattice Boltzmann method
Aydin Nabovati a,*, Edward W. Llewellin b, Antonio C.M. Sousa a,c
a Department of Mechanical Engineering, University of New Brunswick, Fredericton, NB, Canadab Department of Earth Sciences, Durham University, Durham, UKc Department of Mechanical Engineering, University of Aveiro, Aveiro, Portugal
a r t i c l e i n f o
Article history:
Received 22 September 2008
Received in revised form 24 February 2009
Accepted 12 April 2009
Keywords:
A. Fibres
B. Mechanical properties
C. Computational modelling
E. Resin transfer moulding (RTM)
a b s t r a c t
Fluid flow analyses for porous media are of great importance in a wide range of industrial applications
including, but not limited to, resin transfer moulding, filter analysis, transport of underground water
and pollutants, and hydrocarbon recovery. Permeability is perhaps the most important property that
characterizes porous media; however, its determination for different types of porous media is challenging
due its complex dependence on the pore-level structure of the media. In the present work, fluid flow in
three-dimensional random fibrous media is simulated using the lattice Boltzmann method. We deter-
mine the permeability of the medium using the Darcy law across a wide range of void fractions
(0.086 /6 0.99) and find that the values for the permeability that we obtain are consistent with avail-
able experimental data. We use our numerical data to develop a semi-empirical constitutive model for
the permeability of fibrous media as a function of their porosity and of the fibre diameter. The model,
which is underpinned by the theoretical analysis of flow through cylinder arrays presented by [Gebart
BR. Permeability of unidirectional reinforcements for RTM. J Compos Mater 1992; 26(8): 110033], gives
an excellent fit to these data across the range of/. We perform further simulations to determine the
impact of the curvature and aspect ratio of the fibres on the permeability. We find that curvature has
a negligible effect, and that aspect ratio is only important for fibres with aspect ratio smaller than 6:1,
in which case the permeability increases with increasing aspect ratio. Finally, we calculate the permeabil-
ity tensor for the fibrous media studied and confirm numerically that, for an isotropic medium, the per-
meability tensor reduces to a scalar value.
2009 Elsevier Ltd. All rights reserved.
1. Introduction
Permeability prediction, and more generally, the investigation
of the effect of pore structure on the bulk properties of porous
media, has posed a major challenge to researchers and engineers
in a wide range of industrial and academic disciplines. These in-
clude, but are not limited to, resin transfer moulding [1,2], biomed-
ical engineering [35], subsurface flow of oil and groundwater[6,7], filter simulation [8,9] and fuel cell simulations [1012].
Macroscopic approaches for fluid flow simulation in porous
media, either using the Darcy law [13] or more complicated mod-
els [14], require as an input the permeability; however, the analy-
sis of the effect of pore-scale parameters on the macroscopic bulk
properties is a cumbersome task. The pore structure in porous
media is often complex, and complicated flow patterns exist within
the pores and between the grains. Consequently, permeability is
found to be highly medium-specific, hence there is no general
model for permeability as a function of the bulk properties of a
medium. The determination of permeability for a specific material
typically requires time-consuming experimental work.
Most experimental methods of permeability prediction apply a
constant pressure gradient to the porous medium and determine
the average flow velocity from the measured fluid flow-rate. The
mediums permeability is subsequently determined using the
Darcy law [13], as follows:
hui K
l:rp 1
where hui, K, rp and l are the volume-averaged flow velocity, per-meability tensor, pressure gradient vector and the dynamic viscos-
ity of the fluid, respectively. This relationship is valid in the
creeping-flow regime (Reynolds number ( 1).Earlier studies of porous media flow were conducted experi-
mentally and some of the best-known models for the permeability
of porous media are based on experimental data [1315]. In these
studies, primarily due to the macroscopic nature of the experimen-
tal approach, the details of the pore-scale flow-pattern in the
1359-835X/$ - see front matter 2009 Elsevier Ltd. All rights reserved.doi:10.1016/j.compositesa.2009.04.009
* Corresponding author. Tel.: +1 506 452 6128; fax: +1 506 453 5025.
E-mail address: [email protected] (A. Nabovati).
Composites: Part A 40 (2009) 860869
Contents lists available at ScienceDirect
Composites: Part A
j o u r n a l h o m e p a g e : w w w . e l s e v i e r . c o m / l o c a t e / c o m p o s i t e s a
mailto:[email protected]://www.sciencedirect.com/science/journal/1359835Xhttp://www.elsevier.com/locate/compositesahttp://www.elsevier.com/locate/compositesahttp://www.sciencedirect.com/science/journal/1359835Xmailto:[email protected]8/6/2019 Nab Ova Ti 09
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porous medium cannot be captured. In general, studying the effect
of pore-scale parameters on bulk properties requires a large exper-
imental dataset, which is time-consuming and expensive to
generate.
As alternative approaches, analytical and numerical methods
aim to predict the permeability by solving the fluid flow inside
the pores of the porous medium. The numerical procedure echoes
the experimental approach: a pressure gradient is applied; the
fluid flow inside the pores of the medium is solved; the permeabil-
ity of the mediumis then determined using the Darcy law (Eq. (1)).
This approach has two main advantages over the experimental ap-
proach. First, the geometry of the digitally constructed medium
can be varied rapidly and arbitrarily. Second, simulated experi-
ments are typically much quicker to run than their laboratory
counterparts. Together, these benefits allow a more-rapid and
more-thorough exploration of parameter space than can be
achieved in the laboratory.
The very first challenge in the numerical simulation of permeat-
ing flow is that the pore-level structure of the medium is required
as input. Imaging techniques, such as computed tomography
[16,17], have been developed to capture the complex structure of
real porous media; however, these methods may be costly and
time consuming and impose limits on the resolution that can be
achieved. The alternative approach, which has been widely used
in the literature, is to reconstruct the pore-level structure virtually.
The level of the reconstructed structures complexity depends on
the computational resources available and the nature of the prob-
lem under study. The reconstructed medium can be in the form of
ordered or random arrangements of two and three-dimensional
obstacles.
Analytical studies of the pore-level flow, in general, employ the
Stokes equation (a simplified form of the NavierStokes equation,
which is valid for creeping flow) for a specified domain with peri-
odic boundary conditions. Due to the limitations of the methods
applied, the computational domain, which is the building block
of the pore structure, is in the form of a simplified, well-defined
structure in which the grains of the porous medium are repre-sented in the form of two dimensional obstacles [18,19], ordered
sphere packing [20], or ordered packing of cylinders [2124].
Rapid increase in available computing power and the develop-
ment of advanced numerical algorithms mean that detailed
numerical simulations of flow in porous media are now feasible.
Removing the constraints of the analytical approaches, more com-
plex pore geometries, which resemble the real porous-media struc-
tures more closely, can be used in fluid flow simulations. Ordered
or random packing of different geometric configurations, such as
square blocks, spheres, cylinders, and parallelepipeds [25] have
been used in the literature to reconstruct the pore structure. The
choice of the constructing elements depends on the nature and
application of the porous medium to be modeled. Random arrange-
ments of spheres with mono-dispersed, bi-dispersed, or distrib-uted diameter are often used in simulations of flow in geological
materials, including studies of groundwater flow and hydrocarbon
recovery, and flow in packed beds, and rocks [6,7,2628]. Simula-
tions of flow in the preform matrix in resin transfer moulding
(RTM) [24,29,30], and through paper fibres [31,32] and woven
materials [9,3336] often use random arrangements of fibres.
1.1. Porositypermeability relationships for fibrous materials
The key parameter controlling the permeability of fibrous mate-
rials and, indeed, all porous materials is the porosity / = Vpore/
Vsample, where Vsample is the total volume of the sample and Vpore is
the volume not occupied by solid fibres. Several workers have pub-
lished relationships for the permeability of fibrous materials as afunction of their porosity.
Gebart [24] presents a combined theoretical, numerical and
experimental investigation of the permeability of ordered arrays
of fibres. The analytical treatment of creeping flow perpendicular
to the long axis of the fibres is predicated upon the assumptions
that permeability is controlled by the narrow slots formed between
the fibres at their closest approach and that the widthof these slots
varies only slowly. These assumptions are most valid in the limit of
close-packed fibres. Gebart derives the following functional form
for K(/):
K
a2 C
ffiffiffiffiffiffiffiffiffiffiffiffiffiffi1 /c1 /
s 1
!5=22
where a is the fibre radius, /c is the critical value of porosity below
which there is no permeating flow (the percolation threshold) and C
is a geometric factor (Gebart calculates C 16=9ffiffiffi
2p
p and/c = 1 p/4 for a square array, C 16=9
ffiffiffi
6p
p and /c 1 p=2ffiffiffi
3p
for a hexagonal array). Gebart presents numerical results, obtained
using a finite difference solution of the NavierStokes equations,
that show excellent agreement with the relationship up to at least
/ = 0.65.
Koponen et al. [31] used the LBM on a D3Q19 lattice to studycreeping flow through three-dimensional random-fibre sheets,
analogous to paper and non-woven fabrics. They report that the
permeability of such materials is exponentially dependent on the
porosity and independent of whether the fibres were placed ran-
domly or not. They present an empirical relationship for the per-
meability as a function of the porosity, based on a fit to their
data, for porosities in the range 0.4 < / < 0.95:
K
a2
5:55
e10:11/ 13
Clague et al. [37] also studied the permeability of three-dimensional
ordered and disordered fibrous media. They used the lattice Boltz-
mann method (LBM) on a D3Q15 and D3Q19 lattice to simulate
creeping flow through fully three-dimensional random fibre net-
works, in which free overlapping of the fibres was allowed. Both
wall-bounded and unbounded media were considered and the ef-
fect of the wall on the overall permeability of the fibrous media
was investigated. They use a scaling analysis to develop a phenom-
enological relationship between permeability and porosity for both
the bounded and unbounded fibrous media. For the case of an un-
bounded medium, they find:
K
a2 b1
ffiffiffiffiffiffiffiffiffiffiffiffiffiffi1 /c1 /
s 1
!2eb2 1/ 4
where b1 and b2 are curve fitting parameters. For a disordered (ran-
dom) arrangement of fibres, Clague et al. calculate a typical value of
/c = 1p/4 % 0.21 but with a 1r variation that gives minimum andmaximum values of /c = 0 and /c 2 ffiffiffiffipp p % 0:4, respectively.They show an excellent fit to their data, which span the range
0.33 < / < 0.95 (i.e. they do not cover the region near the percola-
tion threshold).
In the present work, fluid flow is simulated in 3D random fi-
brous media at the pore level. We employ the lattice Boltzmann
method for the fluid flow simulation and calculate the permeabil-
ity of the medium using the Darcy law. We cover a wide range of
porosity, from near the percolation threshold to very dilute sys-
tems (0:08 / 0:99). Based on curve fitting of our numericalexperimental results, we propose a semi-empirical constitutive
relationship for the permeability as a function of porosity. We also
investigate the effect of various other pore-level parameters,
including the curvature, diameter and aspect ratio of the fibres,
on the predicted permeability.
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2. Methodology
The complex structure of the pore-level geometry, especially in
media of low porosity, yields small pores and narrow flow pas-
sages. As a rule of thumb, the local flow velocity in these narrow
pores is proportional to the volume-averaged flow velocity divided
by the porosity. The narrow flow passages and locally high veloci-
ties limit the applicability of the conventional computational fluiddynamics approaches. Mesoscopic methods such as the smoothed
particle hydrodynamics (SPH) [38,39], lattice gas automata (LGA)
[40,41] and lattice Boltzmann method (LBM) [4244] have been
successfully used for macroscopic fluid flow simulations, which re-
quire the mesoscopic details of the flow to be considered. The LGA
and SPH methods, in their current state-of-the-art, tend to be com-
putationally costly to perform three-dimensional simulations of
flow in porous media that are of a size adequate to yield physically
meaningful results. Although the early versions of LBM [45] suf-
fered from similar difficulties, later developments of the LBM have
seen dramatic improvements in the computational efficiency, mak-
ing it a suitable tool for mesoscopic, three-dimensional simulations
[42,46,47]. Other attractive features of the LBM are that numerical
operations are spatially local, easing implementation, while solid
boundaries of arbitrary complexity can be included without perfor-
mance penalty. Furthermore, the LBM is well suited to flow simu-
lation at the mesoscopic scale, and is amenable to parallelization.
These characteristics have made the LBM the most popular method
for numerical pore-level analysis; indeed this was one of the first
applications of LBM [48]. The LBM has been shown to be a more
efficient tool for flow simulation in such complex geometries than
conventional fluid dynamic approaches [49,50].
In the present work, three-dimensional fluid flow was simu-
lated in fibrous porous media using LBflow,1 an implementation
of the single-relaxation-time (SRT) LBM on a D3Q15 lattice [51,52].
As in all such implementations, the flow is represented by the prop-
agation of fluid mass through a lattice. The lattice is a discrete
representation of physical space; in the present case a three-dimen-
sional cubic lattice. At any time t, fluid mass can propagate from anode with position r to any of its six orthogonal neighbours or eight
long-diagonal neighbours, or it can remain at the present node. Since
time is also discrete, the propagating fluid arrives at its new location
at time t+ 1, hence, there are i = 15 possible fluid velocities at each
node, represented by the vector ei. The spatial discretization Dx
and the time step Dt define the units of the simulation. The total
density at each node is given by:
qr; t X
i
fir; t 5
where q is also in simulation units (typically initialized to q = 1throughout the lattice). Similarly, the average fluid velocity at each
node is given by:
ur; t P
ifieir; t
qr; t6
In addition to the propagation step, at each node r, at each time step
t, the incoming fluid masses fi undergo collision, in which they re-
lax towards the equilibrium distribution:
feqi qxi 1 ei u
c2su u
2c2s
ei u2
2c4s
" #7
where the weightsx0 = 2/9,x1. . . 6 = 2/9 and x7. . .14 = 1/72, and thelattice pseudo-sound speed cs Dx=
ffiffiffi
3p
Dt. This equilibrium distri-
bution is a discrete analogue of the Maxwell-Boltzmann distribu-
tion for a population of fluid particles having the same density q
and average velocity u as the incoming fluid masses in the simula-
tion. The propagation and collision steps are encapsulated in the
lattice Boltzmann equation:
fir eiDt; t Dt
|fflfflfflfflfflfflfflfflfflfflfflfflfflfflffl{zfflfflfflfflfflfflfflfflfflfflfflfflfflfflffl}propagation
fir; t fir; t f
eqi r; t
s
|fflfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflffl{zfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflfflffl}collision
8
where s is a relaxation parameter, related to the fluid viscosity. Inthe implementation of the LBM adopted in the present work, flowis driven by imposing a constant, uniform body force G on the fluid
at every point, which is physically analogous to a gravitational force
acting on the fluid. This is achieved by adding an extra term gi to
each of the mass components fi prior to propagation. The term giis formulated in such a way that the total mass is conserved but
the momentum is adjusted to account for the force acting on the
mass at the node for the duration of the time step:
gir; t xiDtc2s
G ei 9
This term is added to the right hand side of Eq. (8). The halfway
bounceback method [44] was used to implement the solid wall
boundary condition.
LBflow uses a scripting language to set up the flow simulation;
via an interpreted text file, the user can specify the geometry and
parameters of the simulation. In this study, the geometries of the
porous media of interest are specified as a three-dimensional bin-
ary mask of the simulation lattice. Dimensional quantities for the
simulation are specified in SI units, rather than simulation units.
In this study, the working fluid has the properties of water at
20 C: kinematic viscosity m = 1.004 106 m2 s1, densityq = 998.29kg m3. The driving pressure gradient rp is specifiedin units of Pa m1. Once the flow has settled to steady state, theaverage velocity of the fluid nodes u is output in SI units. The vol-
ume-averaged fluid velocity hui /u is determined allowing thepermeability of the medium to be calculated using the Darcy law,
Eq. (1). Note that the choice of the working fluid properties is
somewhat arbitrary, since the permeability is independent of vis-
cosity, density and driving pressure gradient for creeping flow
(i.e. Reynolds number Re ( 1). This was confirmed numericallyby repeating a typical simulation multiple times for a range of
rp spanning several orders of magnitude, all at low Reynolds num-ber; the calculated permeability was indeed independent of pres-
sure gradient.
The fluid viscosity is related to the relaxation parameters of theSRT LBM:
m s1
2
c2sDt 10
The relaxation parameter represents the degree to which the fluid
populations are relaxed towards the equilibrium value during thecollision step (Eq. (8)). Consequently, the larger the value of the
relaxation parameter, the more rapid is the flow settlement. How-
ever, we should note the use of the halfway bounceback method
for the solid wall boundary condition with the SRT LBM, yields pre-
dictions of the flow field in porous media, and therefore of their per-
meability, that are dependent on the choice of the relaxation
parameter. Consequently, the accuracy of the simulation is depen-
dent on the relaxation parameter. Pan et al. [53] evaluated different
LB methods and solid wall boundary condition treatment methods
for flow simulations in porous media. They showed that results ob-
tained using the SRT LBM with the halfway bounceback method for
the solid boundaries are in good agreement with the results of the
MRT LBM with interpolated bounceback boundaries, and that the
effect of the relaxation parameter dependency is negligible for
s = 1. We set the relaxation parameter equal to 1 in all the1 Available from http://www.lbflow.co.uk.
862 A. Nabovati et al./ Composites: Part A 40 (2009) 860869
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simulations performed. This value represents the best compromise
between simulation accuracy and the rate of flow settlement.
3. Results and discussion
3.1. Validation
To validate our methodology, we simulate creeping fluid flow in
a hexagonal array of infinite, parallel cylinders. The radius of the
cylinders was kept constant and equal to 40 lattice units in a do-
main of l ffiffiffi
3p
l 1, where l was varied between 82 and 230 latticeunits; this yields a medium of porosity between 0.15 and 0.89.
Fig. 1 depicts the schematic of the computational domain unit cell
with periodic boundary conditions on both sides; the gray colour
identifies the simulation domain. Due to the invariance of the do-
main geometry under translation in thez-direction, a fully 3D sim-
ulation can be achieved with a domain 1 lattice unit thick in that
direction by using periodic boundary conditions.
The results of these simulations are presented in Fig. 2, which
compares the permeability, calculated according to the methodol-
ogy presented in Section 2, with the value determined analytically
using the relationship for this geometry presented in [24] (Eq. (2)).
This model, described in Section 1.1, has been widely used for flow
in regular arrays of fibres [54,55]. The agreement over the range of
porosities for which that relationship is valid, i.e. 0.10 < / < 0.65, is
excellent. It is noteworthy that the fit between the data and the
analytical solution is good even beyond the upper limit of validity
claimed by Gebart (dotted line in Fig. 2).
3.2. Flow in fibrous media
To create the fibrous medium structure, randomly oriented,
straight, cylindrical fibres of constant diameter are randomly
placed in a cubic domain with free overlapping. By allowing the fi-
bres to overlap freely, we are able to investigate flow in fibrous
media with porosities across the full range, right down to the per-
colation threshold. Media in which the fibres are not able to over-
lap have a minimum porosity, which is higher than the percolation
threshold. Koponen et al. [31] studied the fluid flow in three
dimensional fibre webs, where flexible fibres were placed ran-
domly in the computational domain without overlapping, the min-
imum reported porosity was higher than 0.4. Nabovati and Sousa
[56] investigated the permeability of sphere packs with and with-
out free overlapping. They found that overlapping has a negligible
impact on permeability for media with porosities higher than 0.85
and leads to a decrease of less than 35% in permeability for low
porosity media. The minimum reported porosity for random pack-
ing of spheres without overlapping was 0.55.
The computational domain comprises a cube of 128 lattice sites
on each side and the periodic boundary condition was applied to
all faces of the cube. The fibres extend to the boundaries of the do-
main. The fibres are placed in the computational domain by using
the following algorithm: (1) a random position vector is chosen
within the computational domain, or one fibre radius of it, as the
origin of the fibres core, (2) a random vector representing the spa-
tial orientation of the fibre core is generated, (3) the fibre core line
is extended from the origin point along the randomly determined
orientation in both directions until it intersects the domain bound-
aries, and (4) lattice sites that are closer to the core line than the
radius of the fibre are designated as solid. The radius of the fibres
is constant along their length and equal to 2, 3, 4, 5 or 6 lattice
units, Dx, depending on the experimental run. Fig. 3 shows a high
porosity sample of the reconstructed fibrous medium; the porosity
of the sample is 0.80.
Fig. 1. Schematic of two dimensional section through the computational unit cell
used for the permeability prediction in hexagonal arrangement of cylinders; flow
domain with periodic boundary conditions on both sides is shown in gray colour.
0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.910
-6
10-4
10-2
100
102
Porosity ()
Present Work
Gebart [24]
K/a2
Fig. 2. Normalized permeability, calculated using the methodology presented in Section 2, is plotted with the analytically-determined relationship (Eq. (2)) presented byGebart in [24] for a hexagonal arrangement of solid cylinders. Gebarts relationship is shown dotted outside the range of values of / for which Gebart claims validity.
Fig. 3. Reconstructed medium with straight fibres and porosity/ = 0.80; the radius
of the fibres is four lattice units and their length is such that they span the
computational domain.
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A pressure gradient is applied in thex-, y- orz-direction and the
velocity field is calculated in the pores of the reconstructed med-
ium. Fig. 4 shows the velocity vectors in a slice of a three-dimen-
sional fibrous medium which has a porosity equal to 0.2; the
pressure gradient, and the mean flow direction, are in the positive
x-direction. We should note that, whilst some pores appear to be
dead-end or isolated in the two-dimensional slice, in the third
dimension, these pores are effectively connected to each other
and they contribute to the fluid flow pattern. As a result, the per-
colation threshold reported to be equal to 0.33 for two-dimen-
sional media made up of random arrangements of squareobstacles [57], in fact, takes a lower value for three-dimensional
media. In the present study, permeating pathways for fluid flow
exist for porosity as low as 0.08.
3.2.1. Effect of fibre radius
Permeability has dimensions of length squared, and it is usual
to normalize permeability by the square of a length scale that is
characteristic of the system; for fibrous media, this is typically
the fibre radius. To validate this approach, we determine the per-
meability of random networks of fibres with radii of 2, 3, 4, 5
and 6 lattice units. Results are shown in Fig. 5. Fig 5 demonstrates:
(1) permeability increases as porosity increases for constant fibre
radius; (2) permeability increases as fibre radius increases for con-
stant porosity. Fig. 5b demonstrates that normalizing the perme-ability by the square of the fibre radius causes the curves for
different fibre radius to collapse onto a single curve, hence, that
this non-dimensionalization is appropriate. Note that the normal-
ized permeability is not completely independent of fibre radius;
the two show an inverse relationship with the normalized perme-
ability for the thinnest fibre typically about 20% higher than for the
fattest on average. We postulate that this dependence is due to the
finite length of the fibres in our simulations giving rise to a variable
aspect ratio as the fibre radius is increased. This is supported by the
results presented later in Section 3.2.4.
3.2.2. Constitutive permeabilityporosity relationship for random fibre
networks
We determine the permeability of around 50 random fibre net-works in the x-, y- and z-direction (giving $150 data points in to-
tal). For each network, the fibres all have the same radius: either 2
or 4 lattice nodes. The permeability of the networks is in the range
0.08 < / < 0.99. Results are plotted in Fig. 6 (note the logarithmic
scale on the permeability axis). The normalized permeability is
approximately exponentially dependent on porosity in the range
0.2 < / < 0.9. At lower and higher porosities, the dependence is
stronger. As expected, the permeability tends towards infinity in
the limit /? 1 and drops towards zero at low (but finite) porosity.
We note that the variation in the data is greatest at very low poros-
ities, where random differences in the placement of the fibres be-
tween different domains lead to large relative changes in thepredicted permeability.
We find that a modified version of the Gebart [24] relationship
provides an excellent fit to data across the full range of porosity
(Fig. 6). We adapt Gebarts original relationship (Eq. (2)) by allow-
ing the three constants it contains to vary:
K
a2 C1
ffiffiffiffiffiffiffiffiffiffiffiffiffiffi1 /c1 /
s 1
!C211
where /c is the critical value of porosity above which permeating
flow can occur (the percolation threshold). C1 and C2 are related
to the geometry of the network (compare with the values deter-
mined by Gebart for a regular array of fibres, presented in Section
1.1). We use the freely-available statistical analysis package SimFit2
to fit Eq. (11) to the data presented in Fig. 6. The fit is carried out in
logarithmic space to avoid biasing the fit towards large values of per-
meability at high porosity. Table 1 shows the best fit values obtained
(R2 = 0.999).
The values are consistent with those determined analytically by
Gebart for a hexagonal array of aligned fibres (Section 1.1); differ-
ences are due to the different geometries of the networks. The va-
lue of/c falls within the range calculated, on statistical grounds, by
Clague et al. [37], for a random network of fibres (Section 1.1).
The published relationships of Koponen et al. [31] and Clague
et al. [37] Eqs. (3) and (4), respectively in Section 1.1 were sim-
ilarly adapted and fitted to the data in Fig. 6. The Koponen relation-
ship provided a very poor best fit to data, and was abandoned. The
Fig. 4. Velocity vectors in a slice of the three-dimensional fibrous medium; the porosity of the sample is 0.2 and the pressure gradient drives flow in the positive x direction.
2 Available from: http://www.simfit.man.ac.uk.
864 A. Nabovati et al./ Composites: Part A 40 (2009) 860869
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best fit of the Clague relationship was as good as the Gebart fit. We
favour the Gebart relationship because it has a sound theoretical
basis, whereas the Clague relationship is purely phenomenological.
To assess the variation of the predicted permeability values due
to the random nature of the reconstructed fibrous porous media,
we performed multiple repeated simulations for media at three
different porosities: $0.1, $0.5 and $0.95, respectively. Due tothe discrete nature of the fibre placement procedure, it is not pos-
sible to create different random media with exactly the same
porosity; hence, there is a variation of around 0.5% for each pre-
scribed porosity. For each porosity, we created 21 media with dif-
ferent random fibre placement and simulated flow in x, y, and z
directions, resulting in 63 permeability determinations for each
porosity. Each dataset is separately plotted against porosity inFig. 7; the permeability predicted using Eq. (11), with the parame-
ter values presented in Table 1, is shown on each plot as a solid
line. Table 2 shows the mean permeability for each dataset and
the permeability normalized by the value predicted using Eq.
(11). The standard deviation is also presented, expressed as a per-
centage of the mean permeability.
From Fig. 7 and Table 2, it can be seen that both the extent of
the variation in permeability and the quality of fit of Eq. (11) de-
pend on the porosity. The standard deviation is small (around
10% of the mean) for mid and high-range porosity; at very lowporosity, the standard deviation is larger (around 50% for /
% 0.1), reflecting the large changes in permeability that arise fromsmall structural differences near the percolation threshold. Eq. (11)
has a tendency to slightly under-predict permeability at lowporos-
ity and to over-predict at high porosity. Given the$6 order of mag-nitude difference in permeability between / % 0.1 and / % 0.95,however, we consider Eq. (11) to provide an accurate and flexible
tool for permeability prediction across the porosity range and note
that the model value is within one standard deviation of the
numerical data across the porosity range.
The literature contains permeabilityporosity data from a num-
ber of laboratory investigations into fibrous media; Jackson and
James [23] provide a summary. In Fig. 8, we compare our perme-
abilityporosity relationship (Eq. (11)) with experimental datafor high porosity fibrous media with randomly oriented straight
0.2 0.4 0.6 0.8 110
-10
10-9
10
-8
10-7
10-6
10-5
Porosity ()
K
(m2)
a = 2 lu
3
4
5
6
0.2 0.4 0.6 0.8 110
-3
10-2
10-1
100
101
Porosity ()
K/a2
(b)(a)
Fig. 5. (a) Numerically-determined permeability as a function of theporosity for fibres with a range of radii. Within each simulation suite, all fibres have thesame radius; (b)
numerically-determined permeability normalized by fibre radius as a function of the porosity.
0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 110
-6
10-4
10-2
100
102
K/a2
Numerically Predicted Values
Proposed Relation, Eq. 11
Porosity ()
Fig. 6. Dimensionless permeabilityas a function of porosity for randomnetworks of straight fibres. Fibre radius is 2 or 4 lattice units in allcases. Thesolid line shows thefit of
our semi-empirical relationship (Eq. (11)) which is adapted from Gebart [24]. Best fit parameters are given in Table 1. The fit (R2 = 0.999) indicates a percolation threshold of
/c% 7.4%.
Table 1
Best fit parameters of Eq. (11) to data presented in Fig. 6; regression coefficient
R2 = 0.999. See main text for details of fitting procedure.
Parameter Best fit value
/c 0.0743
C1 0.491
C2 2.31
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cylindrical fibres of constant diameter presented in that work. The
data were obtained using a range of experimental methods, a
broad spectrum of fibrous materials including filter pads, nylon fi-
bres, Kapron fibres, collagen, metal fibres and polymer fibres, and
various working fluids including water, glycerol and air. Despite
the diversity of these investigations, there is a broad agreement
(within an order of magnitude) among the resulting datasets. Over-
all the agreement between Eq. (11) and the experimental data is
good, especially for porosities higher than approximately 0.75.
3.2.3. Effect of fibre curvature
We investigate the effect of fibre curvature on the permeability
of fibrous media, by replacing straight fibres with randomly curved
fibres as the constituting elements of the medium. We generate the
fibres by constructing a cylinder of constant diameter around a
randomly curved fibre core. The origin of the fibres is chosen ran-
domly. Three different third-order polynomials represent the three
coordinates defining the orientation of the fibre core and they are a
function of a single variable, t:
xi ai;3t3 ai;2t
2 ai;1t ai;0 i 1; 2; 3 12
where the coefficients of these polynomials are chosen randomly in
the range of [1,1], this ensures that fibres are smoothly curved and
avoids tight spirals. The variable tis incremented and decrementedin appropriate steps to extend the fibre in both directions until the
fibre reaches the domain boundaries, producing a smoothly curved
fibre, which crosses the domain.
Fig. 9, shows the permeability we determine from simulations
of flow in media composed of curved fibres. The results are almost
indistinguishable from the results for straight fibres; and the effect
of the fibres curvature on the overall permeability of the medium
can be considered negligible.
3.2.4. Effect of fibre aspect ratio
We investigate the effect of fibre aspect ratio a (length to diam-eter ratio of straight cylindrical fibres of finite length) on perme-
ability for a range of aspect ratios between 1 and 20, for twodifferent values of porosity, namely 0.51 and 0.73. The fibres diam-
4.0
5.0
6.0
7.0
8.0
9.0
0.946 0.947 0.948 0.949 0.950
Porosity ( )
K/a2
0.030
0.035
0.040
0.045
0.050
0.055
0.060
0.497 0.498 0.499 0.500
Porosity ( )
K/a2
(a) (b)
0.0E+00
2.0E-05
4.0E-05
6.0E-05
8.0E-05
1.0E-04
1.2E-04
1.4E-04
0.0995 0.0996 0.0997 0.0998 0.0999 0.1
Porosity ( )
K/a2
(c)
Fig. 7. Dimensionless permeability for three different porosities: (a) $0.95, (b) $0.5, and (c) $0.1. At each porosity, the permeability was determined for 21 different randomnetworks of straight fibres to determine the random variation in permeability. The solid line represents Eq. (11) with the parameters given in Table 1. Note the dramatically
expanded scales compared with Fig. 6. See Section 3.2.2 for discussion.
10-3
10-2
10-1
100
10-4
10-3
10-2
10-1
100
101
102
103
Solid Fraction (1-)
K/a2
Chen (1995)
Ingmanson et al. (1959)
Kirsch & Fuchs(1967)
Stenzel et al. (1971)
Kostornov & Shevchuck (1977)
Jackson and James (1982)
Proposed relation, Eq. 11
Fig. 8. Comparison of dimensionless permeability of fibrous media, calculated
using Eq. (11) with the parameters given in Table 1, with the experimental data
reported by Jackson and James [23]. Readers are directed to that work for full
references to the original experimental studies.
Table 2
Mean permeability and standard deviation for three different porosities: $0.1, $0.5,
and $0.95. See Fig. 7.
Porosity Mean permeability (K/a2) Mean permeability
(normalized to Eq. (11))
Standard
deviation (%)
$0.1 2.58
105 2.09 52
$0.5 4.62 102 1.01 10$0.95 7.50 0.877 11
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eter is constant and equal to 6 lattice units and the aspect ratio is
varied by changing the fibres length. The numerically-determined
values of the permeability are shown in Fig. 10 as a function of the
fibre aspect ratio; the permeability values are normalized by the
permeability calculated using Eq. (11). It can be seen that perme-
ability increases with aspect ratio for a < 6; for a > 6, permeabilityis largely independent of aspect ratio. This finding explains the
imperfect collapse of the data for fibres of varying radius, pre-
sented in Fig. 2, when normalized by the fibre radius. Since the
length of the fibres is finite limited by intersection with the do-
main boundaries the aspect ratio of the fibres in that suite of sim-
ulations varies somewhat with fibre radius.
For a cylinder of diameter d, the ratio of the surface area to the
volume of the fibre (specific surface area) is equal to 1d4 1a. An
increase in aspect ratio therefore yields a decrease of the specific
surface area of the fibres, leading to a reduction in the frictional
drag force and higher values for the permeability.
3.2.5. Permeability tensor
Any experimental or numerical attempt to determine the per-meability tensor and the principle directions of a porous medium
should be performed in three dimensions. This is an expensive
and time consuming task. Neuman [58] proved analytically that
the permeability tensor is a symmetric second order tensor, which
has six distinct elements in general. For isotropic materials, the
three diagonal elements are equal and non-zero and all off-diago-
nal elements are zero. In this case, the permeability can be repre-
sented as a single, scalar value.
Ahn et al. [59], Weitzenbck et al. [60,61] and Parnas et al. [62]
discuss experimental methods and approaches for permeability
tensor measurements. Kolodziej et al. [63] analytically investigated
the permeability tensor of high porosity fibrous porous media. In
their study, fibres had a unidirectional arrangement with non-uni-
form spacing. Nedanov and Advani [64] studied fluid flow in two-
scale fibrous porous media numerically; governing equations of
the fluid flow around and inside the solid and permeable fibres
were developed using the homogenization method and were
solved numerically. They report the diagonal elements of the per-
meability tensor for single and three-ply fabrics. Song et al. [35]calculated the permeability tensor of a three-dimensional, woven
fibrous medium using the finite volume method.
In this study, to evaluate the viability of the LBM for permeabil-
ity tensor determination, the permeability tensor elements of three
samples of different porosities of 0.90, 0.70 and 0.50, respectively,
are determinedbased on the simulated flowfield. For eachporosity,
a pressure gradient is applied in one of the three principle direc-
tions. The mean flow is in the direction of the applied pressure gra-
dient, which builds the diagonal element of the permeability tensor
in the specified direction. We calculated the off-diagonal elements
of the permeability tensor using the net flow in each of the other
two directions, and repeated this procedure for each of the three
directions to obtain the nine elements of the permeability tensor.
The predicted permeability tensors for these media are as follows:
K0:90
1:0866 0:0073 0:0203
0:0073 1:0526 0:0138
0:0206 0:0138 1:0820
264
375 107 m2
K0:70
1:1643 0:0262 0:0021
0:0262 1:1726 0:0006
0:0021 0:0006 1:1632
264
375 108 m2
K0:50
1:8851 0:0478 0:0395
0:0478 1:9017 0:0029
0:0395 0:0029 1:8484
264
375 109 m2
As the media are created with randomly-oriented fibres, there is no
preferential flow direction and the media are expected to be isotro-
pic. In each case, we find that the diagonal elements of the perme-
ability tensor are the same to within $3%; this small difference caneasily be accounted for by the random nature of the network. Fur-
thermore, the off-diagonal elements are approximately symmetri-
cal, and are smaller than the diagonal elements by around two
orders of magnitude. These results support the analysis of Neuman
[58] and demonstrate that it is valid to report a scalar value for per-
meability of these random porous media, and a determination of
the full second order tensor is unnecessary.
4. Conclusion
Three-dimensional fluid flow simulations in fibrous media are
conducted using the SRT LBM; the fibrous media are recon-structed by random placement of cylindrical fibres, with random
0 5 10 15 200.5
0.6
0.7
0.8
0.9
1
Fiber Aspect Ratio
K/Kmodel(Eq.
11)
Phi = 0.505
Phi = 0.730
Fig. 10. Effect of the fibre aspect ratio on the numerically-determined permeability
for two different porosities, 0.51 and 0.73, respectively; permeability values are
normalized by the permeability calculated using Eq. (11) with theparameters givenin Table 1.
0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 110
-4
10-2
100
102
Straight Fibres - Equation 11
Curved Fibres
K/a2
Porosity ()
Fig. 9. Numerically-determined permeabilityof fibrous media as a function of the porosity for media formed of straight (solidline, Eq. (11) with parameters given in Table 1)
and randomly curved fibres (circles, simulation results).
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orientations, within the computational domain. The radius, curva-
ture and length of the fibres are varied systematically. We find that
dividing the permeability by the square of the fibre radius yields an
appropriate non-dimensionalization. We also find that fibre curva-
ture has a negligible impact on the permeability of the medium.
For fibres of finite length with aspect ratios smaller than $6,permeability increases with increasing aspect ratio; this effect is
negligible for values of the aspect ratio greater than 6.
The permeability values that we obtain are compatible with the
available experimental data and, based on the determined values,
we develop a relationship (Eq. (11)) for the permeability as a
function of the materials porosity and the fibre diameter. The
relationship that we present results from a semi-empirical
parameterization of a published analytical relationship for ordered
arrays of fibres [24]. The fit of the relationship to the data is excel-
lent across the range of porosities investigated (0.08 < / < 0.99).
Our analysis shows that the percolation threshold for a three-
dimensional network of randomly oriented fibres is /c = 0.0743 .
The media in this study were created randomly, hence there
was no preferential direction for the flow through the medium;
therefore, the media can be assumed isotropic. Prediction of the
permeability tensor for media of three different porosities sup-
ported this assumption, as the diagonal elements of the numeri-
cally-determined permeability tensors differ by less than $3%,and the off-diagonal elements were two orders of magnitude smal-
ler than the average value of the diagonal elements. This finding
indicates that it is valid to report a scalar value, instead of a second
order tensor, for the permeability of the fibrous media studied.
The results obtained in this study and the general relationship
proposed for the permeability, can be fed to the macroscopic flow
modelling approaches for the industrial applications, e.g. resin
transfer moulding process, where the pore level approach is not
applicable due to the large computational resources requirement.
Acknowledgment
The authors acknowledge the support received from NSERC(Natural Sciences and Engineering Research Council of Canada)
Discovery Grant 12875 (ACMS) and from the Foundation for Sci-
ence and Technology (FCT, Portugal) through the research grant
POCTI/EME/59728/2004 (ACMS). EWL is supported by NERC (UK)
Research Fellowship NE/D009758/2. We thank two anonymous
reviewers for their helpful comments.
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