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JAERJ-Research 96-009 B * n ^ ^j if % m Japan Atomic Energy Research Institute VOL 271&17

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JAERJ-Research96-009

B * n ^ j if % mJapan Atomic Energy Research Institute

VOL 271&17

in. ii t«'?.r

i -cwiti £ * %tt -m tu >* H if; •,

I hi* report t» MM»OI trrfjf»l.ifl>

.iKml .i\.nl.ihttil) of Ilic report* IIHMIIJ be mtilrctKil In Infcrnution

vf fahnicj} tnfotmjtiufc Jjpun Atomic iintity Rf*cjfsb Intitule.

.K N.ik.i-gun. IKir.iWi-kcn JI 'MI , J.ip.in

(I Mv. r /i if -«

JAIJKI-ltesflftrcli 00-009

Vc^h ¥.»!•> II ^ ^ M ^ H

JAIiKI-Ki-swtrcli «0-00»

rubrical ion of Uranium IMu ton him Mixed Carbide and

Nitr ide h i d IMns for the Irradial ion Test in JOVO

Ynsuo AKAI. Tabs l i i M i . Tsitsiin SASAYAMA. Yosfiihiro OKAMOTOKen ichi S1IIOZAWA and Yasuftimi SUZUKI

Department of Chemistry and Fuel Research

Tok;il Research Hstablishtnunl•Ifipan Atomic Hncfgy Kescarcli I n s t i t u t e

Tokai irnira. Naka p n . lli;iraki-kcn

(Kecelveil Jamiiiry 3n. l!)!

One ttraiiititn phi lott him mixed carliidc fuel pin and Un nilridt* fire I pins were faliricittcdfor the i r r a d i a t i o n l e s t in f a s t t e s t r e a c t o r JOVO based on the JAIiKI I'NC j o i n tresearch program e n t i t l e d "Hasic Irradiat ion Test of Carbide and Ni tr ide Fuels for I'aslKeaetors". This paper summarizes I lie r e s u l t s of the study JAIiRl mainly has heen in• li;ir>;c of no far in the program, including the design of fuel pins, preparation of fuelp e l l e t s , fabr icat ion of fuel pins and so on.

Keywords: Cranium. Plutonium. Mixed Carbide. Mixed N i t r i d e . I r r a d i a l i o n T e s t , f u e lI ' d l e i . Fuel I ' in. Fas t Test R e a c t o r .I0V0. Advanced F u e l . I r r a d i a t i o nVertnrmme

»l»*-ti *.i«. U V K W I U I uMlrf lf«% JU.bl'I'NC ioint t iM' .mh

I

2, fflif!(t'>fiffl| 'I

2. 1 Mtt i l '" • • • "•' 22.2 m\\\m\ 2

a i immn uU-y KDMiii 3U-y h©Mia "» • I

3.4 I'JUIWi'l t3.5 WttWfa t

4. m\V's<?>*A\X- • T.}, | B H b * > « l « l « M 74.2 4af!bT>t&M(T: ••• 74. 3 til\&\!&\iW& 71. J m\t'x/)\m s

5. bhfrh • »;« W • o

• a

tit

Contents

1. Introdnct ion ' i"""111" 1

2. t)osi)?n of Fuel Pins *i> v ' i «" 2

2. 1 Basic Design • • »•••• • 2

2.2 Detailed Design 2

3. Preparation of Fuel Pellets • 3

3. 1 Raw Materials 3

a 2 Preparation of Carbide Pellets 3

3.3 Preparation of Nitride Pellets • •» ""•'• ' <t

3. 4 Centerlcss Grind trie •••• * "•• • •••••• • 43. 5 Characterization ••"»»"•"»»•»•» » «...».. ...„.„,„,„.,„,„,„„....... ,\

4. Fatirication of Fuel Pins - 74. 1 Constituent Parts of hie I Pins 71.2 Fatirication of Fuel Pins • 7

1.3 Execution Tests of Welding 7

4.4 Inspection of Fuel Pins 8

5. Postscript • 0

Acknowledgement "'•* 9

References • * • • U

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Table I l!;isk of fuel jdus for irradiation tcstK In .10V0

f'l'.'l

raei f i l le tCoffifr&ition

' •'• U enrichment (ut.%)tVjruJity (£f.D.)Dia/fcter (ram)^taek length (fiffi)

CcRipoditicnDensity (7,T.D.)Diameter (itrti)L'tack length (fwn)

Cladding tut«Mator'iaLOitT'f filnftK?t/?r (tffti)ThiokiwiJS (tun)

Fuel pina>:ar fierv'Jity (5TT.D.)ix-riz-'th (frm)

(UPFUJGI, v ; ,

21.3519.39

857.'*2

200

85

52.5 / 2

Aictonlttc

0.U5

81800

Hitfido-1

'19.2619.39

657.28

200

W857.28

52.5 x 2

Austentfcic8.50.^5

7880O

Nitride-2

(U,Pil)N'19.26

19.39857.H2

200

mm7.H2

52.5 x 2

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81800

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T a b l e 3 Cl u i n i c t c r l s t l o s of c a r b i d e m i d n i t r i d e fuel pel lots

Ditit/jte*' (fun)

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Carbon content (wt.$)Nitrogen content (ut.%)oxygen content (wt.#)C/(U»Ri) or N/(U+hO ratio

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X-tTiy diffraction analysis(U,Pu)C (U,PU)H

Lattice poramotep of fee (run) 0.U9651 O.U89tO 0.H89270-cludod gasea (// C /g) 30 20 20Metallic Impurities (ppffl)

AI 110 70 30Cn 60 U0 noC'd <10 <J0 <J0Co 120 170 90CP 110 60 30Fo 180 50 30Mg 50 30 20Hi 90 30 30V 360 230 50W '(80 1280 530

390 200 I/JO100 80 90

Table I Cluiraclorisiic.'i of carbide and nil ride fuel pins

Total length (an)

Fuol nt.-iek length (rnm)

FlontKt length (rw)

E3cwlrtg (m)

ir*Oig»ht (g)

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321.0

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(I)) Nitride pellet of diameter 7.28mm , 40Mm

(c) Nitride pellet of diameter 7. l rara 40fim

Fi&2 Mitrnslructiirc of fuel pellets

14 -

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: MC-J0Y0-L0

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Fig.3 X-ray diffraction patterns of carbide and nitride fuel pellets

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(a) Carbide p e l l e t

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2mm

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.4 ri-atitormliatirapliy of fuel pellets

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