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Getting All the Light Out: Light Extraction from Organic Light Emitting Devices Yue Qu 1 Prof. Stephen Forrest 1,2,3 1 2018 SSL R&D workshop 1 Department of Electrical Engineering and Computer Science, 2 Physics Department, 3 Department of Materials Science and Engineering, University of Michigan, Ann Arbor

Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

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Page 1: Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

Getting All the Light Out: Light Extraction from Organic Light Emitting Devices

Yue Qu 1

Prof. Stephen Forrest 1,2,3

1 2018 SSL R&D workshop

1Department of Electrical Engineering and Computer Science, 2Physics Department, 3Department of Materials Science and Engineering,

University of Michigan, Ann Arbor

Page 2: Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

Motivation & Background

ηEQE = ηIQE (~100%1) × ηExt ≈ 20%

substrate modes waveguide modes surface plasmon modes

2

1Adachi et al, J. Appl. Phys. 90, 5048–5051 (2001)

2018 SSL R&D workshop

Air mode Substrate mode

Waveguide

SPP

Page 3: Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

Motivation & Background

As ETL increases

SPPs decrease Waveguide modes increase Substrate and air modes

fluctuate

3

0 20 40 60 80 100 120 1400

20

40

60

80

100

Frac

tion

of P

ower

(%)

ETL thickness (nm)

SPP WV

Sub Air

Abs.

2018 SSL R&D workshop

Page 4: Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

Sub-Anode Grid

A multi-wavelength scale dielectric grid between glass and transparent anode (sub-anode grid)

The grid layer is planar and non-intrusive into OLED active region

Waveguided light is scattered into substrate and air modes

4

Qu, Slootsky, Forrest, Nature Photonics (2016)

Cathode

nglass=1.5

nhost norg=1.7, nITO=1.8

ngrid ngrid

2018 SSL R&D workshop

Page 5: Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

Sub-Anode Grid

5

160nm grid/ 70nm ITO/ 2nm MoO3/40nm CBP/15nm CBP:Ir(ppy)3/xnm TPBi/1nm LiF/Al

2018 SSL R&D workshop

Thick-ETL organic structure: 340nm grid/70nm ITO/2nm MoO3/40nm TcTa/15nm CBP: Ir(ppy)3/10nm TPBi/230nm Bphen:Li/Al

Page 6: Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

Sub-Electrode Grid in TE-OLEDs

6 2018 SSL R&D workshop

Substrate Au Ag

SiO2 IZO Organic Capping layer

Metal reflector far away from the EML No excitation of SPPs

Grid >> optical wavelengths

The grid is planar and non-intrusive into the active region

Page 7: Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

control grid

Sub-Electrode Grid in TE-OLEDs

7 2018 SSL R&D workshop

Organic structure: MoO3 30nm/ BPhen: Li 30nm/ Bphen 30nm / CBP : Ir(ppy)3 25nm/ TAPC 40nm /MoO3 30nm/

Glass

Ag Substrate

Organic

IZO 50nm

IZO 50nm

MgF290nm

control grid

grid

control

Page 8: Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

Microlens on Top of TEOLEDs

9 2018 SSL R&D workshop

0 5 10 15 2010-4

10-3

10-2

10-1

100

101

102

J (m

A/c

m2 )

Voltage (V)

450 500 550 600 6500.0

0.2

0.4

0.6

0.8

1.0

MLA control

Inte

nsity

wavelength (nm)

0.1 1 10 1000

10

20

30

40

50

EQ

E(%

)

J (mA/cm2)

Ag

IZO 50nm

Organic

Substrate

SiO2 65nm

IZO 50nm

MLA

Organic structure: HatCN 30nm/ BPhen: Li 30nm/ Bphen 30nm / CBP : (acac)Ir(ppy)2 30nm/ TAPC 40nm / HatCN 30nm/

Page 9: Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

Flexible Corrugated Substrates

10 2018 SSL R&D workshop

Ultra-thin (~μm) Flexible Light extraction from substrate, waveguide and SPP modes

a a

Page 10: Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

Flexible Corrugated Substrates

11

0 5 10 15 2010-7

10-5

10-3

10-1

101

103

glass flat parylene corrugated parylene

J (m

A/c

m2 )

Voltage (V)

0.01 0.1 1 10 1005

10

15

20

25

30

35

glass flat parylene corrugated parylene

EQ

E(%

)

J (mA/cm2)400 450 500 550 600 650 700 750

0.0

0.2

0.4

0.6

0.8

1.0

Inte

nsity

wavelength (nm)

70nm ITO/2nm MoO3/40nm TAPC/25nm CBP: Ir(ppy)2acac/65nm TPBi/LiQ/Al

2018 SSL R&D workshop

Page 11: Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

High RI

Conclusions & Discussions

Four light extraction methods Non-intrusive structures can be better in light extraction Substrates integrated with outcoupling structures are applicable

for both top and bottom emitting OLEDs Wavelength & angle independent outcoupling methodes

12 2018 SSL R&D workshop

Low RI

Scattering layer

Metal/abs. materials

Page 12: Getting All the Light Out: Light Extraction from Organic Light … · 2018. 2. 12. · Getting All the Light Out: Light Extraction from Organic Light Emitting Devices. Yue Qu . 1

Acknowledgements

DoE SSL Program (DE-EE0007626) Universal Display Corporation Lurie Nanofabrication Facility

13 2018 SSL R&D workshop