76
Summer School Recent Developments in Wave Physics of Complex Media Institut d’Etudes Scientifiques de Cargèse 2 – 6 May, 2011 Anderson localization of ultrasonic waves in three-dimensional “mesoglasses” John Page University of Manitoba At Manitoba, we use ultrasound to study mesoscopic wave phenomena in complex media, and to probe the physical properties of mesoscopic materials. - ballistic and diffusive wave transport in random media - field fluctuation spectroscopy (DSS, DAWS…) wave transport & focusing in phononic crystals - wave transport & focusing in phononic crystals - ultrasound in complex materials (e.g., soft matter, foods) www.physics.umanitoba.ca/~jhpage

Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

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Page 1: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Summer SchoolRecent Developments in Wave Physics

of Complex MediaInstitut d’Etudes Scientifiques de

Cargèse

2 – 6 May, 2011

Anderson localization of ultrasonic waves in three-dimensional “mesoglasses”g

John Page University of Manitoba

At Manitoba, we use ultrasound to study mesoscopic wave phenomena in complex media, and to probe the physical properties of mesoscopic materials.

- ballistic and diffusive wave transport in random media- field fluctuation spectroscopy (DSS, DAWS…)

wave transport & focusing in phononic crystals- wave transport & focusing in phononic crystals- ultrasound in complex materials (e.g., soft matter, foods)

www.physics.umanitoba.ca/~jhpage

Page 2: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Mesoscopic wave physics with ultrasound

Wave transport in random media Field fluctuation spectroscopy (e.g., DAWS)

10-3

10-210-5

(b)

m2 )

100

101 <

10-3 10-2 10-1 10010-7

10-6

10-5

10-4

10 3

.002 0.01 0.020.0110-7

10-6 (b)

<r

rel2 (

)> (m

m

(s)

10-4

10-3

10-2

10-1

10

from fits to P() from <2> from g1

~ 2

path 2 > (rad

2)

(s)

Phononic crystals Spectroscopy of complex materials, e.g. foods

Page 3: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Collaborators/Acknowledgements:

• Hefei Hu, Anatoliy Strybulevych, Kurt Hildebrand*, Laura Cobus*, Eric Lee (University of Manitoba, Winnipeg, Canada)Cobus , Eric Lee (University of Manitoba, Winnipeg, Canada)

• Sergey Skipetrov*, Bart van Tiggelen (Université J. Fourier & LPMMC, Grenoble)

• Alexandre Aubry* Arnold Derode (Institut Langevin ESPCI• Alexandre Aubry , Arnold Derode (Institut Langevin, ESPCI, Paris)

Sanli Faez, Ad Langedijk (FOM Institute for Atomic & Molecular Physics, Amsterdam)

* Special thanks for contributions to the slides in this presentation

Page 4: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Outline: Anderson Localization of Ultrasonic WavesSee Physics Today, August 2009

• Introduction to Anderson localizationy y, g

• Localization of elastic waves in 3D

1E-6

1E-5

Experiment Self-consistent Theory Diffusion Theory

nten

sity

I. Why elastic waves?Our samples & their basic

(wave) properties

II. Time-dependent transmission, I(t) 0 100 200 300 400

1E-9

1E-8

1E-7

Nor

mal

ized

In

Time (s)150

200

2 )

(wave) properties

III. Transverse confinement of ultrasonic wavesdue to localization

( )

0 50 100 150 2000

50

100

Exp't Theory = 30 mm = 25 mm = 20 mm = 15 mm

w2 (t)

(m

m2

t (s)

IV. Statistics and Correlations – non-Rayleigh statistics, variance multifractality long-range correlations

t (s)

IV. Coherent Backscattering

variance, multifractality, long-range correlations.

Hu et al., Nature Physics, 4, 945 (Dec, 2008) arXiv:0805.1502• Conclusions

Page 5: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Introduction: Anderson localization of electrons (quantum particles)

2

2 ( ) ( ) ( )V ESchrodinger equation:

( )

E > Ec t d d t t

metal

2 ( ) ( ) ( )2

V Em

r r rV(r) varies randomly in space

P.W. Anderson1958

E = Ec

extended state

(~50 years ago) E < Ec

[# citations > 4200 !]

Page 6: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Introduction: Anderson localization of electrons (quantum particles)

2

2 ( ) ( ) ( )V ESchrodinger equation:

( )

E > Ec t d d t t

metal

2 ( ) ( ) ( )2

V Em

r r rV(r) varies randomly in space

P.W. Anderson1958

E = Ec

extended state

(~50 years ago) E < Ec

"Localization [..], very few believed it at the time, and even fewer saw its importance, among those who failed to fully understand it at first was certainly its author. It has yet to receive adequate mathematical treatment, and one has to resort to the indignity of numerical simulations to settle even the simplest questions resort to the indignity of numerical simulations to settle even the simplest questions about it."P.W. Anderson, Nobel Lecture, 1977

Experiments:Many theoretical breakthroughs: Experiments:Hampered by interactions and finite temperatures

Many theoretical breakthroughs:e.g. Scaling theory (1979) (~30 years ago)

Self consistent theory (1980)

Page 7: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Introduction: Anderson localization of electrons (quantum particles)

2

2 ( ) ( ) ( )V ESchrodinger equation:

( )

E > Ec t d d t t

metal

2 ( ) ( ) ( )2

V Em

r r rV(r) varies randomly in space

P.W. Anderson1958

E = Ec

extended state

(~50 years ago) E < Ec

Localization of classical waves (sound or light)

22 ( ) ( )r r r

e.g., scalar wave equation with disorder:

2 / v 2 > (r)

Sajeev John

where

20

2 2

2

( ) ( )r r r

r 2

v 2 / vo

2 > (r)

Always! j1983

(~25 years ago)

2

0 r2v vdeviations from a uniform medium with velocity v0

Page 8: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Introduction - basic concepts:With sufficient disorder, wave interference can suppress the diffusion coefficient and hence the conductivity. Localized state: confined within a length scale Extended (diffusive) state: extends over the entire sample, Ld

Thouless criterion - distinguishing localized and extended states by their sensitivity to boundary conditions

2 important frequencies (and time scales)• the frequency shift of a mode when boundary conditions are changed from symmetric to antisymmetricchanged from symmetric to antisymmetric.

frequency width is due to time scale T (“Thouless time”) required for change in boundary conditions to be communicated to the wave function ( 1/T ).

• the average frequency separation between neighbouring statesg q y p g gInversely proportional to the density of states [ = 1/( Ld )]H 1/ is called the “Heisenberg time”

Dimensionless Thouless conductance:g > 1 diffusive/extended statesg < 1 localized states

Dimensionless Thouless conductance:

g

Page 9: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Scaling of the Thouless conductance with system size L: What happens if small samples are coupled together to make larger ones?

Extended/diffuse states ( ; states overlap in frequency):

1 1 D 1 dL

2T D L

d LL

2d

g increases with L in 3D

Characteristic diffusion time

2dg L

g increases with L in 3D,g decreases with L in 1D

Localized states ( < ; states well separated in frequency):

1 exp L 1 d

d LL

pT

dL

exp (for )g L L

g always decreases with L

exp (for )g L L

Page 10: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Scaling of the Thouless conductance with system size L: What happens if small samples are coupled together to make larger ones?

Extended/diffuse states:

2dg L g increases with L in 3D,g

Localized states:

g decreases with L in 1D

exp (for )g L L

g always decreases with L

Consequences: • In 3D: g increases with L for diffuse states (large g), but decreases with Lfor localized states (small g)for localized states (small g). transition from diffuse transport to localization at g = gc 1.• In 1D: g always decreases as L increases. No transition all states are localized No transition, all states are localized. • 2D is the “marginal” dimension for localization. Higher order terms indicate that all states are localized in 2D as well (no transition).

Page 11: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Scaling Theory of Localization [Abrahams et al., P.R.L., 42, 637 (1979)]

The scaling of g with L is given by

1

β = d(lng)/d(lnL)e sca g o g t s g e by

2 ln extended statesln ( )

exp ln localized statesd L

g LL

and captured by the scaling function

lnd g-1

p

> 0 extended states

Scaling hypothesis: is a function of g only

lnln

d ggd L

Arrows indicate the direction in which ln g

> 0 extended states < 0 localized states = 0 at gc

Scaling hypothesis: is a function of g only Effect of changing the disorder can be compensated by changing L (g depends on both disorder and L).

varies as L increases

Predictions:• Only in 3D is there a real transition (i.e., a critical point at g = gc) from extended to localized modesextended to localized modes• At gc, g DLd-2 1 is scale independent ( = 0) D 1/L is renormalized• All states in 1D and 2D are localized (if the sample is big enough).

Page 12: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Self-Consistent (SC) Theory [Vollhardt & Wölfle, P.R.L., 45, 842 (1980)]

Wave paths with multiple scattering loops lead to constructive interference, which enhances the probability for the wave to return to the same spot.Consider two wave paths a and b The wave energy isConsider two wave paths a and b. The wave energy is

2 2 2 *2Rea b a b a b

Interference term

Page 13: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Self-Consistent (SC) Theory [Vollhardt & Wölfle, P.R.L., 45, 842 (1980)]

Wave paths with multiple scattering loops lead to constructive interference, which enhances the probability for the wave to return to the same spot.Consider two wave paths a and b The wave energy isConsider two wave paths a and b. The wave energy is

2 2 2 *2Rea b a b a b for different paths, cancels on average (diffusion approximation)

Interference term

Page 14: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Self-Consistent (SC) Theory [Vollhardt & Wölfle, P.R.L., 45, 842 (1980)]

Wave paths with multiple scattering loops lead to constructive interference, which enhances the probability for the wave to return to the same spot.Consider two wave paths a and b The wave energy isConsider two wave paths a and b. The wave energy is

2 2 2 *2Rea b a b a b for different paths, cancels on average (diffusion approximation)

Diffusion slows down and conductivity (transmission) is reduced,

Interference term for loops, doubles the energy locally (time reversed paths)

y ( ) ,becoming scale dependent. SC theory provides physical insight into how localization occurs.

Page 15: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Question: when does the amount of energy returning to the source position become significant?

A simple (approximate) argument can be constructed that this occurs when k 1, where k is the wave vector and is the mean free path.

Ioffe Regel criterion for localization: k 1

Page 16: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Why has it been difficult to observe Anderson localization of electrons experimentally?

For “quantum” particles (electrons), observations are hindered by:

• Need for low temperatures:Lcoh 1/T

(Anderson’s “absence of diffusion” only holds for T = 0)

• Need for small samples:size < L 1 msize < Lcoh 1 m.

• Mutual interactions between electrons

• Electron-phonon interactions

Page 17: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Experiments with classical waves have some advantages.

For “quantum” particles (electrons), observations are hindered by:

• Need for low temperatures:

For light (photons) or sound (phonons),

• Experiments can be done at room• Need for low temperatures:Lcoh 1/T

(Anderson’s “absence of diffusion” only holds for T = 0)

• Experiments can be done at room temperature. Lcoh is independent of T

)

• Need for small samples:size < Lcoh 1 m.

• Samples can be of “human” size:Lcoh is very large.

• No photon photon or phonon• Mutual interactions between electrons

• No photon-photon or phonon-phonon interactions in a linear medium.

• Electron-phonon interactions • Photon-phonon interactions are negligible

(b t it is important to a oid(but it is important to avoid complications due to absorption)

Page 18: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Previous acoustic experiments in 1D:A disordered chain of masses and springs - measure the transverse

Diagonal disorder: vary the positions of the masses

A disordered chain of masses and springs - measure the transverse displacements for different amounts of disorder[He and Maynard, PRL, 57, 3171]:

Diagonal disorder: vary the positions of the masses.

Off-diagonal disorder: vary the sizes of the masses.

Ordered chain

2% site disorder

Localization is easy to observe in 1D!

Page 19: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Previous ultrasonic experiments in 2D:Ultrasound in a disordered plate with random slots [Weaver Wave Motion 12Ultrasound in a disordered plate with random slots [Weaver, Wave Motion, 12, 129-142(1990) ; Lobkis and Weaver, J. Acoust. Soc. Am. 124, 3528 (2008)]:

Measure (with 4 small transducers):Diff (f 660 kH )

b a b a

ab

E E E E ER r t fEE E

1/4

1 2 2 1 distant1/2

adjacent12

, ,

Diffuse (f = 660 kHz)

21

2

Localized (f = 200 kHz)

ba

Page 20: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Previous ultrasonic experiments in 2D:Ultrasound in a disordered plate with random slots [Weaver Wave Motion 12Ultrasound in a disordered plate with random slots [Weaver, Wave Motion, 12, 129-142(1990) ; Lobkis and Weaver, J. Acoust. Soc. Am. 124, 3528 (2008)]:

Measure (with 4 small transducers):

b a b a

ab

E E E E ER r t fEE E

1/4

1 2 2 1 distant1/2

adjacent12

, ,

21

2

Anderson localization near 200 kHz

ba

Localization length ~ 12 cm

Page 21: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Previous experiments with light in 3D:Exponential scaling of the average transmission (for monochromatic waves)Exponential scaling of the average transmission (for monochromatic waves)with thickness L. [Wiersma et al., Nature 390, 671 (1997)]

Diffuse regime: Localized regime

*TL

exp LT

• Difficult to distinguish from effects of absorption ( exp[-L/ℓa])

Page 22: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Previous experiments with microwaves in quasi-1D:Enhanced fluctuations of total transmissionEnhanced fluctuations of total transmission. [Chabanov et al., Nature 404, 850 (2000)]

2 2

Diffuse regime: Localized regime

2

2 1T

T

2

2 const 1T

T

• Chabanov et al. proposed that this criterion for localization is independent of absorption, but their experiments were limited to quasi-1-dimensional samples.

Page 23: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

More recent experiments with light in 3D:Time-dependent transmission through thick samples of TiO particlesTime-dependent transmission through thick samples of TiO2 particles [Störzer et al., PRL 96, 063904 (2006)]

Non-exponential tail at long times: interpreted as a slowing down p gof diffusion with propagation time due to localization.

Current status (~50 years after Anderson’s discovery): • The subject is more alive than ever! j

• Activity in optics, microwaves, acoustics, seismic waves, and atomic matter waves.

Page 24: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Question: Can we convincing observe the localization of ultrasound due to disorder in 3D, and, if so, can we learn something new? N.B.: Scaling theory Only in 3D is there a real transition from extended to localized modes (i.e., a mobility edge) ; unambiguous evidence has been elusive.

Weak disorder (kℓ >> 1): Diffuse propagation DB = ⅓ vE ℓB* (neglect

Strong disorder (kℓ 1): Anderson localization (interference is important!)DB ⅓ vE ℓB (neglect

interference) (interference is important!)

Energy density spreads Energy remains

e.g., After a short pulse of ultrasound is incident on the medium…Localization length

gy y pdiffusively

from the source

Energy remains localized

in the vicinity of the source

Page 25: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Our samples: “Mesoglasses” fabricated by brazing aluminum beads together to form a

lid 3D l ti t ksolid porous 3D elastic network. good control of elastic coupling between beads low intrinsic absorption.

Aluminum volume fraction: = 0.55Monodisperse beads:

radius a = 2 05 mmradius, abead = 2.05 mmSample width >> thickness (L: 8 to 23 mm)

Pulsed ultrasonic transmission measurements (waterproofed samples, in a water tank)

Frequency range: 0.1 to 3 MHz ( ) 6 1a

planartransducer:(far field)

hydrophone

(xi,yi)

incident soundwaves: quasi-planar sample

Page 26: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Coherent transport in disordered Al mesostructures:

Ballistic transport: Average the transmitted field toBallistic transport: Average the transmitted field to recover the weak coherent pulse and measure :

• phase velocity: p kv

• group velocity:• scattering mean free path, ℓ :

Very strong scattering in the

intermediate exp 0 /LI I

d dg kv

Amplitude transmission coefficient: Bandgaps arise from weakly coupled resonances of the aluminum beads (Turner & Weaver, 1998)

frequency regime (0.2 – 3 MHz) :

1 kℓ 2 5of the aluminum beads (Turner & Weaver, 1998) 1 kℓ 2.5(outside the bandgaps)

0.1

mis

sion

t

1E 3

0.01

ude

trans

mco

effic

ient

0.0 0.5 1.0 1.5 2.0 2.5 3.0

1E-3

Am

plitu

Frequency (MHz)

Page 27: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

II. Time-dependent transmission, I(t).• Measure multiply scattered field in many

planartransducer

incident sound(quasi planar)

hydrophone

p y yindependent speckles by scanning the hydrophone.

• Digitally filter the field to limit bandwidth

(quasi-planar)sample

0.2 SPECKLE 1• Digitally filter the field to limit bandwidth (~5% usually)

• Determine I(t) by averaging the squared t itt d l l (N li

0.0

0.1

0.2 SPECKLE 1 SPECKLE 12 SPECKLE 25

Wav

e Fi

eld

(a.u

.)

transmitted pulse envelopes. (Normalize by the peak of the input pulse)

• First compare with the diffusion model, 0 100 200 300 400

-0.2

-0.1W

Time (s)

using realistic boundary conditions (e.g. see Page et al., Phys. Rev. E 52, 3106 (1995) for ultrasonic waves)[z - extrapolation length; z - penetration 1E-3

0.01

nsity

[z0 - extrapolation length; z - penetration depth; a - absorption time]

• For elastic media, the diffusion coefficient D = ⅓ v ℓ* is the energy 1E-6

1E-5

1E-4or

mal

ized

Inte

n

coefficient DB = ⅓ vE ℓ is the energy-density weighted average of longitudinal and transverse waves.

0 100 200 300 4001E-7

1E 6No

Time (s)

Page 28: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Time-dependent transmission at low frequencies:(below the lowest band gap)

Good fit to the predictions of the diffusion approximation for a plane wave source measure D. (Absorption is too small to measure.)

f = 0.2 MHz:

I(t) decays 0.01Experimenty exponentially at

long times

1E 4

1E-3

p Theory

d In

tens

ity

2 2

( ) expwith

Dt tI

1E-5

1E-4

D = 3.0 mm2/sorm

aliz

ed

Normal diffusive

2 202D BL z D

1E-6l* = 2.5 mmR = 0.85L = 14.5 mma ~ infinite (no absorption)

No

Normal diffusive behaviour0 100 200 300 400

1E-7

Time (s)

Page 29: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

I(t) at higher frequencies (e.g. 2.4 MHz)

Find non-exponential decay of I(t) at long times (t >> D ) Looks

Find non exponential decay of I(t) at long times (t D ) Looks like a diffusion process with D(t) decreasing with propagation time.

1E-6

1E-5 Experiment Diffusion Theory

sity

1E-7

zed

Inte

ns

1E-8

Nor

mal

iz

0 100 200 300 400

1E-9

Ti ( )Time (s)

Suggests that sound may be localized

Page 30: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Quantitative analysis of I(t) at high frequencies (2.4 MHz)– fit the (plane wave) data directly with the recently improved self-

i t t th f l li ticonsistent theory of localization [Skipetrov & van Tiggelen (2006)]

Basic idea:The presence of loops increases the return probability as compared to ‘normal’ diffusion

Diffusion slows down

Diffusion constant should be renormalized

Generalization to Open Media:

Loops are less probable near the boundaries

Slowing down of diffusion is spatially heterogeneous

Diffusion constant becomes position-dependent

Page 31: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Quantitative analysis of I(t) at high frequencies (2.4 MHz)– fit the (plane wave) data directly with the recently improved self-

i t t th f l li ti

Mathematical formulation:

consistent theory of localization [Skipetrov & van Tiggelen (2006)]

Diffusion equation

i D r G r r r r

Self consistent equation for the diffusion coefficient

( G(r,r,) – Intensity Green’s function)

, , ,i D r G r r r r

Self-consistent equation for the diffusion coefficient

1 1 3 ( , , )

( , ) ( )B BG r r r

D r D D

Diffusion coefficientBoundary conditions

( () – density of states )

Diffusion coefficient depends on position r

and frequency 0

( , )( , , ) ( , , ) 0B

D rG r r z G r rD

n

Page 32: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Quantitative analysis of I(t) at high frequencies (2.4 MHz)– fit the (plane wave) data directly with predictions of the self

i t t th f l li ti f D( )consistent theory of localization for D(r,) [Skipetrov & van Tiggelen (2006)]

Input parameters: Experiment Self-consistent Theory

Diff i Th

L = 14.5 mm (sample thickness)ℓ = 0.6 mm (scattering mean free

path)R = 0.82 (internal reflection coeff.)

1E-6

1E-5 Diffusion Theory

sity

ℓB* = 2.0 mmL/ = 1.0 = 11 s z0 = ℓB* ⅔ (1+R)/(1-R) = 6.7 ℓB*

vp = 5.0 km/s (phase velocity)kℓ = 1.82

Fitted parameters:1E-7

1E-6

zed

Inte

ns D = 11 s a = 160 s

Fitted parameters:ℓB* (“bare” transport mean free path)L/ ( is the localization length)D or DB (bare diffusion coefficient) (absorption time)

1E-8

Nor

mal

iz

a (absorption time)

0 100 200 300 400

1E-9

Time (s)

Excellent fit at all propagation times.

Page 33: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Quantitative analysis of I(t) at high frequencies (2.4 MHz)– fit the (plane wave) data directly with predictions of the self

i t t th f l li ti f D( )

Experiment Self-consistent Theory

Diff i Th

Localization length :

consistent theory of localization for D(r,) [Skipetrov & van Tiggelen (2006)]

1E-6

1E-5 Diffusion Theory

sity

2

2 46

* ( *) 1B B ckℓB* = 2.0 mmL/ = 1.0 = 11 s

1E-7

1E-6

zed

Inte

ns

Localization regime:

where ( )ck kD = 11 s a = 160 s

1E-8

Nor

mal

iz Localization regime: > 0 , kℓ < (kℓ)c

Diffuse regime:

0 100 200 300 400

1E-9

Time (s)

g < 0 , kℓ > (kℓ)c

Excellent fit at all propagation times with > 0 (L > > L/4) Strong (but indirect) evidence for the localization of sound

Page 34: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Self consistent theory of localization predicts a strong and rapid renormalization of D in our samples:

1 1 ( , , )( , )

where 3 ( ) ,B

B

G r r rD r D

D

DB cannot be

( )( ) D.O.S.

B

=100D-1

measured directly, even for t < D.(D(,z)/DB <<1 for all

=D-1

accessible t).

Best fits have: surprising large DBp g g B(and hence large vE )

Question: Can this be explained by a

=0.1D-1

explained by a reduced density of states (D.O.S.)?

Page 35: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Density of states – direct measurements!

• Unusual behaviour

7 bead sample• Unusual behaviourbelow the first bandgap (~ constant).

F f 0 6 MH

1000

7 bead sample 11 bead sample weakly sintered samples strongly sintered samples

Debye Weyl constant

• For f > 0.6 MHz, average DOS is consistent with standard predictions: 100

sity

of S

tate

sm

-3 M

Hz-1

)

standard predictions:

Debye:D

ens

(cm

D f f 2( ) 12

Weyl (includes surface modes)

0.1 110

Frequency (MHz)

D f fV v

3( ) 12

modes)

sphere sphere L T L T

L L T

V S v v v vD f n f f

v v v v

2 42

3 22

12 2 3 / 3 /2 / 1

Conclude: Large values found for vE cannot be explained by anomalously low DOS (due to short range correlations or bandgap effects)

Page 36: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

III. Transverse confinement (“transverse localization in 3D”)

Experiment (displaced point source technique):Experiment (displaced point source technique):

• Point source (focusing transducer + small aperture)

focusing transducer

hydrophone

sample cross-section

• Point detector, placed a transverse distance away

• Scan x y position of the

hydrophone(on-axis configuration)

• Scan x-y position of the sample to determine I(,t). (off-axis

configuration)cone-shaped aperture

The ratio I( t)/I(0 t) probes the transverse growth (dynamic spreading)The ratio I(,t)/I(0,t) probes the transverse growth (dynamic spreading) of the intensity profile. • Diffuse regime – measure the effective width of the “diffuse halo”, which

f fprovides a method of measuring D independent of boundary conditions and absorption. [Page et al., Phys. Rev. E 52, 3106 (1995)]

2 2 2( , ) exp 4 exp ( )t Dt w tI so the effective width w(t) is exp 4 exp ( )

(0, )Dt w t

tIso the effective width w(t) is

22( ) 4

ln ( , ) (0, )w t Dt

t tI I

Page 37: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Diffuse regime –the effective width of the “diffuse halo” grows linearly in time

Data (from 1995) on a suspension of glass beads in water (kℓ 7)Data (from 1995) on a suspension of glass beads in water (kℓ 7)[Page et al., Phys. Rev. E 52, 3106 (1995)]

2 2 2( , ) exp 4 exp ( )

(0, )t Dt w tt

II

210-4

0

22( ) 4

ln ( , ) (0, )w t Dt

t tI I

120 = 10.2 mm10-7

10-6

10-5 = 0 mm = 10.2 mm = 15.2 mm

ize

Inte

nsity

80

100

= 15.2 mm 4Dt,

D = 0.45 mm2/s

10-9

10-8

10

Nor

mal

i

40

60

w 2 (

mm

2 )

0.2

0.4 = 10.2 mm = 15.2 mm

axis /

I on-a

xis

0 10 20 30 40 50 600

20

10 20 30 40 50 600.0

0.2

I off-a

Measure DB independent of boundary conditions and absorption.

0 10 20 30 40 50 60

t (s)Time (s)

Page 38: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Question: What happens to I(,t) & w(t) in the localization regime? 1E-6 = 0 mm

= 10 mm

1

1E-8

1E-7

= 10 mm = 15 mm = 20 mm = 25 mm = 30 mm

zed

inte

nsity

0.01

0.1

/ I(0

,t)

1E-10

1E-9

Nor

mal

i

1E-4

1E-3 = 10 mm = 15 mm = 20 mm = 25 mm = 30 mm

I(,t)

0 20 40 60 80 100 120 140 160 180 2001E-11

Time (s)0 20 40 60 80 100 120 140 160 180 200

1E-5

Time (s)

200Diffuse regime prediction,

Dynamic transverse width at 2.4 MHz: Localization dramatically

150m

m2 )

4Dt (= 1.25t)

yinhibits the expansion of the intensity profile in the transverse direction. 50

100

= 30 mm = 25 mm = 20 mm

w2 (t)

(m

2 2( , ) exp ( )

(0, )t w tt

II 0 50 100 150 200

0

= 15 mm

t (s)

Page 39: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Quantitative analysis of the dynamic transverse width, w(t):- Fit the data using the new self consistent theory that allows for the

iti d d f th li d diff i ffi i t i 3Dposition dependence of the renormalized diffusion coefficient in 3D. • Excellent fit for all four with:

ℓB* = 2.0 mmBL/ = 1.0 D = 17 s

(a cancels in ratio) 150

200

• Fit is more sensitive to than plane wave I(t)

• Again find > 0 classical100

150

) (m

m2 )

• Again, find > 0 classical wave localization is convincingly demonstrated in this 3D “phononic” mesoglass

50Exp't Theory

= 30 mm = 25 mm = 20 mm

w2 (t)

this 3D phononic mesoglass.

• First direct measurement and theory for the transverse t t f l li d i

0 50 100 150 2000

= 20 mm = 15 mm

t (s) structure of localized waves in 3D. Find w 12-14 mm for this sample

t (s)

Page 40: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

3D Transverse Localization: this animation (prepared by Sergey Skipetrov) shows the “freezing” of the transverse profile at long times ( t ti f I( t)/I( 0) f t > t 100 i thi )(saturation of I(,t)/I(,0) occurs for t > tloc 100 s in this case.)

Theory Experiment Experiment

Page 41: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Decrease of I(,t) with transverse distance is not Gaussian Near the mobility edge (kℓ /(kℓ )c = 0.99 for this sample at this f ) i h t ith t di l tfrequency), w varies somewhat with transverse displacement .The self-consistent theory (solid curves) captures the experimentally observed dependence of w(t) on very well. p ( ) y

1

0 01

0.1

I(0,t)

1E-3

0.01 Expt Theory

t = 10 s t = 25 s t = 50 s

I(,t)

/

1E-4

t 50 s t = 98 s t = 150 s t = 195 s exp[-( /L) 2]

0.0 0.5 1.0 1.5 2.0

/ L

Page 42: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Question: What determines the magnitude of the dynamic transverse width w(t) in transmission?

• For thick samples, w becomes independent of .

• Behaviour at long times: SC theory predictions for the saturated width when L >> : 2when L >> :

[Cherroret, Skipetrov and van Tiggelen, aiXiv:0810.0767v1] 2( ) 2 1 /w t L L

1.0

0.8 L / = 1Exp't Theory

= 30 mm = 25 mm = 20 mm

2( )2 1

wL L

0.4

0.6

L / = 3.6Exp't Theory

= 25 mm

= 15 mm

w 2 /

L 2

0.40

for 3.6L

0.2

= 20 mm = 15 mm

0 50 100 150 2000.0

Time (s)For localized waves, w depends on both L and

Page 43: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

The saturation of w(t) at long times is predicted even at the mobility edge [Cherroret, Skipetrov and van Tiggelen, arXiv:0810.0767v1].

Numerical calculations using the dynamic self-consistent theory:

At the mobility edge: (t ) L

In the diffuse regime: w2(t) = 4D [1 (kl )-2 ]t w(t) Lw2(t) = 4D [1-(kl ) 2 ]t

( L = 100 l )

D i thDeep in the localization regime:

2( )w t

( )2 1 /L L

Page 44: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Similar trends are seen in the experiments (for t /D < 20)• Compare three representative samples with different amounts of disorder

1 0

p p p(same measuring frequency f = 2.4 MHz).

L = 14.5 mm, = 15 mm; L = 23.05 mm, = 12 mm; L = 23.5 mm, = 6.5 mm;

0.8

1.0 L / = 1Exp't Theory

ave = 23 mm

0.6

L / = 2Exp't Theory

ave = 23 mm

2 / L 2

2( ) for / 2

wL

0.4

L / = 3.6

w

2( ) for

/ 3 6wL

0 0

0.2 Exp't Theory ave = 23 mm

/ 3.6L

0 2 4 6 8 10 12 14 16 18 200.0

t / D

Page 45: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

What happens when we vary the frequency?

0.8

1.0

t 1/2

= 25 mm

0.6

t

/ L 2

0.4 0.7 MHz 1.0 MHz1 8 MHz

w 2

0 50 100 150 200 250 300 3500.0

0.2 1.8 MHz 2.4 MHz

0 50 100 150 200 250 300 350

Time (s)

At 0.7 and 1.0 MHz, w 2(t) does not saturate above the mobility edge. (at 0.7 MHz, the time dependence is almost linear)

Should be feasible to measure as the mobility edge is approached

Page 46: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

What happens when we vary the frequency?Plot on log scales to show the time dependence g p

0.70.80.9

1

t 1/2 = 25 mm

0.4

0.50.6

L 2

0.2

0.3

1.0 MHz 1.8 MHz2 0 MHz

w 2 /

L

0.1 t 2/3

2.0 MHz 2.2 MHz 2.4 MHz 2.6 MHz

Near the mobility edge we see

10 100 500

Time (s)

Agrees ith estimatesNear the mobility edge, we seew 2(t) t 2/3 for t < D &w 2(t) t 1/2 for a limited range of t > D

Agrees with estimates of w2(t) using the self-consistent theory.

Page 47: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Summary: Transverse confinement (3D transverse localization)• The dynamic transverse width w 2(t) has completely different properties for

ffdiffuse and localized modes

Diffuse: w 2(t) t and increases without bound.

Localized: w 2(t) saturates at long timesLocalized: w 2(t) saturates at long times. At the mobility edge: w(t) L Deep in the localization regime: 2( ) 2 1 /w t L L

• w 2(t) is independent of absorption its measurement (for any kind of wave) provides a valuable method for assessing whether or not the waves are localized. (No risk of confusing absorption with localization.)

• w 2(t) can be used to measure the localization length .

• Measurements of transverse confinement provide the mostdirect evidence for localizationin 3D to date.

Page 48: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

IV Backscattering experiments – initial results:[with Laura Cobus, Alexandre Aubry and Arnaud Derode – see Laura’s poster for more]

128 l

Average time-dependent backscattered intensity:

128-element transducer array

f = 3.2 MHz

Coherent backscattering cone: due to

= 0.5 mm

Coherent backscattering cone: - due to constructive interference in the backscattering direction of waves travelling along reciprocal paths Simulate far field conditions using planepaths. Simulate far field conditions using plane wave beamforming.

Transverse Confinement of the incoherent i t it G i b f i itintensity: Gaussian beamforming permits measurements of transverse confinement in reflection. Reciprocal paths

Page 49: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Transverse confinement in reflection:• Use Gaussian beamforming [Aubry & Derode, PRE 2007] t f th itt d d i dPRE 2007] to focus the emitted and received waves at the sample surface – measure I(, t) in reflection

•Incoherent background fitted by a Gaussian to measure the transverse width, w.

100

120

140 2

w2 ~ t • Width saturates at long

60

80

100

w2 ~ t1/2

w 2 (m

m2 ) times localization.

• Expect w2(t ) 2 in reflection for thick samples

20

40

w p(c.f., dashed green line – the measured value from transmission measurements t 2 4 MH )

0 20 40 60 80 100 120 1400

Time (s)

at 2.4 MHz)

Page 50: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Coherent backscattering cone:• Simulate far-field conditions using l b f i

0.8

1.0

sity

45us 70us 125 us

plane wave beamforming[Aubry & Derode, JASA (2007)].

• Difficult to separate cone from 0.4

0.6

aliz

ed In

tens

background at early times – preliminary analysis by fitting two Gaussians.

-4 -2 0 2 40.0

0.2

Nor

ma

(degrees)

2.5

3.0

~ t • For diffuse waves the half -width is:

2

1.5

2.0

degr

ees)

-2

~ t1/2 • For localized waves, expect the idth t h i k l idl

tDk)2ln(

22

0.5

1.0

(d cone width to shrink less rapidly, and eventually saturate.

•For t > 50 s, behaviour is

0 20 40 60 80 100 120 1400.0

Time (s)

consistent with the observed transverse confinement of the incoherent intensity.

Page 51: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

The inter-element response matrix Kij exhibits strong coherences along the anti-diagonals:

Matrix K (t = 35 s, f = 2.7 MHz)Matrix K (t 35 s, f 2.7 MHz)

• Coherence along the antidiagonals of K has been demonstrated for single scattering [Aubry and Derode, J. App. Phys. (2009), P.R.L. (2009)]• Here, the coherence along the antidiagonals of K cannot be due to single scattering, since vt/2 > L >> s .

It b l i d b th f t th (th fi t d• It may be explained by the occurrence of recurrent paths (the first and last scattering events along a multiple scattering path are identical) which exhibit the same statistical properties as single scattering

Page 52: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Separation of recurrent paths from the total backscattered signal Alexandre’s idea:

Page 53: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Separation of recurrent paths from the total backscattered signal Spatial intensity profiles:

• Single + recurrent (IS, blue) contribution is broadblue) contribution is broad, and decreases with time. • Classical multiple scattering (IM, red) shows a CB peak on top of a flat plateau, with an enhancement factor of 2.

By identifying and separating the single and recurrent contributions, it should be possible to measure the time-dependent width of the backscattering cone more robustly.

Page 54: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

V. Statistical approach to the localization of elastic waves:

Diffuse ultrasound

0

3.000

3.600

4.200

4.800

5.400

6.000use u t asou d

(speckle pattern for our mesoglass at 0.20 MHz)

1020

30

40

50

010

2030

4050

x (mm)y (mm)0

0.6000

1.200

1.800

2.400

Localized ultrasound (speckle pattern for our mesoglass at 2 4 MH )50

Large fluctuations in the transmitted intensity

mesoglass at 2.4 MHz)

20.00

22.50

25.00

Large fluctuations in the transmitted intensity are characteristic of localized waves.

Signatures of these fluctuations are seen in:

25

30

20

25

yyy

5.000

7.500

10.00

12.50

15.00

17.50are seen in: • Near field speckle pattern• Intensity distribution P(I /I)

15

20

25

10

15

20

y (mm) x (mm)

0

2.500

• Variance• Multifractality

Page 55: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Transmitted intensity distributions for our mesoglass:Measure the intensity I at each point in the near field speckle pattern when the

(a) Data at 0.20 MHz

y p p psample is illuminated on the opposite side with a broad beam. When I is normalized by its average value to get Î = I / I , its distribution is universal.

100(a) Data at 0.20 MHz

Rayleigh distribution: (random wave fields described b i l G i t ti ti ) 2

10-1

100 Experiment, f = 0.20 MHz NvR theory, g' = 11.4 Rayleigh distribution

by circular Gaussian statistics)

ˆ ˆexpP I I10-3

10-2

P( I )

Leading order correction to Rayleigh statistics due to interference (no absorption) [Nieuwenhuizen & van Rossum

10-5

10-4

[Nieuwenhuizen & van Rossum, PRL 74, 2674 (1995)](g = dimensionless conductance):

0 5 10 1510-6

I

Î

21ˆ ˆ ˆ ˆexp 1 4 23

Pg

I I I I Find g = 11.4 >> 1 modes are extended

Page 56: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

(b) Near 2 4 MHz (upper part of intermediate frequency regime) find very

Transmitted intensity distributions for our mesoglass:(b) Near 2.4 MHz (upper part of intermediate frequency regime), find very large departures from Rayleigh Statistics

Fit the entire distribution to predictions by van Rossum and Nieuewenhuizen [R M d Ph 71 313][Rev. Mod. Phys. 71, 313]for a slab geometry in 3D (red curve). Remarkable agreement 10-1

100 Experiment, f = 2.4 MHz NvR theory, g' = 0.80stretched exponential g' = 0 80Remarkable agreement

with experiment.

The tail of intensity di t ib ti b

10-2

10 stretched exponential, g 0.80 Rayleigh distribution

distribution obeys a stretched exponential distribution

ˆ ˆ10-4

10-3

(g is the effective dimensionless conductance.)

ˆ ˆ~ exp 2P gI I

10-6

10-5

Find g = 0.80 < 1, indicating localization.

0 10 20 30 40 5010

Page 57: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Variance of the transmitted intensity – a simpler way to measure the dimensionless conductance g:

Chabanov et al. [Nature 404, 850 (2000)] have proposed that localization is achieved when the variance of the normalized total transmitted intensity ,

satisfies 2

2 2TT̂ T T=

whether absorption is present or not. This corresponds to the localization

22 2ˆvar( )

3 3

TT

gT

condition g 1.

But var( ) and var(Î) are related: ˆˆvar( ) 2var( ) 1TIT̂

Then, the Chabanov-Genack localization criterion gives ˆvar( ) 7 3I

e g for our data at 2 4 MHz:e.g., for our data at 2.4 MHz:

Measure var(Î) = 2.74 0.09

E ll t t ith 0 80 0 08 d f P(Î)

4 0.77 0.4ˆ3 var( ) 1

gI

Excellent agreement with g = 0.80 0.08 measured from P(Î)

Additional evidence that the modes are localized above 2 MHz.

Page 58: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Time dependence of the speckle intensity variance:Point source Broad (quasi-plane-wave) source

25

30o t sou ce oad (quas p a e a e) sou ce

1E-4

1E-3

0.01

t) (a

.u.)25

30

15

20

aria

nce

-5 0 5 10 15 20

1E-7

1E-6

1E-5

speckle 10 speckle 53 speckle 701 speckle 704 speckle 708 average intensity

Inte

nsity

I(t

15

20

aria

nce

5

10 average steady state variance = 3.0

V5 0 5 10 15 20

Time (s)

5

10

V

average steady state variance = 5.66

0 50 100 150 2000

Time (ms)0 50 100 150 200

0

Time (s)

Large peak in variance at early times due to arrival time fluctuations• Large peak in variance at early times – due to arrival time fluctuations.• Variance increases slowly with time at longer times (slower growth than in quasi 1D – microwave observations by Azi Genack’s group).

B th i d it th ith ti l f i t• Both variance and its growth with time are larger for a point source.• Time-dependent variance is less than the stationary variance for the range of times measured.

Page 59: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Time dependence of the speckle intensity variance:Data are consistent with theoretical estimates by Sergey Skipetrov, based

(quasi-mode frequencies n , lifetimes n – for P(), see Skipetrov & van Tiggelen PRL (2006)

ata a e co s ste t t t eo et ca est ates by Se gey S pet o , basedon a mode picture of wave propagation:

n ni t tn nt A e

12, ( )r r Skipetrov & van Tiggelen, PRL (2006) n n

Assuming uncorrelated modes, an estimate of the variance gives

t t f t t LI 2 21( ) var ( ) 1 1 2

E i t l d t

stationaryt t f t t LN

I ( ) var ( ) 1 1 , 2

te 2

Bt D 2where and

Experimental data

8

10

t)

average steady state variance = 5.66

t

ef t t L

e

a b t t t

2,

0

2

4

6

Var

ianc

e,

2(

a b t t t

c d t t t

, 0

,

0 50 100 150 2000

Time (s)

Predictions (valid at long times, t >>D) for typical experimental parameters reproduce the main features in the data

Page 60: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Multifractality (MF) of the wavefunction (with Sanli Faez, Ad Lagendijk):[Faez et al., PRL 103, 155703 (2009) ]

Key idea Unusual spatial structure of the wave functions near the AndersonKey idea - Unusual spatial structure of the wave functions near the Anderson transition: Large fluctuations the moments of the wave function intensity

I(r) = 2(r)/ 2(r)ddr

may depend anomalously on length scale , exhibiting multifractal behaviour(MF each moment scales with a different power- law exponent).

• Many theoretical predictions, but almost no experimental evidenceMany theoretical predictions, but almost no experimental evidenceQuestion: Do the ultrasonic wavefunctions exhibit MF in our samples?

Transmitted speckle patterns I(r) for a fixed point source (at x = y = 0).E it i l f ti t h f

2.425 MHz2.375 MHz

Excite a single wave function at each frequency.

2.35 MHz

5

10

15

5

10

15

5

10

15

-15-10

-50

510

15-15

-10

-5

0

5

y (m

m)

x (mm)

-15-10

-50

510

15-15

-10

-5

0

5

y (m

m)

x (mm)

-15-10

-50

510

15-15

-10

-5

0

5

y (m

m)

x (mm)

Page 61: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

15

Multifractality (MF):Characterizing the length scale dependence: 15

L

0

5

10

mm

)

C a acte g t e e gt sca e depe de ce Vary system size L, or Divide system into boxes of size b,

and vary b with L fixed. 0

5

10

mm

)

b

-15

-10

-5

y (m( < b < L, L/b is the scaling length)

Generalized Inverse Participation Ratios (gIPR): -15

-10

-5

y (m

-15 -10 -5 0 5 10 15

15

x (mm)

Generalized Inverse Participation Ratios (gIPR): The gIPR quantify the non-trivial length scale dependence of the moments of the intensity.

-15 -10 -5 0 5 10 15

15

x (mm)

q

1 1

i

i

qn nq d

q Bi i B

P I I dr r I(r) = 2(r)/ 2(r)ddr (normalized intensity)IBi is the integrated probability inside a box Bi

of linear size bn = (L/b)d is the number of boxes.

( )qP L b ( ) 1q d q with

At criticality

qP L b

MF behaviour: is a continuous function of q (critical states).

( ) 1 qq d q with

normal dimension anomalous dimension

Page 62: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Multifractality (MF):Generalized Inverse Participation Ratios (gIPR): 15

L = Lg

Ge e a ed e se a t c pat o at os (g )Find the “typically averaged” gIPR by box-sampling the wavefunctions (many frequencies) near the surface (d sampling = 2, but sample is 3D) for a single realization 0

5

10

mm

)

b

p gof disorder.

-15

-10

-5

y (m

2( 1) ( )qq qq g gtyp

P L b L b

Representative results at f = 2.40 MHz: -15 -10 -5 0 5 10 15

15

x (mm)

10

Extended states:

468

q = -2 q = -1 q = 0q = 1g

Pq

Extended states:(q) = d(q-1) [i.e., q = 0]

Near criticality:

-202

q q = 2 q = 3lo

g (q), q, both continuous functions of q (MF)

Deep in the localization-1.4 -1.2 -1.0 -0.8 -0.6 -0.4

log (b/Lg)

Deep in the localization regime: (q) = 0

Page 63: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Multifractality (MF):Generalized Inverse Participation Ratios (gIPR): 15

L = Lg

Ge e a ed e se a t c pat o at os (g )Find the “typically averaged” gIPR by box-sampling the wavefunctions (many frequencies) near the surface (dsampling space = 2, but sample is 3D) for a single 0

5

10

mm

)

b

p g prealization of disorder.

-15

-10

-5

y (m

2( 1) ( )qq qq g gtyp

P L b L b

Representative results at f = 2.40 MHz: -15 -10 -5 0 5 10 15

15

x (mm)

10

468

q = -2 q = -1 q = 0q = 1g

Pq

• Determine (q) from the slopes

-202

q q = 2 q = 3lo

g from the slopes

• Subtract off the normal part of (q),

-1.4 -1.2 -1.0 -0.8 -0.6 -0.4 log (b/Lg)

d(q-1), to determine q

Page 64: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Multifractality (MF): the anomalous exponents (from the gIPR)Anomalous exponents qAnomalous exponents q

0.0 Localized ultrasound

-0.5

1-q

Diffuse light

-1.5

-1.0

q, The variation of q with

q gives unambiguous evidence of MF for the

-2 -1 0 1 2 3-2.0

q

localized ultrasonic wave functions

Exact symmetry relation, predicted by Mirlin et al. (PRL 97, 046803, 2006)

=

q

q = 1 – q

Consistent with our data

Page 65: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Multifractality (MF): PDFProbability density function (PDF)Probability density function (PDF)The gIPR are proportional to the moments of the distribution function of the intensities, P (IB), implying

II

( ) ln1( ) , where

ln( / )

d fB

BB

ILb L b

P

f() is called the singularity spectrum [the fractal dimension of the set of points r where I (L/b) ]p ( ) ]

Significance: f() is expected to be independent of (L/b), and give a universal characterization of the MF behaviour.

Relationship with (q):

( ) ( ) fq q f qq

i.e., f() and (q) are related by a Legendre transform

q

Page 66: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

The singularity spectrum f() – relationship with (q)

Start from: P (IB) = probability that box i has IBi between IB and IB + dIBStart from: P (IB) probability that box i has IBi between IB and IB dIB

N(IB) = (Lg/b)dP (IB) = number of boxes with IBi between IB and IB + dIB

Then, the gIPR can be written 300

350

q = 0*, 1B qI

in terms of the PDF as

1

0( ) q

q B B BP I I dIN 200

250

300

B) I

Bq

q q = 0.5 q = 1

*,sharp max at

0

* *( )

B q

q

B

I

BI IN 50

100

150

N(I

B)

( )d fL

0 2 4 6 8 10

0

IBIf both IB* and N(IB*) scale as powers of (Lg/b)

Significance of the exponents and f( ):

( )

( )BLb

IP

Then

( ) ( )* *( )q f q

B g B gI L b I L b, N

Significance of the exponents and f():f() is the fractal dimension of the set of points r where I (L/b)

( ) ( )q q fThen

Page 67: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

The singularity spectrum f() – relationship with (q)

At the peak of N(IB) IBqp N( B) B

*

ln ( ) ln ( )0

ln ln

qB B B

B B

I I Iq

I I

N N(1)

But from

** BBB B II

*

( )* lnwe get

ln

qB

B gg

II L b

L b,

and from ( )* *( ) , we get ln ( ) ( )ln

f q

B g B gI L b I f q L bN N

g

ln ( )

ln lnln ln ln

Bg g

B B B

I f f fL b L b

I I I

N

f

(2)

(1) and (2)

Hence by differentiating with respect to q we also find ( ) ( )q q f

fq

Hence, by differentiating with respect to q, we also find ( ) ( )q q f

q

Page 68: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Multifractality (MF) The parabolic approx and the PDFParabolic approximation:Parabolic approximation:

(1 )q q q 0 5

0.0

q = q (1 - q )with = 0.21( = constant)

The Legendre transformation then yields

-1.5

-1.0

-0.5

q

2( )-3 -2 -1 0 1 2 3 4

-2.0

q

20

0( )( ) ;

4f d d

The PDF in the parabolic approximation: ( )1 d fL

2 2

1( )

1 exp (ln ln ) / 2

BB

Lb

w

II

I I

P

A single parameter log-normal distribution! (w2 and lnIB,c are related)

,exp (ln ln ) / 2B B cB

w I II

Page 69: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Multifractality (MF) PDFThe probability density function

2 2,(ln ) exp (ln ln ) / 2B B B c w I I IP

The probability density function[Histogram of box-integrated intensities, IB , b 2]

Red:Red: diffuse ultrasound(200-300 kHz)

G i-1

0

10.15

posi

tion

Gaussian(centred at 0)

0 2 4 6 8 10 12 14-4

-3

-2

0.10

ln I B) Pe

ak p

b/Blue:Localized Ultrasound(2.35-2.45 MHz)

0.05P (l b/

Log normal (peak shifted to negative ln{ IB / IB })-5 -4 -3 -2 -1 0 1 2

0.00

l I / Ig { B B })ln IB/<IB>

Page 70: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Multifractality (MF)The singularity spectrum, f()The singularity spectrum, f()Measure f() directly, using the method of Chhabra & Jensen [PRL 62, 1327 (1989)], rather than via the Legendre transform.

Red:Red: Diffuse Light• very narrow (almost a 1.5

2.0

delta function) • no shift in the peak from peak = dsampling space = 2

1.0

1 98

2.00f()

Blue:Localized Ultrasound

0.0

0.5

1.94

1.96

1.98

Localized Ultrasound(2.0-2.6 MHz, 700 speckles)• Broad spectrum, indicating MF

0.5 1.0 1.5 2.0 2.5 3.0 3.5-0.5

2.0 2.2 2.41.92

indicating MF• Max is shifted by peak 2 = 0.21 0.02

Question: Is (= 0.21) 1/g ?

Page 71: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Multifractality (MF)Dependence on frequencyp q yThis can be illustrated by the reduced anomalous exponent for q = 2 ( 2)

• MF behaviour is seen 0.1

ssion

throughout the entire frequency range (0.5 – 2.9 MHz)

0 0 1E‐3

0.01

Tran

smis

( )

• 2 is nearly independent of frequency above 1 5 MHz-0.3

-0.2-0.10.0

above 1.5 MHz

• 2 decreases with frequency as the

0 7-0.6-0.5-0.4

2,av

e

bandgaps are approached from below. several “mobility -1.0

-0.9-0.8-0.7

yedges!” 0.5 1.0 1.5 2.0 2.5

Frequency (MHz)

Page 72: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Long range correlations – see Kurt Hildebrand’s poster for more

Spatial and frequency intensity correlations show long-range contributions

10  Scanned point source

Spatial and frequency intensity correlations show long range contributions. Compare near field spatial correlations using a point source and detector:

• When the source position is d th t itt d10 Single point source

 

= 50 m

m)

scanned, the transmitted intensities at all detector positions fluctuate together, due to LDOS fluctuations at

1

2

C S(f, r 

due to LDOS fluctuations at the source positions. Measure essentially infinite-range C0 correlations.

‐0.4

‐0.2• The C0 correlations increase, while the MF exponent 2 decreases,

‐0.8

‐0.6

2

 2 MHz transducer 1 MHz transducer

near the bandgaps• Consistent with recent suggestions that both LDOS

d MF t0.6 0.7 0.8 0.9 1.0 1.1 1.2 1.3 1.4

Frequency (MHz)

average of 1 and 2 MHz results  and MF exponents can

reveal critical behaviour. [Murphy et al, arXiv:1011.0659v1]

Page 73: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

• Large fluctuations in the transmitted intensity for

Statistics - SummaryLarge fluctuations in the transmitted intensity for

localized modes:non-Rayleigh statisticslarge variance var(Î)

g < 115 0

5

10

15

2.35 MHz

large variance, var(Î)

• First experimental observations of wavefunctionltif t lit th A d t iti

-15-10

-50

510

15-15

-10

-5

0

y (m

m)

x (mm)

multifractality near the Anderson transition:scaling of the gIPR, probability density function

( )qqP L b

5

10

15

2.375 MHz

(PDF is log normal)singularity spectrum, f() (peak > d)

-15-10

-50

510

15-15

-10

-5

0

5

y (m

m)

x (mm)

Some questions for future work:

10

15

2.425 MHzSome questions for future work:• Why is the peak in the singularity spectrum is shifted above the sampling dimension by only 0.21 at 2.4 MHz?

What are the effects on MF of open bo ndaries-15

-10-5

05

1015

-15

-10

-5

0

5

10

y (m

m)

x (mm)

• What are the effects on MF of open boundaries, absorption, mixed polarizations?• Can determine critical exponents from MF behaviour?

Page 74: Anderson localization of ultrasonic waves in three ... - 2011 - Ander… · Introduction: Anderson localization of electrons (quantum particles) 2 2 VE() () Schrodinger equation:

Conclusions

We have used ultrasonic experiments and predictions of the self-We have used ultrasonic experiments and predictions of the selfconsistent theory of dynamics of localization to demonstrate/explore the localization of elastic waves in a 3D disordered mesoglass.

Ti d d t t itt d i t it I(t) Time dependent transmitted intensity I(t) non-exponential decay of I(t) at long times.

Transverse confinement in transmission first direct measurements and theory for I(,t), showing how localization cuts off the transverse spreading of the multiple scattering halo.

w 2(t) is independent of absorption and depends on the localization length (and L)

Transverse confinement and coherent backscattering Statistics and correlations: non-Rayleigh

15

20

25

30

10

15

20

25

y (mm) x (mm)

yyy

Statistics and correlations: non-Rayleigh statistics and large variance of the transmitted intensity Î (g = 0.8 < 1 at 2.4 MHz); wavefunctionmultifractality; long range (near-field) correlations

Transverse confinement is a powerful new approach for guiding investigations of 3D Anderson localization for any type of wave.

15multifractality; long range (near-field) correlations.

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