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Diana Adlienė Department of Physics Kaunas University of Technology 4. Particle Generators/Accelerators Joint innovative training and teaching/ learning program in enhancing development and transfer knowledge of application of ionizing radiation in materials processing

4. Particle Generators/Accelerators

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Diana Adlienė

Department of Physics

Kaunas University of Technology

4. Particle

Generators/Accelerators

Joint innovative training and teaching/

learning program in enhancing development

and transfer knowledge of application of

ionizing radiation in materials processing

This project has been funded with support from the European

Commission. This publication reflects the views only of the author.

Polish National Agency and the Commission cannot be held

responsible for any use which may be made of the information

contained therein.

Date: Oct. 2017

Joint innovative training and teaching/ learning program in enhancing development and transfer

knowledge of application of ionizing radiation in materials processing

This presentation contains some information

addapted from open access education and

training materials provided by IAEA

DISCLAIMER

1. Introduction

2. X-ray machines

3. Particle generators/accelerators

4. Types of industrial irradiators

TABLE OF CONTENTS

The best accelerator in the universe…

INTRODUCTION

• Naturally occurring radioactive sources:– Up to 5 MeV Alpha’s (helium nuclei)

– Up to 3 MeV Beta particles (electrons)

• Natural sources are difficult to maintain,

their applications are limited:– Chemical processing: purity, messy, and expensive;

– Low intensity;

– Poor geometry;

– Uncontrolled energies, usually very broad

Artificial sources (beams) are requested!

INTRODUCTION

• Beams of accelerated particles can be used to

produce beams of secondary particles:

� Photons (x-rays, gamma-rays, visible light) are

generated from beams of electrons;

� Neutrons are generated from beams of protons

(spallation neutron sources).

• Primary and secondary beams are used for radiation

processing of materials and/or for analyzis of material

(probe) properties.

RADIATION GENERATORS

Radiation generators are devices that produce energetic beams

of particles which are used for:

– Understanding the fundamental building blocks of nature and the

forces that act upon them (nuclear and particle physics);

– Understanding the structure and dynamics of materials and their

properties (physics, chemistry, biology, medicine);

– Medical treatment of tumors and cancers;

– Production of medical isotopes;

– Sterilization;

– Ion Implantation to modify the surfaces of materials

– National Security: cargo inspection, …

There is active, ongoing work to utilize particle accelerators for

– Transmutation of nuclear waste

– Generating power more safely in sub-critical nuclear reactors

RADIATION GENERATORS/ACCELERATORS

X-ray set

Linear

accelerator

Cyclotron

Neutron

generator

X-RAY MACHINES

• Coolidge in 1913 designed a “hot cathode” x ray tube and his

design is still in use today.

–The main characteristics of the Coolidge tube are its high

vacuum and its use of heated filament (cathode).

–The heated filament emits electrons through thermionic

emission.

–X rays are produced in the target (anode) through radiation

losses of electrons producing characteristic and bremsstrahlung

photons.

–The maximum photon energy

produced in the target equals

the kinetic energy of electrons

striking the target.

X-RAY BEAMS AND X-RAY UNITS

• X-ray beams are produced in energy range between 10

keV and 50 MeV when electrons with kinetic energies

between strike special metallic targets.

• In the target most of the electron’s kinetic energy is

transformed into heat, and a small fraction of the

kinetic energy is emitted in the form of x ray photons

which are divided into two categories:

– Characteristic X rays following electron - orbital

electron interactions

– Bremsstrahlung photons following electron -

nucleus interactions

X-RAY BEAMS AND X-RAY UNITS

• Characteristic X rays result from Coulomb interactions

between the incident electron and atomic orbital electrons of

the target material (collision loss).

• The orbital electron is ejected from its shell and an electron

from a higher level shell fills the resulting orbital vacancy.

• The energy difference between the two shells is:

– Either emitted from the target atom in the form of a

photon referred to as characteristic photon.

– Or transferred to another orbital electron that is ejected

from the target atom as an Auger electron.

X-RAY BEAMS AND X-RAY UNITSCHARACTERISTIC X RAYS

• Characteristic photon and Auger electron eKLM energies;

following a vacancy in the atomic K shell.

Energy of K photon:

Energy of eKLMAuger electron:

α

α

X-RAY BEAMS AND X-RAY UNITSBREMSSTRAHLUNG (CONTINUOUS) X RAYS

• Bremsstrahlung X rays result from Coulomb interactions

between the incident electron and the nuclei of the target

material.

• During the interaction the incident electron is accelerated and

loses part of its kinetic energy in the form of bremsstrahlung

photons.

• The interaction is also referred to as radiation loss producing

braking radiation.

X-RAY BEAMS AND X-RAY UNITSBREMSSTRAHLUNG (CONTINUOUS) X RAYS

• In bremsstrahlung interaction X rays with energies ranging

from zero to the kinetic energy of the incident electron may

be produced, resulting in a continuous photon spectrum.

• The bremsstrahlung spectrum produced in a given X ray

target depends upon:

– Kinetic energy of the incident electron

– Atomic number of the target

– Thickness of the target

• The range R of a charged particle in a particular absorbing

medium is an experimental concept providing the thickness

of the absorber that the particle can just penetrate.

• With regard to the range R of electrons with kinetic energy

EK in the target material of atomic number Z two types of

targets are known:

– Thin targets with thickness much smaller than R.

– Thick targets with thickness of the order of R.

X-RAY BEAMS AND X-RAY UNITSX-RAY TARGETS

• For thin target radiation and electron kinetic energy EK:

– Intensity of emitted radiation is proportional to the

number of photons N times their energy EK.

– Intensity of radiation emitted into each photon

energy interval between 0 and EK is constant.

– The total energy emitted in the form of radiation

from a thin target is proportional to (Z*EK).

X-RAY BEAMS AND X-RAY UNITSX-RAY TARGETS

• Thick target radiation may be considered as a superposition

of a large number of thin target radiations.

• The intensity of thick target radiation spectrum is

expressed as:

• In practice thickness of thick x-ray targets is about 1.1 R to

satisfy two opposing conditions:

– To ensure that no electrons that strike the target can

traverse the target.

– To minimize the attenuation of the bremsstrahlung beam

in the target.

X-RAY BEAMS AND X-RAY UNITSX-RAY TARGETS

X-RAY BEAMS AND X-RAY UNITSCLINICAL X-RAY BEAMS

• A typical spectrum of a clinical x-ray beam consists of:

– Continuous bremsstrahlung spectrum

– Line spectra characteristic of the target material and

superimposed onto the continuous bremsstrahlung

spectrum.

The bremsstrahlung spectrum

originates in the x-ray target.

The characteristic line spectra

originate in the target and in

any attenuators placed into

the x-ray beam.

TYPES OF PARTICLE ACCELERATORS

A wide variety of particle accelerators is in use today.

• The types of machines producing particles are distinguished

by the velocity of particles that are accelerated and by the

mass of particle accelerated.

• Accelerators for electrons differ from accelerators for

protons or heavy ions.

GENERATORS/ACCELERATORS

Example:

A typical method for generating electrons utilizes a thermionic

gun at a potential of about 100 kV. This gives a beam of 100

keV electrons.

Comparison of the velocities of different particles generated at

100 keV kinetic energy shows:

– Electrons: v/c = 0.55

– Protons: v/c= 0.015

– Au1+: v/c= 0.001

This has important implications for the type of acceleration scheme

PROTON AND ELECTRON VELOCITIES vs

KINETIC ENERGY

THE DEVELOPMENT OF ACCELERATORS

• Accelerators have gone through a long development process,

including

– Electrostatic accelerators

– The Van der Graaf accelerator

– The Cyclotron

– The Synchrotron

DIRECT ACCELERATORS:

TRANSFORMER TYPE

Direct accelerators are machines in which accelerated particle moves in a constant electric field gaining the energy (eV) which is equal to the potential difference (V) applied.

This applies for acceleration of electrons, protons and ions

Earliest particle accelerators/generators also called potential

drop generators were the Cockcroft- Walton generator and

the Van der Graaf generator

• Highest voltage achieved is 24 MV

• It is difficult to establish and maintain a static DC

field of 20+ MV

DIRECT ACCELERATORS:

TRANSFORMER TYPE

VAN DER GRAAF GENERATORS

• Van der Graaf generators

(electrostatic generators) are

direct accelerators.

• Generated energy is from the

range 0.5- 5.0 MeV

• Proton current 50 µA, in

pulses - 5 µA.

• Electrostatic generators are

energy stable, accelerated

particles are monoenergetic.

VAN DER GRAAF GENERATORS

VAN DER GRAAF GENERATOR

It was a hit !

Many labs could easily

obtain a Van der Graff.

- Low currents �

- High precision ☺

COCKCROFT-WALTON GENERATOR

COCKCROFT & WALTON GENERATOR

• The 1st stage of Fermilab’s huge accelerator is

a Cockcroft-Walton

Machine

• 750 keV

(Upper limit)

PARTICLE ACCELERATORS

• R. Widerøe (1929) proposed an accelerator by using an

alternating voltage across many alternating “gaps.”

• It was not without a myriad of problems

• - Focusing of beam

• - Vacuum leaks

• - Oscillating high voltages

• - Again, imagination

• His professor refused any further work because it was “sure to

fail.”

• - Widerøe still published his idea in Archiv fur Electrotechnic

ACCELERATION BY REPEATED

APPLICATION OF TIME-VARYING FIELDS

Ising and Widerøe suggested the repeated application of a much smaller

voltage in a linear accelerator by using time-varying fields

In this way, a high particle beam energy could be attained by repeatedly

applying voltage “kicks”

Ising‘s idea Widerøe or Sloan-Lawrence or

interdigital structure

SCHEMATIC OF WIDERØE’S LINAC

ACCELERATION TECHNIQUES: DC FIELD

• The simplest acceleration method: DC voltage

• Can accelerate particles over many gaps: electrostatic accelerator

• Problem: breakdown voltage at ~10MV

DC field still used at start of injector chain

ACCELERATION TECHNIQUES: RF FIELD

• Oscillating RF (radio-frequency) field

• Firstly introduced by Rolf Widerøe

(The principle is known as “Widerøe accelerator” untill now.)

• Particle must see the field only when the field is in the

accelerating direction

• Requires the synchronism condition to hold: Tparticle =½TRF

• Problem: high power loss due to radiation.

vTL )2/1(=

The particles gain energy by surfing on the electric fields

of well-timed radio oscillations

ACCELERATION TECHNIQUES: RF FIELD

ACCELERATION TECHNIQUES: RF CAVITIES

• Electromagnetic power is stored in a resonantvolume instead of being radiated;

• RF power feed into cavity, originating fromRF power generators, like Klystrons

• RF power oscillating (from magnetic toelectric energy), at the desired frequency

• RF cavities requires bunched beams (asopposite to coasting beams)

– particles located in bunches separated inspace

RADIOFREQUENCY POWER GENERATION SYSTEM

• The radiofrequency power

generation system produces

the microwave radiation used

in the accelerating waveguide

to accelerate electrons to the

desired kinetic energy and

consists of two major

components:

– RF power source

(magnetron or klystron)

– Pulsed modulator

FROM PILL-BOX TO REAL CAVITIES

LHC cavity module ILC cavity

(from A.

Chao)

ACCELERATION BY REPEATED APPLICATION OF TIME

VARYING ACCELERATING FIELDS

Two approaches for accelerating with time-varying fields:

an electric field along the direction of particle motion with Radio-

Frequency (RF) Cavities

Circular Accelerators

Use one or a small number of

Radiofrequency accelerating cavities

and make use of repeated passage

through them.

This approach leads to circular

accelerators: Cyclotrons, synchrotrons,

and their variants

Linear Accelerators

Use many accelerating cavities

through which the particle

passes only once

These are linear accelerators.

FROM LINEAR TO CIRCULAR ACCELERATORS?

• Technological limit on the electrical field in an RF cavity

(breakdown);

• Gives a limited ∆E per distance.

• ⇒ Circular accelerators, in order to re-use the same RF cavity

• This requires a bending field FB in order to follow a circular

trajectory

CIRCULAR ACCELERATORS

• Circular accelerators: deflecting forces are needed

• Circular accelerators: piecewise circular orbits with a defined bending

radius ρ

– Straight sections are needed for e.g. particle detectors

– In circular arc sections the magnetic field must provide

the desired bending radius:

• For a constant particle energy we need a constant B field ⇒ dipole magnets

with homogenous field.

SYNCHROTRON

In synchrotrons acceleration isperformed by RF cavities; particlesare accelerated along a closed,circular orbit and the magnetic fieldwhich bends the particles increaseswith time so that a constant orbit ismaintained during acceleration.

The bending field changes with particle beam energy to maintain a

constant radius, so B ramps in proportion to the momentum. The

revolution frequency also changes with momentum.

SYNCHROTRON

The synchrotron concept was first proposed in 1943 by the Australian

physicist Mark Oliphant.

• For an electron synchrotron, the injected beam is already

relativistic, so only the magnetic field changes with beam

energy.

• For a proton synchrotron, the injected beam is not yet

relativistic, so the RF accelerating frequency and the

magnetic field both ramp with energy• RF frequency must stay locked to the revolution

frequency of a particle

• Synchrotrons are used for most HEP experiments (LHC, Tevatron, HERA, LEP, SPS, PS)

STRONG-FOCUSING SYNCHROTRONS

There were two nearly identical very large proton

synchrotrons constructed at the same time 1959-1960:

At the European CERN laboratory

in Geneva (28 GeV)

At the Brookhaven National laboratory on

Long Island (33 GeV).

Both of them are still in operation.

SYNCHROTRON RADIATION

• Charged particles undergoing acceleration emit

electromagnetic radiation

• Main limitation for circular electron machines

– RF power consumption becomes too high

• The main limitation factor for LEP...

– ...the main reason for building LHC !

• However, synchrotron radiations is also useful

COLLIDERS

A collider can be thought of as a fixed-energy synchrotron.

Beams of matter and antimatter particles counter-rotate,

sharing the same beam pipe and are made to collide.

First electron-positron collider, ADA, at

Frascati which was built by Bruno

Touschek in 1960 (eventually reached 3

GeV)

The large hadron collider at

CERN (13 TeV)

LARGE HADRON COLLIDER

The evidence of Higgs boson

was experimentally aproved on

4.07.2012

Protons collide at 14 TeV in this

simulation from CMS,

producing four muons. Lines

denote other particles, and

energy deposited is shown in

blue15.07.2015 The LHCb experiment at

CERN’s Large Hadron Collider has

reported the discovery of a class of

particles known as pentaquarks

CYCLOTRON PRINCIPLE

Lawrence’s Application of Wideroe’s Idea: The Cyclotron

Uniform circular motion is

maintained via centripetal

acceleration:

The radius is:

Ernest Lawrence recognized that

the revolution period and

frequency are independent of

particle velocity:

Therefore, a particle in resonance

with a time varying field applied

to the Dees with frequency given

as above will be accelerated. The

particle is in synchronism with

the time-varying field.

• Such cylcotrons can accelerate

proton energies up to 20-30MeV

CYCLOTRON

• In a cyclotron the particles are accelerated along a spiral

trajectory guided inside two evacuated half-cylindrical

electrodes (dees) by a uniform magnetic field produced

between the pole pieces of a large magnet (1 T).

THE CYCLOTRON PRINCIPLE

� A vertical B-field provides the force to maintain the electron’s circular orbit

� The particles pass repeatedly from cavity to cavity, gaining energy.

� As the energy of the particles increases, the radius of the orbit increases until the particle is ejected

CYCLOTRON

– constant B field

– constant RF field in the gap increases energy

– radius increases proportionally to energy

– limit: relativistic energy, RF phase out of synch

– In some respects simpler than the synchrotron, and often used

as medical accelerators

THE FIRST MILLION VOLT CYCLOTRON

“... we were concerned about how many of the protons would succeed

in spiralling around a great many times without getting lost on the

way."

08/01/32

Lawrence and Livingston at Berkeley

PARTICLE ACCELERATORSBETATRON

• Betatron is a cyclic accelerator in which the electrons are made

to circulate in a toroidal vacuum chamber (doughnut) that is

placed into a gap between two magnet poles.

• Conceptually, the betatron may be considered an analog of a

transformer:

Primary current is the alternating current exciting the magnet.

Secondary current is the electron current circulating in the doughnut.

PARTICLE ACCELERATORSMICROTRON

• Microtron is an electron accelerator that combines the

features of a linac and a cyclotron.

• The electron gains energy from a resonant wave guide cavity

and describes circular orbits of increasing radius in a uniform

magnetic field.

• After each passage through the

wave guide the electrons gain an

energy increment resulting in a

larger radius for the next pass

through the wave guide cavity.

OTHER ACCELERATOR TYPES

Linear accelerators for linear colliders

-

LINEAR ACCELERATORS

Whereas a circular accelerator can make use of one or a small number of RF

accelerating cavities, a linear accelerator utilizes many (hundreds to thousands)

individual accelerating cells.

Again, accelerators for protons or ions “look” quite different from those that

accelerate electrons, because electron beams are already relativistic at low

energy.

Modern proton linear accelerators are based on the Alvarez Drift-Tube Linac.

Alvarez was awarded the 1968 Nobel Prize in Physics for his contributions to

elementary particle physics.

The two largest proton linear accelerators are the LANSCE linac at Los Alamos

(800 MeV) and the Spallation Neutron Source Linac at ORNL (1000 MeV).

LINEAR ACCELERATORS FOR

ELECTRONS

Most electron linacs utilize a structure

known as the Disk-Loaded Waveguide.

Geometry looks somewhat different from

that used for protons since electrons quickly

become relativistic

ACCELERATING CAVITIES

Modern machines use a time-dependent electric field in

a cavity to accelerate the particles

LINACS

Medical linacs are cyclic accelerators that accelerate electrons to

kinetic energies from 4 to 25 MeV using microwave

radiofrequency fields:

– 103 MHz : L band

– 2856 MHz: S band

– 104 MHz: X band

In a linac the electrons are accelerated following straight

trajectories in special evacuated structures called accelerating

waveguides.

LINACS

Schematic diagram of a modern fifth generation linac

LINACSINJECTION SYSTEM

Two types of electron gun producing electrons in linac:

LINACSACCELERATING WAVEGUIDE

Two types of accelerating waveguide are in use:

– Traveling wave structure

– Standing wave structure

ELECTRON

ACCELERATORS/IRRADIATORS

Direct

(transformer)

accelerator

Single cavity

accelerator

Linear

(microwave)

accelerator

DIRECT ACCELERATORS: TRANSFORMER TYPE

Capability for DC power supply (for transformer

accelerators)

Addopted from the lecture of dr. Z.Zimek (ICTJ)

• Single cavity accelerators

TYPES OF INDUSTRIAL IRRADIATORS

• Gamma-irradiators

�Sources:

mainly Co-60 and Cs-137

�Categorization:

from I to IV, specific design based on safety requirements

• Electron-beam irradiators

– Electron energy < 10 MeV

– also use of bremstrahlung

GAMMA IRRADIATORS: CO-60 SOURCE

• Activities ranging from 1 TBq to 100 PBq.

• Relatively long half-life of 5.26 years (source changing

frequency is minimised).

• Co in its solid form is insoluble and non-friable and has a high

melting point (1492 oC) - reduced risk of the spread of

radioactive contamination

beta minus decay with

emission of 2 high energy

gamma photons (1.17 MeV

and 1.33 MeV) beta

particles are absorbed in the

source capsule

GAMMA IRRADIATORS: CS-137 SOURCE

• Half life – 30.7 years.

• Caesium-137 has become less popular in recent years because

its solubility makes it more difficult to contain for long periods.

• It also emits lower energy which means that much larger

amounts of radioactive material are required to produce an

output equivalent to that from cobalt-60.

beta minus decay with

emission of gamma

photons (0.66 MeV, 0.036

MeV and 0.032 MeV)

beta particles are

absorbed in the source

capsule

TYPES OF GAMMA IRRADIATORS

• Category I

– self contained, dry storage irradiator

• Category II

– panoramic, dry storage irradiator

• Category III

– self contained, wet storage irradiator

• Category IV

– panoramic, wet storage irradiator

CATEGORY I

SELF-CONTAINED IRRADIATORS

• Sealed source (Co-60 or Cs-137) is mounted round a tube and

completely enclosed in a dry container constructed of solid

materials and is shielded (lead-steel containement )

• Activity – several Ci (1 Ci = 37 000 000 000 Bq)

• Applications:

• Preservation

(food, seeds, etc.)

• Radiation Effects

(biological research)

• Chemical synthesis

(chemical research)

Sources in here

(do not move)

Sample goes in here

Sample

lowered

CATEGORY I

SELF-CONTAINED IRRADIATORS

CATEGORY II

PANORAMIC SELF-CONTAINED IRRADIATORS

• A controlled human access irradiator in which the sealed

source (Co-60 or Cs-137) is enclosed in a dry container

constructed of solid materials, is fully shielded when not in use

and is exposed within a radiation volume that is maintained

inaccessible during use by an entry control system (maze,

concrete wals)

• Activity – several dozens of Ci

• Application:

• Sterilization (medical supplies)

• Preservation (food)

CATEGORY II

PANORAMIC SELF-CONTAINED IRRADIATORS

Open

Beam Port

CATEGORY III

SELF-CONTAINED WET STORAGE IRRADIATORS

• Sealed Co-60 source is

contained in a water filled

storage pool and is

shielded.

• Human access to the

sealed source and the

volume undergoing

irradiation is physically

restricted in the design

configuration.

• Activity – from several

hundreds to thousands of

CiSterilization (small medical supplies)

CATEGORY IV

SELF-CONTAINED WET STORAGE IRRADIATORS

A controlled human access

irradiator in which the

sealed Co-60 source is

contained in a water filled

storage pool, is fully

shielded when not in use

and is exposed within a

radiation volume that is

maintained inaccessible

during use by an entry

control systemSource rack

Activity – from dozens of thousands of Ci

CATEGORY IV

SELF-CONTAINED WET STORAGE IRRADIATORS

Co-60 source construction

Co-60 source pencil

Pencils

Rack

Source

Storage

CATEGORY IV

SELF-CONTAINED WET STORAGE IRRADIATORS

CATEGORY IV

SELF-CONTAINED WET STORAGE IRRADIATORS

• Water pool for storage

• Concrete walls and maze

during operation

Sterilization of big

packs with

medical suppliers,

pharmacy or

cosmetic products

ELECTRON BEAM IRRADIATORS (EBI)

• Beam energy up to 10 MeV

• Advantage – no induced

radioactivity

• Bremstrahlung from

electron beam interactions

with exposing items is

sometimes used but should

be protected

• Possibility of neutron

production should be taken

into account

Schematic view of electron generator

ELECTRON BEAM IRRADIATORS (EBI)

• Categorization

• Category I

– integrally shielded irradiator unit with interlocks

• Category II

– Irradiator unit housed in shielded room maintained

inaccessible during irradiation

• Applications• Preservation (food, caught fish, etc.)

• Sterilization

• Chemical synthesis (polymerization)

EBI: CATEGORY I

• An integrally shielded unit

with interlocks, where

human access during

operation is not physically

possible owing to the

configuration of the

shielding

• Concrete walls against

electrons and neutrons

• Some lead from

bremstrahlung,

• Aluminium for shielding

against electron beam

EBI: CATEGORY II

A unit housed in shielded rooms that are maintained inaccessible

during operation by an entry control system

– Concrete walls

– Maze for item supply

X-RAY MASCHINE

Forward Peaked Emission of

5.0 MeV X-rays

COMPARISON: BEAM PENETRATION

• The attractive features of X-ray processing for industrial applications,

Greater depth of penetration, allowing for treatment of products with large

volumes.

• Controllable dose rates, which can facilitate monomer polymerization.

• Not a thermal process which eliminates adverse effects on materials due to

the heat

COMPARISON: IONIZING RADIATION

SOURCES

X-RAY PROCESSING THROUGH-PUT

POTENTIAL

ENERGY EVOLUTION

Exponential growth of

energy with time

• Increase of the energy by an

order of magnitude every 6-10

years

• Each generation replaces

previous one to get even higher

energies.

• The process continues…

• Energy is not the only

interesting parameter.– Intensity

– Size of the beam

DEVELOPMENT IN RADIATION

PROCESSING

Continuous increase and development of irradiation facilities:

∼ 250 high activity 60Co gamma and ∼ 1000 EB machines (0.1 –

10 MeV).

Prospect for X-ray application.

NEW DEVELOPMENT IN RADIATION

PROCESSING EQUIPMENT

ADVANCED EB EMITER MODULE

LOW ENERGY EB ACCELERATOR

Diana Adlienė

Department of Physics

Kaunas University of Technology

4. Particle

Generators/Accelerators

Joint innovative training and teaching/

learning program in enhancing development

and transfer knowledge of application of

ionizing radiation in materials processing