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Welcome to the
CHARMS See – TeaFriday, April 21, 2023
Release of Light Alkalis (Li, Na, K) From ISOLDE Targets
Strahinja Lukić, 18.10.2005
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Outline
Release of nuclides from ISOLDE targets
Release measurement technique
Results
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Release of Nuclides from ISOLDE Targets
Nuclide production
Thermal diffusion
Effusion
Ionization
Extraction by 60 kV field
Losses to chemical reactions, leaks, radioactive decay...
Proton beam
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Typical ISOLDE Target
20 cm
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Ion-Sources Surface
Hot transfer line made of a metal with high work function (W, Ta)
Plasma Electron beam ionizing a gas
mixture (Ar+Xe)
Hot or cold transfer line
Laser excitation and ionization using
characteristic wavelengths in 2-3 steps
Chemical selectivity
Surface Ion-Source
EXTRACTION ELECTRODE
http://isolde.web.cern.ch/ISOLDE/
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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ISOLDE Facility LayoutTransmission Losses
http://isolde.web.cern.ch/ISOLDE/
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Release Measurement Using the Tape Station
Proton beam pulses are spaced by 14 - 20 s
Ion beam implanted on a tape at a certain time after the p+ bunch Timing and duration controlled by a
deflector magnet
Tape carries the ions to the detector (1s)
Detection of β, α, γ or n during a specified time
Detector
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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The Release Curve
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Yield and In-Target Rates
The release curve is established for a long lived isotope and applied to the shorter lived isotopes of the same element
The decay losses can be deduced and in-target production rates calculated
But, losses to leaks and chemical reactions impossible to estimate → yields are not always reproducible
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Cross-sections
Production cross-sections can be estimated assuming that: All the nuclides are produced in primary reactions
(approximately correct for Li, Na and K)
Production cross-sections are constant along the target despite the proton energy loss (approximately correct for 1 GeV protons ? Energy loss ~50 MeV, xs variation ~20-30% ?)
mol
atottg
M
Nd
tot
i eCP
110242.6]/1[ 12
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Some Results
Order of magnitude good except data from specific targets
Shape of the distribution approximately good (steeper than in ABRABLA results)
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Some Results
Very few data, incompletely documented
Order of magnitude good
Shape of the distribution approximately good
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Other Results - K
Too few data for potassium in the segment that was treated
Order of magnitude good except in the same specific targets as for sodium
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Other Results - Li
Very difficult element for ISOL Small atom - leaks through solid materials
Fast diffusion – faster than the measurement system?
No sufficiently long-lived isotope – difficult to establish the release curve.
Extrapolate the release curve parameters from K and Na?
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Other Results - Li
Estimated release curves extremely long (not logical for Li) → apparently high decay losses → high xs
Using parameters extrapolated from sodium doesn't seem to work
Possible errors because of the time-dependent background (He)
8Li produced in U-Carbide
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Other Results - Li
No experimental data to compare to.
18-10-2005 Release of the Light Alkalis From ISOLDE Targets
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Conclusions
The method seems to work although it would be difficult to use it for independent cross-section measurements.
The main problem - unpredictable losses
Yield data are scarce, at least in the period that was treated (1993 – 2002)
Systematic measurement of the time-dependent background could help, particularly for lithium