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oak Rldgc Nauonal Laboratory OAK RIDGE NATIONAL LABORATORY UNION CARBIDE CORPORATION for the U.S. ATOMIC ENERGY COMMISSION operated by . 4 c i ORNL- TM- 2343 707630 PREXJMINARY ESTIMATIDN OF EROSION AND RADIOCESIUM REDISPRIBUTION IN A FESCUE MEADOW Roger C. Dahlman and S. I. Auerbach BOX No. FULDER t; f 024544 Publicly Releasable This document has received the necessary patent and technical information reviews and can be distributed without limitation. NOTICE This document contains information of a preliminary nature and wos proparod primarily for internal use at the Oak Rid- National Laboratory. It is subiect to revision or carnction and th&. does not represent a final report. 4-00036 Human Subjects Project

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Page 1: UNION CARBIDE CORPORATION U.S. · or contractor of tho Commission, or employoo of such contractor proparms, disseminates, or provides accoss to, ony information pursuant to his employmnt

oak Rldgc Nauonal Laboratory OAK RIDGE NATIONAL LABORATORY

UNION CARBIDE CORPORATION for the

U.S. ATOMIC ENERGY COMMISSION

operated by .

4

c

i ORNL- TM- 2343 7 0 7 6 3 0

PREXJMINARY ESTIMATIDN OF EROSION AND RADIOCESIUM REDISPRIBUTION

I N A FESCUE MEADOW

R o g e r C. Dahlman and S. I. A u e r b a c h

BOX No.

FULDER

t;

f 024544

Publicly Releasable

This document has received the necessary patent and technical information reviews and can be distributed without limitation.

NOTICE Th is document contains information of a preliminary nature and wos proparod primarily for internal use a t the Oak Rid- National Laboratory. It is subiect to revision or carnction and th&. does not represent a final report.

4-00036 Human Subjects P r o j e c t

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. -

I LEGAL This report was proparad as an account of Gavernmnt sponsarod work.

nor the Commission, nor any porson acting on behalf of tho Commission:

A. Makes any warranty or rapresontation, oxprossod or implied, wi th respoct to tho accurocy.

complotomss, or usofulnoss of the information contained i n th is report, or that tho uso of

any information, apparatus, nmthad, 01 process disclosed i n th is report may not infringe

privatmly o v m d rights; or A s s u m s any l iabi l i t ios wi th r o s p c t to tho use of, or for damages resulting from the US* of

any information. apparatus, mthod, or pacmss disclasod in th is ropwt.

Neither tho United States,

6.

As u w d i n tho abovo, "person acting an bohalf of tho Commission" includes any emplop. or

contractor of the Commission, or mmployoo of such contractor, to tk extent that such emplop.

or contractor of tho Commission, or employoo of such contractor proparms, disseminates, or

provides accoss to, ony information pursuant to h is employmnt 01 contract wi th tho Commission,

or h is employmnt w i th such contractor. L -l

c -,

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ORNL-TM-2 343

C o n t r a c t No. W-7405-eng-26

HEALTH PHYSICS D I V I S I O N

RADIATION EC0IX)GY SECTION

PREUMINARY ESTIMATION OF EROSION AND RADIOCESJXM REDISTRIBUTION

I N A FESCUE MEADOW

R o g e r C. D a h l r n a n and S. I. A u e r b a c h

NOVEMBER 1968

OAK RIDGE NATIONAL LABORATORY

Oak R i d g e , Tennessee

operated by

UNION CARBIDE CORPORATION

for the

U. S. ATOMIC ENERGY COMMISSION

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iii

comms Page

A b s t r a c t . . . . . . . . . . . . . . . . . . . . . . , . . . . . . 1

In t roduc t ion . . . . . . . . . . . . . . . . . . . . . . . . . . . 2

Measurement of Runoff . . . . . . . . . . . . . . . . . . . . . . 3

Es t imated Radiocesium i n Runoff . . . . . . . . . . , . . . . . . 5

Comparison wi th Other Resul t s . . . . . . . . . . . . . . . . . . 7

References . . . . . . . . . . . . . . . . . . . . . . . . . . . . 15

..

1 0 2 4 5 9 1

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PREUMINARY ESTIMATION OF EROSION AND RADIOCESIUM RFDISTRIBUTION

I N A FESCUE MEADOW*

Roger C . Dahlman and S. I. Auerbach

ABSTRACT

The p o t e n t i a l r a d i o a c t i v i t y r e d i s t r i b u t i o n was evaluated f o r

observed and hypo the t i ca l condi t ions of p r e c i p i t a t i o n p r i o r t o

a p p l i c a t i o n of a f a l l o u t simulant t o fescue vegeta t ion . Estimates

from t h i s a n a l y s i s a r e compared with those of t h e rad ionucl ide move-

ment experiment from Area 0807 and a l s o compared wi th p red ic t ions of

e ros ion using t h e Wischmeier and Smith s o i l - l o s s equat ion. Based on

observed e ros ion loss as a func t ion of d i f f e r e n t p r e c i p i t a t i o n events,

approximately .06$ of t h e 137Cs contaminant w i l l move from each

contaminated area annually, and t h e input t o t h e n a t u r a l drainage

2 system w i l l be less than 2 m C i from 4-100 m p l o t s . Th i s es t imate

i s o n e - f o r t i e t h of o t h e r independent p red ic t ions and measurements

because t h e dense fescue vegeta t ion and sod of t h e s imulant-plots

g r e a t l y reduce e ros ion and mineral element loss i n runoff .

*This work i s p a r t o f a cooperat ive p r o j e c t j o i n t l y supported by t h e Off ice of C i v i l Defense, Department of Defense, and t h e U. S. Atomic Energy Commission.

I 0 2 4 5 9 8

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3

MEASUREMENT

Runoff c o l l e c t i n g and measuring

OF RUNOFF

devices have been i n s t a l l e d on

2 of 4 p l o t s which w i l l be contaminated with f a l l o u t s imulant .

s p l i t t e r appra tus (F ig . 1) d iv ides the s t ream of water i n t o equal

volumes, and the q u a n t i t y which d ra ins i n t o t h e polyethylene c o l l e c t o r s

i s used t o c a l c u l a t e t o t a l runoff . Subsamples of s o l i d s and s o l u t i o n

w i l l be taken from the c o l l e c t o r s f o r assay of r a d i o a c t i v i t y . This

procedure w i l l monitor m a t e r i a l s c a r r i e d from the p l o t s i n runoff

and w i l l eva lua te lTICs t r a n s f e r t o t h e n a t u r a l drainage system

ou t s ide the experimental a r ea . Before the runoff e x i t s from the

p l o t i t passes through a bas in i n which sand-size p a r t i c l e s s e t t l e ;

therefore , the simulant-sand w i l l not erode from the area .

This

Surface water runoff from p l o t 2 has been observed s ince

October 1967 and from p l o t 7 s i n c e February 1968.

s h i p between p r e c i p i t a t i o n and runoff i s presented i n Table 1, and

the r e s u l t s show t h a t runoff was a l s o r e l a t e d t o s o i l moisture r e -

charge and r a i n f a l l i n t e n s i t y .

r e spec t ive ly , caused d i s s i m i l a r runoff , ye t t he r e s u l t s can be ex-

p la ined on the b a s i s of s o i l water recharge and r a i n f a l l i n t e n s i t y .

By December 21, 3.6 inches of r a i n f a l l had s a t u r a t e d the s o i l dur ing

the preceding 10 days; then, an in t ense r a i n of s h o r t du ra t ion

(0.6 inches) produced 192 l i t e r s of runoff .

r a i n of 3.9 inches caused n e g l i g i b l e runoff because r a i n f a l l dur ing

t h e preceding 10 days had not s a t u r a t e d the s o i l .

much of t he 3.9 inch r a i n f a l l i n f i l t r a t e d the soil.

s o i l system had the capac i ty t o absorb approximately 4 inches of

The r e l a t i o n -

Two r a i n f a l l events, 4 and 5 inches

On January 12, a s teady

I n t h i s case,

I n gene ra l the

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. . , , _ . . . _ _ . . . " , "

c

5

accentua ted i n win ter when the water t a b l e i s 1 5 t o 30 inches from the

su r face and i s less s e r i o u s i n summer when i t i s over 50 inches deep.

A f a c t o r l i m i t i n g runoff would be vege ta t ive cover.

s tand of dense g r a s s should enhance t h e absorp t ion of water, thus

reducing runof f . Because the observat ions (Table 1) were made during

the win te r period, a t which time t h e r e i s minimal vege ta t ive cover,

In t h i s case the

low evapo t ransp i r a t ion r a t e s , s a t u r a t e d s o i l and high water tab le ,

the magnitude of runoff from p r e c i p i t a t i o n events during the grow-

ing season probably would not exceed t h a t a l ready measured.

Eroded s o l i d s were almost absent from the runoff water. Apparently

t h e dense cover of g r a s s and l i t t e r f i l t e r e d and removed most of the

s o i l from su r face runoff .

of minera l sediments were adsorbed on the i n s i d e of the polyethylene

Small q u a n t i t i e s (< 1 g/5 l i t e r s runoff )

c o l l e c t o r s . But more than 25 l i t e r s of runoff were necessary t o

d e p o s i t a c o l l e c t a b l e q u a n t i t y of s o l i d ma te r i a l . Obviously, e ros ion

of su r face s o i l should not be a s e r i o u s problem i n t h i s experiment,

a l though w e p l an t o examine the minera l s o l i d s f o r sorbed radiocesium.

ESTIMATED RADIOCESIUM I N RUNOFF

Transfer of radiocesium from the f a l l o u t s imulant t o d i f f e r e n t

components of the system w i l l involve many complex r eac t ions , some

of which would be d i s s o l u t i o n i n water, s o r p t i o n on s o i l , a s s imi l a -

t i o n by p lan ts , and t r a n s p o r t throughout t he p r o f i l e v i a p l an t r o o t s .

The important mechanisms a f f e c t i n g t.he i n i t i a l r e d i s t r i b u t i o n of lyCs

w i l l be s o r p t i o n on s o i l and movement of d i sso lved and s o l i d m a t e r i a l s

i n water . From l a b o r a t o r y tes ts it was determined t h a t t he s imulant

w i l l r e l e a s e 10% of the fixed l r / C s fol lowing con tac t w i th water f o r

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7

i

Based on the observed average r a t e of s o i l e ros ion (1 g/5 l i t e r s ) ,

the quan t i ty contained i n 400 l i t e r s of runoff would be 80 g.

q u a n t i t y represented 6.65 x 10

This

$, of the su r face cent imeter of s o i l -3

6 (1.2 x 10 g) i n contac t w i t h the s imulant . The est imated rad io-

cesium t h a t could be removed i n the s o l i d phase i s ca l cu la t ed as 0.04

mCi/plot. Although the g r e a t e s t quan t i ty of r a d i o a c t i v i t y i s c a r r i e d

by s o l i d mater ia l s , the t o t a l loss i n t h i s phase w i l l be n e g l i g i b l e

(0.92 mCi/year from a l l p l o t s ) because the vege ta t ive cover e f f e c t i v e l y

prevents s o i l e ros ion .

The polyethylene c o l l e c t o r s r e t a i n most of the eroded s o i l , and

i n f u t u r e measurements t h i s m a t e r i a l w i l l be removed for rad ioassay

or d i sposa l .

t r a n s f e r r e d d i r e c t l y t o t h e e x t e r i o r drainage system.

are summarized the r a d i o a c t i v i t y movement from p l o t s with c o l l e c t o r s

(480 PCi/year) and without c o l l e c t o r s (1,200 )zCi/year) . the l o s s from p l o t s having no c o l l e c t o r s would be g r e a t e r by a f a c t o r

of 3, t h e r e i s no cause f o r alarm because the p red ic t ed l o s s e s v i a

runoff would c o n s t i t u t e only 0.21% of the 8 c u r i e s of contaminant

i n the 4 p l o t s .

mCi/year) w i l l be r e l eased t o the outs ide dra inage system, and con-

s i d e r i n g the h igh s o r p t i v e capac i ty of l o c a l s o i l f o r cesium, the

contaminant probably w i l l be r e t a ined i n the drainage d i t c h and w i l l

not be c a r r i e d t o the Clinch River.

Thus, contaminated s o i l from only 2 p l o t s w i l l be

I n Table 2

Although

Thus, only a minor quan t i ty of radiocesium (1.7

COMPARISON WITH OTHER RFSULTS

Erosion and runoff va ry g r e a t l y f o r d i f f e r e n t c u l t i v a t i o n p rac t i ces ,

and t h e magnitude of s o i l loss i s a func t ion of many v a r i a b l e s . Because

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9

Appl ica t ion of the s o i l - l o s s equat ion was intended f o r c u l t i v a t e d

crops, and i t possesses l i m i t e d u t i l i t y f o r eva lua t ing e ros ion i n

systems of dense cover and i n t a c t sod.

p e r f e c t l y r e a l i s t i c because n e g l i g i b l e e ros ion occurs i n noncul t iva ted

systems such as pas tu re and meadow. Despi te t h i s l i m i t a t i o n i n a p p l i -

c a b i l i t y we w i l l a t tempt t o p red ic t t h e annual e ros ion loss from a

dense s tand of fescue vege ta t ion using appropr ia te terms i n the

s o i l - l o s s equat ion.

t o e s t a b l i s h some understanding of t h e i r meaning and l i m i t a t i o n s .

Also s e l e c t i o n of va lues f o r some terms i s debatab le ; therefore ,

j u s t i f i c a t i o n f o r our choice of va lues i s presented i n the fol lowing

d iscuss ion .

The au thor s ' i n t e n t was

The terms of t h i s equat ion a r e d iscussed b r i e f l y

1 The r a i n f a l l f a c t o r ( R ) , g iven by Wischmeier and Smith , t h e i r

F ig . 1 was based on s o i l loss from c u l t i v a t e d f i e l d s as a func t ion

of E1 ra ins torm c h a r a c t e r i s t i c s . But t he e f f e c t i v e n e s s of the r a i n -

f a l l ' s e ros ive f o r c e would be reduced considerably for a s o i l i n con-

t a c t w i t h an in t ens ive r o o t system and heav i ly covered with f o l i a g e

and l i t t e r . The r o o t - s o i l mat r ix under e s t ab l i shed g r a s s vege ta t ion

p resen t s a completely d i f f e r e n t environment compared wi th fa l low

s o i l . Roots would r e t a i n s o i l t h a t would be dis lodged and eroded

i n the c u l t i v a t e d condi t ion . Because R va lues f o r t he s t a b i l i z e d

s o i l environment should be l e s s than t h a t f o r fa l low s o i l , we propose

t h a t an R of 200 [ repor ted f o r t h i s a r ea by Wischmeier and Smith ]

would r ep resen t a maximum r a t h e r than average r a i n f a l l e ros ive force .

1

The e r o d i b i l i t y f a c t o r (K) i s a f f e c t e d by phys ica l c h a r a c t e r i s t i c s

of the s o i l . Generally, e r o d i b i l i t y i s d i r e c t l y r e l a t e d t o f ineness

-.

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11

. The r e s u l t s from 2 l o c a l experiments permit a comparison of pre-

d i c t e d and observed s o i l loss . The terms used i n t h e Wischmeier and

Smith equat ion were based on t h e phys ica l and b i o l o g i c a l cha rac t e r -

i s t i c s of small- and s imulant -p lo ts (Table 3 ) and ca l cu la t ed l o s s e s

were compared a g a i n s t measured e ros ion .

pre l iminary runoff d a t a were c o l l e c t e d f o r six months dur ing which

time the ra te of s o i l loss was approximately 1 g/5 l i t e r s which con-

s t i t u t e s 0.5 g/m and e x t r a p o l a t e s t o 1 g/m /year .

condi t ions of severe runoff, the annual s o i l loss i s p red ic t ed on

t h e b a s i s of 20 r a i n f a l l events each producing 400 l i t e r s of runof f ;

then, we would expect 16 g/m /year [(400 l i t e r s / e v e n t ) (20 even t s ) /

( 5 l i t e r s / g ) (100 m2)].

pred ic t ed va lue (12 g/m ) is more than 1OX g r e a t e r than the observed

t o date, (1 g/m ), bu t under very severe condi t ions the expected 2 (16 g/m ) would be s l i g h t l y g r e a t e r than t h a t pred ic ted from the

model. Agreement between observed and p red ic t ed e ros ion l o s s i s

reasonably gocd cons ider ing t h a t t he s o i l - l o s s model was der ived f o r

c u l t i v a t e d systems. Also, w e must remember t h a t topographic f e a t u r e s

of the s imulant -p lo ts approach the lower l i m i t s for which the model

i s app l i cab le .

Considering the s imulant-plots ,

2 2 For a n t i c i p a t e d

2

Using t h e Wischmeier and Smith model t he 2

2

273 Continuous observa t ion of e ros ion from t a l l meadow smal l -p lo ts

over a two-year per iod provide a d d i t i o n a l r e s u l t s f o r c o r r e l a t i n g

p red ic t ed and observed s o i l l o s s .

loss from the vege ta ted system was 72 g/m

l o s s e s of 42 g/m . 13 g/m , an apprec iab le reduct ion i n e ros ion .

Af t e r one year, the observed s o i l

2 compared wi th pred ic ted

2 For the next year the observed loss was only 2

Averaging both years

1 0 2 4 b 0 3

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l e v e l f o r storm e r o s i t i v i t y of t h i s magnitude

Differences i n e r o d i b i l i t y (K) a r e a t t r i b u t e d

i n e a s t e r n Tennessee.

t o v a r i a t i o n i n s o i l

c h a r a c t e r i s t i c s ; Captina--low i n f i l t r a t i o n and f i n e t e x t u r e ; Lindside--

h igh i n f i l t r a t i o n , coarse t e x t u r e .

was recommended by the Soil-Loss P red ic t ion Conference held i n Knoxville,

Tennessee, 1959.

The 0.4 va lue of K f o r Captina

The SL term f o r the s imulant-plot eva lua t ion was taken from

Wischmeier and Smith's s lope e f f e c t c h a r t . Average g rad ien t and s lope

l eng th f o r smal l -p lo ts were determined from r e p l i c a t e d measurements

of m i c r o r e l i e f

s lope length .

a l though they were determined d i f f e r e n t l y . Se l ec t ion of the s imulant-

p l o t C va lue i s descr ibed above ( p . 10) Tamura and Rogowski3 calcu-

l a t e d C from the s o i l - l o s s equat ion assuming t h a t o the r terms a l ready

had been evaluated.

3 and the c a l c u l a t i o n s were 8% ;t 1 f o r 7.5 f t . 2 0.7

The cover f a c t o r s ( C ) were s i m i l a r f o r bo th eva lua t ions ;

A comparison of p red ic t ed and observed r e s u l t s se rves t o t e s t

the model and the choice of terms used i n an eva lua t ion . Long-term

eva lua t ion i s d e s i r a b l e because of v a r i a b i l i t y i n e ros ion responses

a s soc ia t ed with i n d i v i d u a l r a i n f a l l events . Despite the l imi t ed

du ra t ion of observa t ion the re was some agreement between predic ted

and observed e ros ion from both s imulant and smal l p l o t s . For

s i rnulant-plots c o r r e l a t i o n appeared b e t t e r when p red ic t ed e ros ion

was compared with t h e maximum expected assuming extreme condi t ions

of r a i n f a l l e r o s i v i t y . For normal condi t ions , however, the Wischmeier

and Smith model overes t imates e ros ion from a heav i ly vege ta ted sod

( 2 g r e a t e r f o r second year r e s u l t s from smal l -p lo ts 1OX g r e a t e r

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1 5

RFFERFNCES CITED

1. Wischmeier, Walter H,, and Dwlght D. Smith. 1965. Predic t ing

r a in fa l l - e ros ion lo s ses frum cropland e a s t of the Rocky Mountains:

Guide f o r s e l e c t i o n of p rac t i ces f o r s o i l and water conservation.

Agricul ture Handbook No. 282, ARS/USDA, Washington, D . C., 47 pp.

2. Rogawski, A . So, and Tsuneo Tamura. 1965. Movement of l y C s b y

runoff, e ros ion and i n f i l t r a t i o n on the a l l u v i a l Captina s i l t

loam. Health Physics - 11: 1333-1340.

3. Tamura, Tsuneo, and A . S. Rogowski. 1967. Movement of l T C s by

runoff, e ros ion and i n f i l t r a t i o n from a s o i l under d i f f e r e n t

cover condi t ions. Unpublished. Presented a t Symposium on

Pos ta t tack Recovery, November 6-19, 1967, For t Monroe, Vi rg in ia .

1 0 2 4 6 0 5

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k cd a, h .d V =I.

\

0

0 t

0 cu

k 0

+,a I U oa,

.d 0 S V 52

E: 0 C 5 k bo C .d V I a 0 k a k 0

4 8 A

P

(d 0

0 cu %

I024bOb

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LIST OF FIGUFES

Figure 1. View of Splitter Apparatus Used to Measure Runoff from 2 100 m experimental plot.

Figure 2. Predicted Movement of Radiocesium from One Runoff Plot

Shortly After Application of Fallout Simulant.

in Compartments Represent mCi of Ir/Cs/Plot and Other

Numbers

Values Indicate Fractional Transfer Between Compartments.

1 0 2 4 b 0 1 -.

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ORNL-DWG 68-67!9

3c -cssoil -,ooo

**FRACTIONAL TRANSFER BECAUSE SEDIMENTS WILL BE COLLECTED FOR RADIOASSAY. Kd-Cs SO,'n

Predicted Movement o f Radiocesium from One Runoff Plot Shortly After Application o f Fallout Simulant. Numbers in Compartments Represent mci of 137Cs/Plot and Other Values Indicate Fractional Transfer Between Compartments.

F i g . 1

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i 1-2. 3-4.

5 .

6-9. 10. 11.

12-111. 112.

114 113 a

115. 116. 117. 118. 119. EO.

321-220. 221. 222. 223. 224. 225. 226.

ORNL-TM-2343

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Biology Library Cent ra l Research Library ORNL - Y-I2 Technical Library Document Reference Sect ion Laboratory Records Department Laboratory Records, ORNL R . C . ORNL Patent Off i c e S. I. Auerbacn C. E. Baker B. G . Blaylock W . J . Boegly, Jr. W . P. Bonner R. L. Bradshaw T. J. Burnet t H. M. Bu t l e r K. E. Cowser J. W. Curl in R. C. Dahlman D. M. Davis Wallace de Laguna P. B. Dunaway J. W . Elwood F. M. Empson T. Grizzard

228. 229. 230. 231. 232. 233 234. 235 236. 237 238. 239 240. 241. 242. 243. 244. 245. 246. 247. 248. 249. 2%). 251.

S. V. Kaye J. T. Kitchings I11 J. L. Liverman T. F. bmenicK H. G. MacPherson C. R. Malone W . C. McClain R. H. Monheimer K. Z. Morgan D. J. Nelson J. S. Olson R. V. O ' N e i l l L. N. Pe t e r s D. E. Reichle A. F. Shinn J. D. S tory E. G . Struxness C. E. Styron, Jr. Tsuneo Tamura F. G. Taylor W . A . Thomas A. M. Weinberg J. P. Witherspoon

I Martin Witkamp 227. D. G . Jacobs

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252.

253 0

254.

255.

256-260 e

J. N. Wolfe, Environmental Sciences Branch, Division of Biology and Medicine, USAEC, Washington, D. C. J. J. Davis, Environmental Sciences Branch, Division of Biology and Medicine, USAEC, Washington, D. C . R. F. Reitemeier, Environmental Sciences Branch, Division of Biology and Medicine, USAEC, Washington, D. C. W. S. Osburn, Environmental Sciences Branch, Division of Biology and Medicine, USAEC, Washington, D. C. Jack Greene, Off ice of C i v i l Defense, The Pentagon, Washington, /

D. c. 20310

D. c. 20310 261-265. David Benson, Off i c e of C i v i l Defense, The Pentagon, WdShingtOn,

266. C. S. Shoup, Biology Branch, Oak Ridge Operations, USAEC, Oak

267. Carl B e l l , U. T.-AEC Agr i cu l tu ra l Research Laboratory, Oak Ridge,

268. John Cantlon, Department of Botany, Michigan S t a t e University,

269. E. E. C . Clebsch, Department of Botany, Universi ty of Tennessee,

Ridge, Tennessee

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