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Princeton-TAMU Symposium on Quantum Physics and Engineering, in honor of Wolfgang Schleich June 2017 Luis A. Orozco www.jqi.umd.edu Super- and sub-radiance with atoms around an optical nanofibers

Super- and sub-radiance with atoms around an optical

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Page 1: Super- and sub-radiance with atoms around an optical

Princeton-TAMU Symposium on Quantum Physics and Engineering,

in honor of Wolfgang Schleich June 2017

Luis A. Orozco www.jqi.umd.edu

Super- and sub-radiance with atoms around an optical

nanofibers

Page 2: Super- and sub-radiance with atoms around an optical

Graduate Students: J. A. Grover, J. E. Hoffman, S. Ravets (I. d’Optique), P. Solano, B. Patterson. Undergraduate Students: U. Chukwu, C. Ebongue, E. Fenton, B. Friedman, X. Gutierrez, A. Kahn, P. Kordell, E. Magnan, A. Preciado, J. D. Wong-Campos, A. Wood. Professors and Researchers: P. Barberis Blostein, F. K. Fatemi, L. A. Orozco, W. D. Phillips, S. L. Rolston University of Maryland, Institute D’Optique, National Institute of Standards and Technology, Army Research Laboratory, Universidad Nacional Autonoma de Mexico. Supported by: Atomtronics MURI from ARO, DARPA, the Fulbright Foundation, NSF through PFC@JQI, JQI, and ONR.

Page 3: Super- and sub-radiance with atoms around an optical

Christiane Xavier

5 2013

Jeff, Krysten Peter Uchenna Pablo, Jonathan, David

Eliot Alan

6 2015

Sylvain

Jonathan Jeff

3 2012

THE TEAMAdnan

9 2015

Pablo Jeff

102014

1 2016 Burkley

Page 4: Super- and sub-radiance with atoms around an optical

Optical Nanofibers

Page 5: Super- and sub-radiance with atoms around an optical

Optical Nanofibers

Core φ ~ 5 µm Cladding φ ~ 125 µm

Page 6: Super- and sub-radiance with atoms around an optical

Optical Nanofibers

Core φ ~ 5 µm Cladding φ ~ 125 µm

Page 7: Super- and sub-radiance with atoms around an optical

Core φ ~ 5 µm Cladding φ ~ 125 µm

Optical Nanofibers

Page 8: Super- and sub-radiance with atoms around an optical

Core φ ~ 5 µm Cladding φ ~ 125 µm

Optical Nanofibers

Page 9: Super- and sub-radiance with atoms around an optical

50 nm away from the surface 1 atom can block 10% of the light.

Optical Density

Page 10: Super- and sub-radiance with atoms around an optical

Evanescent Coupling γ rad

γ1D Nottoscale

γTot = γ rad +γ1D

Page 11: Super- and sub-radiance with atoms around an optical

Nottoscale

A(!r ) = PI(!r )

α(!r ) = γ1D (!r )

γ0=1neff

σ 0

A(!r )=1neff

OD1(!r )

ONF Single Atom Optical Density

Page 12: Super- and sub-radiance with atoms around an optical

Can we see a collective atomic effect of atoms around the

nanofiber?

Page 13: Super- and sub-radiance with atoms around an optical

Infinite Range Interactions

Not to scale

Page 14: Super- and sub-radiance with atoms around an optical

Infinite Range Interactions

Not to scale

Page 15: Super- and sub-radiance with atoms around an optical

Infinite Range Interactions

Not to scale

Page 16: Super- and sub-radiance with atoms around an optical

Infinite Range Interactions

Vfree ∝exp(ikr)kr

Page 17: Super- and sub-radiance with atoms around an optical

Infinite Range Interactions

Vfree ∝exp(ikr)kr

V1D ∝ exp(ikr)

Page 18: Super- and sub-radiance with atoms around an optical

Infinite Range Interactions

Vfree ∝exp(ikr)kr

V1D ∝ exp(ikr)

Page 19: Super- and sub-radiance with atoms around an optical

Super- and Sub-radiance (a classical explanation)

“When two organ pipes of the same pitch stand side by side, complications ensue which not infrequently give trouble in practice. In extreme cases the pipes may almost reduce one another to silence. Even when the mutual influence is more moderate, it may still go so far as to cause the pipes to speak in absolute unison, in spite of inevitable small differences. Lord Rayleigh (1877) in "The Theory of Sound".

Page 20: Super- and sub-radiance with atoms around an optical

Super- and Sub-radiance (a classical explanation)

We need the response of one oscillator due to a nearby oscillator (interference): !!a1 +γ0 !a1 +ω0

2a1 =32ω0γ0d̂1 ⋅

!E 2!r( )a1,

assuming a1 = a10 expi(ω − i / 2)t

γ = γ0 +32γ0Im d̂1 ⋅

!E 2!r( ){ }, with d̂1 ⋅

!E 2 0( ) = 2

3

ω =ω0 −34γ0 Re d̂1 ⋅

!E 2!r( ){ }

Page 21: Super- and sub-radiance with atoms around an optical

Observation of infinite-range interactions

Page 22: Super- and sub-radiance with atoms around an optical

Probe Beam

The idea behind the experiment

Page 23: Super- and sub-radiance with atoms around an optical

Probe Beam

The idea behind the experiment

We look for modifications of the radiative lifetime of an ensemble of atoms around the ONF.

Page 24: Super- and sub-radiance with atoms around an optical

Probe Beam

The sub- and super-radiant behavior depend on the phase relation of the atomic dipoles along the common mode

The idea behind the experiment

Page 25: Super- and sub-radiance with atoms around an optical

currentnanofiber

α =γ1Dγ0

Coupling Enhancement

Weuseuntrappedatoms!

Page 26: Super- and sub-radiance with atoms around an optical

Measuring the Radiative Lifetime

Page 27: Super- and sub-radiance with atoms around an optical

Measuring the Radiative Lifetime

1 mm

Page 28: Super- and sub-radiance with atoms around an optical

F=1F=2

F’=2F’=3

F’=1F’=0

De-pump Re-pump Probe

De-pump

Probe

Re-pump

Preparing the Atoms

Page 29: Super- and sub-radiance with atoms around an optical

F=1F=2

F’=2F’=3

F’=1F’=0

De-pump Re-pump Probe

Preparing the Atoms

20 30 40 50 60 70-30

-25

-20

-15

-10

-5

0

Atom-surface position [nm]

Frecuencyshift

[MHz] Δ

Δ

Page 30: Super- and sub-radiance with atoms around an optical

Atomic distribution with optical pumping

Distribution of atoms with optical pumping

0 50 100 150 200 2500.0

0.2

0.4

0.6

0.8

1.0

Atom-surface distance (nm)

Densitydistribution(arb.unit)

Page 31: Super- and sub-radiance with atoms around an optical

-4

-3

-2

-1

0

Log 10

cou

nt r

ate

0 5 10 15 20 25 30t/τ

0

Two distinct lifetimes

Page 32: Super- and sub-radiance with atoms around an optical

-4

-3

-2

-1

0

Log 10

cou

nt r

ate

0 5 10 15 20 25 30t/τ

0

Two distinct lifetimes

τ ≈ 7.7τ 0

τ ≈ 0.9τ 0

Page 33: Super- and sub-radiance with atoms around an optical

Two distinct lifetimes

τ ≈ 7.7τ 0

τ ≈ 0.9τ 0

-4

-3

-2

-1

0

Log 10

cou

nt r

ate

0 5 10 15 20 25 30t/τ

0

Page 34: Super- and sub-radiance with atoms around an optical

Decay time vs detunning

No radiation trapping for long lifetime

Page 35: Super- and sub-radiance with atoms around an optical

Decay time vs detunning

No radiation trapping for short lifetime

-4 -2 0 2 40.91.01.11.21.3

Δ/γ0

γ/γ 0

Page 36: Super- and sub-radiance with atoms around an optical

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0 5 10 15 20- 6

- 5

- 4

- 3

- 2

- 1

0

time (in units of τ0)

Log 1

0no

rmal

ized

coun

t ra

te

Page 37: Super- and sub-radiance with atoms around an optical

-4

-3

-2

-1

0

Log 10

cou

nt r

ate

0 5 10 15 20 25 30t/τ

0

Two distinct lifetimes

τ ≈ 7.7τ 0

τ ≈ 0.9τ 0

Page 38: Super- and sub-radiance with atoms around an optical

N dependence

γsup = γ rad + Nγ1D

Page 39: Super- and sub-radiance with atoms around an optical

N dependence

γsup = γ rad + Nγ1D

Superradiance depends on the atom number!

Page 40: Super- and sub-radiance with atoms around an optical

Measurment of N

-20 -10 0 10 200.6

0.7

0.8

0.9

1.0

frequency (MHz)

Transmission

Probe

OD = N ⋅OD1(!r0 )

Page 41: Super- and sub-radiance with atoms around an optical
Page 42: Super- and sub-radiance with atoms around an optical

The slope (0.02) is smaller than γ1D (0.10) because it is an average over different realizations, non all of them superradiant.

Page 43: Super- and sub-radiance with atoms around an optical

Sub-radiance???

γsup = γ rad + Nγ1D

Page 44: Super- and sub-radiance with atoms around an optical

Infinite-range subradiance is limited!

Subradiance???

γ sub = γ rad −γ1D

γsup = γ rad + Nγ1D

γ radγ1D

Page 45: Super- and sub-radiance with atoms around an optical

-4

-3

-2

-1

0

Log 10

cou

nt r

ate

0 5 10 15 20 25 30t/τ

0

Sub-radiance??? γ rad

γ1D

γ ≈ 0.13γ0

γ sub = γ rad −γ1D ≈ 0.9γ0

The subradiant decay rate we measure is too slow!

Page 46: Super- and sub-radiance with atoms around an optical

Understanding the Signal

Page 47: Super- and sub-radiance with atoms around an optical

Understanding the Signal

Page 48: Super- and sub-radiance with atoms around an optical

Polarization dependent signal

VerDcallypolarizedprobe Horizontallypolarizedprobe

Page 49: Super- and sub-radiance with atoms around an optical

Polarization dependent signal

Vertically polarized probe Horizontally polarized probe

Page 50: Super- and sub-radiance with atoms around an optical

Subradiant Signal

-  Interaction distance smaller than λ: all modes get cancelled.

-  Interaction distance greater than λ: only one mode gets cancelled

We measure

γ sub = γ rad −γ1D ≈ 0.9γ0γ sub = 0.13γ0

Page 51: Super- and sub-radiance with atoms around an optical

Super-radiant Signal

-  Interaction distance smaller than λ: all modes get enhanced.

-  Interaction distance greater than λ: only one mode gets enhanced

We measure

γsup = γ rad + Nγ1Dγsup =1.1γ0

Page 52: Super- and sub-radiance with atoms around an optical

Fitting the Simulation

-4

-3

-2

-1

0

Log 10

nor

mal

ized

cou

nt ra

te

-4-2024

Nor

mal

ized

Res

idua

ls

(a)

(b)

0

-1

-2

-3

-4

t/τ0

0 5 10 15 20 25 30

0 5 10 15 20

t/τ0

Log 10

nor

mal

ized

cou

nt ra

te

Page 53: Super- and sub-radiance with atoms around an optical

Fitting the Simulation

Page 54: Super- and sub-radiance with atoms around an optical

Long distance modification of the atomic radiation

Page 55: Super- and sub-radiance with atoms around an optical

Long distance modification of the atomic radiation

We have atomic densities low enough to observe mostly infinite-range interactions

Page 56: Super- and sub-radiance with atoms around an optical

nanofiber

Left MOT

Splitting the MOT in two

Right MOT

≈ 400λ

Page 57: Super- and sub-radiance with atoms around an optical

Right MOT

Left MOT

Both MOTs

Evidence of infinite-range interactions

Page 58: Super- and sub-radiance with atoms around an optical

Observations: About one in 50 of the decays is super-radiant. Quantitative agreement with simulations.

Page 59: Super- and sub-radiance with atoms around an optical

Summary •  We have seen collective atomic effects (sub- and

super- randiance) monitoring the mode of the nanofiber. Superadiance shows long-range dipole-dipole interactions (many times the wavelength) scaling with the optical density (number of atoms). Subradiance is between nearby atoms.

•  New platform for exploring long-range interactions. •  Many Body physics without the Markov

approximation.

Page 60: Super- and sub-radiance with atoms around an optical

Thanks!

Page 61: Super- and sub-radiance with atoms around an optical