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1855-15
School and Workshop on Highly Frustrated Magnets and StronglyCorrelated Systems: From Non-Perturbative Approaches to
Experiments
Frederic Mila
30 July - 17 August, 2007
Institute of Theoretical PhysicsEcole Polytechnique Fédérale de Lausanne,
Switzerland
Strong coupling approaches and effective Hamiltonian
StrongStrong couplingcouplingapproachesapproaches andand
effective effective HamiltonianHamiltonianF. F. MilaMila
InstituteInstitute ofof TheoreticalTheoretical PhysicsPhysicsEcoleEcole Polytechnique FPolytechnique Fééddééralerale de de LausanneLausanne
ScopeScope•• Introduction: Introduction: whywhy strongstrong couplingcoupling??•• BriefBrief reviewreview ofof degeneratedegenerate perturbation perturbation
theorytheory•• FrustratedFrustrated magnetsmagnets in in zerozero fieldfield: : couplingcoupling
triangles, triangles, tetrahedratetrahedra,,……•• LaddersLadders andand coupledcoupled dimersdimers in a in a fieldfield•• PerturbingPerturbing IsingIsing modelsmodels•• Alternatives to Alternatives to degeneratedegenerate perturbationperturbation
Heisenberg modelHeisenberg modelStandard analytical approach: expansion in 1/S
Spin-waves around classical GS
Problem: frustration highly degenerate GS
No natural starting point for 1/S
Alternative?
StrongStrong couplingcoupling II
1) Suppose
2) Write with
StrongStrong couplingcoupling IIII
3) If GS of H0 degenerate, treat V withdegenerate perturbation theory
Effective Hamiltonian
Small parameters:
NB: often useful to assume some parameters are small even if they are not (like 1/S for S=1/2!)
ExamplesExamples
JJ’
Weakly coupled triangles
Trimerized kagome
Heisenberg model with Ising anisotropy
Perturbation around Ising limit
DegenerateDegenerate Perturbation Perturbation TheoryTheory
Second Second orderorderExtremely useful, yet not totally standard
HigherHigher orderorder II
HigherHigher orderorder IIII
Standard Standard exampleexample: : superexchangesuperexchange
Hubbard model
½-filling 1 e-/ site
2nd order perturbation
Heisenberg model
One triangleOne triangle
CoupledCoupled trianglestriangles
JJ’
Pseudo-spin‘chirality’
Spin
First-order perturbation in J’
Triangular lattice
SpinSpin--chiralitychirality meanmean--fieldfield decouplingdecoupling
Relevant degrees of freedom selected
Reasonable to use mean-field
Degenerate GS
Dimer coverings oftriangular lattice
OtherOther examplesexamples
•• TetrahedraTetrahedra: GS : GS isis a a twotwo--foldfold degeneratedegeneratesinglet singlet pure pure ‘‘chiralitychirality’’ effective effective modelmodel
•• OddOdd rings: rings: likelike for a triangle, GS for a triangle, GS consistsconsistsofof twotwo doublets doublets spinspin--chiralitychirality modelmodel
•• UnitsUnits withwith nonnon--degeneratedegenerate singlet GS in a singlet GS in a magneticmagnetic fieldfield singlet singlet degeneratedegenerate withwithlowestlowest triplet triplet atat criticalcritical fieldfield
DimersDimers in a magnetic fieldin a magnetic fieldIsolated dimers
Coupled dimers
Magnetization of spin laddersMagnetization of spin ladders
CuHpCl Chaboussant et al, EPJB ‘98
DimersDimers in a magnetic fieldin a magnetic field
Isolated dimersCoupled dimers
2 states/rung degenerate GS
Frustrated laddersFrustrated ladders
Metal-insulator transition for V=2t (J’=J/3)
Magnetization PlateauMagnetization Plateau
D. Cabra et al, PRL ‘97K. Totsuka, PRB ‘98
T. Tonegawa et al, PRB ‘99F. Mila, EPJB ‘98
Frustration
Kinetic energy
Repulsion
Metal-insulator transition
Magnetization plateau
Magnetization of SrCuMagnetization of SrCu2(BO(BO3))2
Kageyama et al, PRL ‘99
ShastryShastry--Sutherland modelSutherland model
Ground-state Product of singlets on J-bonds (Shastry, Sutherland, ’81)
Triplets Almost immobile and repulsive (Miyahara et al, ’99)
(Miyahara et al, ’00)Plateaux
Frustrated Coupled Frustrated Coupled DimersDimers
Triplet Hopping Triplet Repulsion
Quantum Quantum DimerDimer ModelsModelsSquare lattice (Rokhsar-Kivelson, ’88)
Assume dimer configurations are orthogonal
RK ’88Leung et al, ‘96
QDM on triangular latticeQDM on triangular lattice
Spin liquid with gapped spectrumand topological degeneracy
Equivalent spin model? Yes! The QDM is theeffective model of an Ising model in transverse field
FullyFully FrustratedFrustrated IsingIsing modelmodel
Ground states: 1 unsatisfied bond/hexagon
ExampleExample ofof a a groundground statestate
Bond unsatisfied if J>0
For that ground state, unsatisfied bondslie on dashed lines
MappingMapping onto QDM Hilbert onto QDM Hilbert spacespace
Hexagonal lattice= dual lattice oftriangular lattice
Draw a bond on the triangular lattice acrossall unsatisfied bonds dimer covering
AddAdd a transverse a transverse fieldfield
One spin flip outside ground state manifold
TwoTwo spin flipsspin flips
Stay in ground state manifold
Flip two spinson neighboring
unsatisfied bonds
In In termsterms ofof dimersdimers
Flip dimersaround flippable
plaquette
2nd order perturbation theory in Γx
Ising model , QDM with flip term / Γx2/J
Alternative I : Canonical TransformationAlternative I : Canonical Transformation
Advantages
- Possible for non degenerate GS- Systematic expansion- Gives access to full spectrum
Drawbacks
- Not universal: needs to find S - Necessary condition: all linear
corrections must vanish
Standard example: Hubbard Heisenberg
Alternative II: COREAlternative II: CORE
CORE: Contractor Renormalization
1) Find numerically low-energy spectrum of largestaccessible system
2) Fit it numerically with effective Hamiltonian of smallersub-units
Advantages
- Very flexible- Universal- Best effective model from
quantitative point of view
Drawbacks
- Not well suited for analyticaltreatment of effective model
- Physics of effective model nottransparent
ConclusionsConclusions
•• Effective Effective HamiltonianHamiltonian: : oftenoften a a goodgood wayway to to understandunderstand physicsphysics atat a qualitative a qualitative levellevel
•• If If naturalnatural smallsmall parameterparameter, THE , THE methodmethod to to bebe recommendedrecommended
•• SeveralSeveral waysways ofof derivingderiving an effective an effective HamiltonianHamiltonian. . DegenerateDegenerate perturbation perturbation theorytheory veryvery simple simple andand recommendedrecommended if if firstfirst or second or second orderorder sufficientsufficient