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Positronium and e+-e- Annihilation
Gam
ma-G
am
ma C
orr
ela
tion
s 2
10 32 ( ) 1.25 10 sec
#
n n
n principal quantum
7 33 ( ) 1.4 10 secn n 2
2 0 2 3
0
372
2.818 , . .
e erc
r fm class el radius
Eg/2E0 1
dN/dEg
Eg/2E0 1
dN/dEg
Decay at rest: 2Eg≈E0 ≈ 1.022 MeV2-body decay q12≈1800
3-body decaycontinuumin Eg and q12
2-body decayline spectrumin Eg and q12
q12
Para Positronium
Ortho Positronium
0I
1I
0E eV
48 10E eV
1
s
2
s
2
s
1
s
Gam
ma-G
am
ma
Corr
ela
tion
s3
Radiation Detectors for Medical Imaging
e e 2 (511 keV )
Positron e+ (anti-matter) annihilates with electron e- (its matter equivalent of the same mass) to produce pure energy (photons, g-rays). Energy and momentum balance require back-to-back (1800) emission of 2 g-rays of equal energy
g Detectors (NaI(Tl))
Positron emission tomographic (PET) virtual slice through patient’s brain
Administer to patient radioactive water: H2
17O radioactive acetate: 11CH3COOX
Observe 17O or 11C b+ decay by
ANSEL Angular Correlation Experiment
Gam
ma-G
am
ma C
orr
ela
tion
s 4
Top left: PET imaging experiment setup with two 1.5”x1.5” NaI(Tl) detectors (BICRON) on a slotted correlation table. A “point-like” 22Na g source can be hidden from view.Top right: 22Na g spectrum measured with NaI1.Bottom right: - g g angular correlation measurement.
Second correlation setup: NaI(Tl) vs. HPGe
Gam
ma-G
am
ma
Corr
ela
tion
s 5
E1-E2-Dt Multi-Parameter Measurement
-g g cascade (60Ni) or PET experiment, full 3D energy-time distribution.
Dela
y v
ar.
TFA/CFTD
Gate Generator
PreAmp
Amp Energy 1
Relative Time
PreAmp
TFA/CFTD
Gate Generator
Amp
TACDt
Energy 2
Start
Stop
Counter
Counter
DAQ
Pulse Generator Counter
Pulser
Dead time measurement
Gam
ma-G
am
ma
Corr
ela
tion
s 6
E1-E2 Dual-Parameter Measurement
-g g cascade (60Ni) or PET experiment, full 2D spectrum
Dela
y v
ar.
TFA/CFTD
Gate Generator
PreAmp
Amp Energy 1
Strobe
PreAmp
TFA/CFTD
Gate Generator
Amp Energy 2
Pulse Generator Counter
Pulser
Dead time measurement
Coin
cid.
OR
DAQ
2D Parameter MeasurementG
am
ma-G
am
ma
Corr
ela
tion
s 7
2D Scatter Plot:Each point represents one event {E1, E2}
E2
E1
Projection on E2 axis
Projection
on E1 axis
Gam
ma-G
am
ma
Corr
ela
tion
s 8
Gated E1-E2 Coincidence Measurement
-g g cascade (60Ni) or PET experiment, gates on g1 and g2 lines
Dela
y v
ar.
SCAGate
Generator
Amp Energy 1
Strobe
Amp
SCA
Gate Generator
Energy 2
Pulse Generator Counter
Pulser
Dead time measurement
Coin
cid.
OR
DAQ
Gam
ma-G
am
ma
Corr
ela
tion
s 9
Absolute Activity Measurement
1 1 2 2
12 1 2 12 12
1 2 1 2
12 12
/
N A P N A P individual rates
P P P N A P coincidence rate
N N A P A PA singles coinc
N A P
N1
N2
N12
TFA/CFTD
Gate Generator
Pre Amp
Pre Amp
TFA/CFTD
Gate Generator
Coin
cid
en
ce Counter
Coinc.
Counter 1
Counter 2
1
2
Activity A
Activity A [disintegrations/time], independent radiation types i =1,2 detection probabilities Pi
Symmetries of the Nuclear Mean Field
Gam
ma-G
am
ma C
orr
ela
tion
s 1
1
1,...,
,
1: ( )
,
2
,( ) ( )
( )
ˆ
A
i ji j
central potential no angle depe
Invariance against space inversion rotati
Nuclearmean fieldU U r r
per nucleon A
U r U r
Conservation of parity and angular momentum
quantum dualit
nd
y
ons
n
H
e ce
2
1
22 2 2
2
2 2
ˆ ˆ ˆ ˆˆ( ) , 0 ,2
ˆ ˆ ˆ: ( ) ( )( )
ˆ ˆ ˆ ˆ ˆ( ) ( ) ( );
Ai
ii i
ix ix i ii
z i z i i z i i
pU r H H R
m
because p p and U r U rx
and R U r U R r U r and R p p
Potential
Bound States
r
Y(r)
0
Nucleon-nucleon forces are dominantly radial
1 2 1 2( , ) ( )U r r U r r
r
U r
r n=0
n=1
n=2
Gam
ma-G
am
ma C
orr
ela
tion
s 1
2
Stationary Nuclear States
ˆ
2
ˆ: ( )
ˆ ˆ ˆ ˆ ˆ ˆ, ( ) 0
ˆ ( ) (
, 0 ,
)i
Lz z
n n n
z z
z z z
Hj r E j r sta
Operator for rotations R e
H R H L H
tio
L
nary states
2 2ˆ ( , ) ( 1) ( , )
ˆ ( , ) ( , )
ˆ ( ) ( )
m m
z m m
m m
L Y Y
L Y m
Parity
Y
Y Y
Consequences of space-inversion and rotational invariance:Stationary states eigen states are also eigen states of
Radial (r) and angular ( , q f) degrees of freedom are independent Separate d.o.f in Schrödinger Equ. Product wave functions
r
U r
ˆ ˆˆ , zand L LH
, , ( , , ) ( ) ( , )n mn m r j r Y
Spherical Harmonics or (axial symmetry)Legendre Polynomials
r n=0
n=1
n=2
Ip
2+
1-
0+
En
Gam
ma-G
am
ma C
orr
ela
tion
s 1
3
Electromagnetic Nuclear Transitions
Conserved: Total energy (E), total angular momentum (I) and total parity (p):
222
.
( ) ( , )mi
Initial Nucl State
j r Y
Ip
2+
1-
0+
Ei
Ip
2+
1-
0+
Ef
i fi fi fE E E I I I
111
.
( ) ( , )mf
Final Nucl State
j r Y ( ) ( , )I
mE
Photon WF
r Y
Consider here only electric multipole transitions.Neglect weaker magnetic transitions due to changes in current distributions.
t-Dependent Electromagnetic Radiation Fields
Gam
ma-G
am
ma C
orr
ela
tion
s 1
4
Point Charges
NuclearCharge
Distribution
Monopole ℓ = 0
Dipole ℓ = 1
Quadrupole ℓ =2
Protons in nuclei = moving charges emits elm. radiation
Heinrich Hertz
Propagating Electric Dipole Field
E. Segré: Nuclei and Particles, Benjamin&Cummins, 2nd ed. 1977
Gam
ma-G
am
ma C
orr
ela
tion
s 1
5
Selection Rules for Electromagnetic Transitions
Conserved: Total energy (E), total angular momentum (I) and total parity (p):
i fi fi fE E E I I I
iiI
f
fI
iI
z
mi
mf
fI
mg
,
.
, ,
[ 1( )]
, 1 , 1
:
fi i
i f
i fi f
i f
i
f
i
i
f
Angular momenta I I
direction undetermined
Projections conserved
m m m m m
Electric dipole radiation
I
I I I m m
I
m
I I
Coupling of Angular Momenta
Quantization axis : z direction. Physical alignment of I possible (B field, angular correlation)
Gam
ma-G
am
ma C
orr
ela
tion
s 1
6
Spherical Harmonics P1|m|cos (m )f
z
x
yq
f
r
Plot Re Ylm P1
|m|cos (m )f
( , , ) 1, ( ), cos( )
sin( ) cos( )
sin( ) sin( )
cos( )
mLr r P m
x r
y r
z r
11y
10y
2 21 1
0 1
1/3 2 1/3
( ) ( 0) ( ) ( 1) ( )W P m Y P m Y
21 21
21 20
1( ) 1 cos
2
( ) sin
Y
Y
Emission in z direction
Emission perpend. to z
-g g Angular Correlations
Gam
ma-G
am
ma C
orr
ela
tion
s 1
7
Simple example: cascade 0 1 0Mostly Dm=±1 emitted in z-direction
0
I
1
0
1
2
0, 1
0
m
0
Det 1
Det 2
Q1=0
Q2
g1
g2
1 2 21 2 1 1
21211
2
( ) (0) ( )
( ) ( )
11 cos
2
m m
m
W W W
W Y
Det 1: Define z, select transition with maximum g intensity for q1=0.
Det 2: Measure emission patterns with respect to this z direction determine Dm.
22 2 21 2 0 0
22
( ) cos cos
1 cos ....
nn n n
n nW A P A
A
General Expression for - g g angular correlation
Typically: n ≤ 2. Legendre Polynomials Pn(cosq)
E2 -g g Angular Correlations
Gam
ma-G
am
ma C
orr
ela
tion
s 1
8
2 2
4
2 4
4 2 0
2
1 0.1020 cos 0.0091 cos
E ETheoretical
highest order P
W P P
Anisotropy
max0 0
201
(90 ) (180 ):
(180 )
n
nn
W WA A
W
Example: Rotational E2-g cascade, Dm=±2 maximally emitted in z-direction
After: G. Musiol, J. Ranft, R. Reif, D. Seeliger, Kern-u. Elementarteilchenphysik, VCH 1988