28
Alicia Mullins From: Sent: To: Subject: Attachments: Follow Up Flag: Flag Status: Timothy McCartin Wednesday, August 24, 2005 3:58 PM Bret Leslie; [email protected]; James Rubenstone Re: Inventory spreadsheet Inventoryl Myrs.XLS Follow up Flagged All: The attached file has some of my plot in addition to the calculation -,most should be easy to follow - call if you have questions. Sheet 1 has some general information that I used - and Sheet 3 has the actual calculations that are somewhat clear I hope >>> David Pickett <dpickettccnwra.swri.edu> 08/24/05 11:32 AM >>> Tim, At the team meeting, you offered to share your inventory spreadsheet. I'd sure like to see it. Thanks, David

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Alicia Mullins

From:Sent:To:Subject:Attachments:

Follow Up Flag:Flag Status:

Timothy McCartinWednesday, August 24, 2005 3:58 PMBret Leslie; [email protected]; James RubenstoneRe: Inventory spreadsheetInventoryl Myrs.XLS

Follow upFlagged

All:

The attached file has some of my plot in addition to the calculation -,most should be easy to follow - call if youhave questions. Sheet 1 has some general information that I used - and Sheet 3 has the actual calculationsthat are somewhat clear I hope

>>> David Pickett <dpickettccnwra.swri.edu> 08/24/05 11:32 AM >>>Tim,

At the team meeting, you offered to share your inventory spreadsheet.I'd sure like to see it.

Thanks,

David

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Date: Wed, 24 Aug 2005 15:57:50 -0400From: Timothy McCartin <[email protected]>Subject: Re: Inventory spreadsheetTo: Bret Leslie <[email protected]>,[email protected],James Rubenstone <[email protected]>

Message-id: <[email protected]>MIME-version: 1.0X-Mailer: Novell GroupWise Internet Agent 6.5.4Content-type: multipart/mixed; boundary="=_PartD8FA9A2E.0_="X-IronPort-AV: i="3.96,138,1122868800"; d="xls'32?scan'32,208,32";a="l 1915:sN HT1 62760030"

Original-recipient: rfc822;[email protected]

SolubilityLimits.xls Jan. 2005

Nuclide At. Mass Ci/MTU Ci/MTU Ci/ggrams at 10 yrs. at 1000 y

g/MTU "T-Half (yr) Sol. Limit Sol. Limit TPA5.0 DCF 100L @ SL 10k-4 Rel.

mrem/yrat 1000 y g/liter Pci/liter mr/yr/(pCi/l) - mrem/yr

Tc-991-129

Cm-246U-238

Cm-245Am-241Np-237

Am-243Pu-239

Pu-240

Pu-242

U-234Th-230Ra-226Pb-210

Cs-135

Ni-59

C-14

Se-79

CI-36

Nb-94

Pu-238

99 1.23E+01 1.43E+01 1.72E-02 8.31E+02129 2.95E-02 3.52E-02 1.73E-04 2.03E+02

246238

245241237

243239

240

242

234230226210

135

59

14

79

36

94

2.56E-02, 6.19E-023.19E-01 3.16E-01

1.25E-01 3.19E-011.64E+03 1.06E+032.87E-01 1.24E+00

1.54E+01 2.33E+013.08E+02 3.56E+02

5.08E+02 4.90E+02

2.06E+00

1.13E+00 2.52E+001.29E-04 2.1OE-023.67E-07 3.76E-034.72E-08 3.75E-03

3.51 E-01 5.26E-01

2.46E+00 2.40E+00

1.33E+00 1.26E+00

3.80E-01 4.48E-01

1.17E-02 1.13E-02

5.04E-01 8.19E-01

3.09E-013.34E-07

1.72E-013.45E+007.18E-04

1.99E-01

6.23E-02

2.29E-01

3.82E-03

6.37E-032.02E-029.89E-017.74E+01

1.15E-03

7.97E-02

4.48E+00

6.96E-02

3.31 E-02

1.90E-01

2.OOE-019.46E+05

1.86E+003.07E+021.73E+03

1.17E+025.71 E+03

2.14E+03

5.40E+02

3.96E+021.04E+003.80E-034.84E-05

4.57E+02

3.01 E+01

2.81 E-01

6.43E+00

3.41 E-01

4.31 E+00

2.1OE+051.60E+07

4.70E+034.50E+09

8.50E+034.30E+022.10E+06

7.40E+032.40E+04

6.50E+03

3.87E+05

2.40E+057.70E+041.60E+032.20E+01

2.30E+06

7.60E+04

5.70E+03

6.50E+04

3.OOE+05

2.OOE+04

9.90E+011.29E+02

2.40E-047.60E-03

2.40E-041.20E-042.10E-02

1.20E-041.20E-04

1.20E-04

1.20E-04

7.60E-032.30E-042.30E-056.60E-05

1.35E+02

1.10E-01

1.40E+01

7.90E+01

3.60E+01

9.30E-07

1.70E+122.23E+10

7.40E+072.53E+03

4.11E+074.13E+081.51 E+07

2.38E+077.46E+06

2.74E+07

4.57E+05

4.83E+074.63E+062.27E+075.1OE+09

1.55E+ 11

8.75E+09

6.26E+13

5.49E+12

1.19E+12

1.76E+05

0.201 1.21E+02 1.91E-031.07E-03 4.91E+01 4.14E-03

2.70.186

2.732.663.24

2.642.58

2.58

2.58E+00

0.2070.4

0.9673192

5.16E-03

1.53E-04

1.52E-03

6.35E-03

2.21E-03

5.21 E-03

5.40E+001.27E-05

3.03E+002.97E+011.32E+00

1.70E+005.20E-01

1.91 E+00

3.19E-02

2.70E-015.01 E-025.93E-015.40E+02

2.16E+01

3.62E-02

2.57E+03

9.42E+02

7.10E+01

2.49E-05

4.52E-021.59E-02

2.35E-017.62E+021.09E+00

1 .66E+012.48E+02

3.42E+02

1.44E+00

1.41 E-012.27E-039.83E-043.97E-03

7.34E-04

9.93E-05

5.18E-04

7.69E-04

6.75E-06

1.15E-03

Nuclide

Tc-991-129

Cm-246U-238

Cm-245Am-241Np-237

Am-243Pu-239

Pu-240

Pu-242

U-234Th-230Ra-226Pb-210

Cs-135

Ni-59

C-14

Se-79

CI-36

Nb-94

238 2.11E+03 1.97E+00 1.71E+01 1.15E-01 8.78E+01 1.20E-04 2.05E+09 2.34E+00 1.30E+02 1.25E+00 Pu-238

Radionulcide Inventory (relative to total inventory at specific times)

60

50

40

20

-I.

o 304-

0

0

10

IIPu

E3UM11Th

12 Tc 99

0 Np 237

1OOK 300K 500K 700K 1M

Time (years)

WlOKo3 50K13 1OOK

Radionulcide Inventory (relative to total inventory at specific times)

U)0•I-

U

100

90

80

70

60

50

40

30

20

10

0

83

93

54

43

0 Am 241

F Pu

DITc 99

* Np 237

10 0 0

1K

31 0 0

10K

Time (years)

11

26M-

2 05 4

50K 1OOK

Total Inventory (relative to inventory at 1,000 years)100

100 -r

80

U)

4-0

C.

60 1

40

26

20

62

0 !

1K 10K 50K 1OOK

Time (years)

Inventory at 1,000 Years

60

50

54

43

40 1

0

AD

CL

30 -

20 1

10 1

I0-

0 0

Pu Tc 99 U Np 237 Am 241

Inventory at 10,000 Years

100-93

70 -- _ __- _ __ _ _ -_ __ --- _ _ _ _ __ _ _ _ _ __ _ _ _ _ _

S60 _ _ _ _ _ _ _ _ _ _ _ _ _ _

40

30

20

10-.

a,3 0______0__

0

Pu Tc 99 U Np 237 Am 241

Inventory at 100,000 Years

6056

50+-

40

"C.

a.1

30 4---26

20

10

54

00 !

Pu Tc 99 U Np 237 Am 241

Inventory at 500,000 Years

40

35

30

25

0 20

IL

0

15

10-

37

17

1211

00 i

Pu Tc 99 u Np 237 Am 241

Inventory at I Million Years

40

35

30

34

25 4

0 20

10

15

17

15

11

00 !

Pu Tc 99 u Np 237 Am 241

Ci Inventory Inventory

Time1K10K50K

Time100K300K500K700K1M

Pu U Th Np 237 Tc 99

Pu U Th Np 237 Tc 9922.74542 2.209321 1.296452 1.413829 10.311.270967 1.378576 1.337341 1.32351 5.3299750.842986 0.912334 0.851305 1.238961 2.7544130.58904 0.65066 0.494425 1.159813 1.423419

0.344181 0.456672 0.210333 1.05E+00 0.528796

Time Pu1K10K50K

Time PU100K300K500K700K1M

43.393.482.7

56.411.011.511.911.3

U Th Np 237 Tc 99 Cs 1350.1 0.0 0.1 0.70.6 0.0 0.3 2.82.2 0.8 1.3 10.8

U Th Np 237 Tc 99. Cs 1355.5 3.2 3.5 25.6

11.9 11.5 11.4 45.912.4 11.6 16.9 37.513.2 10.0 23.5 28.915.0 6.9 34.4 17.3 1:

0.00.10.5

1.34.1

6.28.62.8

*Time1K10K50K100K300K500K700K1M

%i Overall Inventory

99.825.55.82.10.60.40.30.2

% Inventory

Time1K10K50K100K300K500K700K1M

Pu Tc 99 U Np 237 Am 24143.3 0.7 0.1 0.1 54.193.4 2.8 0.6 0.3 0.082.7 10.8 2.2 1.3 0.056.4 25.6 5.5 3.5 0.011.0 45.9 11.9 11.4 0.011.5 37.5 12.4 16.9 .0.011.9 28.9 13.2 23.5 0.011.3 17.3 15.0 34.4 0.0

Time1K10K50K1OOK300K500K700K1M

Time1K10K50K1OOK300K500K700K1M

Time1K10K50K1OOK300K500K700K1M

Time1K10K50K1OOK300K500K700K1M

Tc 990.72.8

10.825.645.937.528.917.3

U0.10.62.25.5

11.912.413.215.0

Np 2370.10.31.33.5

11.416.923.534.4

Am 24154.10.00.00.00.00.00.00.0

March 3,2005 Inventory _1 Myrs .XLS

1K as INPUT

Nuclide At. Mass T-Half (yr) lambdagrams (1/yr)

Tc-99 99 2.1OE+05 3.30E-061-129 129 1.60E+07 4.33E-08Cm-246(1) 246 4.70E+03 1.47E-04U-238(1) 238 4.50E+09 1.54E-10Cm-245(2) 245 8.50E+03 8.15E-05Am-241(2) 241 4.30E+02 1.61E-03Np-237(2) 237 2.10E+06 3.30E-07Am-243(3) 243 7.40E+03 9.37E-05Pu-239(3) 239 2.40E+04 2.89E-05Pu-240 240 6.50E+03 1.07E-04Pu-242 242 3.87E+05 1.79E-06U-234(4) 234 2.40E+05 2.89E-06Th-230(4) 230 7.70E+04 9.OOE-06Ra-226(4) 226 1.60E+03 4.33E-04Cs-135 135 2.30E+06 3.01E-07Ni-59 59 7.60E+04 9.12E-06C-14 14 5.70E+03 1.22E-04Se-79 79 6.50E+04 1.07E-05CI-36 36 3.OOE+05 2.31E-06Nb-94 94 2.OOE+04 3.47E-05TOTALS=

Ci/g

1.72E-021.73E-043.09E-013.34E-071.72E-01

3.45E+007.18E-041.99E-016.23E-022.29E-013.82E-036.37E-032.02E-029.89E-011.15E-037.97E-02

4.48E+006.96E-023.31 E-021.90E-01

g/MTUat 1000 y8.31 E+022.03E+022.OOE-019.46E+051.86E+003.07E+021.73E+031.17E+025.71 E+032.14E+035.40E+023.96E+021.04E+003.80E-03

4.57E+023.01 E+012.81E-016.43E+003.41 E-014.31 E+009.59E+05

Ci/MTUat 1000 y1.43E+013.52E-026.19E-023.16E-013.19E-011.06E+031.24E+002.33E+013.56E+024.90E+022.06E+002.52E+002.1OE-023.76E-035.26E-01

2.40E+001.26E+004.48E-011.13E-028.19E-011.96E+03

% of % ofTotal Totalat 1K yrs overall

0.73 0.730.00 0.000.00 0.000.02 0.020.02 0.02

54.08 54.080.06 0.061.19 1.19

18.16 18.1625.00 25.00

0.11 0.110.13 0.130.00 0.000.00 0.000.03 0.030.12 0.120.06 0.060.02 0.020.00 0.000.04 0.04

99.78 99.78

10 K as INPUT

Nuclide At. Massgrams

T-Half (yr) lambda Ci/g(1 /yr)

Tc-991-129Cm-246(1)U-238(1)Cm-245(2)Am-241(2)Np-237(2)Am-243(3)Pu-239(3)Pu-240Pu-242U-234(4)Th-230(4)Ra-226(4)Cs-1 35Ni-59C-14Se-79CI-36Nb-94TOTALS=

991292462382452412372432392402422342302261355914793694

2.10E+051.60E+074.70E+034.50E+098.50E+034.30E+022.10E+067.40E+032.40E+046.50E+033.87E+052.40E+057.70E+041.60E+032.30E+067.60E+045.70E+036.50E+043.OOE+052.OOE+04

3.30E-064.33E-081.47E-041.54E-108.15E-051.61 E-033.30E-079.37E-052.89E-051.07E-041.79E-062.89E-069.OOE-064.33E-043.01 E-079.12E-061.22E-041.07E-052.31 E-063.47E-05

1.72E-021.73E-043.09E-013.34E-071.72E-01

3.45E+007.18E-041.99E-016.23E-022.29E-013.82E-036.37E-032.02E-029.89E-011.15E-037.97E-02

4.48E+006.96E-023.31 E-021.90E-01

g/MTU Ci/MTUat 10K y at 10K y8.07E+02 1.39E+012.03E+02 3.52E-025.31 E-02 1.64E-029.46E+05 3.16E-018.92E-01 1.53E-014.77E-02 1.64E-012.03E+03 1.46E+005.04E+01 1.OOE+014.46E+03 2.78E+028.19E+02 1.88E+025.31E+02 2.03E+003.86E+02 2.46E+001.07E+01 2.16E-012100E-02 1.98E-02

4.55E+02 5.25E-012.77E+01 2.21E+009.41E-02 4.22E-015.84E+00 4.07E-013.34E-01 1.11E-023.15E+00 6.OOE-019.56E+05 5.01E+02

% ofTotalat 10K yrs

2.770.010.000.060.030.030.292.00

55.5137.460.400.490.040.000.100.440.080.080.000.12

99.94

% ofTotaloverall

0.710.000.000.020.010.010.070.51

14.199.570.100.130.010.000.030.110.020.020.000.03

25.55

50 K as INPUT

Nuclide At. Massgrams

Tc-991-129Cm-246(1)U-238(1)Cm-245(2)Am-241(2)Np-237(2)Am-243(3)Pu-239(3)Pu-240Pu-242U-234(4)Th-230(4)Ra-226(4)Cs-1 35Ni-59C-14Se-79CI-36Nb-94TOTALS=

99129246238

245241237243239240242234230226135

5914793694

T-Half (yr) lambda(1/yr)

2.1OE+05 3.30E-061.60E+07 4.33E-084.70E+03 1.47E-044.50E+09 1.54E-108.50E+03 8.15E-054.30E+02 1.61E-032.1OE+06 3.30E-077.40E+03 9.37E-052.40E+04 2.89E-056.50E+03. 1.07E-043.87E+05 1.79E-062.40E+05 2.89E-067.70E+04 9.00E-061.60E+03 4.33E-042.30E+06 3.01E-077.60E+04 9.12E-065.70E+03 1.22E-046.50E+04 1.07E-053.00E+05 2.31E-062.00E+04 3.47E-05

Ci/g

1.72E-021.73E-043.09E-013.34E-071.72E-01

3.45E+007.18E-041.99E-016.23E-022.29E-013.82E-036.37E-032.02E-029.89E-011.15E-037.97E-02

4.48E+006.96E-023.31 E-021.90E-01

% of % ofg/MTU Ci/MTU Total Totalat 50K y at 50K y at 50K yrs overall

7.07E+022.03E+021.46E-04

9.46E+053.42E-021.82E-03

2.OOE+031.19E+001.43E+031.15E+014.94E+023.44E+024.27E+011 .59E-01

4.50E+021.92E+017.26E-04

3.82E+003.05E-017.88E-01

9.52E+05

1.22E+013.51 E-024.50E-053.16E-015.87E-036.28E-031.44E+002.37E-01

8.89E+012.64E+001.89E+002.19E+008.62E-011.57E-015.18E-011.54E+003.26E-032.66E-011.01 E-021.50E-011.13E+02

10.770.030.000.280.010.011.270.21

78.692.331.671.940.7601140.461.360.000.240.010.13

100.30

0.620.000.000.020.000.000.070.014.540.130.100.110.040.010.030.080.000.010.000.015.78

100 K as INPUT

% ofg/MTU Ci/MTU Total

% ofTotalNuclide At. Mass

gramsT-Half (yr) lambda Ci/g

(1/yr)

Tc-991-129Cm-246(1)U-238(l)Cm-245(2)Am-241 (2)Np-237(2)Am-243(3)Pu-239(3)Pu-240Pu-242U-234(4)Th-230(4)Ra-226(4)Cs-1 35Ni-59C-1 4Se-79CI-36Nb-94TOTALS=

99129246238245241237243239240242234230226135

5914793694

2.1OE+051.60E+074.70E+034.50E+098.50E+034.30E+022.1OE+067.40E+032.40E+046.50E+033.87E+052.40E+057.70E+041.60E+032.30E+067.60E+045.70E+036.50E+043.OOE+052.OOE+04

3.30E-064.33E-081.47E-041.54E-108.15E-051.61 E-033.30E-079.37E-052.89E-051.07E-041.79E-062.89E-069.OOE-064.33E-043.01E-079.12E-061.22E-041.07E-052.31 E-063.47E-05'

1.72E-021.73E-043.09E-013.34E-071.72E-,01

3.45E+007.18E-041.99E-016.23E-022.29E-013.82E-036.37E-032.02E-029.89E-011.15E-037.97E-024.48E+006.96E-023.31 E-021.90E-01

at 100K y at 100K y at 100K yrs overall

6.OOE+02 1.03E+01 25.592.02E+02 3.50E-02 0.099.13E-08 2.82E-08 0.00

9.46E+05 3.16E-01 0.785.79E-04 9.95E-05 0.003.09E-05 1.07E704 0.001.97E+03 1.41 E+00 3.511.10E-02 2.19E-03 0.01

3.37E+02 2.10E+01 52.135.56E-02 1.27E-02 0.03

4.52E+02 1.73E+00 4.282.97E+02 1.89E+00 4.706.42E+01 1.30E+00 3.225.77E-01 5.71E-01 1.42

4.43E+02 5.11E-01 1.271.22E+01 9.73E-01 2.411.66E-06 7.45E-06. 0.00

2.24E+00 1.56E-01 0.392.72E-01 8.99E-03 0.021.39E-01 2.65E-02 0.07

9.51E+05 4.03E+01 99.91

0.530.000.000.020.000.000.070.001.070.000.090.100.070.030.030.050.000.010.000.002.05

300 K as INPUT

% ofg/MTU Ci/MTU Total

% ofTotalNuclide At. Mass

gramsTc-991-129Cm-246(1)U-238(1)Cm-245(2)Am-241(2)Np-237(2)Am-243(3)Pu-239(3)Pu-240Pu-242U-234(4)Th-230(4)Ra-226(4)Cs-1 35Ni-59C-14Se-79CI-36Nb-94TOTALS=

99129246238245241237243239240242234230226135

5914793694

T-Half (yr) lambda(1/yr)

2.1OE+05 3.30E-061.60E+07 4.33E-084.70E+03 1.47E-044.50E+09 1.54E-108.50E+03 8.15E-054.30E+02 1.61E-032.1OE+06 3.30E-077.40E+03 9.37E-052.40E+04 2.89E-056.50E+03 1.07E-043.87E+05 1.79E-062.40E+05 2.89E-067.70E+04 9.OOE-061.60E+03. 4.33E-042.30E+06 3.01E-077.60E+04 9.12E-065.70E+03 1.22E-046.50E+04 1.07E-053.OOE+05 2.31E-062.OOE+04 3.47E-05

1.72E-021.73E-043.09E-013.34E-071.72E-01

3.45E+007.18E-04S1.99E-01

6.23E-022.29E-013.82E-036.37E-032.02E-029.89E-011.15E-037.97E-02

4.48E+006.96E-023.31 E-021.90E-01

Ci/gat 300K y at 300K y

3.1OE+02 5.33E+002.01E+02 3.47E-021.41 E-20 4.38E-21

9.46E+05 3.16E-014.78E-11 8.21E-122.55E-12 8.80E-121.84E+03 1.32E+008.05E-1 1 1.60E-1 11.04E+00 6.51E-023.04E-11 6.96E-123.16E+02 1.21E+001.67E+02 1.06E+006.62E+01 1.34E+002.25E-01 2.23E-01

4.17E+02 4.81E-011.97E+00 1.57E-014.55E-17 2.04E-162.65E-01 1.85E-021.71 E-01 5.66E-031.36E-04 2.59E-05

9.50E+05 1.16E+01

at 300K yrs overall45.950.300.002.720.000.00

11.410.000.560.00

10.409.16

11.531.924.141.350.000.160.050.00

99.65

0.270.000.000.020.000.000.070.000.000.000.060.050.070.010.020.010.000.000.000.000.59

500 K as INPUT

% ofg/MTU Ci/MTU Total

% ofTotalNuclide At. Mass

gramsT-Half (yr) lambda Ci/g

Tc-991-129Cm-246(1)U-238(l)Cm-245(2)Am-241 (2)Np-237(2)Am-243(3)Pu-239(3)Pu-240Pu-242U-234(4)Th-230(4)Ra-226(4)Cs-1 35Ni-59C-1 4Se-79CI-36Nb-94TOTALS=

99129246238245241237243239240242234230226135

5914793694

2.1OE+051.60E+074.70E+034.50E+09

-8.50E+034.30E+022.1OE+067.40E+032.40E+046.50E+033.87E+052.40E+057.70E+041.60E+032.30E+067.60E+045.70E+036.50E+043.OOE+052.OOE+04

(l/yr)3.30E-064.33E-081.47E-041.54E-108.15E-051.61 E-033.30E-079.37E-052.89E-051.07E-041.79E-062.89E-069.00E-064.33E-043.01 E-079.12E-061.22E-041.07E-052.31 E-063.47E-05

1.72E-021.73E-043.09E-013.34E-071.72E-01

3.45E+007.18E-041.99E-016.23E-022.29E-013.82E-036.37E-032.02E-029.89E-011.15E-037.97E-02

4.48E+006.96E-023.31 E-021.90E-01

at 500K y at 500K y1.60E+02 2.75E+001.99E+02 3.44E-022.19E-33 6.78E-349.46E+05 3.16E-013.95E-18 6.78E-192.11E-19 7.26E-191.72E+03 1.24E+005.88E-19 1.17E-193.24E-03 2.02E-041.66E-20 3.80E-21

2.21E+02 8.43E-019.37E+01 5.96E-014.22E+01 8.51 E-012.32E-01 2.30E-013.93E+02 4.53E-013.18E-01 2.53E-021.25E-27 5.58E-273.14E-02 2.19E-031.08E-01 3.57E-031.33E-07 2.53E-08

9.49E+05 7.35E+00

at 500K yrs overall37.480.470.004.300.000.00

16.860.000.000.00

11.478.11

11.583.126.160.340.000.030.050.00

99.97

0.140.000.000.020.000.000.060.000.000.000.040.030.040.010.020.000.000.000.000.000.37

700 K as INPUT

Nuclide At. Massgrams

Tc-991-129Cm-246(1)U-238(1)Cm-245(2)Am-241 (2)Np-237(2)Am-243(3)Pu-239(3)Pu-240Pu-242U-234(4)Th-230(4)Ra-226(4)Cs-1 35Ni-59C-1 4Se-79CI-36Nb-94TOTALS=

99129246238245241237'243239240242234230226135

5914793694

T-Half (yr) lambda(1/yr)

2.1OE+05 3.30E-061.60E+07 4.33E-084.70E+03 1.47E-044.50E+09 1.54E-108.50E+03 8.15E-054.30E+02 1.61 E-032.10E+06 3.30E-077.40E+03 9.37E-052.40E+04 2.89E-056.50E+03 1.07E-043.87E+05 1.79E-062.40E+05 2.89E-067.70E+04 9.OOE-061.60E+03 4.33E-042.30E+06 3.01E-077.60E+04 9.12E-065.70E+03 1.22E-046.50E+04 1.07E-053.00E+05 2.31E-062.00E+04 3.47E-05

Ci/g

1.72E-021.73E-043.09E-0i3.34E-071.72E-013.45E+007.18E-041.99E-016.23E-022.29E-013.82E-036.37E-032.02E-029.89E-011.15E-037.97E-024.48E+006.96E-023.31 E-021.90E-01

g/MTU Ci/MTUat 700K y at 700K y

8.28E+01 1.42E+001.97E+02 3.42E-023.40E-46 1.05E-46

9.46E+05 3.16E-013.26E-25 5.60E-261.74E-26 6.00E-261.61E+03 1.16E+004.30E-27 8.55E-281.00E-05 6.26E-079.07E-30 2.08E-301.54E+02 5.89E-015.26E+01 3;35E-012.45E+01 4.94E-011.48E-01 1.46E-01

3.70E+02 4.26E-015.13E-02 4.09E-033.41E-38 1.53E-373.73E-03 2.59E-046.79E-02 2.25E-031.30E-10 2.47E-11

9.49E+05 4.93E+00

% ofTotalat 700K yrs

28.870.690.006.410.000.00

23.530.000.000.00

11.956.79

10.032.978.640.080.000.010.050.00

100.01

% ofTotaloverall

0.070.000.000.020.000o000.060.000.000.000.030.020.030.010.020.000.000.000.000.000.25

10K as OUTPUT

lk to 10k totalDecay Prod. gm/MTU

total % ofCi/MTU Total

% ofTotalNuclide g/MTU

Tc-991-129Cm-246(1)

2.84E+00 U-238(1)0.14 Cm-245(2)

Am-241(2)Np-237(2)Am-243(3)

8.48E+02 Pu-239(3)43.27 Pu-240

Pu-242U-234(4)Th-230(4)Ra-226(4)Cs-1 35Ni-59C-14Se-79CI-36Nb-94

at 10K yr gm

8.07E+02 0.2.03E+02 0.5.31E-02 0.

9.46E+05 18.92E-01 0.1.54E-04 41.72E+03 3.5.04E+01 0.4.40E+03 5.8.19E+02 0.5.31E+02 0.3.86E+02 0.9.59E-01 9.7.70E-05 1

4.55E+02 0.2.77E+01 0.9.41 E-02 0.5.84E+00 0.3.34E-01 0.3.15E+00 0.

at 10k yr at 1Okyr at 1Okyr Overall

OOE+00OOE+00OOE+00.47E-01OOE+00.75E-0206E+02OOE+0077E+01OOE+00OOE+00OOE+0075E+00.99E-02OOE+00OOE+00OOE+00OOE+00OOE+00OOE+00

8.07E+022.03E+025.31 E-029.46E+058.92E-014.77E-022.03E+035.04E+014.46E+038.19E+02-5.31 E+023.86E+021.07E+012.OOE-024.55E+022.77E+019.41 E-025.84E+003.34E-013.15E+009.56E+05

1.39E+013.52E-021.64E-023.16E-011.53E-011.64E-01

1.46E+001.OOE+012.78E+021.88E+022.03E+002.46E+002.16E-011.98E-025.25E-012.21 E+004.22E-014.07E-011.11E-026.OOE-015.01 E+02

2.750.010.000.060.030.030.291.99

55.0737.160.400.490.040.000.100.440.080.080.000.12

99.15

0.710.000.000.020.010.010.070.51

14.199.570.100.130.010.000.030.110.020.020.000.03

25.55

50K as OUTPUT

Decay

Nuclide g/MTU1Ok to 50k total totalDecay Prod. gm/MTU Ci/MTU

Tc-991-129Cm-246(1)

2.77E+00 U-238(1)0.55 Cm-245(2)

Am-241(2)Np-237(2)Am-243(3)

4.68E+02 Pu-239(3)93.37 Pu-240

Pu-242U-234(4)Th-230(4)Ra-226(4)Cs-1 35Ni-59C-14Se-79CI-36Nb-94

to 50K yr gm

7.07E+02 0.'2.03E+02 0.'1.46E-04 0.'

9.46E+05 53.42E-02 0.'4.74E-30 12.00E+03 41.19E+00 0.'1.41E+03 2.1.15E+01 0.'4.94E+02 0.'3.44E+02 0.'7.47E+00 3.5.95E-10 14.50E+02 0.'1.92E+01 0.'7.26E-04 0.3.82E+00 0.'3.05E-01 0.'7.88E-01 0.'

0OE+00OOE+0000E+00.29E-020OE+00.82E-03.71 E-020OE+0012E+0100E+000OE+000OE+0052E+01.59E-010OE+000OE+000OE+0000E+000OE+000OE+00

at 50k yr

7.07E+022.03E+021.46E-04

9.46E+053.42E-021.82E-03

2.OOE+031.19E+001.43E+031.15E+014.94E+023.44E+024.27E+011.59E-01

4.50E+021.92E+017.26E-043.82E+003.05E-017.88E-01

9.52E+05

at 50kyr

1.22E+013.51 E-024.50E-053.16E-015.87E-036.28E-031.44E+002.37E-01

8.89E+012.64E+001.89E+002.19E+008.62E-011.57E-0-1.5.18E-011.54E+003.26E-032.66E-011.01 E-021.50E-011.13E+02

% ofTotal

at 50kyr

10.770.030.000.280.010.011.270.21

78.692.331.671.940.760.140.461.360.000.240.010.13

100.30

% ofTotal

Overall

0.620.000.000.020.000.000.070.014.540.130.100.110.040.010.030.080.000.010.000.015.78

100K as OUTPUT

Decay 50k to 100k totalNuclide g/MTU Decay Prod. gm/MTU

total % ofCi/MTU Total

% ofTotal

to 100K yr

Tc-99 6.OOE+021-129 2.02E+02Cm-246(1) 9.13E-08

2.50E+00 U-238(1) 9.46E+052.22 Cm-245(2) 5.79E-04

Am-241(2) 1.81 E-38Np-237(2) 1.97E+03Am-243(3) 1.10E-02

9.34E+01 Pu-239(3) 3.37E+0282.70 Pu-240 5.56E-02

Pu-242 4.52E+02U-234(4) 2.97E+02Th-230(4) 2.72E+01Ra-226(4) 6.21 E-1 1Cs-1 35 4.43E+02Ni-59 1.22E+01C-14 1.66E-06Se-79 2.24E+00CI-36 2.72E-01Nb-94 1.39E-01

gm

0.OOE+000.OOE+000.OOE+001.45E-04

0.00E+003.09E-051.79E-03

O.OOE+003.90E-010.00E+000.OOE+000.00E+003.70E+015.77E-010.OOE+000.OOE+000.OOE+000.00E+000.OOE+000.00E+00

at 100k yr at 100kyr

6.OOE+022.02E+029.13E-089.46E+055.79E-043.09E-051.97E+031.10E-023.37E+025.56E-02

4.52E+022.97E+026.42E+015.77E-01

4.43E+021.22E+011.66E-062.24E+002.72E-011.39E-019.51 E+05

1.03E+013.50E-022.82E-083.16E-019.95E-051.07E-041.41 E+002.19E-03

2.10E+011.27E-021.73E+001.89E+001.30E+005.71iE-015.11E-019.73E-017.45E-061.56E-018.99E-032.65E-02

4.03E+01

at 100kyr Overall

25.59 0.530.09 0.000.00 0.000.78 0.020.00 0.000.00 0.003.51 0.070.01 0.00

52.13 1.070.03 0.004.28 '0.094.70 0.103.22 0.071.42 0.031.27 0.032.41 0.050.00 0.000.39 0.010.02 0.000.07 0.00

99.91 2.05

300K as' OUTPUT

Ci% Decay 100k to 300k total total % of % ofSubtotals Nuclide g/MTU Decay Prod. gm/MTU Ci/MTU Total Total

to 300K yr 6m at 300k yr at 300kyr at 300kyr Overall

Tc-99 3.1OE+02 O.OOE+00 3.1OE+02 5.33E+00 45.95 0.271-129 2.01E+02 0.OOE+00 2.01E+02 3.47E-02 0.30 0.00Cm-246(1) 1.41E-20 0.OOE+00 1.41E-20 4.38E-21 0.00 0.00

2.21 U-238(1) 9.46E+05 9.13E-08 9.46E+05 3.16E-01 2.72 0.02 1.385.48 Cm-245(2) 4.78E-11 0.OOE+00 4.78E-11 8.21E-12 0.00 0.00 11.88

Am-241(2) 2.99E-145 2.55E-12 2.55E-12 8.80E-12 0.00 0.00Np-237(2) 1.84E+03 2.89E-05 1.84E+03 1.32E+00 11.41 0.07Am-243(3) 8.05E-11 0.OOE+00 8.05E-11 1.60E-11 0.00 0.00

22.75 Pu-239(3) 1.04E+00 4.93E-05 1.04E+00 6.51E-02 0.56 0.00 1.2756.44 Pu-240 3.04E-11 0.OOE+00 3.04E-11 6.96E-12 0.00 0.00 10.96

Pu-242 3.16E+02 0.OOE+00 3.16E+02 1.21E+00 10.40 0.06U-234(4) 1.67E+02 0.OOE+00 1.67E+02 1.06E+00 9.16 0.05Th-230(4) 1.06E+01 5.56E+01 6.62E+01 1.34E+00 11.53 0.07Ra-226(4) 1.36E-38 2.25E-01 2.25E-01 2.23E-01 1.92 0.01Cs-135 4.17E+02 0.OOE+00 4.17E+02 4.81E-01 4.14 0.02Ni-59 1.97E+00 0.OOE+00 1.97E+00 1.57E-01 1.35 0.01C-14 4.55E-17 0.OOE+00 4.55E-17 2.04E-16 0.00 0.00Se-79 2.65E-01 0.OOE+00 2.65E-01 1.85E-02 0.16 0.00CI-36 1.71E-01 0.OOE+00 1.71E-01 5.66E-03 0.05 0.00Nb-94 1.36E-04 0.OOE+00 1.36E-04 2.59E-05 0.00 0.00

9.50E+05 1.16E+01 99.65 0.59

500K as OUTPUT

Decay 300k to 500k total total % of % ofNuclide g/MTU Decay Prod. gm/MTU Ci/MTU Total Total

to 500K yr gm at 500k yr at 500kyr at 500kyr Overall:

Tc-99 1.60E+02 0.OOE+00 1.60E+02 2.75E+00 37.48 0.141-129 1.99E+02 O.OOE+00 1.99E+02 3.44E-02 .0.47 0.00Cm-246(1) 2.19E-33 0.OOE+00 2.19E-33 6.78E-34 0.00 0.00U-238(1) 9.46E+05 1.41E-20 9.46E+05 3.16E-01 4.30 0.02Cm-245(2) 3.95E-18, 0.OOE+00 3.95E-18 6.78E-19 0.00 0.00Am-241(2) 2.47E-152 2.11E-19 2.11E-19 7.26E-19 0.00 0.00Np-237(2) 1.72E+03 2.39E-12 1.72E+03 1.24E+00 16.86 0.06Am-243(3) 5.88E-19 0.OOE+00 5.88E-19 1.17E-19 0.00 0.00Pu-239(3) 3.24E-03 3.61E-13 3.24E-03 2.02E-04 0.00 0.00Pu-240 1.66E-20 0.OOE+00 1.66E-20 3.80E-21 0.00 0.00Pu-242 2.21E+02 0.OOE+00 2.21E+02 8.43E-01 11.47 0.04U-234(4) 9.37E+01 0.OOE+00 9.37E+01 5.96E-01 8.11 0.03Th-230(4) 1.09E+01 3.12E+01 4.22E+01 8.51E-01 11.58 0.04Ra-226(4) 5.29E-39 2.32E-01 2.32E-01 2.30E-01 3.12 0.01Cs-135 3.93E+02 0.OOE+00 3.93E+02 4.53E-01 6.16 0.02Ni-59 3.18E-01 0.OOE+00 3.18E-01 2.53E-02 0.34 0.00C-14 1.25E-27 0.OOE+00 1.25E-27 5.58E-27 0.00 0.00Se-79 3.14E-02 0.OOE+00 3.14E-02 2.19E-03 0.03 0.00CI-36 1.08E-01 0.OOE+00 1.08E-01 3.57E-03 0.05 0.00Nb-94 1.33E-07 0.OOE+00 1.33E-07 2.53E-08 0.00 0.00

9.49E+05 7.35E+00 99.97 0.37

700K as OUTPUT

Ci% Decay 500k to 700k totalSubtotal. Nuclide g/MTU Decay Prod. gm/MTU

total % ofCi/MTU Total

to 700K yr gm

Tc-99 8.28E+01 0.00E+001-129 1.97E+02 0.00E+00Cm-246(1) 3.40E-46 0.00E+00

9.12E-01 U-238(1) 9.46E+05 2.19E-3312.41 Cm-245(2) 3.26E-25 0.OOE+00

Am-241(2) 2.04E-159 1.74E-26Np-237(2) 1.61 E+03 1.97E-1 9Am-243(3) 4.30E-27 0.OOE+00

8.43E-01 Pu-239(3) 1.OOE-05 2.64E-2111.47 Pu-240 9.07E-30 0.OOE+00

Pu-242 1.54E+02 0.OOE+00U-234(4) 5.26E+01 0.OOE+00Th-230(4) 6.97E+00 1.75E+01Ra-226(4) 5.46E-39 1.48E-01Cs-135 , 3.70E+02 0.OOE+00Ni-59 5.13E-02 0.OOE+00C-14 3.41E-38 0.OOE+00Se-79 3.73E-03 0.OOE+00CI-36 6.79E-02 0.OOE+00Nb-94 1.30E-10 0.OOE+00

at 700k yr

8.28E+011.97E+023.40E-469.46E+053.26E-251.74E-26

1.61 E+034.30E-271.O0E-059.07E-301.54E+025.26E+012.45E+011.48E-01

3.70E+025.13E-023.41 E-383.73E-036.79E-021.30E-10

9.49E+05

at 700kyr

1.42E+003.42E-021.05E-463.16E-015.60E-266.OOE-261.16E+008.55E-286.26E-072.08E-305.89E-013.35E-014.94E-011.46E-014.26E-014.09E-031.53E-372.59E-042.25E-032.47E-1 1

4.93E+00

at 700kyr

28.870.690.OQ6.410.000.00

23.530.000.000.00

11.95

6.7910.032.978.640.080.000.010.050.00

100.01

% ofTotal

Overall

0.070.000.000.02 6.51E-010.00 13.200.000.060.000.00 5.89E-010.00 11.950.030.020.030.010.020.000.000.000.000.000.25

IM as OUTPUT

Ci

SubtotalDecay 700k to 1 M total

Nuclide g/MTU Decay Prod. gm/MTU

total % of % ofTotalCi/MTU Total

L

P

Tc-991-129Cm-246(1)

6.51E-01 U-238(1)13.20 Cm-245(2)

Am-241(2)Np-237(2)

•u Am-243(3)5.89E-0. Pu-239(3)

11.95 Pu-240Pu-242U-234(4)Th-230(4)Ra-226(4)Cs-1 35Ni-59C-1 4Se-79CI-36Nb-94

to 1M yr gm at 1M yr at 1M yr

3.07E+01 0.00E+00 3.07E+01 5.29E-011.95E+02 0.00E+00 1.95E+02 3.37E-022.07E-65 0.OOE+00 2.07E-65 6.41 E-669.46E+05 3.40E-46 9.46E+05 3.16E-017.74E-36 O.00E+00 7.74E-36 1.33E-36

1.65E-236 4.13E-37 4.13E-37 1.42E-361.46E+03 1.58E-26 1.46E+03 1.05E+002.69E-39 0.00E+00 2.69E-39 5.35E-401.73E-09 1.07E-30 1.73E-09 1.08E-1 01 .1 6E-43 0.OOE+00 1.16E-43 2.65E-44

9.01E+01 0.OOE+00 9.01E+01 3.44E-012.21 E+01 0.00E+00 2.21 E+01 1.41 E-011.64E+00 8.77E+00 1.04E+01 2.1OE-015.33E-58 3.49E-02 3.49E-02 .3.45E-023.38E+02 0.00E+00 3.38E+02 3.89E-013.32E-03 0.00E+00 3.32E-03 2.65E-044.89E-54 0.00E+00 4.89E-54 2.19E-531.52E-04 0.00E+00 1.52E-04 1.06E-053.39E-02 0.00E+00 3.39E-02 1.12E-033.96E-15 0.OOE+00 3.96E-15 7.53E-16

9.48E+05 3.05E+00

at 1M yr Overall

17.34 0.031.11 0.000.00 0.00

10.36 0.020.00 0.000.00 0.00

34.44 0.050.00 0.000.00 0.000.00 0.00

11.28 0.024.61 0.016.90 0.011.13 0.00,

12.76 0.020.01 0.000.00 0.000.00 0.000.04 0.000.00 0.00

99.98 0.16

U4.57E-01

14.97

Pu3.44E-01

11.28