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Aerosol and Air Quality Research, 16: 2950–2963, 2016 Copyright © Taiwan Association for Aerosol Research ISSN: 1680-8584 print / 2071-1409 online doi: 10.4209/aaqr.2015.07.0461 Numerical Study of the Transport and Convective Mechanisms of Biomass Burning Haze in South-Southeast Asia Muhammad Yaasiin Oozeer 1* , Andy Chan 1 , Maggie Chel-Gee Ooi 1 , Antonio Maurício Zarzur 2 , Santo Valentin Salinas 3 , Boon-Ning Chew 3 , Kenobi Isima Morris 1 , Wee-Kang Choong 1 1 Faculty of Engineering, University of Nottingham Malaysia Campus, Semenyih, Selangor, Malaysia 2 Associate Laboratory for Computing and Applied Mathematics, National Institute for Space Research, São José dos Campos, São Paulo, Brazil 3 Centre for Remote Imaging, Sensing and Processing (CRISP), National University of Singapore, 119076, Singapore ABSTRACT This study aims to identify the vertical transport mechanisms that uplifted the forest fire emissions from Sumatra to the upper troposphere during the June 2013 haze crisis. WRF-Chem is used to simulate the formation and transport of biomass-burning haze during the study period of 18 th to 26 th June 2013. The South-Southeast Asian synoptic weather patterns and their effects on the transport of biomass-burning emissions from Sumatra to Peninsular Malaysia were studied computationally to explain the phenomenon. Results show that PM 10 emissions were lifted to 200 hPa height (approximately 12 km) over the Strait of Malacca on 24 th June. The two identified vertical transport mechanisms confirmed a previously conjectured convergence over the Strait of Malacca and orographic lifting over Peninsular Malaysia. These mechanisms were able to uplift the biomass-burning emissions to the upper troposphere and this could have significant long-range transport and global climatic effects. Keywords: WRF-Chem; Southeast Asia; Biomass burning; Vertical transport mechanism; Deep convection. INTRODUCTION Biomass burning is a prominent recurrence in Southeast Asia (SEA). Intense forest fires have often been the result of intentional bush-burning that aims to clear the land for agricultural purposes (Quah and Johnston, 2001). In some regions of Indonesia such as Southwest Kalimantan and Southeast Sumatra, where fire prone peat swamp forests exist, extensive forest fires have occurred during the dry Southwest monsoon season (May–October) of 1994 and 1997 (Nichol, 1997, 1998). 1994 and 1997 were both El-Nino Southern Oscillation (ENSO) years and the intensification of the dry conditions over Indonesia has been an important contributing factor to the strong forest fires which occurred during that time (Heil and Goldammer, 2001). Biomass burning has been reported to be a significant source of ozone precursor gases such as nitric oxide (NO), carbon monoxide (CO) and hydrocarbons (Crutzen et al., 1985). In SEA, biomass-burning haze (BBH) has been identified as an important source of tropospheric ozone * Corresponding author. Tel.: +60122747617 E-mail address: [email protected] (Fujiwara et al., 1999; Liu et al., 1999; Chan et al., 2000, 2003) while aerosols from such burning have been found to contribute largely to ‘Atmospheric Brown Clouds’ (Ramanathan and Crutzen, 2003). More importantly, BBH reduces air quality and imposes a very negative effect on human health (Dawud, 1998; Aditama, 2000; Kunii et al., 2002; Wiwanitkit, 2008; Hyer and Chew, 2010; Kim Oanh et al., 2011). Quah (2002) reviewed the issues and policy responses to the severe damage of BBH on the regional environment and the economy during the 1997 episode and has highlighted the need for prompt and effective measures in face of the biomass burning problem. Therefore the impact of BBH over SEA on the atmospheric environment, economy and general well-being cannot be overstated and is receiving more and more attention, not only regionally but globally. One of the most important phenomena in large-scale haze is deep convection (Lin et al., 2009). This is the most frequently mentioned mechanism for the transport of biomass-burning products up in the troposphere. Deep convection is able to carry biomass air pollutants to higher altitudes over SEA and is a leading candidate to explain climate change in context (Folkins et al., 1997; Chan et al., 2003). A strong convection mechanism responsible for the uplifting of biomass-burning emissions over Indonesia, New Guinea and Malaysia has also previously been at the center of discussions (Folkins et al., 1997). Lin et al. (2009)

Numerical Study of the Transport and Convective …...2002; Wiwanitkit, 2008; Hyer and Chew, 2010; Kim Oanh et al., 2011). Quah (2002) reviewed the issues and policy responses to the

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  • Aerosol and Air Quality Research, 16: 2950–2963, 2016 Copyright © Taiwan Association for Aerosol Research ISSN: 1680-8584 print / 2071-1409 online doi: 10.4209/aaqr.2015.07.0461

    Numerical Study of the Transport and Convective Mechanisms of Biomass Burning Haze in South-Southeast Asia Muhammad Yaasiin Oozeer1*, Andy Chan1, Maggie Chel-Gee Ooi1, Antonio Maurício Zarzur2, Santo Valentin Salinas3, Boon-Ning Chew3, Kenobi Isima Morris1, Wee-Kang Choong1 1 Faculty of Engineering, University of Nottingham Malaysia Campus, Semenyih, Selangor, Malaysia 2 Associate Laboratory for Computing and Applied Mathematics, National Institute for Space Research, São José dos Campos, São Paulo, Brazil 3 Centre for Remote Imaging, Sensing and Processing (CRISP), National University of Singapore, 119076, Singapore ABSTRACT

    This study aims to identify the vertical transport mechanisms that uplifted the forest fire emissions from Sumatra to the upper troposphere during the June 2013 haze crisis. WRF-Chem is used to simulate the formation and transport of biomass-burning haze during the study period of 18th to 26th June 2013. The South-Southeast Asian synoptic weather patterns and their effects on the transport of biomass-burning emissions from Sumatra to Peninsular Malaysia were studied computationally to explain the phenomenon. Results show that PM10 emissions were lifted to 200 hPa height (approximately 12 km) over the Strait of Malacca on 24th June. The two identified vertical transport mechanisms confirmed a previously conjectured convergence over the Strait of Malacca and orographic lifting over Peninsular Malaysia. These mechanisms were able to uplift the biomass-burning emissions to the upper troposphere and this could have significant long-range transport and global climatic effects. Keywords: WRF-Chem; Southeast Asia; Biomass burning; Vertical transport mechanism; Deep convection. INTRODUCTION

    Biomass burning is a prominent recurrence in Southeast Asia (SEA). Intense forest fires have often been the result of intentional bush-burning that aims to clear the land for agricultural purposes (Quah and Johnston, 2001). In some regions of Indonesia such as Southwest Kalimantan and Southeast Sumatra, where fire prone peat swamp forests exist, extensive forest fires have occurred during the dry Southwest monsoon season (May–October) of 1994 and 1997 (Nichol, 1997, 1998). 1994 and 1997 were both El-Nino Southern Oscillation (ENSO) years and the intensification of the dry conditions over Indonesia has been an important contributing factor to the strong forest fires which occurred during that time (Heil and Goldammer, 2001).

    Biomass burning has been reported to be a significant source of ozone precursor gases such as nitric oxide (NO), carbon monoxide (CO) and hydrocarbons (Crutzen et al., 1985). In SEA, biomass-burning haze (BBH) has been identified as an important source of tropospheric ozone * Corresponding author.

    Tel.: +60122747617 E-mail address: [email protected]

    (Fujiwara et al., 1999; Liu et al., 1999; Chan et al., 2000, 2003) while aerosols from such burning have been found to contribute largely to ‘Atmospheric Brown Clouds’ (Ramanathan and Crutzen, 2003). More importantly, BBH reduces air quality and imposes a very negative effect on human health (Dawud, 1998; Aditama, 2000; Kunii et al., 2002; Wiwanitkit, 2008; Hyer and Chew, 2010; Kim Oanh et al., 2011). Quah (2002) reviewed the issues and policy responses to the severe damage of BBH on the regional environment and the economy during the 1997 episode and has highlighted the need for prompt and effective measures in face of the biomass burning problem. Therefore the impact of BBH over SEA on the atmospheric environment, economy and general well-being cannot be overstated and is receiving more and more attention, not only regionally but globally.

    One of the most important phenomena in large-scale haze is deep convection (Lin et al., 2009). This is the most frequently mentioned mechanism for the transport of biomass-burning products up in the troposphere. Deep convection is able to carry biomass air pollutants to higher altitudes over SEA and is a leading candidate to explain climate change in context (Folkins et al., 1997; Chan et al., 2003). A strong convection mechanism responsible for the uplifting of biomass-burning emissions over Indonesia, New Guinea and Malaysia has also previously been at the center of discussions (Folkins et al., 1997). Lin et al. (2009)

  • Oozeer et al., Aerosol and Air Quality Research, 16: 2950–2963, 2016 2951

    have identified leeside troughs over Indochina as major contributors to the uplifting of the tracer in a tracer modelling study while Cheng et al. (2013) have identified that biomass-burning emissions were lifted due to thermal forcing-induced upward motion and high terrain in the northern part of SEA. While the uplifting mechanisms have been studied in Indochina, there is a need to identify the convective mechanisms responsible for the uplifting of biomass-burning emissions in Southern SEA, as literature in this region on the mechanisms remain scarce.

    Intense biomass burning occurred over Sumatra in June 2013. Satellite imageries show that large scale forest fires from Sumatra were mainly responsible for the occurrence of haze in the region (NASA, 2013). Data obtained from the Malaysian Department of Environment (DOE) also show that Air Pollution Index (API) readings exceeded the hazardous level of 300 on several occasions in Peninsular Malaysia during the haze episode (Department of Environment Malaysia, 2013). In this study, the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem; Grell et al., 2005) was used to study the haze crisis that hit South-SEA in June 2013. Particular attention was given to PM10 emissions since PM10 concentrations usually exceed those of other gases emitted during forest fires and the WHO (World Health Organization) guidelines (Radojević and Hassan, 1999). Most studies on BBH have been restricted to immediate dispersion and haze trajectories to neighboring countries (Lin et al., 2009) when measurements have showed that deep convection in SEA can lift biomass-burning emissions up in the troposphere (Folkins et al., 1997). It is therefore important to get a better understanding of the uplifting mechanisms, and this is a gap that this study aims to fill.

    This study aims to: (1) study the transport of BBH in SEA, in particular Peninsular Malaysia, by integrating the appropriate weather and pollutant datasets as well as forest fire hotspot data for the June 2013 forest fire study period into WRF-Chem, (2) identify weather conditions that caused and intensified the transport of BBH from Sumatra to Malaysia during the forest fire episode, (3) demonstrate the influence of the topography on air motion and therefore the transport of BBH over the study area, and (4) identify regions of deep convection near and downwind of the forest fire hotspots and analyze horizontal and vertical BBH plume dispersion. The achievement of these objectives will improve our understanding of the transport mechanisms of BBH in South SEA and will hopefully help to develop more effective inter-governmental policies on the issue. More importantly, this study may help in the formulation of emission control policies which aim at reducing emissions at times when the transport of biomass burning emissions are likely to be carried over regions of deep convection, thus limiting long range transport of these emissions. DATA AND METHODS Observations

    API readings obtained from the Malaysian DOE (DOE Malaysia, 2013) showed that a major haze episode hit Malaysia during the second half of the month of June 2013.

    The air pollutants included in the calculation of API in Malaysia are ozone (O3), carbon monoxide (CO), nitrogen dioxide (NO2), sulphur dioxide (SO2) and suspended particulate matter of less than 10 microns in size (PM10) and a summary of the API categories is listed in Table 1. The observed data indicate that the haze episode became apparent on 15th June when API readings were first categorized as ‘Unhealthy’ in Melaka City and Muar during that period. ‘Hazardous’ readings were first recorded on 20th June in Muar while Melaka City was hit with readings reaching 415 on 23rd June and Port Klang with a maximum API reading of 487 on 25th June. The highest API reading of 746 was recorded on 23rd June at Muar. ‘Unhealthy’ API readings were recorded in several regions of Malaysia until the highest API readings classified as ‘Moderate’ were recorded on 27th June, marking the end of the haze episode. The forest fires which were responsible for the occurrence of haze were detected by the Moderate Resolution Imaging Spectrometer (MODIS) and the hotspot satellite data for 19th, 20th, 23rd and 24th June 2013 are illustrated in Fig. 1. The red spots represent the fire hotspots and the daily observed fire count is indicated at the bottom left corner of each panel. Domain Setup and Data Integration

    The WRF-Chem model (Grell et al., 2005) was used to simulate BBH over SEA during the June 2013 haze episode. The model domain is shown in Fig. 2. It consists of a 27-km grid resolution outer domain with 180 × 117 grid points and a nest (d02) set at 9-km grid resolution with 190 × 190 grid points. The outer domain covers Indonesia and the Southern part of Indochina, including Malaysia, while the nest focuses on Sumatra and Peninsular Malaysia. The vertical level configuration was adapted from Lin et al. (2009) and consists of 35 sigma levels which were most tightly packed near the surface. The lowest level was set at about 16 m above the surface while the model top was set at 50 hPa. The meteorological initial and boundary conditions were obtained from the NCEP FNL (Final) Operational Global Analyses (2000) with 1 × 1 grid spacing at 6-hour intervals. To ensure that the model did not violate the Courant-Friedrichs-Levy (CFL) stability criterion (Courant et al., 1928) the time step of the simulation was set at 120 seconds (less than the recommended maximum of 6 × grid spacing). The model results were output every hour.

    The trace gas and aerosol emissions fields were pre-processed using an adapted version of PREP-CHEM-SRC (Freitas et al., 2011). PREP-CHEM-SRC integrates emissions inventories and forest fire hotspots onto a specified domain. Table 1. Summary of the ranges of index values and the corresponding categories for the Malaysian API system (Department of Environment Malaysia, 2015).

    API Category < 50 Good

    51–100 Moderate 101–200 Unhealthy 201–300 Very Unhealthy

    > 300 Hazardous

  • Oozeer et al., Aerosol and Air Quality Research, 16: 2950–2963, 2016 2952

    Fig. 1. Fire hotspots (shown as red spots) detected from MODIS satellite data on 19th, 20th, 23rd and 24th June 2013 (NASA, 2013). The fire count is indicated at the bottom left hand corner of each panel. The biomass burning emissions were estimated using the Brazilian Biomass Burning Emissions Model (3BEM; Longo et al., 2010) and were injected into the atmosphere using the plume rise model described in Freitas et al. (2006, 2007, 2010). The forest fire hotspots database integrated in the model includes a combination of the MODIS fire locations database (U.S. Naval Research Laboratory, 2013) and the Wildfire Automated Biomass Burning Algorithm (WFABBA) database (University of Wisconsin-Madison, 2013). In order to include Emissions Database for Global Atmospheric Research (EDGAR) version 4.2 in the simulations an additional script was required to convert the data to the appropriate format (HDF5). Two-way nested 24 h WRF-Chem simulations were initialized at 00UTC on 16 June 2013 and the emission inventories had to be updated for each day of simulation. In addition, each simulation was restarted from the previous run to ensure that the chemistry was initialized from the previous 24 h forecast. 11 individual days of simulation were run and the first 2 days of run were treated as spin-up. Model Chemistry and Physics

    The Morrison double-moment microphysics scheme (Morrison et al., 2009) which is capable of predicting the mixing ratios and the number concentrations of five species, namely, cloud droplets, cloud ice, snow, rain and graupel, was used to represent the resolved-scale cloud physics. The longwave and shortwave radiative processes were represented by the Rapid Radiative Transfer Model for general circulation models (GCMs) longwave and shortwave radiation schemes (RRTMG; Mlawer et al., 1997; Pincus

    et al., 2003) respectively. These two radiation schemes can interact with WRF-Chem to include aerosol scattering. Convective parameterization was performed by the Grell 3D cumulus scheme, which is an improved version of the Grell-Devenyi (GD) cumulus scheme (Grell and Dévényi, 2002). In addition, the Grell 3D cumulus scheme allows for feedback from parameterized convection to the radiation schemes. The Noah land-surface model (Chen and Dudhia, 2001) was used to obtain moisture and thermal fluxes form the surface while the Mellor-Yamada-Janjić (MYJ) scheme (Janjić, 1996, 2002) was the selected planetary boundary layer scheme for the simulations. The Regional Acid Deposition Model, 2nd generation (RADM2) (Stockwell et al., 1990) gas phase chemistry mechanism was used with the Georgia Tech/Goddard Global Ozone Chemistry Aerosol Radiation and Transport (GOCART) model (Chin et al., 2000). The aerosol direct effect was turned on by activating aerosol radiative feedback in the simulation. RESULTS AND DISCUSSION Model Evaluation

    The model was first evaluated by comparing the vertical profile at Sepang to sounding data provided by the Department of Atmospheric Science at the University of Wyoming (University of Wyoming, 2013). Vertical profiles can be compared by studying the change of potential temperature θ (K) with change in geopotential height Z (km). The potential temperature and the geopotential height corresponding to the location of the Sepang weather station (2.71°N, 101.70°N) were extracted for 18th to 26th June 2013 and compared to the sounding data. Table 2 shows the correlation coefficients (r) and the Root Mean Square Error (RMSE) obtained from the comparison of the model and sounding data vertical profiles. The evaluation results show that the model performs very well when the vertical profiles were compared within a maximum geopotential height of 12 km. The correlation coefficients were all higher than 0.98 and the highest RMSE observed was only 3.98 K. While the study of deep convection is of major concern in this work, the tropopause which resides at an approximate geopotential height of 16 km to 18 km over Sepang falls out of the boundaries of our region of interest. The model developed and presented in this work therefore proves to be an effective tool in simulating atmospheric conditions in South-SEA. Figs. 3 and 4 show the vertical profiles and scatterplot of potential temperature values for 19th and 24th June at Sepang station. Plots for these 2 dates were chosen since the most intense hotspot activity occurred on the 19th and 24th June as shown in Fig. 1. In addition, high PM10 concentrations were recorded on these 2 days as shown in Fig. 5. Fig. 4 shows that the correlation coefficient and RMSE for the observed and simulated potential temperature were 0.987 and 3.98 K respectively on 19th June and 0.994 and 3.00 K respectively on 24th June.

    The simulated aerosols were evaluated by comparing the PM10 readings at 4 of the 52 air quality monitoring stations operated by the Malaysian DOE (DOE Malaysia, 2013), namely, Johor (CAS 019), Perak (CAN 041), Kuala

  • Oozeer et al., Aerosol and Air Quality Research, 16: 2950–2963, 2016 2953

    Fig. 2. (a) Model domain and (b) Simulation nest with cross-sections XX’ and YY’.

    Table 2. Correlation coefficient, RMSE and Average Percentage Error of vertical derived from WRF-Chem and sounding data.

    Date Vertical profile (0 km-12 km) Correlation Coefficient (r) RMSE (K) Average Percentage Error (%) 18/06/2013 0.992 2.92 0.69 19/06/2013 0.987 3.98 0.87 20/06/2013 0.987 3.49 0.72 22/06/2013 0.991 3.26 0.75 23/06/2013 0.993 2.56 0.60 24/06/2013 0.994 3.00 0.80 25/06/2013 0.989 3.34 0.79 26/06/2013 0.996 3.73 0.93

  • Oozeer et al., Aerosol and Air Quality Research, 16: 2950–2963, 2016 2954

    Fig. 3. Comparison of Vertical profiles at Sepang station on (a) 19th June 2013 and (b) 24th June 2013.

    Fig. 4. Scatterplots of potential temperature θ (K) at Sepang station on (a) 19th June 2013 and (b) 24th June 2013.

  • Oozeer et al., Aerosol and Air Quality Research, 16: 2950–2963, 2016 2955

    Fig. 5. Comparison of observed and model simulated PM10 emissions for the period 19th to 25th June 2013 at (a) Johor, (b) Perak, (c) Kuala Lumpur and (d) Klang. Lumpur (CAC 058) and Klang (CAC 011). These stations were selected for evaluation since the southwest region of Peninsular Malaysia was the most affected during the haze episode and their locations are shown in Fig. 2(b). Klang (CAC 011) is located near Port Klang. The grid index corresponding to the geographical location of each air quality monitoring station was first determined and the model value for the PM10 concentration at the estimated grid index was calculated by bi-linear interpolation from the surrounding four model grid points. Fig. 5 shows the comparison of observed and model simulated PM10 emissions for the period 19th to 25th June 2013. The highest correlation (r = 0.504) was observed for readings at Johor where emissions were well simulated throughout the 7 days. The model succeeded at reproducing the diurnal variation of PM10 concentrations at all 4 stations. However, PM10 concentrations were underestimated over Perak despite maintaining a positive correlation (r = 0.213), which suggests that this discrepancy may have occurred as a result of overestimated vertical transport over the region of Perak. In addition, the errors present in the biomass burning emission inventories may have limited model performance for the study region and contributed to the visible uncertainties in Fig. 5.

    Meteorological Conditions The variations in sea level pressure (SLP) and wind

    patterns during the haze episode are shown in Fig. 6. Southwesterlies prevailed over Sumatra and Peninsular Malaysia since the Southwest monsoon season occurs from the month of May to October in SEA. These southwesterlies were intensified by the presence of a low pressure belt that usually forms between latitude 10°N and 15°N. This low pressure belt is also known as the Northern Intertropical Convergence Zone (ITCZ). On 18th June, there was a gradual intensification of the low pressure belt which drew stronger winds from the Indian Ocean and by 19th June two major low pressure systems formed over the Gulf of Thailand near Cambodia and over the South China Sea. The Southern ITCZ, which separates the southwesterlies from the Indian Ocean and the southeast trade winds, could be observed near Southern Peninsular Malaysia towards the Northeast in Figs. 6(b) and 6(c). The occurrence of the low pressure systems was verified through NASA’s Worldview interactive tool (NASA, 2013).

    On 20th June, as the low pressure system over Cambodia moved eastward towards the South China Sea and it began to merge with the already existing low pressure system in

  • Oozeer et al., Aerosol and Air Quality Research, 16: 2950–2963, 2016 2956

    Fig. 6. SLP (hPa) (shaded colours) and wind fields (m s–1) (arrows) at 06 UTC (a–h) from 18th to 25th June.

  • Oozeer et al., Aerosol and Air Quality Research, 16: 2950–2963, 2016 2957

    that region as shown in Fig. 6(c). The winds over Peninsular Malaysia gradually shifted from blowing to the northeast to an easterly direction while weak winds prevailed over southern Peninsular Malaysia and Singapore. By 21st June, a stronger low pressure system formed from the two smaller low pressure systems and southwesterlies were established over southern Peninsular Malaysia while westerlies predominated over northern Peninsular Malaysia and Thailand. The low pressure system further intensified on 22nd June and began to travel towards the west over Vietnam but gradually lost in intensity on 23rd June. The southwesterlies blowing from Sumatra over Peninsular Malaysia gradually shifted to southerlies and southeasterlies on 23rd and 24th June respectively as shown on Figs. 6(f) and 6(g). A new low pressure system gradually formed over the South China Sea, resulting in a high pressure region over Sumatra. Southeasterlies also blew along the Strait of Malacca while northwesterlies blew over the Gulf of Thailand as a result of the low pressure system on 25th June as shown in Fig. 6(h).

    High pressure over Sumatra may have inhibited precipitation over Sumatra and contributed to the intensification of the forest fires in Riau. In fact, Reid et al. (2012) reported that decreased precipitation and increased severe fire events were observed in Borneo and Sumatra when tropical cyclones occurred over the northern South China Sea. The fires might also have been sustained by dry warm air flowing over the Barisan Mountains onto Riau. As moist air coming from the Indian Ocean is force-lifted over the windward side of the mountain, moisture is lost to cloud formation thus resulting in dry air which warms up as it flows down over the leeward side of the mountain.

    The mountain flow can be observed on Figs. 7–9. Horizontal PM10 Emissions Transport

    In order to study the horizontal and vertical extent of the haze plume during the 2013 episode, PM10 plots were extracted from the simulation results. Fig. 10 shows the horizontal PM10 plume at 998 hPa height (~16 m) over Sumatra and Peninsular Malaysia during the haze episode.

    On 16th and 17th June few fire hotspots were observed over Riau, Sumatra with little emission being carried over the Southwest coast of Peninsular Malaysia (not shown). The number of hotspots increased on the 18th and reached a high on 19th June as shown in Fig. 1. Emissions increased drastically on the 19th and were initially transported over Malaysia by southwesterlies and thereafter by westerlies. Fig. 10(c) shows that on 20th June more haze was transported over Peninsular Malaysia where Muar was the most affected city on that day. Forest fires were still predominant on Sumatra on 21st June and biomass-burning emissions were still transported to Peninsular Malaysia with a shift in the plume direction from easterly direction to northeasterly direction due to the wind shift. Fig. 10(d) shows that emissions occurred over Batu Pahat, Melaka and Seremban due to the shift in direction of the plume flow and the API readings increased accordingly over these regions. The location of these regions can be seen on Fig. 2(b).

    Fire hotspots were still prominent over Sumatra on 22nd and 23rd June. The emissions were transported in a north-northeasterly direction from Sumatra to Malaysia on 22nd June and the most affected city was Muar where a maximum reading of 1050 µg m–3 to 1200 µg m–3 was recorded from

    Fig. 7. Wind fields (m s–1) (arrows), Vertical PM10 plume (µg m–3) (shaded colors-left) and Vertical Wind Speed (cm s–1) (shaded colors-right) on 19th June along XX’.

  • Oozeer et al., Aerosol and Air Quality Research, 16: 2950–2963, 2016 2958

    Fig. 8. Wind fields (m s–1) (arrows), Vertical PM10 plume (µg m–3) (shaded colors-left) and Vertical Wind Speed (cm s–1) (shaded colors-right) on 24th June at (a) 14 UTC and (b) 19 UTC along XX’. 21 UTC to 00 UTC. The API reading at that time peaked at 746 in Muar. The haze plume then started to shift northwards and Melaka and Muar were observed to be the most affected cities on 23rd June as shown in Fig. 10(f). The API reading at Melaka peaked at 415 at 03 UTC on that day. Increased hotspot activity over Riau was observed on 24th June and the south-southwesterlies transported the PM10 emissions over the western coast of peninsular Malaysia, Port Klang in particular, as shown on Fig. 10(g). Hotspot activity drastically reduced on 25th June over Sumatra and

    on 26th June the PM10 plume dissipated due to reduced forest fire activity on Riau, marking the end of the June 2013 haze episode as shown in Fig. 10(h). Vertical PM10 Emissions Transport and Deep Convective Motion

    One of the main objectives of this study is to identify regions of deep convection near and downwind of the forest fire hotspots that were responsible for the transport of BBH to higher altitudes, which is not easily observed

  • Oozeer et al., Aerosol and Air Quality Research, 16: 2950–2963, 2016 2959

    Fig. 9. Wind fields (m s–1) (arrows), Vertical PM10 plume (µg m–3) (shaded colors-left) and Vertical Wind Speed (cm s–1) (shaded colors-right) at 14 UTC on (a) 19th and (b) 24th June along YY’. through measurements. Fig. 2(b) shows the nest (d02) with lines XX’ and YY’ which represent the vertical cross-sections studied in this section. Depending on the day of simulation, their center points correspond to high emission spots and the cross-sections can therefore show vertical convective conditions above those regions. In addition, the cross-sections also lie along the direction of plume flow (Fig. 10) and can therefore depict the advective conditions involved. Hence the vertical cross-sections serve to identify the air motion responsible for the uplifting of the emissions and

    their transport from Sumatra to Peninsular Malaysia. Table 3 shows the location and orientation of each cross-section.

    The vertical PM10 emission plume and vertical velocity along the two cross-sections were plotted for every day of the haze episode. The wind fields were calculated from the horizontal velocity along a particular cross-section and 10 times the vertical velocity (10*W). The most intense hotspot activity during the June 2013 episode occurred on 19th and 24th June and it was found that emissions reached the highest altitude on these 2 days. Hence only the results obtained

  • Oozeer et al., Aerosol and Air Quality Research, 16: 2950–2963, 2016 2960

    Fig. 10. Horizontal PM10 plume (µg m–3) at 998 hPa height (a–h) from 18th to 26th June 2013 and (i) location of relevant regions.

    Table 3. Location and orientation of vertical cross-section on nest (d02).

    Cross-section Centre grid point on nest (x, y) Angle

    (°) Regions crossed

    XX’ (99, 112) 0 Riau in Sumatra and between Melaka and Sepang over Peninsular Malaysia

    YY’ (102, 112) 60 Between Muar and Batu Pahat over Peninsular Malaysia

  • Oozeer et al., Aerosol and Air Quality Research, 16: 2950–2963, 2016 2961

    for 19th and 24th June are presented and discussed in this section. The identified uplifting mechanisms are illustrated and discussed below. Figs. 7 and 8 show the vertical PM10 plots along XX’ while Fig. 9 illustrate the PM10 plots along YY’.

    The most prominent vertical transport of PM10 was found to take place over the Strait of Malacca on 19th and 24th June along both cross-sections. Fujita et al. (2010) described the mechanism by which a morning maximum in the diurnal precipitation was formed by the convergence of cold outflows from Sumatra and Peninsular Malaysia over the Strait. These outflows are generally produced by precipitation systems from the previous evening and converge over the Strait at around midnight. Fig. 7 shows that PM10 emissions reached at least 350hPa over the Strait near 2°N at 11 UTC on 19th June due to strong vertical motions that reached the upper troposphere above that region. As the direction of plume flow switched northward on 24th June, PM10 concentrations along the cross-section XX’ increased as compared to 19th June. At 14 UTC, the PM10 plume had reached a height of 500 hPa over the strait while a second PM10 band over Malaysia near 3.3°N reached at least the 200 hPa (~12 km) in the upper troposphere as shown in Fig. 8(a). This deep convective transport can be attributed to a strong orographic effect which occurs as the wind is force-lifted over the slope on the West coast of Malaysia and its mountains deeper inland. As the morning precipitation maximum forms (Fujita et al., 2010) at 18 UTC, a higher concentration PM10 plume rises to at least 200 hPa over the Strait of Malacca as shown in Fig. 8(b) confirming further the transport of biomass burning emissions to the upper troposphere in the region.

    Fig. 9(a) shows the transport of PM10 emissions along YY’ at 14 UTC on 19th June. Much higher concentrations of PM10 were observed along YY’ as compared to XX’ for the same day since YY’ followed the direction of plume flow on 19th June. A residual layer was formed between 950 hPa and 850 hPa as the plume was transported in a northeasterly direction. However, a very distinguishable peak which reached 500 hPa was still formed over the Strait of Malacca thus demonstrating the strong influence of convection in this region. In contrast, while a similar peak was formed on the 24th closer to the coast of Sumatra, lower PM10 concentrations were observed in the residual layer which extended from 900 hPa to 750 hPa, due to the switch in the direction of plume flow. This is shown in Fig. 9(b). CONCLUSION

    In order to study the 2013 SEA BBH case, WRF-Chem simulations were performed to identify the weather conditions that caused and intensified the transport of haze from Sumatra to Peninsular Malaysia. The model was run from 16th to 26th June 2013 and was evaluated by comparing the simulation vertical profile at Sepang to sounding data and PM10 emissions to readings recorded by the Malaysian DOE. The prevailing convective conditions were also studied to understand how far deep convection affected vertical haze plume dispersion over the region.

    The results showed that southwesterlies from the Indian

    Ocean were mostly responsible for the transport of biomass-burning haze from Sumatra to Peninsular Malaysia. Variations in the wind direction occurred as low pressure systems forming the Northern Intertropical Convergence Zone travelled eastward and westward. The haze plume was directed over the southern part of Peninsular Malaysia during the first half the episode and then shifted northward to affect the west coast of Malaysia during the second half. Muar and Melaka city were found to be the two most affected cities during the haze episode.

    To study the vertical haze plume dispersion and the regions of deep convection, the results were plotted along vertical cross-sections for 19th and 24th June. The PM10 plume was lifted to at least 350 hPa and 200 hPa on 19th and 24th June respectively due to the convergence of outflows from Sumatra and Peninsular Malaysia over the Strait of Malacca. Orographic lifting over the West coast of Malaysia and the Malaysian mountains also lifted the haze plume to at least 200 hPa. The uplifting of the biomass-burning emissions to such heights could have long range transport effects if the emissions are carried aloft by the prevailing upper level winds. ACKNOWLEDGMENT

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    Received for review, July 15, 2015 Revised, November 17, 2015

    Accepted, January 5, 2016