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Neutron Detection with Diamond Detectors ( 252 Cf source measurement) 2 nd ADAMAS workshop GSI Darmstadt, 15 th -17 st -December-2013 Jose Due˜ nas, Lu´ ıs Acosta & Ismael Martel Dpto. F´ ısica Aplicada Universidad de Huelva. Francisco Manchado & Pepe S´ anchez Hostipal Juan Ram´on Jim´ enez Jose Due˜ nas ([email protected]) Neutron detection with DD UHU Dpto. F´ ısica Aplicada 1 / 10

Neutron Detection with Diamond Detectors · Jose Duenas,~ Lu s Acosta & Ismael Martel Dpto. F sica Aplicada Universidad de Huelva. Francisco Manchado & Pepe S anchez Hostipal Juan

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Page 1: Neutron Detection with Diamond Detectors · Jose Duenas,~ Lu s Acosta & Ismael Martel Dpto. F sica Aplicada Universidad de Huelva. Francisco Manchado & Pepe S anchez Hostipal Juan

Neutron Detection with Diamond Detectors(252Cf source measurement)

� 2nd ADAMAS workshop ≺GSI Darmstadt, 15th-17st -December-2013

Jose Duenas, Luıs Acosta & Ismael Martel Dpto. Fısica Aplicada Universidad de Huelva.

Francisco Manchado & Pepe Sanchez Hostipal Juan Ramon Jimenez

Jose Duenas ([email protected]) Neutron detection with DD UHU Dpto. Fısica Aplicada 1 / 10

Page 2: Neutron Detection with Diamond Detectors · Jose Duenas,~ Lu s Acosta & Ismael Martel Dpto. F sica Aplicada Universidad de Huelva. Francisco Manchado & Pepe S anchez Hostipal Juan

Motivation & Outline

1 Motivation.Identification of neutrons by means of n-C interaction.Neutron detection in Hospital environment.PhD thesis of Francisco Manchado.

2 Some typical neutron detectors.3 Experimental lab setup.

252Cf neutron source.Chamber + electronics setup.

4 Preliminary results.Low energy part (< 2 MeV).Contributions above 2 MeV.

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Page 3: Neutron Detection with Diamond Detectors · Jose Duenas,~ Lu s Acosta & Ismael Martel Dpto. F sica Aplicada Universidad de Huelva. Francisco Manchado & Pepe S anchez Hostipal Juan

Neutron interactions with matter

Main interaction

Neutrons have not electriccharge (neutral), which makedirect detection a “bit” difficult.

Main interations: Scattering andabsorption.

Classic expression for kineticenergy v = 1.383× 107

√E .

3He, 235U and 10B commonlyused in detectors due to largeabsorption cross sections for theproduction of charged particleswith low-speed neutrons.

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Page 4: Neutron Detection with Diamond Detectors · Jose Duenas,~ Lu s Acosta & Ismael Martel Dpto. F sica Aplicada Universidad de Huelva. Francisco Manchado & Pepe S anchez Hostipal Juan

Detectors for neutrons

Different types

Solid, liquid, or gas-filled media.

Some examples:

gas-filled (3He) counterscintillatorsfission chambers

Detectors with neutron-activematerial added:

Gadolinium.10B.6Li; thermal neutrons via(n,α) reaction.6LiF on diamond [M. Angelone et al.

NIMA 595 (2008) 616].

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Page 5: Neutron Detection with Diamond Detectors · Jose Duenas,~ Lu s Acosta & Ismael Martel Dpto. F sica Aplicada Universidad de Huelva. Francisco Manchado & Pepe S anchez Hostipal Juan

252Cf neutron source

Spontaneous fission neutron source

Table: Main composition of the neutronsource (Oak Ridge National Lab).

Nuclide Mass % Activity %

249Cf 9.297 0.103250Cf 18.505 5.456251Cf 7.186 0.0309252Cf 65.012 94.412

Half line of 2.7 years.

Active diameter of 5 mm.

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Page 6: Neutron Detection with Diamond Detectors · Jose Duenas,~ Lu s Acosta & Ismael Martel Dpto. F sica Aplicada Universidad de Huelva. Francisco Manchado & Pepe S anchez Hostipal Juan

Electronic chain setup

Lab setup

scCVD-500 µm; 4 mm × 4 mm; 300 V; leakage no readable (< 1 nA).

Mesytec MSI-8 preamplifier + shaper (1 or 2 µs shaping time).

Mesytec MHV high voltage supply and MNV for electronics bias.

Canberra 16K 1 µs ADC. USB interfase. GenieTM software.

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Page 7: Neutron Detection with Diamond Detectors · Jose Duenas,~ Lu s Acosta & Ismael Martel Dpto. F sica Aplicada Universidad de Huelva. Francisco Manchado & Pepe S anchez Hostipal Juan

Chamber setup

In the chamber

Chamber to ambient pressureexcept for the α calibration.

Detector connected directly tothe lemo feedthrough.

Several Al layers around thechamber to avoid contaminationand also noise.252Cf source far from detector.

Thick lead shield (3.2 mm) justin front of the source to stop αparticles.

Measurement in dark.

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Page 8: Neutron Detection with Diamond Detectors · Jose Duenas,~ Lu s Acosta & Ismael Martel Dpto. F sica Aplicada Universidad de Huelva. Francisco Manchado & Pepe S anchez Hostipal Juan

252Cf spectra for long term acquisition Low energy part

Spectrum time progression

energy (MeV)0.6 0.8 1 1.2 1.4 1.6 1.8 2

co

un

ts

0

2000

4000

6000

8000

10000

12000

42 days acquisition

21 days acquisition

1.5 days acquisition

Other spectrum from 252Cf,using a setup with a pcCVD anda Si for coincidence, see bottomright [S. Oberstedt NIMA 714 (2013) 31].

pulse hight (channel)0 50 100 150 200 250 300 350

co

un

ts

310

410

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Page 9: Neutron Detection with Diamond Detectors · Jose Duenas,~ Lu s Acosta & Ismael Martel Dpto. F sica Aplicada Universidad de Huelva. Francisco Manchado & Pepe S anchez Hostipal Juan

252Cf spectra for long term acquisition Contributions above 2 MeV

Spectrum time progression

energy (MeV)0.6 0.8 1 1.2 1.4 1.6 1.8 2

co

un

ts

0

200

400

600

800

1000

1200 42 days acquisition

21 days acquisition

1.5 days acquisition

energy (MeV)3.5 4 4.5 5 5.5 6 6.5 7 7.5

co

un

ts

0

2

4

6

8

10

12

14

16

42 days acquisition

21 days acquisition

1.5 days acquisition

No found anything like it in literature, quite often 12C(n,α)9Be &T(d,n)4He at 14.8 MeV.

Could one of the contact layer (DLC/Pt/Au) interacting with n?

Need for n reaction simulation.

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Page 10: Neutron Detection with Diamond Detectors · Jose Duenas,~ Lu s Acosta & Ismael Martel Dpto. F sica Aplicada Universidad de Huelva. Francisco Manchado & Pepe S anchez Hostipal Juan

Summary and future work

Summary

Characterization with 252Cf source.

Our scCVD-500 µm proved to be able to detect neutrons.

Also proved the stability behavior for 41 days nonstop measurement.

Near future

Simulation will be done to identify the possible reactions.

Experiment, propably at CNA accelerator Sevilla, with the rightreaction to produce neutrons.

Design the proper diamond detector (either fast or slow neutrons).

Study the integration of the system.

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