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K. Reich, M. Schecter, B.I. Shklovskii,
University of Minnesota
Part 1: Two-dimensional electron gas in STO
2
Dielectric constant of STO
3
The origin LAO-STO 2DEG
J. Mannhart et al, MRS Bull. 33 1027 (2008)
4
Thomas-Fermi accumulation layer
5
Landau Hamiltonian
6
Thomas-Fermi accumulation layer. Linear dielectric response
7Ya. I. Frenkel, Ioffe Institute, 1928
TF-Linear results:
9
TF-Nonlinear results
10
TF results for d combined
11
Justification of TF approach
12
Experimental density profile of electrons n(x) (Y. Yamada, H. K. Sato, Y. Hikita, H. Y. Hwang, and Y. Kanemitsu, Applied Physics Letters 104, 151907 (2014)) obtained by time-resolved photoluminescence. Fitting with our theory is shown by the solid line: d = 250b = 9 nm.
13
FIG. 2. Fitting by (x+d)^{-12/7} obtained by infrared ellipsometry in A. Dubroka, M. Rossle, K. W. Kim, V. K. Malik, L. Schultz, S. Thiel, C. W. Schneider, J. Mannhart, G. Herranz, O. Copie, M. Bibes, A. Barthelemy, and C. Bernhard, Phys. Rev. Lett. 104, 156807 (2010). The fitting parameter d =142b = 5 nm.
Experimental density profile of electrons n(x)
14
Part 2:Spherical charge in STO
Han Fu, K. Reich,B.I. Shklovskii
University of Minnesota.
C. Cen, S. Thiel, G. Hammerl, C. W. Schneider, K. E. Andersen, C. S. Hellberg, J. Mannhart, and J. Levy, Nature Materials 7, 298 (2008)
Drawing on LAO/STO
16
• κ = 20000
• At Z > Zc , collapse happens!
Thomas-Fermi "atom" in STO
17
Collapse of the "atom" and charge renormalization
• Electrons collapse to the center
• At large nuclear charge Z, the final net charge is renormalized to Z*
18
Known collapse phenomena • Supercritical nucleus Z > 1/α = 137
α = e2/ћc
• Narrow-band gap semiconductors, Weyl semimetals, and graphene αeff= e2/ћvκ, ε=pv
I. Pomeranchuk and Y. Smorodinsky (1945) Y. B. Zeldovich and V. S. Popov (1972)
E. B. Kolomeisky, J. P. Straley, and H. Zaidi, (2013)M. M. Fogler, D. S. Novikov, and B. I. Shklovskii, (2007), Levitov (2007), M. F. Crommie, (2012)
Relativistic origin
• Ek = pc ≈ ћc/r, U = -Ze2/r |U/Ek| = Zα,
• Z > 1/α → collapse happens,
Zn
S
A. B. Migdal, V. S. Popov, D. N. Voskresenskii (1977).
E. B. Kolomeisky, J. P. Straley,
H. Zaidi (2013). SZZn
20
A different origin in STO:nonlinear dielectric response
20000,4
20
3
20
3
P
AP
P
APPE
PPED 44 3DE
62
1)(
1)(
rrE
rrE
5
1)(
1)(
rr
rr
21
A different origin in STO:nonlinear dielectric response
22
Collapse and charge renormalizaton
• As Z increases, collapse strengthens
• Degenerate gas
2
2
5
243
)(,)(R
aeRE
R
eaZRe k
a
RZc
,/
)(1.0)(
2/3
3
bb ae
r
arn
2/92/7
*0
2 5.0)(4 ZZ
ZZrnrdrS
cZa
RZ
7/9*
23
Collapse and charge renormalization in STO
Zc ≈ R/a Z* ≈ (R/a)9/7
Zn
S
*ZSZZn at Z >> Z*
24
Redistribution of electron density
Collapsed, Saturn-like
uncollapsed
linearnonlinear
aB
Potential profile
• Double-layer structure
Fermi level
Fermi sea
Similar to supercharged nuclei border studied by A. B. Migdal, V. S. Popov, D. Voskresenskii (1977).
26
Finite temperature
• Thermal ionization at finite T• s = kB ln (n / n0),
n0=2 / λ3, λ ~ T-1/2, n=Zi N
I = Zie2/κri = Zi2e2/κ2ab,
ri=κab/Zi
I=sT • Zi > Z* at T > 8 K, Inner tail ionized at T > 450 K
T < 10 K
d
T > 10 K
Temperature-induced metal-insulator crossover
28
Thank you
29
Electron layer width d from accumulation to inversion
30
Role of dispersion term