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Giacomo Prando
Research threads
1. Magnetism in flatland
2. Iridium oxides – thin films
3. Many-body localization and Floquet time-crystals (“Incontri del martedì”, 27.11.2018)
4. Orbital-selectivity in iron-based pnictides
13.09.2018 – Pavia, “Congresso interno di Dipartimento”
Giacomo Prando
Research threads
1. Magnetism in flatland
2. Iridium oxides – thin films
3. Many-body localization and Floquet time-crystals (“Incontri del martedì”, 27.11.2018)
4. Orbital-selectivity in iron-based pnictides
13.09.2018 – Pavia, “Congresso interno di Dipartimento”
In the beginning was graphene
Nat. Mater. 6 183 (2007)
A truly two-dimensional material with exceptional mechanical and electronic properties
“Relativistic” condensed matter physics
+ Massive bunch of novel physical phenomena
Prospects for two-dimensional electronics
Mind the gap, please – TM dichalcogenides
Versatile materials complementing graphene
Mechanical exfoliation in
atomic trilayers is possible
Scalable devices based on Lego-like architectures (vdW heterostructures)
Chem. Rev. 113 3766 (2013); Nature 499 419 (2013); Nat. Rev. Mater. 2 17033 (2017)
Superconductivity in flatland
Gate-induced superconductivity in atomically thin layers of MoS2
Nat. Nanotech. 11 339 (2016)
Ising superconductivity in atomically thin layers of NbSe2
Nat. Phys. 12 139+144 (2015)
Magnetism in flatland Cr2Ge2Te6 , Nature 546 265 (2017)
CrI3 , Nature 546 270 (2017)
Magnetism – really in “flatland”?
CrI3
I
Cr
3 μB
+ Samples are not atomically-thin + Samples are on substrates + Ising-like anisotropy for magnetic moments ...Mermin-Wagner theorem is safe.
“Flatland” or not – interesting physics
Electrical control of magnetism in CrI3
Nat. Nanotech. 13 544+549 (2018); Nat. Mater. 17 406 (2018)
“Flatland” or not – scalable spintronic devices
M
M
Ins
Tunnelling magnetoresistance
Magnetic tunnel junction
Science 360 1214+1218 (2018)
Nat. Mater. 11 372 (2012)
“Flatland” or not – scalable spintronic devices
M
M
Ins
Tunnelling magnetoresistance
Magnetic tunnel junction
Science 360 1214+1218 (2018)
Nat. Mater. 11 372 (2012)
Sizeable ferromagnetic signal from VSe2 monolayers
+ Strong magnetism (15 μB per V)
+ The effect persists at room temperature
+ VSe2 is non-magnetic in the bulk
Nat. Nanotech. 13 289 (2018)
TM dichalcogenides – Ferromagnetism in VSe2
Experimental tools – spin-polarized muons
Sample: Se[50nm]/VSe2[ML]/MoS2[substrate]
Conventional-NMR signal: proportional to nuclear magnetization. Inconvenient
Muon spin rotation with positive muons
Contemp. Phys. 40 175 (1999)
Experimental tools – spin-polarized muons
Paul Scherrer Institute, Switzerland
After muon implantation in the sample:
Quantum sensor of local magnetism.
No need of external magnetic fields.
Journ. Phys. C 20 3187 (1987); Contemp. Phys. 40 175 (1999)
Experimental tools – spin-polarized muons
Journ. Phys. C 20 3187 (1987); Contemp. Phys. 40 175 (1999)
Experimental tools – spin-polarized muons
Space- and time-resolved detection of positrons: Information on local magnetism
Journ. Phys. C 20 3187 (1987); Contemp. Phys. 40 175 (1999)
Experimental tools – spin-polarized muons
Low-energy positive muons
Unique spectrometer – tuning of muons’ kinetic energy possible
Control over implantation depth over tens of nm.
Optimal conditions for probing magnetism in nanostructures.
VSe2
Unpublished experimental results (July 2018) – spin-polarized muons
Sample: Se[50nm]/VSe2[ML]/MoS2[substrate] (black dots)
Temperature dependence: reminiscent of strong magnetic signal
Reference sample: Se[50nm]/MoS2[substrate] (pink squares)
The same behaviour is observed without VSe2
Experimental results (July 2018) – open questions
+ Signal loss due to muonium (μ+e-)
+ Muon spin rotation needs large samples (2 cm): are we dealing with a homogeneous device?
+ Nominally-identical substrates result in different properties:
any insight leading to better control in the growth?
New measurements at Leibniz-IFW in Dresden by means of different experimental tools
Work in progress!
Nat. Nanotech. 13 289 (2018)
Giacomo Prando
Research threads
1. Magnetism in flatland
2. Iridium oxides – thin films
3. Many-body localization and Floquet time-crystals (“Incontri del martedì”, 27.11.2018)
4. Orbital-selectivity in iron-based pnictides
13.09.2018 – Pavia, “Congresso interno di Dipartimento”
3d electrons – cuprates
Hubbard model
Crossover from antiferromagnetic insulator to Fermi liquid
Phys. Rev. Lett. 101 076402 (2008); Nature 464 183 (2010)
5d electrons – iridates
“Spin-orbital Mottness”
Phys. Rev. Lett. 101 076402 (2008) Phys. Rev. Lett. 108 177003 (2012)
Spin and orbital degrees of freedom are entangled
Sizeable coupling between
lattice and magnetism
5d electrons – iridates
Phys. Rev. Lett. 102 017205 (2009); Journ. Phys. Cond. Matt. 25 422202 (2013); Ann. Rev. CMP 7 195 (2016)
Structural strain-induced modifications in PLD-grown heterostructures (PoliMi) Both static and dynamic (piezo) strain
RIXS: spectrum of magnetic excitations (PoliMi)
PRIN – iridate thin films
Phys. Rev. B 92 024405 (2015); Phys. Rev. B 95 115111 (2017)
Basic magnetic properties: low-energy muons (UniPv)
PRIN – iridate thin films
Phys. Rev. B 92 024419 (2015)
Magnetic anisotropy: (anti)ferromagnetic resonance (UniPv)
PRIN – iridate thin films
Phys. Rev. B 94 024412 (2016)