Gem*Star Aps Dnp

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    A D N A

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    1GEM STA R

    Green Energy-MultiplierSub-critical, Thermal-spectrum,Accelerator-driven, Recycling Reactor

    GEM STA R

    R. Bruce Vogelaar

    Virginia TechOctober 28, 2011APS - DNP

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    The Inconvenient TruthAl Gore

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    Global Warming is happening now

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    nuclear energy will probably beconfirmed in most of today's nuclearcountries as a low carbon energy source

    needed to limit imports of oil and gas andto meet fast growing energy needs

    Carre previous talk

    and everyone puts a brave face on it;sans any other alternative for the past 40years

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    but there are otherinconvenient truthsWaste

    long-lived fission products andactinides

    bury in Yucca Mountain? (now cancelled!)

    burn with accelerators?burn in next generation reactors?

    store on sitecurrent practice

    Weapons Proliferationenrichmentreprocessing

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    Probabilistic Risk Assessment (PRA)of Core Damage Frequency (CDF)

    E v e n

    t s / R e a c

    t o r - Y e a r

    Safety

    SMR claim 10 -8 events per reactor-year

    thats 1 event in 1,000,000 reactors over 100 years

    is there a credibility issue?

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    current prices for electricity(estimated by Black and Veatch, Overland Park, Kansas)

    cents/kwhCoal without CO 2 capture 7.8Natural gas at high efficiency 10.6Old nuclear 3.5New nuclear 10.8Wind in stand alone 9.9Wind with the necessary base line back-up 12.1Solar source for steam-driven electricity 21.0Solar voltaic cells; higher than solar steam electricity

    *NYT, Sunday (3/29/09) by Matthew Wald

    GEM*STAR: 4.5 per kWh with natural uranium fuel

    Cost

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    Paradigm Shift

    ReprocessingThermalReactorsEnrichment

    NaturalUranium

    FastReactors

    GeologicStorage

    Liquid FuelRecycling Reactor

    Withsupplemental neutrons

    Natural uranium orLWR spent fuel

    GeologicStorageEnd-of-life waste remnant reduced

    by x10 and delayed by centuriesNo enrichment, no reprocessing

    GEM STA R

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    what would an accelerator based nuclear energy deployment look like

    UraniumOre

    Enrichment

    FuelFabrication

    AdvancedBurner

    Reactor

    FuelSeparation

    TransmutationFuel

    Fabrication

    Fission Products and Process Losses

    LightWater

    Reactor

    High-LevelWasteRepository

    Low-LevelWaste

    DisposalStorage

    Strontium, Cesium and Uranium

    TransmutationReprocessing

    RecyclingLiquid-fuelSubcritical

    Reactor

    reduce and defer waste

    Fluorination

    Accelerator or fusion neutrons

    GNEP

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    The cost of neutrons has dropped dramatically

    1.00E+05

    1.00E+06

    1.00E+07

    1.00E+08

    1.00E+09

    1.00E+10

    1.00E+11

    1.00E+12

    1950 1960 1970 1980 1990 2000 2010 2020

    Year

    N e u t r o n c o s t

    ( $ p e r g r a m

    )

    Electrosta tic tandemwith stopping lengthdeuterium target

    LAMPF withW target

    SNS withHg target

    GEM*STARwith U target

    Electron linac w ithW target

    ~40 grams of neutrons will produce 1GWe for one year

    ($432M @ 5 /kWh)

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    Proton Driven Sub-Critical System

    electric thermaltbeam fissiont

    beam beamn f tbeam1 f n t

    walla 1 f n tnet electric power out

    power on targetelectric wall

    walla 1 f n t

    1a

    t m

    Ewall Ebeama Eelectric

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    a

    Design criteria: large m (fissions per neutron),limiting the need to maximize a (accelerator efficiency)

    uranium fuel (un-reprocessed LWR spent fuel is actually better) molten salt eutectic improved neutron utilization & target design

    This is what the GEM*STAR project achieves.Results in multiple advantages over existing (orplanned) nuclear energy systems.

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    Solid Fuel Issues

    volatile fission-product build-upwithin cladding

    much more centrallypeaked for driven

    systems

    non-uniform fuelconsumption

    thermal shock due to beam trips (~800 320)

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    Molten Salt Eutectic Fuel

    ThF 4

    UF 4

    LiF : UF 4LiF

    850

    950

    1050

    750 650

    1111 o

    1035 o845o

    568 o

    565 o

    500 o

    490o

    550

    Uranium or Thoriumfluorides form eutecticmixture with 7LiF salt.

    High boiling point lowvapor pressure

    Proven in ORNLMSRE reactorusing ModifiedHastelloy-N(235 U, 239 Pu, 233 U)

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    consider a clear liquid which releases heat when

    exposed to light, eventually turning a dark purpleInitial fill

    with continuous feed-and-bleed beginning here

    color and heat output remainsconstant indefinitely

    equilibrated isotope fractionsthroughout core and throughout time

    increasing light exposure

    feed

    bleedfast internal mixing

    10 -6 less volatile fission-productbuild-up in core

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    For 50 years, and even today, people argue for fast-spectrum systems.

    Why?

    Faster burn-up of heavy actinides.

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    But Using Thermal Spectrum0.01 0.2 eV

    highest tolerance for fission products: spin structure and resonance spacing reducescapture cross-section at thermal energies:

    -fission (239 Pu)-capture (f.p.)

    151 Sm (transmuted rapidly to low c nuclei) 135 Xe (continuously removed as a gas)

    more than compensates for slower fission ofheavy actinides (which are burned anyway)

    ~ 100 (vs ~ 10 @ 50 keV)

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    extracts many times more fission energy,

    without additional long-lived actinides

    Feed material:

    LWR spent fuel 20 GWy

    Acc 1 40 GWy

    Acc 2 60 GWy

    etc

    major reduction and deferral of waste

    Relative Wasteafter 2 passes

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    Recycling

    first pass(40+ years)

    second pass(40+ years)

    each can be usedto start anotherpre-equililbrated

    core every 5 years

    subsequent passes (fusion n source?)

    40 years worth of LWR spent fuel

    under-coreinterim storage

    under-coreinterim storage

    under-coreinterim storage

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    Existing Proton Beam Power

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    Target Considerations

    GEM*STAR Internal Target

    diffuse (or multiple) beam spots molten salt used for heat removal high neutron yield from uranium

    (but minimize target fission) spent target fluorinated and used as fuel

    minimize impact on local reactivity

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    -0.005

    0.000

    0.005

    0.010

    0.015

    0.020

    0.025

    0.030

    0

    30

    60

    90

    120

    150

    180

    210

    240

    270

    300

    330

    360

    0.00 0.50 1.00 1.50 2.00 2.50 3.00

    F l u e n c e

    ( n / b )

    N

    e t E l e c

    t r i c P o w e r O

    u t / P o w e r o n

    T a r g e

    t

    Fissioned Fraction (%)

    Fuel: Natural Uranium (MCNPX)

    GEM*STAR Split Design

    Traditional Graphite (0.6 ppm B)

    Fluence

    equiv. to a LWRburning 0.5% ofnatural uranium

    running at peak gives 91%Pu-239 plutonium

    running at x60 gives 70%Pu-239 plutonium

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    0.000

    0.005

    0.010

    0.015

    0.020

    0.025

    0.030

    0.035

    0.040

    0

    50

    100

    150

    200

    250

    300

    350

    400

    0.00 0.50 1.00 1.50 2.00 2.50 3.00 3.50

    F l u e n c e

    ( n / b )

    N e

    t E l e c

    t r i c P o w e r

    / P o w e r o n

    T a r g e

    t

    Additional Fission Fraction (%)

    GEM*STAR split designTraditional Graphite100 * keff + 50Fluence

    feed LWRspent fuel

    fissionproductfraction

    SuperCritical

    Fuel: un-reprocessed Light-Water-Reactor spent fuel

    running at x140 gives45% Pu-239 plutonium

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    High Temperature MSAdvantages over LWRs

    no high-pressure containment vessel 34% 44% efficiency for thermal to electric

    conversion (low-pressure operation)

    match to existing coal-fired turbines, enablesstaged transition for coal plants, addressingpotential cap-and-trade issues

    synthetic fuels via modified Fischer-Tropschmethods very attractive (much morerealistic than hydrogen economy)

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    What are the obstacles?GEM*STAR uses liquid fuel but NRC is onlycomfortable with solid fuel, despite MSRE successExisting commercial deployed fleet of LWRsEngineers in nuclear industry have little experience withaccelerators; physicists using accelerators have little

    experience with nuclear power plants littlecooperation in base programs (vague talk about adistant ATW application)current focus (in US) only on existing and newmodular reactors (scaled down versions of existingdeployed technology)

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    advantages seem clearhowever:

    DOE NE Report to Congress, April 2010, Nuclear EnergyResearch and Development Roadmap does not include the wordaccelerator even once .

    DOE Science (HEP & NP) ADS Report (September 17, 2010) Finding #2: Accelerator-driven sub-critical systems offer the potential for safely

    burning fuels which are difficult to incorporate in critical systems, for examplefuel without uranium or thorium . [ WHY not U ??? ]

    Finding #3: Accelerator driven subcritical systems can be utilized to efficientlyburn minor actinide waste .

    Finding #4: Accelerator driven subcritical systems can be utilized to generatepower from thorium-based fuels

    MIT Energy Initiative;OBamas Blue Ribbon Panel 100 year horizon, no new direction, yet continue DOE-NE funding at current level

    DOE NE thinking about an ADS demonstration in 2050 (ie, when Im 90 )

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    ADS Technology Readiness AssessmentTransmutation

    Demonstration

    Industrial Scale

    Transmutation

    Power

    GenerationFront End System PerformanceReliability

    AcceleratingSystem

    RF Structure Development and PerformanceLinac Cost Optimization

    ReliabilityRF Plant Performance

    Cost Optimization Reliability

    Beam Delivery PerformanceTarget Systems Performance

    ReliabilityInstrumentationand Control

    Performance

    Beam Dynamics Emittance/halo growth/beamlossLattice design

    Reliability Rapid SCL Fault RecoverySystem Reliability Engineering Analysis

    34

    Green: ready, Yellow: may be ready, but demonstrationor further analysis is required, Red: more development isrequired.

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    Table was based on outdated criteria, permitting modest R&D butdeferring ADS for power to distant future.

    helps motivate Intensity Frontier (ie: Project X at Fermilab) ;but higher efficiency via higher-power beams is not a requirement;$100s of millions are going into solar and wind which have far greater outages.

    DOE-NE: It takes about 20 years to validate any new fuel system, so 2050

    is the earliest one might imagine for ADS.based on input from solid-fuel manufacturers;but consider how this might change if a new system actually addressed waste,proliferation, LWR spent fuel usage, and safety (thus becoming politically,publicly, and financially desirable).

    Table 1: Range of Parameters for Accelerator Driven Systems for four missions

    described in this whitepaper

    Transmutation Demonstration

    Industrial Scale

    Transmutation

    Industrial Scale Power Generation

    with Energy Storage

    Industrial Scale Power Generation without

    Energy Storage Beam Power 12 MW 10 75 MW 10 75 MW 10 75 MW Beam Energy 0.5 3 GeV 12 GeV 12 GeV 12 GeV Beam trips (t > 5 min) < 50/year < 50/year < 50/year < 3/year Availability > 50% > 70% > 80% > 85%

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    People (and agencies) are legitimatelyafraid that if they blink theyll lose what

    they already have.

    How to proceed in this environment?

    ARPA-E: nothing nuclear at allNEUP: low relevance

    start with liquid transport fuel demonstrationusing other green energy (~$7M);transition it to nuclear (GEM*STAR)

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    ADNA (Accelerator Driven Neutron Applications, Inc)

    commercial project for liquid transportation fuel generate funds for demonstration facility

    GEM*STAR Consortium continue to engage funding agencies and raise

    awareness (DOE, ARPA-E, DTRA, NSF, NNSA, Foundations, Federal and State governments, etc) Virginia research facility Powerful motivation for existing and NEW multi-

    disciplinary research avenues