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Evaluation of the GMI Combo Model Yasuko Yoshida and Bryan Duncan Goddard Earth Science & Technology (GEST) Center, UMBC

Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

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Page 1: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

Evaluation of the GMI Combo Model

Yasuko Yoshida and Bryan Duncan

Goddard Earth Science & Technology (GEST) Center, UMBC

Page 2: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

Introduction

We are evaluating Combo simulation results using surface, aircraft and satellite measurements.

Three simulations:

1 ) GEOS-4-DAS (2004-5)

2) FVGCM (1994-1998 SSTs)

3) GEOS-4-Forecast (July 2004-June 2005) –preliminary results

Page 3: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

Projects

Impact of European pollution on surface ozone in northern Africa and Middle East

Impact of 2004 boreal fires on US air quality

Differences in transport between GEOS-4-DAS, GEOS-4-Forecast, and FVGCM meteorological fields

Page 4: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

ObservationsAircraft missions:• Japan Airlines (JAL) - CO• Measurements of OZone and water vapor by Airbus In-service airCraft

(MOZAIC) – CO, O3

Surface measurements: • NOAA Global Monitoring Division (GMD) - CO• U.S. Environmental Protection Agency (EPA) – O3

• Cooperative Programme for Monitoring and Evaluation of Long-range Transmission of Air Pollutants in Europe (EMEP) – O3

Satellite instruments:• The Aura Microwave Limb Sounder (MLS) – CO• The Ozone Monitoring Instrument (OMI) – NO2

• Atmospheric Infrared Sounder (AIRS) – CO ; see Joanna’s presentation• OMI-MLS – Tropospheric Column O3 ; see Mark Schoeberl’s

presentation ; Jerry Ziemke’s product

Page 5: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

GMD CO (1994-98) vs

GMI FVGCM (1994-98 SSTs)

⇒ Simulated CO OK in local summer/fall : photochemistry Dominates

⇒ Simulated CO too low in local winter/spring : transport dominates

A potential partial fix?Jennifer estimates that seasonality may be too low for Chinese emissions.

Page 6: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

GMD CO (2004-2005) vs

GMI DASvs

Forecast (12 and 24 hr)

⇒ Models OK in summer/fall but too low in winter/spring

⇒ DAS and Forecasts similar in the higher NH

Page 7: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

GMD CO (2004-2005) vs

GMI DASvs

Forecast (12 and 24 hr)

⇒ DAS and Forecast different in the tropics: due to different convections?

Page 8: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

0 4 8 12 16 20

lon_dim

0 60 120 180 240 300-90

-70

-50

-30

-10

10

30

50

70

90

0

2

4

6

8

10

12

14

16

18

20

22

24

lon_dim

0 60 120 180 240 300-90

-70

-50

-30

-10

10

30

50

70

90

Precipitation Jul 2004

GMI DASvs

Forecast

[mm/day]

Forecast

DAS

⇒ DAS shows much more (about x2) precipitation than Forecast over ITCZ and SPCZ

⇒ DAS has excessive convection

ITCZ

SPCZ

Page 9: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

⇒ DAS is higher than Forecast at the higher SH : Transport from tropics dominates

GMD CO (2004-2005) vs

GMI DASvs

Forecast (12 and 24 hr)

⇒ DAS and Forecast different in the tropics: due to different convections?

Page 10: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

EMEP Day-time O3 (2004) vs

GMI (GEOS-4-DAS 2004)

⇒ Simulated surface O3 in Europe is generally OK, especially from winter to spring.

⇒ Simulated O3 is too high in summer – grid resolution

A potential partial fix?Turn back on HO2 uptake onaerosols.

Page 11: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

EPA Day-time O3 (2004) vs

GMI (GEOS-4-DAS 2004)

⇒ East coast of US - similar story as in Europe, but worse over-prediction in summer:• grid resolution• isoprene nitrate formation uncertainties (EPA is working on issue).

Page 12: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

O3 Difference (DAS Model – EPA) of Monthly Mean (2004)

Page 13: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

CO Latitudinal Distribution ComparisonGEOS-4-DAS: 2004 and 2005

JAL : Tokyo ⇔ Sydney

Jan

50

100

150

200

CO

[p

pb

]

JALModel

Apr

50

100

150

200

Jul

30oS 20oS 10oS 0o 10oN 20oN 30oNLatitude

50

100

150

200

CO

[p

pb

]

Oct

30oS 20oS 10oS 0o 10oN 20oN 30oNLatitude

50

100

150

200

Too low Chinese Emissions?

Page 14: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

20

50

100

150

CO

[p

pb

]

DJF JAL (94-98)Model (94-98)

MAM

30oS 20oS 10oS 0o 10oN 20oN 30oNLatitude

20

50

100

150

CO

[p

pb

]

JJA

30oS 20oS 10oS 0o 10oN 20oN 30oNLatitude

SON

CO Latitudinal Distribution ComparisonFVGCM : 1994-1998 SSTs

JAL : Tokyo ⇔ Sydney

Climatological BB emissions misses boreal fire?

Page 15: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

CO Cruise Plots MOZAIC vs GMI (GEOS-4-DAS)

N = 623R2 = 0.77|bias| = 24%

N = 523R2 = 0.70|bias| = 12%

N = 433R2 = 0.16|bias| = 23%

N = 585R2 = 0.66|bias| = 24%

N = 406R2 = 0.59|bias| = 20%

N = 381R2 = 0.19|bias| = 18%

OSAKA->VIENNA jul 5 2004

0 100 200 300 400 500 600 7000

0

50

100

150

200

CO

[p

pb

]

35

40

45

50

55

60

65

Lat

itu

de

[N]

1000

800

600

400

200

Pre

ssu

re [

hP

a]

MOZAICGMI_DASLatitudePressure

PEKIN->MUNCHEN jul 19 2004

0 100 200 300 400 500 600 7000

0

50

100

150

200

CO

[p

pb

]

40

42

44

46

48

Lat

itu

de

[N]

1000

800

600

400

200

Pre

ssu

re [

hP

a]

WASHINGTON->VIENNA jul 14 2004

0 100 200 300 400 5000

0

50

100

150

200

CO

[p

pb

]

40

45

50

55

Lat

itu

de

[N]

1000

800

600

400

200

Pre

ssu

re [

hP

a]

MUNCHEN->LOS ANGELES jul 15 2004

0 100 200 300 400 500 600 700 8000

0

50

100

150

200

CO

[p

pb

]

35

40

45

50

55

60

65

Lat

itu

de

[N]

1000

800

600

400

200

Pre

ssu

re [

hP

a]

DELHI->VIENNA jul 3 2004

0 100 200 300 400 5000Time [min]

0

50

100

150

200

CO

[p

pb

]

30

35

40

45

Lat

itu

de

[N]

1000

800

600

400

200

Pre

ssu

re [

hP

a]

MUNCHEN->DELHI jul 29 2004

0 100 200 300 400 5000Time [min]

0

50

100

150

200C

O [

pp

b]

30

35

40

45

Lat

itu

de

[N]

1000

800

600

400

200

Pre

ssu

re [

hP

a]

Latit

ude

[N]

Latit

ude

[N]

Latit

ude

[N]

Latit

ude

[N]

Latit

ude

[N]

Latit

ude

[N]

Time [min]Time [min]

Page 16: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

jan

0 50 100 150

0

1000

2000

3000

4000

nu

mb

er o

f d

ata

po

ints O

3 threshold = 120 ppbv

below thrabove thr

apr

0 50 100 150

0

500

1000

1500

2000

2500

jul

0 50 100 150

0

500

1000

1500

2000

oct

0 50 100 150

0

500

1000

1500

2000

0 50 100 150

0

1000

2000

3000

4000

nu

mb

er o

f d

ata

po

ints O

3 threshold = 150 ppbv

0 50 100 150

0

500

1000

1500

2000

2500

0 50 100 150

0

500

1000

1500

2000

0 50 100 150

0

500

1000

1500

2000

0 50 100 150CO [ppb]

0

1000

2000

3000

4000

nu

mb

er o

f d

ata

po

ints O

3 threshold = 180 ppbv

0 50 100 150CO [ppb]

0

500

1000

1500

2000

2500

0 50 100 150CO [ppb]

0

500

1000

1500

2000

0 50 100 150CO [ppb]

0

500

1000

1500

2000

CO Histogram Comparison: MOZAIC vs GMIEurope ⇔ North America (2005) Stratosphere

MOZAIC CO (Tropospheric)

MOZAIC CO (Stratospheric)

DAS model CO (Tropospheric)

DAS model CO (Stratospheric)

Troposphere

Page 17: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

MLS CO vs GEOS-4-DAS for March 2005

Page 18: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

MLS CO (March 2005) vs FVGCM (March 1994-98 Mean)

Page 19: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

MLS (March 2005) vs GMI FVGCM (March 1994-8 Mean)

20°N-20°S at 100 hPa

Probability Distribution of CO:

⇒ Distributions are generally OK. (MLS CO is known too high)

Page 20: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

Probability distributions (20°S-20°N) of MLS CO (March 2005), DAS (March 2005) and FVGCM (March 1994-98 Mean)

• 15-20 ppbv CO is observed by ER-2 STEP in LS, so FVGCM is reasonable• In LS, DAS is closer to MLS due to biases of both model and observations.• DAS causes more vertical mixing

Page 21: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

Probability distributions (20°S-20°N) of MLS CO, DAS, FVGCM and Forecast (12- and 24- hour)

• Both Forecast runs are close to FVGCM in UT.• In LS, Forecasts are between FVGCM and DAS.• There is no difference between the two Forecast runs in UT.

Page 22: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

Tropospheric O3: OMI-MLS* vs DAS (March 2005)

0.0 11. 22. 33. 44. 56. 67. 78. 89. 100.

0.0 3.4 6.9 10.3 13.8 17.2 20.7 24.1 27.6 31.

• Model captures the general features well, but overestimates the observations over the tropical Atlantic, northern Africa, near the Himalayas.

*Jerry Ziemke’s product.

[days][ppbv]

Page 23: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

Tropospheric O3: OMI-MLS vs DAS (August 2005)

0.0 11. 22. 33. 44. 56. 67. 78. 89. 100.

0.0 3.4 6.9 10.3 13.8 17.2 20.7 24.1 27.6 31.

• Model overestimates the observations from west Asia to entire China, and also over northeastern US.

•Middle East ozone maximum not obvious in observations.

[days][ppbv]

Page 24: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

Surface CO comparisons using GMD observations show that our model CO is too low during local winter and spring indicating possible problems with transport and/or seasonality of emissions.

Latitudinal distribution comparisons of CO using JAL data show the GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo.

For surface O3 comparisons, the GMI model show high biases during summer over western Europe and the northeastern US, partly reflecting uncertainties in our isoprene chemistry and problems of grid resolution.

Based on histogram comparisons of CO using MOZAIC data, our model overestimates stratospheric CO, but underestimates tropospheric CO especially in winter and spring.

Conclusions

Page 25: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

The model Comparison to MLS CO is reasonable, if we take into account the known high bias of current MLS CO concentrations.

The model reproduces very well the seasonal cycles and latitudinal distributions of tropospheric O3 columns except high emission regions such as China.

The intermodel comparisons using CO histograms with DAS, FVGCM and Forecast fields show that DAS gives the fastest vertical transport to the LS, and Forecast yields similar results as FVGCM in the UT, but higher in the LS.

Conclusions

Page 26: Evaluation of the GMI Combo Model · 2017. 1. 24. · GMI DAS and FVGCM both underestimate the CO especially close to emission regions near Tokyo. For surface O 3 comparisons, the

OMI NO2 product vs GMI

AIRS CO vs GMI

OMI-MLS O3 vs GMI

On going evaluation