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Emerging Modules for ASMs: Emerging Modules for ASMs: Chemistry – Chemistry – Aerosols – Aerosols – Clouds Clouds J-P Blanchet, É. Girard, C. Jones, J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof, P. Du, Stefanof, P. Du, A.Tatarevic, P. Dehasse, Y. Melin, D. Simjanoski, C. Jouan, J. A.Tatarevic, P. Dehasse, Y. Melin, D. Simjanoski, C. Jouan, J. Dorais, G. Dueymes Dorais, G. Dueymes S-A. Demers-Giroux, J.-N. Blanchet S-A. Demers-Giroux, J.-N. Blanchet Department of Earth and Atmospheric Sciences (SCTA) Department of Earth and Atmospheric Sciences (SCTA) Institute of Environmental Sciences (ISE) Institute of Environmental Sciences (ISE) University of Quebec at Montreal (UQAM) University of Quebec at Montreal (UQAM) and collaboration with and collaboration with S. Gong S. Gong MSC MSC Presented at the Presented at the International collaboration in Arctic System Modelling Workshop International collaboration in Arctic System Modelling Workshop July 16–17 July, University of Quebec at Montreal July 16–17 July, University of Quebec at Montreal Funding Agencies Partners

Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

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Page 1: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Emerging Modules for ASMs: Emerging Modules for ASMs: Chemistry – Chemistry – Aerosols – CloudsAerosols – Clouds

J-P Blanchet, É. Girard, C. Jones, J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof, P. Du,P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof, P. Du,

A.Tatarevic, P. Dehasse, Y. Melin, D. Simjanoski, C. Jouan, J. Dorais, G. DueymesA.Tatarevic, P. Dehasse, Y. Melin, D. Simjanoski, C. Jouan, J. Dorais, G. DueymesS-A. Demers-Giroux, J.-N. BlanchetS-A. Demers-Giroux, J.-N. Blanchet

Department of Earth and Atmospheric Sciences (SCTA)Department of Earth and Atmospheric Sciences (SCTA)Institute of Environmental Sciences (ISE)Institute of Environmental Sciences (ISE)

University of Quebec at Montreal (UQAM)University of Quebec at Montreal (UQAM)

and collaboration withand collaboration with

S. GongS. GongMSCMSC

Presented at the Presented at the International collaboration in Arctic System Modelling WorkshopInternational collaboration in Arctic System Modelling Workshop

July 16–17 July, University of Quebec at MontrealJuly 16–17 July, University of Quebec at Montreal

Funding AgenciesPartners

Page 2: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Aerosol Impact on the Weather and Climate SystemAerosol Impact on the Weather and Climate System

To be completed …

PermafrostSoil Moisture

Sea Ice

Sea Ice

Snow Cover

River Flow

Cold WinterTemperatures

ForestFires

Sea

Ice

Exp

ort

IndustrialAerosols

WarmSummer

DMSaerosol

L

Sea Ice

Smoke

Bio aerosolsClimateHydrologyAir Quality

Page 3: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

AVHRR T 20 yr Summer Temperature Trend NASA/Goddard Space Flight Center

Scientific Visualization Studio, Larry Stock, Robert Gersten based on data analysis by Joey Comiso (NASA)

Sea ice-albedo feedback (+)

Snow-albedo feedback (+)

A rapidly declining perennial sea ice cover in the Arctic, Geophysical Research Letters, Vol. 29, No. 20, October 2002

http://svs.gsfc.nasa.gov/search/Keyword/Arctic.html

Mean Annual Trend °C / yr

Page 4: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

AVHRR T 20 yr Winter Temperature Trend 1982-2002 NASA/Goddard Space Flight CenterScientific Visualization Studio, Larry Stock, Robert Gersten (2003)

Raatz, 1991

CGCM1/IS92a-Winter

2040-60 minus 1975-95

Mean Annual Trend °C / yr

Page 5: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Evidences of Evidences of aerosol alterations in the Arcticaerosol alterations in the Arctic

Bigg (1980) observed Bigg (1980) observed sulfuric acid coatingsulfuric acid coating on on nearly all other aerosol nearly all other aerosol particles during winterparticles during winter

Boris observed Boris observed reduced reduced ice nuclei activityice nuclei activity by 100 by 100 to 10000 fold in crystal to 10000 fold in crystal counts during counts during anthropogenic Arctic anthropogenic Arctic haze event.haze event.

Reaction on calcium fluorideRef.: Bigg, 1980

Page 6: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

NARCM: Aerosol Size-Specie ResolvedNARCM: Aerosol Size-Specie Resolved

• Flexible model structure• Multi-components Simulations• Physically based size distribution• Numeric diffusion for particle growth• Computational intensive (large bin no.)

Gong, Barrie and Blanchet et al. 2003, JGR

Size

Mas

s

CanadianAerosol ModuleGong et al (1997, 2003)

D yn am icsP h ysics

S em i-lagran giantracer tran sp ort

C R C MC a na d ia n R e g io na l C lim a t M o d e l

A eroso l sou rcef u n ction

A eroso l p rocesses

C A MC a na d ia n A e r o so l M o d ule

N A R C MN o r the r n A e r o so l C lim a te M o d e l

• Saltation• Sea spray • Chemistry• Incloud oxydation• DMS• Volcano• Anthropogenic

• Nucleation• Condensation• Coagulation• Sedimentation• Wet deposition• dry deposition

65 full 4D tracers

12 size bins X 5 species

Page 7: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Model and Validation Structure

+

Canadian Regional Climate Model (GEM-Arctic)

Canadian Aerosol Module (CAM)+

Chemistry (GEM-AQ) +

Mixed Phase Cloud Resolving (GEM-CRM)

EarthCARE Instrument Simulator (Radar+Lidar+Rad+MLS)

+

Leve

l 2: V

alid

atio

n -

Clo

sure

A-Train: CloudSat-CALIPSO-MLS

Le

vel 1

Standard ProductsAlgorithms

PEARL / SHEBA / IPY

Laboratory

Instrumented Flights

New dedicated satellite instrument : TICFIRE

Page 8: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

A-Train : CloudSat – CALIPSO – AQUA – AURA – AIRSA-Train : CloudSat – CALIPSO – AQUA – AURA – AIRS

Ref.: CALIPSO Web site

CALIPSO

CloudSat

Page 9: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

PEARLab (CANDAC) at Eureka on PEARLab (CANDAC) at Eureka on Ellesmere Island in the Canadian ArcticEllesmere Island in the Canadian Arctic

(80 deg N, 86 deg W, 610 meters)(80 deg N, 86 deg W, 610 meters)

Methodology:

Compare Model Simulations to ground site measurements from Eureka, Alert, Spitsbergen, and Barrowand satellite data…

Cloud RadarLidar HSRL

µwave RadiometerAt sea level

Also at 610m

Page 10: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

A-Train and PEARL ObservationsA-Train and PEARL Observations

PEARL

Page 11: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Observed Simulated

Monthly Mean Aerosol – Observed vs Simulated

Amount

Occurrence

Page 12: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Statistics for TIC – AerosolsJanuary & July 2007

Ref.: Grenier, Blanchet and Munoz-Alpizar (JGR, 2009)

Page 13: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Spain

Ala

ska

Kab

ul

Page 14: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Spain

Ala

ska

Kab

ul

Page 15: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Spain

Ala

ska

Kab

ul

TIC-2B

TIC-2A

TIC-1

Page 16: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Is there a 4th General Circulation Cell during extreme cold pole conditions?

A dynamics-aerosol-clouds-radiationInteraction on planetary scale

Lows drift NBring aerosol

Form TIC

Precipitate

Rad-CoolingAv. Pot. Energy

Page 17: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Summary Aerosol links air chemistry to climate via alteration

of cloud, precipitation, radiation and circulation in important ways.

Spreading over 5 orders of magnitudes, aerosol physics need adequate size and species resolution for treatment (6D).

Including explicit aerosol may now be optional, but will become essential for proper climate simulations.

Due to time and spatial scales, arctic aerosols are an important research topic.

Page 18: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Further at MOCA-2009

M 13.9 Stefanof et al (Monday 17h00)

M 13.10 Grenier et al (Monday 17h15)

M 13.12 Munoz et al (Monday 17h45)

J 03.17 Blanchet et al (Tuesday 9h30)

J 02.5 Blanchet et al (Wednesday 14h30)

M 12.1 Bertram et al (Thursday 10h30)

M 12.5 Girard et al (poster M557 Thursday)

J 02.2 Dorais et al (Poster J283 Wednesday)

J 02.1 Simjanovski et al (Poster J282 Wednesday)

Page 19: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Cold- Dry anomaly

Fast growing Ice

Aerosol lifting

Aerosol index

Page 20: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Process #1 – Adiabatic CoolingDynamics

Time Scale : ~ 6 – 24 hours

DT ≈ -10 to -20°C

Page 21: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Process #2 – Direct IR CoolingEmission from Ice Clouds

TIC-2B TIC-1

Time Scale : ~ 1 – 5 days

Heating Rate

0

2

4

6

8

10

12

14

16

18

20

-5.0 -4.0 -3.0 -2.0 -1.0 0.0 1.0 2.0 3.0

00:00-03:00

03:00-06:00

06:00-09:00

09:00-12:00 TIC-2B

DT ≈ -3 to -8°C

TIC 1

0

2

4

6

8

10

12

14

16

18

20

-5.0 -4.0 -3.0 -2.0 -1.0 0.0 1.0 2.0 3.0

12:00-15:00

15:00-18:00

18:00-21:00

21:00-24:00 TIC-1

DT ≈ 0 to +2°C

Page 22: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Process #3 – Indirect IR CoolingEmission due to Lost Water Vapour

Time Scale : ~ 1 – 2 weeks

DT ≈ -5 to -10°C

PCP-Water ~ 1 mm Model Bias + 0.3 mm

DRY Anomaly

Page 23: Emerging Modules for ASMs: Chemistry – Aerosols – Clouds J-P Blanchet, É. Girard, C. Jones, P. Grenier, R. Munoz-Alpizar, T. Ayash, A. Stefanof, C. Stefanof,

Net Effect of all 3 Processes

Total Cooling ≈ -30 to -40°C

TIC-2B TIC-1

Process #1: Dynamics

Process #2: Direct IR

Process #3: Indirect IRDry radiation

Dry adiabatic