13
A review of studies on fluid flow passing through an ideal aggregate Part I: Models with an uniformly permeable porous layer Rong Yuan Qingdao University College of Mathematics 308 Ningxia Road, Qingdao, Shandong 266071 P. R. China [email protected] Abstract: This is a review of studies on fluid flow passing through an isolated ideal aggregate with a porous layer with the uniformly permeability. Fluid flows are governed by the Brinkman’s extension of Darcy’s law and continuity equation. These equations with appropriate boundary conditions are analytically solved by introducing stream functions, respectively. The comparisons between Kim & Yuan’s cell model with a porous layer with the uniformly permeability and other previous works are investigated. Key–Words: ideal aggregate; porous media; uniformly permeability; drag force 1 Introduction Fluids are substances whose molecular structure of- fers no resistance to external shear forces: even the smallest force causes deformation of fluid particles. Fluid flow is caused by the action of externally ap- plied forces. Common driving forces include pressure differences, gravity, shear, rotation, and surface ten- sion. The effect of the driving forces differ consid- erably when fluids pass objects with different perme- abilities so that fluid behavior changes significantly. Therefore, study of the hydrodynamics of fluid flow passing impermeable or porous objects is important in the theory of fluid dynamics. Porous media can be found in many instances in natural and engineered systems such as soil and rocks in nature; animal and plant tissues in biology [10, 17]; and aggregates formed during sedimentation and granular filtration in water and wastewater treat- ment. When fluid flows pass through these porous medium, the characteristics of flows are closely re- lated to the hydrodynamic properties of the porous medium. For example, in water and wastewater treat- ment using membrane filtration, the product flow and membrane life-span are affected by hydrodynamic properties of the porous medium such as permeabil- ity and selectivity. Therefore, study for hydrodynam- ics of fluid flow passing through porous media is very important in real applications. Fluid flow relative to aggregates of fine parti- cles is also of significance in processes of conven- tional water and wastewater treatment such as coagu- lation/flocculation, sedimentation, and granular filtra- tion as well as advanced treatment such as membrane filtration [1, 13, 22, 25, 26, 28, 31, 41, 43, 44]. There are four pressure-driven membrane sepa- ration process: Microfiltration (MF), Ultrafiltration (UF), Nanofiltration (NF) and Reverse Osmosis (RO). MF removes contaminants from a fluid by passage through a microporous membrane. A typical micro- filtration membrane pore size range is 0.1 to 10µm. UF is a variety of membrane filtration in which hy- drostatic pressure forces a liquid against a semiper- meable membrane. Suspended solids and solutes of high molecular weight are retained, while water and low molecular weight solutes pass through the mem- brane. This separation process is used in industry and research for purifying and concentrating macromolec- ular (10 3 - 10 6 Da) solutions, especially protein so- lutions. NF is a relatively recent membrane process used most often with low total dissolved solids water such as surface water and fresh groundwater to soften water (polyvalent cation removal) and remove disin- fection by-product precursors such as natural organic matter and synthetic organic matter. NF is widely used in food processing applications such as dairy for simultaneous concentration and partial (monovalent ion) demineralization. RO is a separation process that uses pressure to force a solution through a membrane that retains the solute on one side and allows the pure solvent to pass to the other side. More formally, it is the process of forcing a solvent from a region of high solute concentration through a membrane to a region of low solute concentration by applying a pressure in excess of the osmotic pressure. This is the reverse WSEAS TRANSACTIONS on MATHEMATICS Rong Yuan E-ISSN: 2224-2880 690 Issue 6, Volume 12, June 2013

A review of studies on fluid flow passing through an ideal ... · Part I: Models with an uniformly permeable porous layer Rong Yuan Qingdao University College of Mathematics 308

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Page 1: A review of studies on fluid flow passing through an ideal ... · Part I: Models with an uniformly permeable porous layer Rong Yuan Qingdao University College of Mathematics 308

A review of studies on fluid flow passing through an ideal aggregatePart I: Models with an uniformly permeable porous layer

Rong YuanQingdao University

College of Mathematics308 Ningxia Road, Qingdao, Shandong 266071

P. R. [email protected]

Abstract: This is a review of studies on fluid flow passing through an isolated ideal aggregate with a porouslayer with the uniformly permeability. Fluid flows are governed by the Brinkman’s extension of Darcy’s law andcontinuity equation. These equations with appropriate boundary conditions are analytically solved by introducingstream functions, respectively. The comparisons between Kim & Yuan’s cell model with a porous layer with theuniformly permeability and other previous works are investigated.

Key–Words: ideal aggregate; porous media; uniformly permeability; drag force

1 IntroductionFluids are substances whose molecular structure of-fers no resistance to external shear forces: even thesmallest force causes deformation of fluid particles.Fluid flow is caused by the action of externally ap-plied forces. Common driving forces include pressuredifferences, gravity, shear, rotation, and surface ten-sion. The effect of the driving forces differ consid-erably when fluids pass objects with different perme-abilities so that fluid behavior changes significantly.Therefore, study of the hydrodynamics of fluid flowpassing impermeable or porous objects is importantin the theory of fluid dynamics.

Porous media can be found in many instancesin natural and engineered systems such as soil androcks in nature; animal and plant tissues in biology[10, 17]; and aggregates formed during sedimentationand granular filtration in water and wastewater treat-ment. When fluid flows pass through these porousmedium, the characteristics of flows are closely re-lated to the hydrodynamic properties of the porousmedium. For example, in water and wastewater treat-ment using membrane filtration, the product flow andmembrane life-span are affected by hydrodynamicproperties of the porous medium such as permeabil-ity and selectivity. Therefore, study for hydrodynam-ics of fluid flow passing through porous media is veryimportant in real applications.

Fluid flow relative to aggregates of fine parti-cles is also of significance in processes of conven-tional water and wastewater treatment such as coagu-lation/flocculation, sedimentation, and granular filtra-

tion as well as advanced treatment such as membranefiltration [1, 13, 22, 25, 26, 28, 31, 41, 43, 44].

There are four pressure-driven membrane sepa-ration process: Microfiltration (MF), Ultrafiltration(UF), Nanofiltration (NF) and Reverse Osmosis (RO).MF removes contaminants from a fluid by passagethrough a microporous membrane. A typical micro-filtration membrane pore size range is 0.1 to 10µm.UF is a variety of membrane filtration in which hy-drostatic pressure forces a liquid against a semiper-meable membrane. Suspended solids and solutes ofhigh molecular weight are retained, while water andlow molecular weight solutes pass through the mem-brane. This separation process is used in industry andresearch for purifying and concentrating macromolec-ular (103 - 106 Da) solutions, especially protein so-lutions. NF is a relatively recent membrane processused most often with low total dissolved solids watersuch as surface water and fresh groundwater to softenwater (polyvalent cation removal) and remove disin-fection by-product precursors such as natural organicmatter and synthetic organic matter. NF is widelyused in food processing applications such as dairy forsimultaneous concentration and partial (monovalention) demineralization. RO is a separation process thatuses pressure to force a solution through a membranethat retains the solute on one side and allows the puresolvent to pass to the other side. More formally, it isthe process of forcing a solvent from a region of highsolute concentration through a membrane to a regionof low solute concentration by applying a pressure inexcess of the osmotic pressure. This is the reverse

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of the normal osmosis process, which is the naturalmovement of solvent from an area of low solute con-centration, through a membrane, to an area of highsolute concentration when no external pressure is ap-plied. The membrane here is semipermeable, meaningit allows the passage of solvent but not of solute.

MF and UF are widely used for particulate re-moval, capable of separating particulate materialsranging from 10 nm to 10 microns. In the processesof MF/UF, particles within the feed stream are sub-jected to a drag force and accumulate near the mem-brane surface and tend to axially migrate to the out-let of the membrane. The boundary layer concentra-tion modifies the solution properties of viscosity anddensity, and solute molecular diffusivity [29]. DuringMF and UF processes, flux decline occurs due to var-ious fouling phenomena such as concentration polar-ization, deposition and adsorption of retained soluteson membrane surfaces, and pore blocking/plugging ofmembranes.These phenomena result in a decreasingdriving force on permeation due to enhanced resis-tances against solvent transport through membranes[4, 5, 11, 12, 38, 39]. In MF and UF processes, aggre-gate cake formation is one pattern of matter-stackingphenomena on the membrane surfaces, while otherpatterns cause distinguishable behaviors of permeateflux decline [2, 3, 6, 8, 9, 18, 24, 32, 33, 34, 35, 36,37, 47, 48].

The major limiting factor of filtration perfor-mance is the ratio of permeate flux (with appropri-ate water quality) to operation/maintenance cost, of-ten increasing due to membrane fouling. When co-agulation/flocculation of the conventional water andwastewater treatment is used as a pretreatment or co-process of MF/UF applications, a higher permeateflux is observed because deposited aggregates gener-ate much more porous and permeable structures thanthose of cake layers composed of individual colloidalparticles. This phenomenon, so-called aggregate-enhanced membrane filtration (AEMF),[14, 19, 20,23, 28, 31, 42, 45, 46], has significant potential in opti-mizing MF/UF processes and possibly minimizing theoperation/maintenance cost, but it has not been fullyaddressed with rigorous fundamentality. An in-depthanalysis of fluid flow relative to the aggregates will,therefore, lead to a better understanding of AEMF.

2 Drag force exerted on isolatedspherical objects

The study for hydrodynamics of fluid flow relative toan impermeable sphere dates back to about 150 yearsago [40]. Fluid flow was governed by the Stokes equa-

tion and continuity equation. Almost 100 years later,Brinkman [7] studied fluid flow passing through anisolated sphere of uniform permeability. In 1987 [27],Masliyah, et al. combined Stokes’ and Brinkman’smodels together and studied the creeping flow past asolid sphere with a uniformly porous shell.

2.1 Stokes’ model

In 1851 [40], Stokes studied the effect of the internalfriction of fluids on the motion of pendulums. As oneof the applications of the theory, he investigated thehydraulic resistance of a sphere moving uniformly ina homogeneous fluid, which can be obtained as a lim-iting case of the resistance to a ball pendulum.

Let u be the fluid velocity and ur,uθ and uϕ thecomponents of the velocity along the spherical coor-dinate system of r, θ and ϕ, respectively, p the pres-sure, and µ the viscosity of the fluid. When the fluidis homogeneous, incompressible, and Newtonian, thegoverning equations are

µ∇2u = ∇p (1)

and continuity equation

∇ · u = 0 (2)

Besides the general equations of Eqs.(1) and (2),boundary equations of the fluid flow need to be con-sidered. For convenience, there will be no occasionto consider the case of a free surface, only that of thecommon surface of the fluid and a solid. If the fluidimmediately in contact with a solid could flow pastit with a finite velocity, it would follow that the solidwas infinitely smoother with respect to its action onthe fluid than the fluid with respect to its action on it-self. Let R be the radius of the solid whose center islocated at the origin of spherical coordinates (r, θ, ϕ).The fluid flow approaches in the +Z direction withvelocity V , as depicted in Figure 1, due to the axi-symmetry of the fluid flow relative to an isolated per-meable sphere. The boundary conditions are as fol-lows:

ur (R, θ) = 0 (3a)uθ (R, θ) = 0 (3b)

limr→+∞

ur (r, θ) = V cos θ (3c)

limr→+∞

uθ (r, θ) = −V sin θ (3d)

To solve the governing equations of Eqs. (1) and(2) with boundary conditions (3), Stokes introduced astream function ψ(r, θ) which satisfies the following

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+Z

r

ur

R

θ

V

Approaching

fluid

Solid

space

Figure 1: Coordinate system for axi-symmetric fluidflow relative to a solid sphere

equations:

ur = − 1

r sin2 θ

∂ψ

∂θ(4a)

uθ =1

r sin θ

∂ψ

∂r(4b)

Then the governing equations (1) and (2) become thefollowing partial differential equations in a form of thestream function ψ(r, θ):

E4ψ = 0 (5)

where E2 is a differential operator defined as

E2 =∂2

∂r2+

sin θ

r2∂

∂θ

(1

sin θ

∂θ

)(6)

The general solution of Eq. (5) is:

ψ =1

2V

(A

r+Br + Cr2 +Dr4

)sin2 θ (7)

where coefficients A,B,C and D are determined byusing the boundary conditions (3) as follows:

A =R3

2, B = −3R

2, C = 1, and D = 0 (8)

Stokes [40] also calculated the drag force exerted onthe solid sphere

F = 2πR2

∫ π

0(−τrr cos θ + τrθ sin θ)|r=R sin θdθ

(9)

where τrr and τrθ are normal and tangential compo-nents of the stress tensors of fluid flow, respectively.They are defined as follows:

τrr = −p+ 2µ∂ur∂r

(10a)

τrθ = µ

(1

r

∂ur∂θ

+∂uθ∂r

− uθr

)(10b)

Using Stokes’ law, the dimensionless drag force Ω isintroduced as

Ω =F

6πµV R2(11)

then, it is represented as

Ω = −2B

3R(12)

components of the flow velocity are

ur =

(1 +

1

2

R3

r3− 3

2

R

r

)cos θV (13)

and

uθ =

(−1 +

1

4

R3

r3+

3

4

R

r

)sin θV (14)

and, therefore the dimensionless drag force is

ΩS = 1 (15)

2.2 Brinkman’s model

Brinkman [7] studied a solution of long chainmolecules in which each polymer molecule forms amolecular cluster. He also studied sedimentation ve-locity of the molecular cluster and the viscosity ofsuch solutions. According to this model, each molecu-lar cluster is represented by a porous sphere which hasa constant hydraulic permeability. Similar to Stokes’smodel, let R be the radius of the porous sphere whichcenters at the origin of spherical coordinates (r, θ, ϕ),and the flow approaches to the sphere in the +Z direc-tion with a uniform velocity V , as shown in Figure 2Let u be the fluid velocity outside the porous sphere,u∗ = (u∗r , u

∗θ, u

∗ϕ) the velocity of fluid through the

porous sphere. The azimuthal component of u∗, u∗ϕ,is zero due to the spherical symmetry. According toBrinkman, the fluid flow through the porous sphere isgoverned by the extension of Darcy’s law (so calledBrinkman’s extension of Darcy’s law or Brinkman’sEquation [7]. The governing equations outside andinside of the porous sphere are

µ∇2u = ∇p, r > R (16a)

µ∗∇2u∗ − µ∗

κu∗ = ∇p∗, 0 < r < R(16b)

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+Z

r

ur

R

θ

V

Approaching

fluid

Uniformly

porous sphere

Figure 2: Coordinate system for axi-symmetric fluidflow relative to a porous sphere

respectively, and the continuity equations are,

∇ · u = 0, r > R (17a)∇ · u∗ = 0, 0 < r < R (17b)

where p and p∗ are pressures, µ and µ∗ viscositiesof fluid, and κ is the permeability of the uniformlyporous sphere.

It is assumed that the velocity of fluid flow atthe center of the porous sphere is finite, the normaland tangential components of velocity and stress ten-sor across the porous sphere interface are continuous,and the flow is unidirectional far from the permeablesphere. So the boundary conditions are

limr→0

u∗r is finite (18a)

limr→0

u∗θ is finite (18b)

ur (R, θ) = u∗r (R, θ) (18c)uθ (R, θ) = u∗θ (R, θ) (18d)τrr (R, θ) = τ∗rr (R, θ) (18e)τrθ (R, θ) = τ∗rθ (R, θ) (18f)

limr→∞

ur = V cos θ (18g)

limr→∞

uθ = −V sin θ (18h)

where τrr∗ and τrθ∗ are normal and tangential com-ponents of the stress tensors inside the porous sphere,

respectively, which are defined as follows:

τ∗rr = −p∗ + 2µ∗∂u∗r∂r

(19a)

τ∗rθ = µ∗(1

r

∂u∗r∂θ

+∂u∗θ∂r

−u∗θr

)(19b)

With the incompressibility of the Newtonian fluid im-plied in Eq. (17), it has been proven that the continu-ity of the normal stress is equivalent to that of the fluidpressure [14, 23]:

p∗ (R, θ) = p (R, θ) (20)

Similar to Eq. (4), ψ∗ (r, θ) is defined

u∗r = − 1

r2 sin θ

∂ψ∗

∂θ(21a)

u∗θ =1

r sin θ

∂ψ∗

∂r(21b)

Then, the governing Eqs.(16) and (17) are combinedinto the 4th order partial differential equations

E4ψ = 0, r > R (22a)

E4ψ∗ − 1

κE2ψ∗ = 0, 0 < r < R (22b)

where E2 is defined by the Eq. (6). The generalsolutions of Eq. (22) are

ψ = −κV2

(A

ξ+Bξ + Cξ2 +Dξ4

)sin2(θ),

ξ > β (23a)

ψ∗ = −κV2

[E

ξ+ Fξ2 +G

(cosh ξ

ξ− sin ξ

)+H

(sinh ξ

ξ− cosh ξ

)]sin2(θ),

0 < ξ < β (23b)

where ξ = r/√κ and β = R/

√κ. Using boundary

conditions of Eq. (18), one can determine coefficientsA−H as follows:

A =β3

JB

[−2β2 + 3

(β2 + 2

)(1− tanhβ

β

)](24a)

B = −3β3

JB

(1− tanhβ

β

)(24b)

C = 1 (24c)D = 0 (24d)E = 0 (24e)

F =3

JB

(1− tanhβ

β

)(24f)

G = 0 (24g)

H =6β2

JB· 1

coshβ(24h)

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where JB = 2β2 + 3

(1− tanhβ

β

). The dimen-

sionless drag force ΩB is:

ΩB = −2B

3β=

2β2(1− tanhβ

β

)2β2 + 3

(1− tanhβ

β

) (25)

For a impermeable solid sphere, κ → 0, i.e., β → ∞and tanhβ/β → 0. In this case, ΩB of Eq. (15)converges to ΩS(= 1).

2.3 Masliya et al.’s model

Masliya et al [27] studied creeping flow past a solidsphere with a porous shell by combining the Stokesand Brinkman models. The dimensionless radiusof solid core and shell thickness, normalized by thesquare root of the shell permeability, govern the fluidflow inside and outside the porous shell. In the lim-iting cases, the analytical solution describing the flowpast the composite sphere reduces to those for flowpast a solid sphere (Stokes’ case [40]) and a homoge-neous porous sphere (Brinkman’s case [7]).

Let b be the outer radius of the porous shell ofthe isolated composite sphere and a the radius of thesolid impermeable sphere surrounded by the porousshell. It is assumed that the porous shell is homoge-neous and isotropic with a constant permeability κ.The creeping flow of the Newtonian fluid of viscosityµ is assumed to be steady and axi-symmetric. For con-venience, the authors considered the sphere to be sta-tionary having its center at the origin of spherical co-ordinates (r, θ, ϕ), while a constant fluid is approach-ing in the +Z direction at velocity V , as shown in Fig-ure 3. Let u = (ur, uθ, uϕ) and u∗ = (ur

∗, uθ∗, uϕ

∗)denote the velocity vectors of fluid flow through theoutside of the composite sphere and the porous shell,respectively. The governing equations are as follows:

µ∇2u = ∇p, r > b (26a)

µ∗∇2u∗ − µ∗

κu∗ = ∇p∗, a < r < b (26b)

the continuity equations of

∇ · u = 0, r > b (27a)∇ · u∗ = 0, a < r < b (27b)

where µ, µ∗, p, p∗ and κ have the same meaningsas described above. The pressure profiles of p and p∗satisfy the following equation:

p (b, θ) = p∗ (b, θ) (28)

+Z

r

ur

b

a

θ

V

Approaching

fluid

Solid sphere

Uniformly

porous layer

Figure 3: Coordinate system for axi-symmetric fluidflow relative to a composite sphere comprising asolid impermeable sphere surrounded by a uniformlyporous shell

andµ = µ∗ (29)

is assumed [14, 24].For the present problem, the boundary conditions

are described as follows:

u∗r (a, θ) = 0 (30a)u∗θ (a, θ) = 0 (30b)ur (b, θ) = u∗r (b, θ) (30c)uθ (b, θ) = u∗θ (b, θ) (30d)τrr (b, θ) = τ∗rr (b, θ) (30e)τrθ (b, θ) = τ∗rθ (b, θ) (30f)limr→∞

ur = V cos θ (30g)

limr→∞

uθ = −V sin θ (30h)

In the limit of a = b = R, Eq. (30) is identical to Eq.(18)

To solve the governing equation (26) and (27)with the boundary conditions of Eq. (30), the streamfunctions ψ and ψ∗ of Eq. (23) satisfy the followingpartial differential equations:

E4ψ = 0, r > b (31a)

E4ψ∗ − 1

κE2ψ∗ = 0, a < r < b (31b)

The general solutions of the stream functions ψ (ξ, θ)and ψ∗ (ξ, θ) can be expressed as follows, which are

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similar to Eq. (7) and Eq. (23), respectively.

ψ = −κV2

(A

ξ+Bξ + Cξ2 +Dξ4

)sin2(θ),

ξ > β (32a)

ψ∗ = −κV2

[E

ξ+ Fξ2 +G

(cosh ξ

ξ− sin ξ

)+H

(sinh ξ

ξ− cosh ξ

)]sin2(θ),

α < ξ < β (32b)

where ξ = r/√κ, α = a/

√κ and β = b/

√κ. In

terms of functional forms, Eqs. (7) and (32a) areidentical using r and ξ, respectively; Eqs. (23b) and(32b), of the same form, are applied to different radi-cal ranges.

Using the boundary conditions of Eq. (30), thesecoefficients from A to H are determined as follows:

B =1

2JM

[(3α3 − 9β α2 + 9α+ 6β3

)sinh∆

+(−3β α3 + 9α2 − 9β α− 6β4

)cosh∆

](33)

where

JM =(3α2 − 3

)sinh∆

+(α3 + 3α+ 2β3 + 3β

)cosh∆− 6α

(34)and

∆ = β − α

Note that the expression for B in Eq. (33) is anotherform of B in Eq. (21) in Masliya et al.’s paper [27].

H =1

JM

[−3

(α3 + 2β3

)coshα

+9α (−β sinhβ + coshβ+α sinhα− coshα)]

(35)

G =(sinhα− α coshβ)H − 3α

α sinhβ − coshα(36)

F =G coshα+H sinhα

3α(37)

E = 2B + 2Fβ3 (38)

= 1 (39)

D = 0 (40)

A = −Bβ2 + E + Fβ3 + (coshβ − β sinhβ)G+(sinhβ − β coshβ)H − β3

(41)Masliya et al. calculated the dimensionless drag forcedefined as

ΩM =2B

3β(42)

and the expression of ΩM is

ΩM =1

3JM

[(−3α3 + 9β α2 − 9α− 6β3

)sinh∆

+(3β α3 − 9α2 + 9β α+ 6β4

)cosh∆

](43)

If a = b = R and R → ∞, then ∆ = 0 and α = β =R/

√κ→ ∞, and then ΩM → ΩH .

3 Drag force exerted on cells withuniformly porous layer

In 1958 [16], Happel put Stokes’ sphere into a spher-ical cell to develop an cell model to study fluidflow passing through a swarm of equal-sized parti-cles swarm. In 1973 [30], Neale et al. followed Hap-ple’s approach to research fluid flow passing througha swarm of permeable spheres by adding Brinkman’smodel in a cell. In 2005 [21], Kim and Yuan includedMasliyah’s sphere in a cell to study the creeping flowover a swarm of the equal-sized composite spheresand provided the most general solution that includedthe five previous studies.

3.1 Happel’s cell model

Happel [15] studied the motion of particles relative toa fluid flow to predict the effect of concentration ofparticles on their rate of steady sedimentation underthe influence of gravity. The model assumed that par-ticles are spherical, mono-dispersed and smooth. TheNavier-Stokes equations without inertia terms wereused to describe the fluid motion. A random assem-blage consist of a number of cells, each of which con-tains a spherical particle surrounded by a fluid enve-lope; each envelope contains the same amount of fluidas the relative volume of fluid to the particle volumein the assemblage. Happel developed a sphere-in-cellmodel to describe the motion of fluids relative to bedsof spherical particles.

Happel’s cell model considered two concentricspheres: the inner sphere of a radius a representinga spherical particle, and the outer sphere of radius bthe cell containing fluid and the particle at the center.It is assume that the fluid approaching in the +Z di-rection at velocity V is steady and axi-symmetric, andthis two concentric spheres are stationary having theircenter at the origin of spherical coordinates (r, θ, ϕ),as illustrated in Figure 4 The motion of fluid is gov-erned by Stokes’ equation with continuity equation asfollows:

µ∇2u = ∇p, a < r < b (44a)∇ · u = 0, a < r < b (44b)

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+Z

r

ur

b

a

θ

V

Approaching

fluid

Solid sphere

Void space

Figure 4: Coordinate system for axi-symmetric fluidflow relative to two concentric spheres comprising asolid impermeable sphere surrounded by shell of fluid

where the axi-symmetry of the fluid gives a 2-D prob-lem. To solve the partial differential equations (44), itis assumed that the internal sphere moves with a freesurface. The boundary condition is described as fol-lows:

ur (a, θ) = 0 (45a)uθ (a, θ) = 0 (45b)ur (b, θ) = V cos θ (45c)τrθ (b, θ) = 0 (45d)

the limit of b → ∞, Eqs. (45) are identical to Eqs.(3) with a = R .

Introducing a stream function ψ (r, θ) defined byEq. (4), the governing equation Eq. (44) becomes anordinary differential equation as follows:

E4ψ = 0, a < r < b (46)

where E2 is the differential operator defined by Eq.(6). Using the boundary conditions Eq. (45), the so-lution for Eq. (46) is calculated as

ψ = −V b2

2

(A

r+Br + Cr2 +Dr4

)sin2 θ, a < r < b

(47)where

A =b3η3

−2− 3 η5 + 3 η + 2 η6(48)

B = −b(3 + 2 η5

−2− 3 η5 + 3 η + 2 η6(49)

C =3 η5 + 2

−2− 3 η5 + 3 η + 2 η6(50)

and

D = − η3

b2 (−2− 3 η5 + 3 η + 2 η6)(51)

where η = a/b. The solutions to components of thevelocity u = (ur, uθ) are

ur =

(−A

r3− B

r− C − r2D

)cos θV (52)

and

uθ =

(−1

2

A

r3+

1

2

B

r+ C + 2 r2D

)sin θV (53)

The dimensionless drag force ΩH is given as

ΩH = −2

3

2 η5 + 3

2 η6 − 2 + 3 η − 3 η5(54)

The volume fraction of spherical particles in the as-semblage can be described as ϕ = (a/b)3 = η3. TheΩH is represented as a function of ϕ as

ΩH = −2

3

2ϕ5/3 + 3

2ϕ2 − 2 + 3ϕ1/3 − 3ϕ5/3(55)

3.2 Neale et al.’s cell model

Neale et al. [30] discussed what Sutherland andTan (1970) investigated analytically regarding the sed-imentation characteristics of an isolated permeablesphere and came to the principal conclusion that in-ternal permeation could be neglected, even at overallporosities in excess of 0.9. Neale et al. comparedseveral possible solutions for the problem of creep-ing flow relative to an isolated permeable sphere, andfound that the most satisfactory solution was basedupon Brinkman’s extension of Darcy’s Law. Thissolution was generalized, using Happel’s model, tocover the problem of flow relative to a swarm of per-meable spheres.

For mathematical simplicity, they introduced asimple model that includes a permeable sphere ofradius a composed of homogeneous and isotropicporous material of permeability κ. The fluid flow wasassumed to be steady and axi-symmetric. The spher-ical particle was assumed to be stationary having itscenter at the origin of spherical coordinates (r, θ, ϕ),while the flow approaches in the +Z direction withvelocity V , as depicted in Fig. 5 The fluids outside

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+Z

r

ur

b

a

θ

V

Approaching

fluid

Uniformly

porous sphere

Void space

Figure 5: Coordinate system for axi-symmetric fluidflow relative to an isolated permeable sphere

and inside the permeable sphere were governed byNavier-Stokes equation and Brinkman’s extension ofthe Darcy equation as follows,

µ∇2u = ∇p, a < r < b (56a)

µ∗∇2u∗ − µ∗

κu∗ = ∇p∗, 0 < r < a (56b)

respectively, with continuity equations in correspond-ing regions

∇ · u = 0, a < r < b (57a)∇ · u∗ = 0, 0 < r < a (57b)

where u = (ur, uθ, uϕ), u∗ =(u∗r, u

∗θ, u

∗ϕ

); and µ,

µ∗, p, p∗, and κ∗ were defined as noted earlier with theassumption of the axi-symmetric nature of the perme-able sphere, the azimuthal coordinate ϕ may hence-forth be suppressed. The boundary conditions wereexpressed as follows:

limr→0

u∗r is finite (58a)

limr→0

u∗θ is finite (58b)

ur (a, θ) = u∗r (a, θ) (58c)uθ (a, θ) = u∗θ (a, θ) (58d)τrr (a, θ) = τ∗rr (a, θ) (58e)τrθ (a, θ) = τ∗rθ (a, θ) (58f)ur (b, θ) = V cos θ (58g)τrθ (b, θ) = 0 (58h)

where τrr, τrθ , τ∗rr and τ∗rθ were defined by Eq. (10)and Eq. (19).

To solve the governing Eqs. (56)-(57) withboundary conditions of Eq. (58), we introduce streamfunctions ψ and ψ∗ into Eq. (4) and Eq. (21), respec-tively, which should satisfy the following ordinary dif-ferential equations:

E4ψ = 0, a < r < b (59a)

E4ψ∗ − 1

κE2ψ∗ = 0, 0 < r < a (59b)

where E2 is defined in Eq. (6). By using the bound-ary conditions of Eq. (58), the general solutions for ψand ψ∗ are expressed as follows:

ψ =κV

2

(A

ξ+Bξ + Cξ2 +Dξ4

)sin2(θ),

β < ξ < β/η (60a)

ψ∗ =κV

2

[E

ξ+ Fξ2 +G

(cosh ξ

ξ− sin ξ

)+H

(sinh ξ

ξ− cosh ξ

)]sin2(θ),

0 < ξ < β (60b)

where ξ = r/√κ, β = a/

√κ and η = a/b. Coeffi-

cients A,B,C,D,E, F,G and H in Eq. (60) are de-termined by using boundary conditions from Eq. (58)as follows:

A = − 1

JNEN

[β5 + 6β3 − tanhβ

β

(3β5 + 6β3

)](61)

B =1

JNEN

[3β3 + 2β3η5 + 30βη5

−tanhβ

β

(3β3 + 12β3η5 + 30βη5

)](62)

C = −η Bβ

− 1 (63)

D = −η5A

β5(64)

E = 0 (65)

F = − B

β3− 10D (66)

G = 0 (67)

H =1

JNEN

[6β2 (sechβ)

(1− η5

)](68)

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where

JNEN = 2β2 − 3β2 η + 3β2η5 − 2β2η6

+90β−2η5 + 42 η5 − 30 η6 + 3

−tanhβ

β

(−3β2 η + 15β2η5

−12β2η6 + 90β−2η5

+72 η5 − 30 η6 + 3)

(69)

Similarly, the dimensionless drag force is calculatedas follows:

ΩNEN =2B

3β(70)

where the subscript NEN of ΩNEN represents theinitials of the last names of Neale, Epster and Nader[30].

3.3 Kim and Yuan’s cell model

Kim and Yuan (2005b) developed a model to evalu-ate hydrodynamic cake resistance due to filtered ag-gregates. An aggregate is modeled as a hydrodynam-ically and geometrically equivalent solid core with aporous shell. Creeping flow past a swarm of the com-posite spheres was solved using Stokes’ equation andBrinkman’s extension of Darcy’s law. They analyt-ically calculated the dimensionless drag force ΩKY

exerted on the composite sphere. In certain limitingcases, ΩKY converged to pre-existing analytical solu-tions for (i) an isolated impermeable sphere (Stokes’Model [40], (ii) an isolated uniformly porous sphere(Brinkman’s Model [7]), (iii) an isolated compositesphere (Masliya et al.’s Model [27]), (iv) a swarm ofimpermeable spheres (Happel’s Model [16]), and (v)a swarm of uniformly porous spheres (Neale et al.’sModel [30]).

From a hydrodynamic point of view, the flowthrough a uniform porous sphere can be categorizedinto two representative types: a slow interior flowdriven by fluid pressure and a fast exterior flow due toshear stress around the permeable sphere surface [43].This phenomenon is more apparent in a fractal ag-gregate whose central region is typically much denserthan its edge. Therefore, in their work, a fractal aggre-gate characterized by its radius and fractal dimensionis simplified to an impermeable inner core and an uni-formly permeable outer shell. Following Neale et al.’s(1973a) approach, they positioned the simplified ag-gregate at the center of the tangential stress-free cell[30], applied proper boundary conditions, and calcu-lated the hydrodynamic drag force exerted on a swarmof the model aggregates.

A primary assumption used in this study is that asolid spherical core surrounded by a uniformly porous

shell is hydrodynamically equivalent to a fractal ag-gregate with radially varying permeability. For mathe-matical convenience, the composite sphere is assumedto be stationary having its center at the origin of spher-ical coordinates (r, θ, ϕ), while the flow approaches inthe −Z direction with a constant velocity V . The ra-dius of the impermeable core is a; the outer radius ofthe porous shell with permeability κ is b (b > a); andthe radius of the hypothetical spherical cell of the freetangential stress is c (c > b). The creeping flow ofNewtonian fluid with absolute viscosity µ is consid-ered to be steady and axi-symmetric, as shown in Fig.6.

+Z

r

ur

b

ca

θ

V

Approaching

fluid

Solid sphere

Uniformly

porous layer

Void space

Figure 6: Coordinate system for axi-symmetric fluidflow relative to a composite sphere consisting of animpermeable solid sphere and a porous shell with tan-gential stress-free surface

The governing equations of incompressible New-tonian creeping flow in the void space and the porousshell covering the solid core are Stokes’ equation andBrinkman’s extension of Darcy’s law, respectively,

µ∇2u = ∇p, b < r < c (71a)

µ∗∇2u∗ − µ∗

κu∗ = ∇p∗, a < r < b (71b)

with continuity equations of

∇ · u = 0, b < r < c (72a)∇ · u∗ = 0, a < r < b (72b)

From the assumption of the axi-symmetric nature ofthe permeable sphere problem, the azimuthal coordi-nate ϕ was not considered. As we mentioned above,

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it has been proven that the continuity of the normalstress is equivalent to that of the fluid pressure [14,24], i.e.

p (b, θ) = p∗ (b, θ)

The boundary conditions are set as follows:

u∗r (a, θ) = 0 (73a)u∗θ (a, θ) = 0 (73b)u∗r (b, θ) = ur (b, θ) (73c)u∗θ (b, θ) = uθ (b, θ) (73d)τ∗rr (b, θ) = τrr (b, θ) (73e)τ∗rθ (b, θ) = τrθ (b, θ) (73f)ur (c, θ) = V cos θ (73g)τrθ (c, θ) = 0 (73h)

where τrr, τrθ , τ∗rr and τ∗rθ were defined by Eq. (10)and Eq. (19). To solve the governing equations (71)with the boundary conditions (73), stream functionsψ(r, θ) and ψ∗(r, θ) defined by Eqs. (4) and (21) areused. Then the problem is to solve the following ordi-nary differential equations:

E4ψ = 0, b < r < c (74a)

E4ψ∗ − 1

κE2ψ∗ = 0, a < r < b (74b)

where E2 is a partial differential operator defined byEq. (6). The functional form of ψ and ψ∗ are ex-pressed as follows with valid radial regions:

ψ =κV

2

(A

ξ+Bξ + Cξ2 +Dξ4

)sin2(θ),

β < ξ < γ (75a)

ψ∗ =κV

2

[E

ξ+ Fξ2 +G

(cosh ξ

ξ− sin ξ

)+H

(sinh ξ

ξ− cosh ξ

)]sin2(θ),

α < ξ < β (75b)

where ξ = r/√κ, α = a/

√κ, β = b/

√κ and γ =

c/√κ. Using the boundary conditions of Eqs. (73),

the coefficientsA−H are analytically solved, as givenin Appendix A.

Using the definition of the dimensionless dragforce ΩKY :

ΩKY (α, β, γ) =2B

3β(76)

they calculate some limiting cases of ΩKY :(i) If α → β (or κ → 0) and c → ∞, then

Stokes’s equation is obtained, i.e.

limγ→∞

limα→β

ΩKY (α, β, γ) = ΩS = 1 (77)

(ii) If α → 0 and γ → ∞, then Brinkman’sequation [7] is replicated, i.e.,

limγ→∞

limα→0

ΩKY (α, β, γ) = ΩB (78)

(iii) If γ → ∞, then Masliya’s expression [27] isreproduced, i.e.,

limγ→∞

ΩKY (α, β, γ) = ΩM (79)

(iv) If α → β (or κ → 0) and η = c/b, thenHappel’s formula [16] is retrieved, i.e.,

limα→β

ΩKY (α, β, γ) = ΩH (80)

(v) If α → 0, then Neale et al.’s work [30] isobtained, i.e.,

limα→0

ΩKY (α, β, γ) = ΩNEN (81)

The above comparison is summarized in the fol-lowing figure.

ao

Stoke, 1851

b

ao

Masliya, et al, 1987

b

o

Brinkman, 1949

c

ao

Happel, 1958

b

c

ao

Kim & Yuan, 2005a

b

c

o

Neale, et al, 1973

==========⇒

c→

∞,b→

a

======⇒

c→

==========⇒

c→

∞,a→

0

====⇒b → a====⇒a → 0

Figure 7: Comparisons between Kim & Yuan’s cellmodel with a porous layer with the uniformly perme-ability and other previous works

Appendix: Expressions of the coeffi-cients from A to H of stream functionsin Kim and Yuan’s cell model

A = −Bβ2 − Cβ3 −Dβ5 + E + Fβ3

+(coshβ − β sinhβ)G+(sinhβ − β coshβ)H

(82)

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B =1

JKY

[(−9

2αβ − 3

2β α3

−3β4 +9

2α2

)cosh∆

+

(3

2α3 − 9

2β α2

+9

2α+ 3β3

)sinh∆

]C

+

[15β3α+

(−15

2β3α

−30β4 +45

2β2α2

−5β6 − 15

2β3α3

)cosh∆

+

(30β3 − 15

2β3α2 +

45

2β2α

+15

2α3β2 + 15β5

)sinh∆

]D

(83)

where

JKY = −6α+(−3 + 3α2

)sinh∆(

3α+ 3β + 2β3 + α3)cosh∆

(84)

C =1

C0

[(−1

3

(12− 12α2

)sinh∆

−1

3

(−4α3 − 8β3 − 12β

−12α) cosh∆− 8α

)γ5

+

(−1

3

(15β3α2 − 60β3 − 30β5

−15α3β2 − 45β2α)sinh∆

−1

3

(60β4 − 45β2α2 + 15β3α

+5β3α3 + 10β6)cosh∆

+ 10β3α

)γ2

−1

3

(288β5 + 360β3 + 90β4α

+60β7 + 30β4α3

−360β3α2 − 18α2β5)sinh∆

−1

3

(−360β3α− 168β6 − 6α3β5

+90α2β4 − 360β4 − 12β8

−18αβ5 − 120β3α3)cosh∆

− 240β3α− 72αβ5

]D

+

[−4α+

(−2 + 2α2

)sinh∆

+

(2α+

4

3β3 +

2

3α3 + 2β

· cosh∆]γ3

(85)

where

C0 =

[(2− 2α2

)sinh (∆)

+

(−2

3α3 − 2α− 2β

−4

3β3)cosh∆ + 4α

]γ3

+[(−2β3 − α3 − 3α

+ 3β α2)sinh∆

+(2β4 − 3α2 + β α3

+3αβ) cosh∆] γ2

+(4β5 + 8β3 + 2α3β2

+6β2α− 2β3α2)sinh∆

+

(−2β3α− 4

3β6 + 6β2α2

−8β4 − 2

3β3α3

)cosh∆ + 4β3α

(86)

D =1

D0

[(−12β3 − 6β5 + 3β3α2

−9β2α− 3α3β2)sinh∆

+(2β6 + 12β4 − 9β2α2 + β3α3

+3β3α)cosh∆− 6β3α

(87)

where

D0 =[(−6 + 6α2

)sinh∆− 12α

+(2α3 + 6β + 4β3 + 6α

)cosh∆

]γ6

+[(9α− 9β α2 + 3α3 + 6β3

)sinh∆

+(9α2 − 6β4 − 3βα3 − 9αβ

)cosh∆

]γ5

+[−108αβ5 − 360β3α− 30β7

+(−15β4α3 − 144β5

−180β3 + 180β3α2

+9α2β5 − 45β4α)sinh∆

+(−45α2β4 + 180β4 + 180β3α

+84β6 + 3α3β5 + 9αβ5

+60β3α3 + 6β8)cosh∆

+(24β8 + 270β3α+ 60β6

−6β6α2 + 90β3α3 − 270α2β4

+36αβ5 + 12α3β5)sinh∆

+(−4β9 − 60β7 + 36α2β5

−6αβ6 − 90β4α3 − 270β4α− 2β6α3

+270β3α2)cosh∆ + 120αβ6

(88)E = 20Dβ3 + 2B + 2Fβ3 (89)

F =1

3

G coshα+H sinhα

α(90)

G = −(α coshβ − sinhα)H

α sinhβ − coshα

− 15αβ2D + 3αC

α sinhβ − coshα

(91)

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and

H =1

JKM

[9α2 sinhα− 9β α sinhβ

+(−9α− 6β3 − 3α3

)coshα

+9α coshβ]C+[45α2β2 sinhα+ 45αβ3 sinhβ

+45β2α coshβ+(−45β2α− 30β5 − 15α3β2

−90β3)coshα

]D

(92)

Acknowledgements: The research was supportedby the US National Science Foundation (CBET-0444931(CAREER) and CBET-0552413), and Qing-dao Univeristy (grant No.06300371). The authorwould like to thank Prof. Albert S. Kim for his supportand help when the author was studying at Universityof Hawaii at Manoa.

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