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A new statistical scission-A new statistical scission-point model fed with point model fed with
microscopic ingredientsmicroscopic ingredients
A new statistical scission-A new statistical scission-point model fed with point model fed with
microscopic ingredientsmicroscopic ingredients
Sophie HeinrichSophie Heinrich
CEA/DAM-Dif/DPTA/Service de Physique NucléaireCEA/DAM-Dif/DPTA/Service de Physique Nucléaire
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Workshop on the Theories of Workshop on the Theories of Fission and Related PhenomenaFission and Related PhenomenaESNT Workshop May 9- 12,ESNT Workshop May 9- 12, 2006 2006
Workshop on the Theories of Workshop on the Theories of Fission and Related PhenomenaFission and Related PhenomenaESNT Workshop May 9- 12,ESNT Workshop May 9- 12, 2006 2006
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
A new statistical scission-point A new statistical scission-point modelmodel
PreamblePreamble
A new statistical scission-point A new statistical scission-point modelmodel
PreamblePreamble
Our goalOur goal::
To reconsider the original Wilkins scission-point model (1976)in order to provide some fission fragments properties,
sustaining it with microscopic ingredients,and avoiding ad hoc parameters.
(Thesis work)
ObservationsObservations::
Wide amplitude process
Dramatic importance of shell effects of the fission fragments.
Reorganization of the nucleus internal structure
System’s “history” is simulated by a statistical statistical equilibriumequilibrium at the
scission pointscission point.Static Approach
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Fundamental HypothesisFundamental HypothesisFundamental HypothesisFundamental Hypothesis
Many reachable observables
We have:• Experimental data with new insight (exotic nuclei, super heavy nuclei) and wide energy range (SPIRAL , GSI, …)
• A need of predictions for nuclear data(used directly or as a guide for reaction models)
Why a renewal of the static approach ?Why a renewal of the static approach ? Why a renewal of the static approach ?Why a renewal of the static approach ?
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
We should provide:• Fission fragments distributions (mass, energy …)
• Fragments properties (deformation, isospin …)
Without phenomenological ajustement.
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
• Huge increase in computer processing power (CCRT, Ter@tec)
• Very good microscopic description for individual (deformed) energy levels
• New level densities
• Better comprehension of scission-point features
Possible improvements to scission-point model
Why a renewal of the static approach ?Why a renewal of the static approach ? Why a renewal of the static approach ?Why a renewal of the static approach ?
Fission fragments distributions are entirely determined at ScissionScission PointPoint by the energy available in the system of the complementary fragment pairs...
If scission point can be precisely characterized, there is no If scission point can be precisely characterized, there is no more ajustable parameter !more ajustable parameter !
Heavy fragment Light fragment
Tips distance
H L
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Scission-point ModelScission-point ModelScission-point ModelScission-point Model
Energy at the scission point =
Individual microscopic energy (Individual microscopic energy (HF + Gogny forceHF + Gogny force)) for each fragments
++ Nuclear interactionNuclear interaction between the 2 fragments
++ Coulombian interactionCoulombian interaction between the 2 fragments
Available Energy of the system =
E( compound system before fission ) – E( scission )E( compound system before fission ) – E( scission )
)(* )( relEdispo EE Available energy:
Relative probability of a given fragment pair :Relative probability of a given fragment pair :
dEhhll
hlhZ
lZ
hA
lA
llE)*,(),(
),,,,,(
),(*
0
Phase space:
hlT
τZZAAV
hlhl ddZZAAPl h
coll
hlhlhlpot
1
0
1
0
),,,,,,(
min min
)exp(),,,(
Wilkins et al.CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Basic equation Basic equation Basic equation Basic equation
If we can precisely evaluate If we can precisely evaluate DD at the scission point, at the scission point, there is no more adjustable parameters.there is no more adjustable parameters.
Heavy fragment
Light fragment
Tips Distance DD
H L
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Scission-point ModelScission-point ModelScission-point ModelScission-point Model
Evolution of 228Th distributions
D = 1fm
to 10fm
How to choose D ???
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Tips-Distance EffectTips-Distance EffectTips-Distance EffectTips-Distance Effect
Fusion path
Potential barrier
S P
Exit
Point
~ D
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Fission PathFission PathFission PathFission Path
Z Axis (fm)
radi
us
(fm
)
Q20
Selection of the Exit Points :
Strong modification of total binding energy Hexadecapolar moment drop Nucleon density at the neck < 0.01 nuc.fm-3 :
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Correlation between Scission-point and Correlation between Scission-point and Exit-pointExit-pointCorrelation between Scission-point and Correlation between Scission-point and Exit-pointExit-point
D ~ 4 to 6fm
Fit on 2 ellipsoids
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Mass and charge distributionsMass and charge distributions
228 Thorium228 Thorium
D = 5fm
Excitation energy of fissioning nucleus = 10MeV
Direct access to mass and charge yields.
Outline of involved deformations.
CEA DAM/DPTA/SPN/MED/Sophie Heinrich Journées de physique nucléaire 2006
222->228222->228ThoriumThorium
K-H. Schmidt et al.
N=132
N=134
N=136
N=138
Competition between the symmetric and the asymmetric fission for isotopes from A=222 to A=228.
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Mean Values Mean Values Mean Values Mean Values
hl
E
ddd
Ehhll
hZ
lZ
hA
lAP
ll
)*,(),(...
),,,(
),(*
0............
X
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Total Kinetic Energy : <VTotal Kinetic Energy : <Vcoulcoul + V + Vnucnuc>>Total Kinetic Energy : <VTotal Kinetic Energy : <Vcoulcoul + V + Vnucnuc>>
5UZ
A
A
Average kinetic energy for one fragment
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Average TKE of a specific fragment pairAverage TKE of a specific fragment pair Average TKE of a specific fragment pairAverage TKE of a specific fragment pair
We can pick a specific fragment pair …
… and calculate the TKE of the system distribution.
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Average deformation and excitation Average deformation and excitation energiesenergies
Average deformation and excitation Average deformation and excitation energiesenergies
A
Z
A
Average deformation of one fragment
Average excitation energy of one fragment with respect to the mass
Saw-tooth curve
Spherical/deformed and proton/neutron shell effects are well reproduce (Gogny force works fine).
Most probable configurations: reliable predictions for nuclear data with a parameter coming from microscopic calculation.
Peak width too short: needs dynamical consideration.
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
What have we learned ?What have we learned ?What have we learned ?What have we learned ?
Many observables are available : mean TKE, mean excitation energy,... and can be used for further evaluations (number of emitted neutron, …)
We still suffer from a lack of description about what happens before the scission-point (prescission energy, emission of particules,…).
Rethink the whole definition of scission point.
Include temperature microscopic calculation (no more shell effect).
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Still to be done :Still to be done :Still to be done :Still to be done :
Try out microscopic level densities.
J.L. Sida J.L. Sida (PhD Director)(PhD Director)H. GoutteH. GoutteJ.F. BergerJ.F. BergerM. GirodM. GirodS. HilaireS. Hilaire
P. RomainP. RomainB. MorillonB. MorillonP.MorelP.MorelM. DupuisM. DupuisF. ChappertF. Chappert
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Cast & Crew :Cast & Crew :Cast & Crew :Cast & Crew :
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Level Density : G S MLevel Density : G S MLevel Density : G S MLevel Density : G S M
Generalized Superfluid ModelGeneralized Superfluid Model : : Critical energy, critical temperature, …etc, corresponding to phase transition between normal and superfluid phase.
Level DensityLevel Density ::
02 ETaE critcritcrit
4/504/1
)(2
)(12
)2(1 )(
0
EEaE e
EEa
oc
2
2
11)(~
aTe
WAaaaT
E > Ecrit
:
E < Ecrit :
DE e
S
oc
)2(1 )(
2
21
1)(~critcrit
Ta
critTa
eWAaaa
critcrit
First interpretation : liquid drop fission…
Equal mass fragments :
Actually, we often observe a heavy and a light fragment…
We need to consider quantum effects
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Experimental resultsExperimental resultsExperimental resultsExperimental results
Multi-valley symmetric valley asymmetric valley
Time dependant Time dependant Potential Energy SurfacePotential Energy Surface
Time dependant Time dependant Potential Energy SurfacePotential Energy Surface
ElongationAsymmetry
En
erg
y
Exit Points Héloïse Goutte
CEA/DAM Theoretical Nuclear Structure Lab.
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Dynamical CalculationsDynamical CalculationsDynamical CalculationsDynamical Calculations
CEA DAM/DPTA/SPN/MED/Sophie Heinrich ESNT Workshop May 9-12 2006
Microscopic Description of the Microscopic Description of the NucleusNucleus
Microscopic Description of the Microscopic Description of the NucleusNucleus
1 Nucleus = N nucleons with strong interaction
Force N-N ? No direct calculationfrom QCD
N body physics
Can be resolved up to N = 10 - 12For N >> 10 : approximation needed
Shell Model• Effective residual interaction• Valence space• Symmetry conservation
Mean field Approach• No core• Separation between internal structure and collective excitation(mean field and beyond)
Naked force
Effective force
Zero rangeFinite range
Phenomenological Effective Force