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Welcome to the 10th East Asia Symposium on Superconductor Electronics Dear colleagues and friends, It is our great honor and pleasure to organize the 10th East Asia Symposium on Superconductor Electronics (EASSE-2019), which will be held in Beijing, China from Oct. 8 to Oct. 11, 2019. Following the tradition of this series, the coming symposium will bring together the researchers on superconductor electronics across East Asia to exchange and share our research ideas and results, as well as to meet old friends and make new friends, so that we shall further strengthen the collaboration between us and promote the research and applications of superconductor electronics in East Asia. Not only the capital of China but also a city vibrant with life and energy, Beijing has many new things to offer, even to frequent visitors, in addition to its numerous historical scenic spots. And October is the best time in a year to see it as well as the other parts of China. Do come to EASSE-2019. We shall do our best to make your participation fruitful and rewarding, both professionally and socially. B.S. CaoSymposium Chair

10th East Asia Symposium on Superconductor Electronics · Superconductor Electronics Dear colleagues and friends, It is our great honor and pleasure to organize the 10th East Asia

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Welcome to the 10th East Asia Symposium on

Superconductor Electronics

Dear colleagues and friends,

It is our great honor and pleasure to organize the 10th East Asia Symposium on

Superconductor Electronics (EASSE-2019), which will be held in Beijing, China

from Oct. 8 to Oct. 11, 2019. Following the tradition of this series, the coming

symposium will bring together the researchers on superconductor electronics

across East Asia to exchange and share our research ideas and results, as well as

to meet old friends and make new friends, so that we shall further strengthen the

collaboration between us and promote the research and applications of

superconductor electronics in East Asia.

Not only the capital of China but also a city vibrant with life and energy, Beijing

has many new things to offer, even to frequent visitors, in addition to its numerous

historical scenic spots. And October is the best time in a year to see it as well as

the other parts of China.

Do come to EASSE-2019. We shall do our best to make your participation fruitful

and rewarding, both professionally and socially.

B.S. Cao,Symposium Chair

Sponsors

Tsinghua University

Nanjing University

Western Superconducting Technologies Co.,Ltd.

Chinese Institue of Electronis

National Natural Science Foundation of China

Ministry of Science and Technology of the People’s Republic of China

Ministry of Education of the People’s Republic of China

The 10th East Asia Symposium on Superconductor

Electronics (EASSE-2019)

International Steering Committee

S. Ohshima ( Yamagata University, Yonezawa ), Chairman

B.S. Cao ( Tsinghua University, Beijing )

J. Chen ( Nanjing University, Nanjing )

H.E. Horng ( National Taiwan Normal University, Taipei )

N. Khare ( Indian Institute of Technology, Delhi )

H.J. Lee ( Pohang University of Science and Technology, Pohang )

Y.H. Lee (KRISS, Daejeon )

K. Nakajima (Yamagata University, Yonezawa)

Y.K. Park ( University of Science and Technology, Daejeon )

K. Tanabe ( ISTEC, Tokyo )

T. Venkatesan ( National University of Singapore, Xiamen University Malaysia )

L.M. Wang ( National Taiwan University, Taipei )

P.H. Wu ( Nanjing University, Nanjing )

International Advisory Committee

Z.G. Khim( Seoul National University, Seoul )

S. Kuriki( Hokkaido University, Sapporo )

C.K. Ong( National University of Singapore, Xiamen University Malaysia)

Organizing Committee

B.S. Cao ( Tsinghua University, Beijing ), Chairman

Y.R. Li ( Sichuan University, Chengdu ), Co-Chairman

J. Chen ( Nanjing University, Nanjing ), Co-Chairman

B. Wei ( Tsinghua University, Beijing ), Co-Chairman

D.K. Chen ( CETC, Hefei )

J. Li ( IOP, CAS, Beijing )

Y.P. Liu ( IOP, CAS, Beijing )

L.X. You ( SIMIT, CAS, Shanghai )

F.R. Wang ( Peking University, Beijing )

D.N. Zheng ( IOP, CAS, Beijing )

Topics

1) Materials and Device Fabrication;

2) RF Components and Devices;

3) SQUIDs and Applications;

4) Detectors and Applications;

5) Digital;

6) Quantum Information;

7) Cryogenic and Electrical Systems;

8) Novel Devices;

9) Metrology and Standard;

10) Topological Devices.

Conference Venue: Unisplendour International Center (October 9th 8:30 - 11:40)

Conference Venue: Jinchunyuan (October 9th 14:00 - 21:00, October 10th, October 11th)

EASSE 2019 – Program Tuesday 8 October, 2019

14:00 18:00 Registration (Location: Jinchunyuan)

18:00 20:00 Reception (Location: Jinchunyuan restaurant)

Wednesday 9 October, 2019 Conference Venue: Unisplendour International Center (October 9th 8:30 - 11:40)

Opening ceremony (Chair: Jian Chen)

8:30 8:40 Welcome address by professor Qikun Xue, vice president of Tsinghua University

8:40 8:50 Opening address by professor Peiheng Wu, Nanjing University

8:50 9:00 Welcome by professor Bisong Cao, Tsinghua University

9:00 9:30 Group photo of EASSE2019 & Coffee break

9:30 10:00 Memorial to Prof. Tsutomu Yamashita

Session I (Chairs: Yang Yu, Akira Fujimaki) Superconducting Computing & Circuits

10:00 10:20 Akira Fujimaki Numerical and Experimental Analysis on π-Shifted

SQUIDs for Logic Circuits and Memories Page 1

10:20 10:40 Mutsuo Hidaka Improvements of superconducting digital circuit

fabrication process Page 2

10:40 11:00 Kai Xu Generation of multicomponent atomic Schrödinger

cat states of up to 20 qubits Page 3

11:00 11:20 Yang Yu Simulation and manipulation of topological bands

using superconducting quantum circuits Page 4

11:20 11:40 Zhirong Lin Real-time detection of an itinerant microwave

photon using dressed-state engineering Page 5

12:00 13:00 Lunch (Location: Jinchunyuan restaurant)

Conference Venue: Jinchunyuan (October 9th 14:00 - 21:00, October 10th, October 11th)

Session II (Chairs: Huabing Wang, Masayoshi Tonouchi) Meeting Room 3 Microwave

14:00 14:20 Lu Ji Growth and properties analysis on epitaxial 2 inch

Tl-2212 superconducting films Page 6

14:20 14:40 Haiwen Liu

Compact and High Performance Microwave

Superconducting Bandpass Filters Using Microstrip

Multimode Resonators

Page 7

14:40 15:00 Liang Sun Development of the Ultra-wideband HTS Microstrip

Filters Page 8

15:00 15:20 Ming-Jye Wang Toward Full RF-Bandwidth mm-Wavelength

Receiver for Astronomical Telescope Page 9

15:20 15:40 Sansheng Wang

High quality uniform REBCO film growth by the

metalorganic deposition using trifluoroacetates and

its modifications for large-power microwave

devices application

Page 9

15:40 16:00 Xuehui Guan Novel Spiraled D-CRLH High Temperature

Superconducting Filter with a Dual-Passband Page 11

16:00 16:20 Coffee break

Session III (Chairs: Hideo Itozaki, Jinjin Li) Meeting Room 2 SQUIDs

14:00 14:20 Saburo Tanaka

Development of High-Tc SQUID Metallic

Contaminant Detection System for Li-ion Battery

Components

Page 12

14:20 14:40 Xiaoming Xie SQUID Systems for Bio-imaging/testing and

Geophysical Prospection Page 13

14:40 15:00 Jen-Jie Chieh Nonn-invasive and Fast Imaging Tumors by SQUID Page 14

16:00 16:20 Coffee break

Session IV (Chairs: Haiwen Liu,Ming-Jye Wang) Meeting Room 3 Junctions

16:20 16:40 Huabing Wang Josephson junctions with novel barrier layers Page 18

16:40 17:00 Hu-Jong Lee Strong proximity Josephson coupling in

heterojunctions of 2D materials Page 19

17:00 17:20 Akinobu Irie Spin-dependent behaviors in Ferromagnet/Intrinsic

Josephson junctions/Ferromagnet Hybrids Page 20

17:20 17:40 Masayoshi Tonouchi Ultrafast optical response and vortex generation in

high-Tc superconductors Page 21

18:00 19:00 Dinner (Location: Jinchunyuan restaurant)

Session V (Chair: Masataka Ohkubo) Meeting Room 2 Standard

16:20 16:40 SangYoung Lee

Two-resonance-mode dielectric resonator method

as an International Standard for the Intrinsic Surface

Impedance of High-Tc Superconductor Films

Page 22

16:40 17:00 Jinjin Li

The Development of Large-scale Josephson

Junction Array Devices for the Quantum Voltage

Standard at NIM

Page 23

17:00 17:20 Myung-Ho Bae Quantum metrology triangle for future electrical

standard Page 24

18:00 19:00 Dinner (Location: Jinchunyuan restaurant)

Biosusceptometry and Magnetic Nanoparticles

15:00 15:20 Shu-Hsien Liao High-Tc SQUID based NMR for breast cancer and

liver cancer diagnosis Page 15

15:20 15:40 Kenji Sakai Estimation of electrochemical impedance using

HTS-SQUID based magnetic measurement system Page 16

15:40 16:00 Li-Min Wang

Characterization of High-Tc dc-SQUID

Magnetometers: Fabrication with Sputtered YBCO

Films Deposited on Recycled SrTiO3 Bi-crystal

Substrates

Page 17

Poster Session (Chairs: Dongning Zheng, Takashi Tachiki) Meeting Room 3

19:00 21:00

Hirofumi Yamasaki

Correlation between the critical current density and

surface resistance in YBCO thin films—

reexamined

Page 46

Fang Li

Vortex manipulation with dots and antidots on

superconductivity of REBa2Cu3O7-δ films growth

by trifluoroacetate metal organic deposition method

Page 47

Xiaoqing Sun Effects of Ionic Accumulation in Nerve Conduction Page 48

Teppei Ueda Property of HTS Josephson Junction irradiated by

Ga Focused Ion Beam Page 49

Guofeng Zhang LTS SQUID magnetometers and gradiometers Page 50

Yifeng Pei LTS SQUID Based Transient Electromagnetic

System for Geophysical Prospecting Page 51

Yingyi Shao Control of roughness and stress of Nb films for

Nb/Al‐AlOx/Nb Josephson junctions Page 52

Zuyu Xu Tunable Josephson junction based on black

phosphorus Page 53

Shixian Chen Novel Nb-based Josephson junctions using

Bi2Sr2CaCu2O8+δ as barriers Page 54

Fajun Li Proximity Effects on Mo/Cu Bilayers Page 55

Sifan Wang Development of Mo/Cu TES Devices Page 56

Yeru Wang Characterization of Sputtered Molybdenum Thin

Films Page 57

Takahiro Murakami Bi-2212 mesas made of Bi-2212 thin film for THz

emission with superior heat dissipation. Page 58

Zaidong Qi High-power terahertz emission from

Bi2Sr2CaCu2O8 intrinsic Josephson junction stacks Page 59

Runfeng Su Characterization of superconducting NbN hot-

electron bolometers as THz direct detectors Page 60

Herng-Er Horng The application of high-Tc SQUID-based low-field

NMR in human liver tumor discrimination Page 61

Steering Committee (Chair: Shigetoshi Ohshima) Meeting Room 2

18:00 19:00 Steering Committee

Thursday 10 October,2019 Session VI (Chairs: Yoshihiko Takano, Akinobu Irie) Meeting Room 3 THz

8:40 9:00 Takashi Tachiki

Investigation of radiation properties of THz-wave

oscillators using Bi-2212 intrinsic Josephson

junctions for oscillator-array design

Page 25

9:00 9:20 Akira Kawakami 2 THz Hot Electron Bolometer Mixer using a

Magnetic Thin Film Page 26

9:20 9:40 Hsiao-Wen Chang Development of NbN Hot Electron Bolometer

Mixer Operating at 1.5 THz Page 27

9:40 10:00 Kensuke Nakajima Applications of superconducting thin films for

extensive use in terahertz functional devices. Page 28

10:00 10:20 Nobuyuki Yoshikawa Extremely Energy-Efficient Circuit Technology

based on Adiabatic Quantum Flux Parametron Page 29

10:20 10:40 Coffee break

Standardization Session (Chairs: SangYoung Lee, Masataka Ohkubo) Meeting Room 2

8:40 10:20 Shigetoshi Ohshima TC90/WG8&WG14 Page 30

10:20 10:40 Coffee break

Session VII (Chair: Kensuke Nakajima) Meeting Room 3 Others

10:40 11:00 Yoshihiko TAKANO Discovery of new superconductors under high

pressure using materials informatics Page 31

11:00 11:20 Hideki Ichinose Specimen Thinning for HRTEM via Photon

illumination Page 32

11:20 11:40 Chong Kim Ong Electrical signal transmission in Neural Functions Page 33

12:00 13:00 Lunch (Location: Jinchunyuan restaurant)

Session VIII (Chair: Nobuyuki Yoshikawa) Meeting Room 2 SNSPD

10:40 11:00 Lixing You Superconducting nanowire single photon

detectors for quantum information Page 34

11:00 11:20 Hirotaka Terai Recent progress in research and development of

superconducting nanowire single-photon detectors Page 35

11:20 11:40 Labao Zhang The original seeds of dark counts of SNSPD Page 36

12:00 13:00 Lunch (Location: Jinchunyuan restaurant)

13:00 18:00 Lab tour

18:00 21:30 Conference Banquet (Location: Laoshe Teahouse)

Friday 11 October,2019 Session IX (Chairs: Lixing You, Hirotaka Terai) Meeting Room 3 TES

8:40 9:00 Wei Cui Superconducting Detectors and Electronics for

Astronomical Applications Page 36

9:00 9:20 Yong Hamb Kim Metallic magnetic calorimeters for astroparticle

physics applications Page 38

9:20 9:40 Shuo Zhang Introduction to cryogenic particle detectors for

Shanghai Light source Facility Page 39

9:40 10:00 Takekazu Ishida Neutron imaging using a superconducting detector Page 40

10:00 10:20 Masataka Ohkubo

A challenge to chemical-state nanoscale-imaging

with superconductor-tunnel-junction X-ray detector

for aviation industry

Page 42

10:20 10:40 Coffee break

Session X (Chair:Hu-Jong Lee) Meeting Room 3 SQUIDs

10:40 11:00 Hideo Itozaki High Tc Scanning SQUID Microscope Page 44

11:00 11:20 Anjan Kumar Gupta Optimization of constriction based Nb µ-SQUIDs

for probing nano-magnetism Page 45

11:20 11:40 Neeraj Khare

11:40 12:00 Shigetoshi Ohshima Closing Remarks

12:00 13:00 Lunch (Location: Jinchunyuan restaurant)

Abstract Book

1

Numerical and Experimental Analysis on -Shifted

SQUIDs for Logic Circuits and Memories

A. Fujimaki1, Y. Takeshita1, D. Hasegawa1, F. Li1, K. Sano1,

M. Tanaka1, and T. Yamashita1,2

1Department of Electronics, Nagoya University, Nagoya.

2JST-PRESTO

[email protected]

We have successfully demonstrated -shifted SQUIDs (-SQUIDs) made up of two

conventional Nb/AlOx/Nb Josephson junctions and a single -shifted magnetic Josephson

junctions (hereinafter junctions). The junctions have a sandwich structure of a Nb/PdNi/Nb

trilayer. We confirm that modulation patterns of the critical currents to external magnetic fields

in -SQUIDs are shifted by a field corresponding to half of magnetic flux quantum as shown

in Figure 1.

The -SQUIDs function as an essential element of the half flux quantum (HFQ) logic circuit.

Figure 1 indicates that the -SQUIDs can be regarded as single junctions with reduced critical

currents. In addition, the phase change in a single switching of -SQUIDs is , so that HFQ

logic circuits can be built up by replacing conventional single junctions of the rapid single flux

quantum (RSFQ) circuits with -SQUIDs [1]. Numerical analysis of the HFQ circuits made

up of 100-A-junctions shows that the energy consumption is reduced below 0.05 aJ/junction,

which is 1-2 orders of magnitude smaller than that of the RSFQ circuit.

The -SQUIDs have two stable states corresponding to a clockwise and counter-clockwise

circulating current without any field. The potential barrier height between the two states can be

controlled by adjusting a loop inductance of the -SQUID or a critical current of an inserted

additional junction. The low barrier height enables us to make a large capacity matrix memory

driven by an impulse like an SFQ pulse [2].

The detail of the numerical and experimental analysis will be given at the symposium.

Fig. 1 Experimentally obtained modulation pattern of critical current of a -SQUID

[1] T. Kamiya, et al., IEICE Trans. Electron. E101-C (2018) 385.

[2] Fujimaki, et al., 17th Int. Supercond. Electron. Conf., 2019, Riverside, CA, USA.

-15 -10 -5 0 5 10 15

0.20

0.15

0.10

0.05

0

-0.05

-0.10

-0.15

-0.20

Critic

al

cu

rren

t [m

A]

Applied magnetic flux density [µT]

2

Improvements of superconducting digital circuit

fabrication process

M. Hidaka1

1National Institute of advanced industrial science and technologies (AIST), Tsukuba.

[email protected]

Superconducting digital circuits are attractive for their high-speed and low-dissipation

characteristics. AIST is routinely fabricating Nb-based superconducting digital circuits and also

investigating advanced fabrication process toward higher performances and various

applications. For examples, 106 GHz clock operation of a single-flux-quantum (SFQ) processor

was demonstrated using Josephson junctions (JJs) of 20 kA/cm2 critical current density (Jc)

[1], circuits area of adiabatic quantum flux parametron (AQFP) were reduced 40% by a

double gate layer device structure [2] and outputs of superconducting strip photon detectors

(SSPD) were effectively combined by a monolithic SFQ readout circuit [3]. We found out main

origin of SFQ circuit defects was small particles underneath JJs. Replacement of deposition

method of SiO2 from bias sputter to chemical vapor deposition (CVD) which generates much

fewer particles than that by bias sputter achieved dramatically improvement of SFQ circuit

integration level [4].We are also developing quantum annealing circuits based on the digital

fabrication process with Jc of 0.1 kA/cm2 which is 100 times smaller compared with ordinary

digital circuits [5].

A part of his presentation is based on results obtained from a project commissioned by the New

Energy and Industrial Technology Development Organization (NEDO) and JSPS-KAKENHI

18H05211, 18H05245.

[1] M. Tanaka, M. Kozaka, Y. Kita, A. Fujimaki, S. Nagasawa, and M. Hidaka (2015). IEEE Trans. Appl.

Supercond., Vol. 25, pp. 1–4.

[2] T. Ando, S. Nagasawa, N. Takeuchi, N. Tsuji, F. China, M. Hidaka, Y. Yamanashi, and N. Yoshikawa, (2017).

Supercond. Sci. Technol., Vol. 30, 075003.

[3] H. Terai, S. Nagasawa, S. Miyajima, T. Yamashita, S. Miki, M. Yabuno, and M. Hidaka (2016). ASC2016,

3EOr1B-03

[4] M. Hidaka, S. Nagasawa, T. Satoh and K. Hinode (2015). ,IEEE Xplore, 10.1109/ISEC2015.

[5] M. Maezawa, G. Fujii, M. Hidaka, K. Imafuku, K. Kikuchi, H. Koike, K. Makise, S. Nagasawa, H. Nakagawa,

M. Ukibe, and S. Kawabata (2019). J. Phys. Soc. Jpn., 061012.

3

Generation of multicomponent atomic Schrödinger

cat states of up to 20 qubits

Chao Song1†, Kai Xu2†, Hekang Li2†, Yu-Ran Zhang2,5, Xu Zhang1,

Wuxin Liu1, Qiujiang Guo1, Zhen Wang1, Wenhui Ren1, Jie Hao3,

Hui Feng3, Heng Fan2*, Dongning Zheng2*, Da-Wei Wang1,

H. Wang1*, Shi-Yao Zhu1

1Department of Physics, Zhejiang University, Hangzhou.

2Institute of Physics, Chinese Academy of Sciences, Beijing.

3Institute of Automation, Chinese Academy of Sciences, Beijing.

5Beijing Computational Science Research Center, Beijing.

*Corresponding author. E-mail: [email protected] (H.F.); [email protected] (D.N.Z.);

[email protected] (H.W.).

†These authors contributed equally to this work.

Multipartite entangled states, especially the Greenberger-Horne-Zeilinger (GHZ) states, are a

fundamental resource for numerous applications in quantum information science, but the

generation of such states remains an outstanding challenge due to their intrinsic fragilities.

Therefore, the creation of multiqubit GHZ states serves as an important benchmark for

characterizing the controllability and scalability of experimental quantum platforms [1,2]. We

report the deterministic generation of an 18-qubit GHZ state and multicomponent atomic

Schrödinger cat states of up to 20 qubits on a quantum processor, which features 20

superconducting qubits, also referred to as artificial atoms, interconnected by a bus resonator.

By engineering a one-axis twisting Hamiltonian, the system of qubits, once initialized,

coherently evolves to multicomponent atomic Schrödinger cat states—that is, superpositions of

atomic coherent states including the GHZ state—at specific time intervals as expected. We

measure a GHZ state fidelity F = 0.525 ± 0.005 for 18 qubits, confirming genuine 18-partite

entanglement. Our approach on a solid-state platform should not only stimulate interest in

exploring the fundamental physics of quantum many-body systems, but also enable the

development of applications in practical quantum metrology and quantum information

processing.

[1] Omran et al., Generation and manipulation of Schrödinger cat states in Rydberg atom arrays. Science 365,

570-574 (2019).

[2] K. X. Wei et al., Verifying multipartite entangled GHZ states via multiple quantum coherences.

arXiv:1905.05720 [quant-ph].

4

Simulation and manipulation of topological bands

using superconducting quantum circuits

Xinsheng Tan1, Yuxin Zhao1,2, Danwei Zhang3, Mengmeng Li1, Haifeng Yu1, Hui Yan3,

Shiliang Zhu1,3, Yang Yu1, Zidan Wang2,

1National Laboratory of Solid State Microstructures, School of Physics, Nanjing University,

China 2Department of Physics, The University of Hong Kong

3Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials,

SPTE, South China Normal University, Guangzhou 510006, China

Topological band theory has attracted much attention since several types of topological metals

and semimetals have been explored. These robustness of nodal band structures are symmetry-

protected, whose topological features have deepened and widened the understandings of

condensed matter physics. Meanwhile, as artificial quantum systems superconducting circuits

possess high controllability, supplying a powerful approach to investigate topological

properties of condensed matter systems. We realize Hamiltonians with topological symmetry

by mapping momentum space to parameter space in a superconducting quantum circuit[1-4].

By measuring energy spectrum of the system, we observe the gapless band structure of

topological semimetals, shown as Dirac points or Weyl points in momentum space. The phase

transition from topological semimetal to topological insulator can be realized by continuously

tuning the parameter in Hamiltonian. Our work open a platform to simulate the relation between

the symmetry and topological stability in condensed matter systems.

[1] Xinsheng Tan, Yuxin Zhao, Qiang Liu, Guangming Xue, Haifeng Yu, Z. D. Wang, Yang Yu, Npj Quantum

Materials 2, 60 (2017).

[2] Xinsheng Tan, Dan-Wei Zhang, Qiang Liu, Guangming Xue, Hai-Feng Yu, Yan-Qing Zhu, Hui Yan, Shi-

Liang Zhu, Yang Yu, Phys. Rev. Lett. 120, 130503 (2018).

[3] Xinsheng Tan, Mengmeng Li, Danyu Li, Kunzhe Dai, Haifeng Yu, Yang Yu, Appl. Phys. Lett. 112, 172601

(2018).

[4] Xinsheng Tan, Yuxin Zhao, Qiang Liu, Guangming Xue, Haifeng Yu, Zidan Wang, Yang Yu, Phys. Rev.

Lett. 122, 010501 (2019).

5

Real-time detection of an itinerant microwave

photon using dressed-state engineering

Zhirong Lin1,2

1CAS Center for Excellence in Superconducting Electronics, Shanghai Institute of

Microsystem and Information Technology, Shanghai, China

2 Center for Emergent Matter Science, RIKEN, Wako, Japan

[email protected]

Several schemes for single microwave photon detection have been proposed and demonstrated

lately in circuit quantum electrodynamics [1-4]. However, most experimental demonstration to

date are performed in the time-gated mode. In this presentation, we demonstrate a real-time

detection of itinerant microwave photons. In our setup, a superconducting flux qubit is coupled

to two resonators, which have substantial difference in the dispersive shifts. Under an adequate

choice of the frequency and the power of the qubit drive, one resonator is used to form an

impedance-matched Λ system that deterministically captures incoming photons, and the other

is used for continuous monitoring of the event. We observe a quantum jump produced by an

itinerant microwave photon and attain a single-photon-detection efficiency of ~0.35. The

detection efficiency of this detector is limited by the relatively short qubit relaxation time.

[1] K. Inomata*, Z. R. Lin*, et al. (2016). Single microwave-photon detector using an artificial Λ-type three-

level system. Nature Commun., 7, 12303.

[2] S. Kono et al. (2018). Quantum non-demolition detection of an itinerant microwave photon. Nature Physics,

14, 546.

[3] Jean-Claude Besse et al. (2018). Single-Shot Quantum Nondemolition Detection of Individual Itinerant

Microwave Photons. Phys. Rev. X, 8, 021003.

[4] Raphaël Lescanne et al. (2019). Detecting itinerant microwave photons with engineered non-linear

dissipation. arXiv:1902.05102

6

Growth and properties analysis on epitaxial 2 inch

Tl-2212 superconducting films

X. L. Liang, J. Xin, T. Xue, M. He, S. L. Yan, and L. Ji

School of Electronic Information and Optical Engineering, Nankai University, Tianjin.

[email protected]

The extensive use of large-area high temperature superconducting (HTS) thin films has

emerged in superconducting microwave devices. The interest in the Tl-based HTS films arises

from their higher critical temperature (Tc), which avoids the demands for more cryogenic device.

This paper introduces a developed two-step method without additional Tl source to fabricate

high-quality Tl2Ba2CaCu2O8 (Tl-2212) films on 2 inch LaAlO3 substrates. This method enables

the preparation of Tl-2212 films to be less complicated and more repeatable, which can promote

the theoretical research and practical application of Tl-based films. Based on the high

reproducibility of this fabricating process, the obtained 2 inch Tl-2212 films have excellent

quality, the superconducting properties of Tc, the critical current density Jc (77K, zero field) and

surface resistance (Rs) of 2 inch samples can be studied easily. The Tc value of sample films

prepared at different conditions varies from 99 to 103 K, and Jc of films ranges from 0.7 to

1.8MA/cm2. Systematic experiment reveals that the oxygen content affects the Tc of the films,

and the surface roughness of the films is closely related to Jc values. The variation of Rs

(calculated at 12GHz) with temperatures on Tl-2212 films was also observed, which is a helpful

guideline for the application of microwave devices based on Tl-2212 films.

7

Compact and High Performance Microwave

Superconducting Bandpass Filters Using Microstrip

Multimode Resonators

Haiwen Liu

School of Electronics and Information Engineering, Xi'an Jiaotong University, Xi'an

As the key passive component in the radio-frequency (RF) front-end, bandpass filter (BPF) with

compact size and high performance are in great demand for enhancing system functionality. Meanwhile,

high-temperature superconducting (HTS) materials are becoming more and more attractive in the

context of designing microwave filters because of their lower losses and excellent performance.

In past few years, several types of high performance HTS BPFs have been designed for demonstration.

For circuit size miniaturization, various microstrip multimode resonators have been proposed, such as

the multi-stub-loaded resonators and square ring loaded resonator. At first, a series of the second-order

multiband HTS filters have been presented based on the multi-stub-loaded resonators [1], [2]. The

measured insertion losses are all extremely small, but the selectivity and stopband performance need to

be improved because of the low-order design. Therefore, a newly dual-mode hairpin ring resonator is

proposed and applied to constitute an eighth-order dual-band HTS BPF [3]. The configuration of the

designed filter and the obtained frequency responses are respective shown in Fig. (a) and (b). As

predicted, the band edge selectivity and the attenuation in stopband are highly enhanced.

In addition, the differential circuits have been received much attention recently due to their ability of

lower electromagnetic noise and crosstalk. So, based on the HTS technology, a fourth-order differential

dual-band HTS BPF has been designed using the proposed square ring loaded resonator [4]. The layout

of the differential filter is depicted in Fig. (c) and the simulated results as well as the measured results

are shown in Fig. (d). It is seen from Fig. (d) that a favorable common-mode (interference signal)

suppression over a wide frequency range is obtained.

With the advantages of ultra-low in-band insertion losses and high selectivity, these proposed filters are

attractive for potential applications in multiband communication systems requiring high-sensitivity and

high anti-interference properties.

[1] H. W. Liu, J. H. Lei, X. H. Guan, L. Sun, and Y. S. He, “Compact triple-band high-temperature

superconducting filter using multimode stub-loaded resonator for ISM, WiMAX, and WLAN Applications,”

IEEE Transactions on Applied Superconductivity, vol. 23, no. 6, Art. ID. 1502406, Dec. 2013.

[2] H. W. Liu, P. Wen, Y. L. Zhao, B. P. Ren, X. M. Wang, and X. H. Guan, “Dual-band superconducting

bandpass filter using quadruple-mode resonator,” IEEE Transactions on Applied Superconductivity, vol. 24,

no. 2, pp. 130-133, Apr. 2014.

[3] H. W. Liu, B. P. Ren, S. X. Hu, X. H. Guan, P. Wen, and J. M. Tang, “High-order dual-band superconducting

bandpass filter with controllable bandwidths and multitransmission zeros,” IEEE Trans. Microw. Theory

Tech., vol. 65, no. 10, pp.3813-3823, Nov. 2017.

[4] B. P. Ren, Z. W. Ma, H. W. Liu, X. H. Guan, X. L. Wang, P. Wen, and M. Ohira, “Differential Dual-Band

Superconducting Bandpass Filter Using Multi-Mode Square Ring Loaded Resonators With Controllable

Bandwidths,” IEEE Transactions on Microwave Theory and Techniques, vol. 67, no. 2, pp. 726-737, Feb.

2019.

8

Development of the Ultra-wideband HTS Microstrip

Filters

Y. Wu1, L. Sun1, C. Li1, X. Zhang1, J. Wang1, X. Wang1, Y. Bian1, G. Li1, H. Li1, and Y. He1

1 Beijing National Laboratory of Condensed Matter Physics and Institute of Physics, Chinese

Academy of Sciences

[email protected]

Ultra-wideband (UWB) technology is been known as with advantages such as high

communication speed, low power consumption and high anti-jamming performance. It has been

widely used in radio astronomy observation, deep space exploration and wireless

communication. As a key unit in front-end of RF receivers, UWB filters have been developed

massively. In this talk, UWB filters developed on high temperature superconducting microstrip

lines are presented. Firstly, a wideband filter for radio astronomy observation, which has a

fractional bandwidth (FBW) of 37.8%, is introduced. By adopting a hairpin-like structure,

resonators can generate strong coupling, and push its first spurious resonant peak away from

the passband. Then, a UWB filter for deep space exploration, which has an FBW of 65%, is

presented. λ/4 hair-pin resonators were used in this filter instead of regular /2 resonators,

which not only minimized the size of the filter, but also eliminated the effect of second

harmonic resonance of /2 resonators. Finally, a filter with an FBW of 108% for wireless

communication is introduced. The filter is realized by cascading a high-pass filter and a low-

pass filter, with a low noise amplifier inserted between the high-pass filter and the low-pass

filter to improve the matching between the filters.

9

Toward Full RF-Bandwidth mm-Wavelength

Receiver for Astronomical Telescope

M. J. Wang1*, T. J. Chen1, W. C. Lu1, Y. B. Chang1, Y. D. Huang1, C. E. Tong2, L. Zeng2, P.

Grime2

1Institute of Astronomy and Astrophysics, Academia Sinica, Taipei, Taiwan

2Harvard-Smithsonian Center for Astrophysics, Cambridge, MA 02138, USA

[email protected]

The construction and operation of cutting-edge astronomical telescope is very expensive.

Improving the sensitivity and efficiency is an important issue for detecting system development.

For radio telescope receiver, the simultaneous observation bandwidth is the key parameter. For

total power detection mode, the sensitivity is proportional to 1 √𝐵𝑊⁄ , i.e. wider bandwidth

resulting in higher sensitivity. For the spectrum detection mode, the wider bandwidth can

observe more emission lines in one integration and speed up the observation.

In a mm-wavelength receiver, the RF signal coupled through feed horn can be up to 100GHz.

However, the observation bandwidth is dependent on the intermediate frequency (IF)

bandwidth of receiver with single tone local oscillator (LO) source in the regular system

configuration. Cooled low noise amplifier (CLNA) and superconductor-insulator-

superconductor (SIS) mixer are the two critical components. After years effort, the wSMA

receiver has demonstrated the-state-of-art ultrawide bandwidth of 32 GHz [1]. Further

extending the bandwidth of CLAN and SIS mixer becomes difficult due to the impendence

match issue.

A possible approach to extend the simultaneous observation bandwidth further is using multi-

receivers pumped at different LO frequencies. The RF signal is divided into several sub-bands

by superconducting bandpass filters. The individual sub-band RF signal is detected by an SIS

mixer which is pumped by the LO source at the center frequency of sub-band. The observation

bandwidth of this detection scheme could be increased by a factor of the number of sub-bands.

In my presentation, I will include the detail scheme of full RF-bandwidth receiver, the

developed ultrawide wSMA receiver, and some preliminary works on bandpass filter in mm-

wavelength.

[1] C. Edward Tong, et. al. “Development of SIS Receivers with Ultra-wide Instantaneous Bandwidth for

wSMA”, 29th IEEE International Symposium on Space THz Technology (ISSTT2018), Pasadena, CA, USA,

March 26-28, 2018

High quality uniform REBCO film growth by the

metalorganic deposition using trifluoroacetates and

10

its modifications for large-power microwave devices

application

S.S.Wang1,3*, Z.L.Zhang1, F. Li1,B. Wei2, B.S.Cao2,L.K.Gao3,J.Liu3

1. Key Laboratory of Micro-nano Measurement, Manipulation and Physics (Beihang

University), Ministry of Education, Beijing 100191, China

2. Department of Physics, Tsinghua University, Beijing 100084, China

3.Beijing Dingchen Superconducting Technology Co., Ltd.

E-MAIL: [email protected]

A need exists for the large-area superconducting REBa2Cu3O7-x (REBCO) films with high

critical current density for microwave communication. Trifluoroacetic metalorganic (TFA-

MOD) method is a promising low cost technique for large-scale production of REBCO films,

because it does not need high vacuum device and is easily applicable to substrates of various

shape and size. In my group, double-sided REBCO films with maximum 3-inch diameter were

prepared on LaAlO3 substrates by TFA-MOD method. Inductive critical current densitiy Jc,

microwave surface resistance Rs, as well as the microstructure were characterized, and low Rs

(10GHz) below 0.3 mΩ at 77K were obtained. A newly homemade furnace system was used to

epitaxially grown REBCO films, which can improve the uniformity of YBCO film significantly

by gas supply and temperature distribution proper design. Results showed that the large area

YBCO films were very uniform in microstructure and thickness distribution, an average

inductive Jc in excess of 3MA/cm2 can be obtained steadily. And the REBCO film filter has

been prepared to work at temperatures lower than 74K. These results are very close to the

highest value of YBCO films made by conventional vacuum method, so we show a very

promising route for large-scale production of high quality large-area REBCO superconducting

films at a lower cost.

Also, we will report some recent research work about REBCO film modification and its flux

pinning behavior, as well as microwave properties. Especially, we have developed a new

modification to get very high critical current density of above 10 MA/cm2 by four probe

measurement, which will be very useful for next-step large-power filter and transmitter

fabrication.

11

Novel Spiraled D-CRLH High Temperature

Superconducting Filter with a Dual-Passband

B. Ren1, X. Guan1, H. Su1, P. Wen2 and H. Liu2

1School of Information Engineering, East China Jiaotong University, Nanchang.

2School of Electronics and Information Engineering, Xi’an Jiaotong University, Xi’an.

[email protected]

With the development of multifunctional communication technology, dual-band bandpass

filters are widely exploited, including dual-band bandpass filters with high temperature

superconducting (HTS) technology [1][2][3]. In this study, a novel HTS dual-band bandpass

filter using spiraled Dual Composite Right-Left Handed (D-CRLH) resonator is presented. The

new proposed resonator is constructed by microstrip spiral coupled lines and microstrip high-

impedance lines[4]. Compared with the conventional CRLH resonator, this type of the

resonators is much smaller, and no grounded via is need, which simplifies the fabricating

process.

Moreover, an equivalent circuit model of the spiraled Dual Composite Right-Left Handed (D-

CRLH) resonator for dual-band application is given. Then, according to the transmission matrix

of the transmission line, the dispersion characteristics of the D-CRLH resonator is obtained and

analyzed, which makes it suitable for implementing the miniaturized high-performance filter.

For demonstration, a D-CRLH HTS filter with a dual-passband is designed on a 0.5mm thick

MgO wafer with double sided YBa2Cu3O7 films. Transmission zeros have been obtained in

the stopband of the filter, improving the stopband characteristics of the filter.

[1] Ji, L., Ma, J., Sun, J., Wang L., Li, Y., and Liu, B. (2012) Design and performance of dual-

band high temperature superconducting filter, Science China Information Sciences,

55(4):956-961 [2] Guan, X., Su, H., Liu, H., Wen, P., Liu, W., Gui, P., and Ren, B. (2019) Miniaturized high

temperature superconducting bandpass filter based on D-CRLH resonators, IEEE

Transactions on Applied Superconductivity, 29(5), 1501504

[3] Ma, P., Wei, B., Hong, J., Cao, B., Guo, X., and Jiang, L., (2017) Design of dual-mode

dual-band superconducting filters,”IEEE Trans. Appl. Supercond., 27(7):1502809.

[4] Li, C., Sun L., Wang, J., Bian, Y., Yu T., Li, F., Li, C., Li H., Gu, C.-Z. and He, Y. (2013)

A VHF band HTS filter based on modified single-spiral resonators for radio astronomy

application, Science China Physics, Mechanics & astronomy, 56(5): 910–915.

12

Development of High-Tc SQUID Metallic

Contaminant Detection System for Li-ion Battery

Components

S. Tanaka1, M. Sagawa I. Furukubo, K. Hayashi and T. Ohtani2

1Toyohashi University of Technology, Toyohashi, Japan.

2Nikka Densoku Limited, Kawagoe, Japan

[email protected]

For manufacturers producing Li-ion batteries or its components, problems with metallic

contaminants are critical issues. When contamination occurs, the manufacturer of the product

can suffers a great loss from a recalling the tainted product. The lower detection limit for

practical X-ray imaging is in the order of 1 mm. A detection system using a SQUID is a

powerful tool for sensitive inspections [1]. The battery component, e.g. battery slurry should be

also tested. Therefore we proposed and developed a detection system using RF SQUIDs. In this

system, an object with a contaminant was magnetized by a permanent magnet, and then the

remanent field of the contaminant detected by the SQUID. A microscope-type SQUID cryostat

was developed so that the SQUID could approach the target as close as 1 mm [2]. We did not

use a real slurry in this experiment, but the dependence of the sensitivity on the position of the

metallic sample was evaluated supposing a pseudo slurry tube with a 50 mm diameter. A

stainless steel test piece of 50m x 50m L was drawn by an electric motor with a speed of

20 m/min. As a result, the test piece with stand-off distance of 26 mm was detected with a

signal-to-noise ratio of more than 3. This result suggests the system is a promising tool for the

detection of contaminants in practical use.

[1] S. Tanaka, T. Ohtani, U. Yosuke, T. Chigasaki, and Y. Hatsukade, "Metallic Contaminant Detection System

using Multi-Channel Superconducting Quantum Interference Device (SQUID)," Solid State Phenomena, vol.

215, 465-469, 2014.

[2] S. Tanaka, K. Matsuda, O. Yamazaki, M. Natsume, and H. Ota, "Development of High Tc Microscope with

Flux guide," Supercond. Sci. and Technology, vol. 15, 146-149, 2002.

13

SQUID Systems for Bio-imaging/testing

and Geophysical Prospection

S.L. Zhang1,2, H. Dong1,2, L.L. Rong1,2, L.X. You1,2, X.M. Xie1,2

1Center for excellence in superconducting electronics

2Shanghai Institute of Microsystem and Information Technology

[email protected]

In this talk, I will give an overview of low Tc SQUID based system development for

bio-imaging and geophysical prospection, at the Shanghai Institute of Microsystem

and Information Technology, Chinese Academy of Sciences (SIMIT, CAS). We have

jointly developed China’s first 4-9 channel MCG systems with Medi Medical

(Shanghai) equipment, Ltd. and received CFDA certificate. Preclinical research

shows that the equipment has good potentiality as a diagnostic tool for Coronary

heart disease [1]. We have developed multichannel ultra-low field magnetic

resonance systems with noise around 1 fT/Hz1/2 and electromagnetic coil generated

pre-polarization field around 80 mT, overcoming the challenges of ambient field

fluctuation, field gradients, powerline and its harmonics, etc [2-3]. The relaxation

times (T1 and T2) and the images of bio-samples were then successfully acquired. We

have developed China’s first ground based low Tc SQUID receiver for transit

electromagnetic method (TEM) with low noise (7 fT/Hz) and high stability in

unshielded environment. Joint explorations were carried out with a mining company.

The surveying results were in excellent agreement with drilling results at different

places. We have also developed China’s first low Tc SQUID based air-borne full

tensor magnetic gradient measurement system. After optimizations, the systems were

tested at various environment, reaching a noise level of 50 pT/m (0.01-5Hz, rms).

[1] R. Tao, S. Zhang , X. Huang, M. Tao, J. Ma, S. Ma, C. Zhang, T. Zhang, F. Tang, J. Lu, C. Shen,

and X. Xie, (2019). IEEE Trans. Biomed. Eng., 66 1658-1667.

[2] C. Liu, B. Chang, L. Qiu, H. Dong, Y. Qiu, Y. Zhang, H.-J. Krause, A. Offenhäusser, and X.

Xie, J. Magn. Reson. (2015) 257 8-14

[3] X. Huang, H. Dong, Y. Qiu, B. Li, Q. Tao, Y. Zhang, H.-J. Krause, A. Offenhäusser and X. Xie,

(2018). J. Magn. Reson. 286 52-59

14

Nonn-invasive and Fast Imaging Tumors by SQUID

Biosusceptometry and Magnetic Nanoparticles

J.J. Chieh1, K.W. Huang2, C. K. Yeh

3, S. H. Liao1, Y. Y. Lee1, P. Y. Hsiao1, H. C. Yang1, and H.

E. Horng1

1Institute of Electro-Optical Science and Technology, Taiwan Normal University,Taipei

2Department of Surgery and Hepatitis Research Center, Taiwan University Hospital,Taipei

3Department of Biomedical Engineering and Environmental Sciences, Tsing Hua University, Hsinchu

[email protected]

INTRODUCTION For intraoperative imaging in operating theaters or preoperative imaging in

clinics, compact and economic integration rather than large and expensive equipment is

required to coregister structural and functional imaging. However, current technologies, such

as those integrating optical and gamma cameras or infrared and fluorescence imaging, involve

certain drawbacks, including the radioactive biorisks of nuclear medicine indicators and the

inconvenience of conducting measurements in dark environments. A novel dual-imaging model

system integrating an optical camera and magnetic scanning superconducting-quantum-

interference device (SQUID) biosusceptometry (SSB) was proposed. The simultaneous

coregistration of low-field magnetic images of MNP distributions and optical images of

anatomical regions enabled the tumor distribution to be determined easily and in real time. To

simulate targeted MNPs within animals, fewer reagents than the injected dose were contained

in a microtube as a sample for the phantom test. The positioning and discrimination of liver

tumors implanted on the backs and livers of rats were verified by conducting in vivo and ex

vivo tests. The results of tissue staining verified the feasibility of using this method to determine

the distribution of liver tumors.

MATERIAL AND METHODS Labeled MNPs on target tumors are magnetized under a DC

magnetic field. The US chips and pickup coils are used to vibrate MNPs and detect the

ultraweak magnetic signals of MNPs, respectively. The US excitation and magnetic detection

devices are integrated in a small probe. Consequently, labeled MNPs on target tumors were

imaged for tumor imaging by mechanically moving the integrated probe in 2D or by electrically

varying the US focus in 3D. One animal test was verified that anti-AFP MNPs were bound to

liver tumors by directly injecting a magnetic reagent (1.6 emu/g and 750 µl) into a liver tumor

(12 × 7 × 12 mm in length, width, and height) implanted on the back of an anesthetized rat.

RESULTS One animal test was verified that anti-AFP MNPs were bound to liver tumors by

directly injecting a magnetic reagent (1.6 emu/g and 750 µl) into a liver tumor (12 × 7 × 12 mm

in length, width, and height) implanted on the back of an anesthetized rat.

CONCLUSION The utilized DC magnetic field in targeted regions including tumors not only

magnetizes MNPs for magnetic imaging but also attracts more MNPs to target tumors faster,

critical for many MNP-based biomedical applications, like imaging, drug delivery, etc. [1] J. J. Chieh, , et al., J. Nanobiotechnol. 13: 11,2015.

[2] K.W. Huang, J.J. Chieh*, et al., Nanotechnology,27, 235101,2016.

[3] K.W. Huang, J.J. Chieh*, et al., ACS Nano, 11, 3030–3037, 2017.

15

High-TC SQUID based NMR for breast cancer and

liver cancer diagnosis

Shu-Hsien Liao1, Yu-Ting Liao1, Hao-Wei Huang1 Yan-Cheng Chen1, Jhih-Hao Chen1, Kai-

Wen Huang2 Herng-Er Horng1

1Institute of Electro-Optical Science and Technology, National Taiwan Normal University,

Taiwan.

2Graduate institute of Clinical medicine, National Taiwan University, Taiwan

[email protected]

In this study, a high-Tc SQUID-detected nuclear magnetic resonance spectrometer was set-up

to discriminate Breast tumor and liver tumor. For NMR and MRI measurement we apply three dimensional gradient field to cancel the field inhomogeneity in our lab to obtain a narrow

linewidth NMR spectrum of 0.8 Hz from a 0.5-ml water specimen. For NMR measurement, the

Larmor frequency is varying with time due to the variation of static field from environment.

Therefore, the time-domain frequency adjusted average method guided by a fluxgate was used

to correct the frequency variation and average the NMR signal in time domain. For tumor

discrimination, the T1 relaxation time of normal tissue and tumor tissue were demonstrated.

Furthermore, the receiver operating characteristic curve was applied to determinate the

threshold value of T1 relaxation time. The sensitivity and specificity for breast cancer and liver

cancer diagnosis were preformed. Our high-Tc SQUID based low-field MRI system shows the

feasibility for cancer diagnosis.

16

Estimation of electrochemical impedance using HTS-

SQUID based magnetic measurement system

K. Sakai, T. Kiwa and K. Tsukada

Graduate School of Interdisciplinary Science and Engineering in Health Systems,

Okayama University, Okayama

[email protected]

Electrochemical impedance spectroscopy (EIS) is widely used to analyze the electrochemical

reactions of devices and the EIS is useful for improving the performance of devices because the

precise electrochemical reactions can be analyzed by EIS. In the conventional measurement

method of EIS, the impedance was measured by the voltage and current between the electrodes

attached to the measurement sample. Because of this, the obtained impedance is the averaged

values between the electrodes and it is difficult to evaluate the EIS of localized region inside

the sample. Thus, we have proposed to estimate the localized EIS (LEIS) by detecting a

magnetic field from a current flowing in the sample. However, the applied voltage for EIS

measurement should be low to avoid the nonlinear response of sample, hence the magnetic field

generated from the sample is also small due to the small current. To detect this small magnetic

field, a highly sensitive measurement system using a high-temperature-superconductor

superconducting quantum interference device (HTS-SQUID) was developed [1].

In this study, the magnetic signal from the current measured by changing the frequency of

applied voltage was compared with AC impedance measured by the conventional method and

the estimation of LEIS is discussed. To demonstrate the estimation of LEIS, a dye-sensitized

solar cell with different catalysis in one cell was prepared. As a result, the detected magnetic

signal depended on the measured area at which the catalysis material is different and the

tendency of each magnetic signal was similar to the EIS of solar cell prepared with each single

catalysis. This result indicates that the estimation of LEIS will be possible using the proposed

method.

[1] K. Sakai, T. Kizu, T. Kiwa, K. Tsukada, “Analysis of AC Impedance in Localized Region Using Magnetic

Field Distribution Measured by HTS-SQUID”, IEEE Trans. Appl. Supercond., Vol. 28, 1600905 (2018)

17

Characterization of High-TC dc-SQUID

Magnetometers: Fabrication with Sputtered YBCO

Films Deposited on Recycled SrTiO3 Bi-crystal

Substrates

Tien-Wei Yang , and Li-Min Wang

Department of Physics/Graduate Institute of Applied Physics, National Taiwan University,

Taipei 10617, Taiwan.

Fabrication of high-performance high-Tc superconducting quantum interference devices

(SQUIDs) with low flux noise, high-throughput yield, and low cost is still challenging [1,2].

High-temperature-Tc dc-SQUID magnetometers have been fabricated using sputtered

YBa2Cu3Oy (YBCO) films grown on recycled 22.6°-tilted bi-crystal SrTiO3 (STO) substrates.

First, high-quality recycled STO bi-crystal substrates have been obtained via an optimum

polishing process, showing a surface roughness of ~0.2 nm after this process and a reduced

width of the artificial bi-crystal boundary on the surface of recycled STO substrates. During

sputtering deposition, optimum growth temperature of YBCO thin film is controlled to make a

smooth surface on the artificial boundary. The critical temperature and surface roughness of

YBCO thin film are 89 K and 2 nm, respectively. The surface morphology of Josephson

junctions in the fabricated high-Tc SQUIDs has been probed by AFM and SEM images. The

dc-SQUID magnetometers are designed with a directly-coupled pickup coil. The I-V curves,

field modulation pattern, and the flux noise spectrum have been used to characterize the SQUID

magnetometers. With optimum processes for thin-film growth and device fabrication, the

throughput yield is higher than 90% for devices with a modulation voltage VPP > 20 μV and the

field noise spectrum below 75 fT/Hz1/2 at 1 kHz, and 260 fT/Hz1/2 at 10 Hz at temperature 77

K. The factors of influence on the noise properties are investigated.

[1] S. Ruffieux, M. Xie, M. Chukharkin, C. Pfeiffer, A. Kalabukhov, D. Winkler and J. F. Schneiderman (2017),

Feedback solutions for low crosstalk in dense arrays of high-Tc SQUIDs for on-scalp MEG, Supcond. Sci.

Technol., 30, p 054006.

[2] Kuen-Lin Chen, Su-Hsien Liao, Yan-Hong Chen, Herng-Er Horng, Li-Min Wang, and Hong-Chang Yang

(2015), Low-Noise Serial High-Tc YBa2Cu3Oy Superconducting Quantum Interference Devices Based on

Bicrystal Junctions, IEEE Transactions on Applied Superconductivity, 25, p1600107.

18

Josephson junctions with novel barrier layers

Huabing Wang*,Zuyu Xu, Wei Chen, Shixian Chen, Wanghao Tian, Yangyang Lv,

Xianjing Zhou, Sining Dong, Jun Li, Yonglei Wang, and Peiheng Wu

Research Institute of Superconductor Electronics (RISE), Nanjing University, Nanjing.

*[email protected]

Hybrid Josephson junctions incorporating various barrier layers provide prospects for the

realization of fundamental studies of exotic physical phenomena as well as the applications to

superconducting quantum devices. Recently, interest in the Josephson coupling with novel

barrier layers (such as semiconductors, graphene, topologic insulators, etc) has been utilized

for field-effect supercurrent transistors, superconducting quantum chips and accessing the

Majorana fermionic excitation states [1,2]. Nonetheless, these effects require the formation of

homogeneous and barrier-free interfaces between the superconductor and barrier layers. To

overcome the obstacles, we have developed an in-situ fabrication system which enables us to

minimize oxidization and interfacial degradation of hybrid Josephson junctions. Here, some

experimental results on the novel barrier layers in contact with superconductors are reported,

we show the strong Josephson coupling through the barrier layers proved by the Shapiro steps

and Frounhofer-like patterns. In addition, the electrostatic field is exploited to modify the

supercurrent of Josephson junctions. Our in-situ fabrication technique introduces a powerful

tool to investigate the peculiar behavior of Josephson junctions with novel barrier layers and

also to improve the Josephson coupling for applications in superconducting hybrid quantum

devices.

We gratefully acknowledge financial support by the National Natural Foundation of China

(Grants No.61727805, 11234006).

[1] Heersche, H.B., Jarillo-Herrero, P., Oostinga, J.B., Vandersypen, L.M. & Morpurgo, A.F. (2008). Bipolar

supercurrent in graphene. Nature 446, 56-59 .

[2] Rokhinson, L.P., Liu, X. & Furdyna, J.K. (2012). The fractional a.c. Josephson effect in a semiconductor–

superconductor nanowire as a signature of Majorana particles. Nature Physics 8, 795-799.

[3] Zhu, Y.Y. at el. (2019). Isotropic Josephson tunneling in c-axis twist bicrystals of Br2Sr2CaCu2O8+ᵹ.

Preprint at https://arxiv.org/abs/1903.07965

19

Strong proximity Josephson coupling in

heterojunctions of 2D materials

Hu-Jong Lee

Department of Physics, POSTECH, Pohang 37673, Republic of Korea

Realization of proximity coupling in Josephson junctions, incorporating various two-

dimensional (2D) van der Waals materials including graphene, has recently attracted much

research interest. In this talk, I will focus on the short-ballistic (SB) strong Josephson coupling

realized in vertical and planar proximity Josephson junctions with mono-layer graphene as the

thin normal-conducting spacer. The short-ballistic junction characteristics provide highly

robust coherent states to be utilized for possible quantum-device applications. Here, for vertical

graphene Josephson junctions (GJJs), the SB strong proximity coupling is realized by

shortening the channel length down to the thickness of mono-layer graphene between two

superconducting-layer electrodes. For planar GJJs, the SB strong coupling is realized via the

ballistic conducting channel of a boron-nitride-encapsulated graphene layer. I will also discuss

how the Josephson effect is utilized to study fundamental material properties such as the robust

surface conduction in a topological insulator and the edge conduction in 2D materials such as

quantum spin Hall insulators and graphene. For details on the topics, one may refer to Ref. [1].

[1] Gil-Ho Lee and Hu-Jong Lee, Proximity coupling in superconductor–graphene heterostructures, Reports on

Progress in Physics 81, 056502 (2018).

20

Spin-dependent behaviors in Ferromagnet/Intrinsic

Josephson junctions/Ferromagnet Hybrids

A. Irie1, R. Kimura1, K. Murata1, K. Yamaki1, Yu. M. Shukrinov2, and I. R. Rahmonov2

1School of Engineering, Utsunomiya University, Utsunomiya.

2BLTP, JINR, Dubna.

[email protected]

Since many interesting spin-related phenomena have been observed in different variation of

Ferromagnet/Superconductor (F/S) structures [1,2], F/S hybrids have attracted much attention

in recent years not only from a fundamental interest but also from an application point of view.

Most of experimental studies with respect to the spin-dependent properties of such systems

have been performed using low Tc superconductors such as Nb and Al. On the other hand, it is

also important and interesting to clarify the spin-dependent transport properties in such systems

using high Tc superconductors because they can lead to the design of new spintronics device

operating at higher temperature.

We have investigated the influence of the ferromagnet magnetization on the transport

properties of intrinsic Josephson junctions (IJJs) in Co/Au/BSCCO/Au/Co hybrid structure

under applied magnetic fields. Due to their extremely thin superconducting layer of 0.3 nm, the

spin-polarized current injection into IJJs is expected to significantly influence their

superconducting behavior. The current-voltage characteristic at 77 K in a zero-field showed the

multiple quasiparticle branches with hysteresis similar to that of conventional intrinsic

Josephson junctions. On the other hand, it was observed that the critical current shows a clear

asymmetric field dependence with respect to the direction of the field sweep, resulting in

hysteretic behavior. By comparing the field dependence of critical current with magnetization

curve of the sample, we found that the critical current is strongly suppressed in the antiparallel

configuration of the relative magnetization orientation of upper and lower Co layers in F/IJJs/F

structure due to the accumulation of spin-polarized quasiparticles in intrinsic Josephson

junctions. The observed suppression of the critical current is as large as more than 20%. The

experimental data were analyzed qualitatively using the sine -Gordon model.

[1] A.I. Buzdin, Rev. Mod. Phys., vol.77, no.3, pp.935–976, 2005.

[2] J. Linder and J.W.A. Robinson, Nature physics, vol.11, no.4, pp.307–315, 2015.

21

Ultrafast optical response and vortex generation

in high-Tc superconductors

Masayoshi Tonouchi

Institute of Laser Engineering, Osaka University, Osaka, Japan

[email protected]

High Tc superconductors (HTSCs) is one of the most attractive perovskite oxides in terms of

fundamental science and future applications such as in quantum information and THz devices.

Superconductivity develops as the result of various scatterings with minimum ensemble free

energy. Unveiling its complicated carrier dynamics has been considered to be the most

important physics for HTSC science. However, in comparison with semiconductors, tools to

probe it are rather limited because one cannot observe usual photoluminescence from HTSCs,

suggesting that transient physics in HTSCs is still premature field. Here, we explain that the

observation of THz emission helps to understand such carrier dynamics. Upon illumination of

HTSCs with femtosecond optical pulses, one can generate THz waves as a consequence of

optical modulation of supercurrent. One can expect from the THz waveforms in time domain

that major part of nonequilibrium states lasts only one picosecond. However, actual carrier

dynamics may last much longer, including avalanche pair breaking. To study the carrier

dynamics, pump and probe THz emission spectroscopy (PPTES) is employed. PPTES detects

THz emission electric field excited by the probe fs optical pulses which follow the pump pulses.

The transient phenomenon takes around 10 picoseconds in total, which is much longer than

expected from the waveforms. Phenomenological explanation is that, the initial pair breaking

is the avalanche process with multi scattering which decreases the transport supercurrent,

simultaneously the rest of pairs start to accelerate, and the supercurrent recovers. Namely, we

observe that the supercurrent modulation ends within 2 picoseconds. However, there still

remain nonequilibrium states. The emission THz field is enhanced due to the increase of

transmittance of the THz waves during avalanche pair breaking process and in the YBCO films

and after the enhancement point, quasiparticles relax into the cooper pairs while emitting

phonons. We can estimate various time constants for those scattering by PPTES.

Another interesting optical response is optical vortex generation in HTSCs. Illumination

with the fs optical pulses evaporates the supercurrent partially and locally in the HTSC films

carrying the transport supercurrent, and, as a consequence, the magnetic flux is allowed to exist.

This means that the photons change the initial conditions for superconducting state similar to

the field-cooled one. Distribution of the vortices reflects the special distribution of the fs

photons. Thus a single fs laser beam pattern can be captured by the optical-vortex generation.

In this talk, we review such ultrafast optical response and vortex generation in HTSCs [1]

[1] Rana D. R. and Tonouchi M. (2019), Terahertz Emission Functionality of High-Temperature

Superconductors and Similar Complex Systems, Advanced Optical Materials in press.

22

Two-resonance-mode dielectric resonator method as

an International Standard for the Intrinsic Surface

Impedance of High-TC Superconductor Films

S.Y. Lee1, S.H. Lee1, H.S. Jung2 and J.H. Lee2

1Department of Physics, Konkuk University, Seoul.

2SuNam Co., Ltd, Anseong

[email protected]

Two-resonance-mode dielectric resonator (DR) method has been published as an IEC

international standard, IEC 61788-15 Ed. 1, for measurements of the intrinsic surface resistance

(RS) and the intrinsic surface reactance (XS) of high-TC superconductor (HTS) films [1].

However, descriptions on uncertainty analysis for the RS and the XS, which are missing in IEC

61788-15 Ed. 1, need to be included in the second edition of the standard. We describe

uncertainty analysis for the RS and XS based on the measured uncertainties in the quality factors

(uQ) and the resonant frequencies (uf) for the TE021 and the TE012 modes of a sapphire resonator.

For this purpose, we first estimate uncertainties in the complex conductivity σ (= σ1 – iσ2) from

uQ and uf, which are used to estimate uncertainties in RS and XS using the relation of ZS =

(iωμ0/σ)1/2 with ω and μ0 denoting the angular frequency and the permittivity of vacuum,

respectively. The sapphire resonator is designed such that the two resonance modes, TE021 and

TE012, appear next to each other with no parasitic modes appearing between the two modes.

Also, the tan δ of the sapphire rod used for the dielectric resonator should be extremely low for

realizing low uncertainties in the RS and the XS.

We also review applicability of the two-resonance-mode DR method for measuring the

thickness of metallic and superconductive films, as well as the tan δ of low-loss dielectrics at

cryogenic temperatures, YBa2Cu3O7-δ films and Pt films were tested for the thickness

measurements, with high-purity Si and Ge being used for the dielectrics. The thickness of Pt

films as thin as 10 nm could be measured non-invasively, with a tan δ value as low as 10-7 being

measured with accuracy at cryogenic temperatures. We also review use of the DR method for

investigating homogeneity in the RS over the area of large HTS films

[1] IEC 61788-15, Ed. 1, Superconductivity – Part 15: Electronic characteristic measurements – Intrinsic surface

impedance of superconductor films at microwave frequencies (IEC, 2011).

23

The Development of Large-scale Josephson

Junction Array Devices for the Quantum Voltage

Standard at NIM

Jinjin Li, Wenhui Cao, Yuan Zhong, Lanruo Wang, Qing Zhong, Xueshen Wang

National Institute of Metrology, Beijing, China.

[email protected]

The integrated Josephson junction array devices are the core part of the quantum voltage

standards. The National Institute of Metrology of China (NIM) has been developing Nb/NbxSi1-

x/Nb array devices for the quantum voltage metrology since 2010. Many progresses have been

made. A 400,000 array device with a 4-junction vertically stacked structure is realized. Good

dc V-I characteristics are obtained. The superconducting on-chip microwave circuit which

consists of power divider, filters, biases, on-chip inductors, capacitors, resistors and tapered

transmission lines is realized. The 0.5 V quantum voltage device has been realized in 2018. The

device includes on-chip microwave circuit system and ~26,000 Josephson junctions. The output

voltage is about 0.46 V under 17.46 GHz microwave irradiation. The quantum voltage system

based on this device is directly compared with the programmable Josephson quantum voltage

standard based on the device of National Institute of Standard and Technology of USA (NIST).

The difference of reproducible quantum voltage is on the 10-10 V level , which indicates that

the device has good performance. The NIM device can provide stable quantum voltage and can

be used to carry out dc voltage calibration. The 1 V quantum voltage device has been realized

in 2019. The output voltage is about 1.17 V under 18.36 GHz microwave irradiation. Low

voltage noise which is as good as NIST is obtained. We also developed the device for the

two-channel micro-volt quantum voltage system. High precision system with absolute

uncertainty better than 10-9 V is realized. The system has already been applied to low voltage

calibration.

24

Quantum metrology triangle for future electrical

standard

Myung-Ho Bae

Korea Research Institute of Standards and Science, Daejeon 34113, Republic of Korea

[email protected]

The international system of units (SI) such as kelvin (K), kilogram (kg), mole (mol) and ampere

(A) were recently redefined, based on the physical constants such as Boltzmann constant k,

Plank constant h, Avogadro Number NA and elementary charge e. For instance, ampere will be

defined by taking the elementary charge to be fixed as 1.602176634x10-19 coulomb in the new

SI. Thus one ampere is the electric current corresponding to the fow of 1/(1.6021766208x10-

19) elementary charges per second. However, the realization of one ampere based on the new

definition is too far to go with the current technology. A practical way to realize the one ampere

at laboratories will be to use the Ohm's law between the quantum Hall resistance (QHR)

standard and the Josephson voltage standard (JVS). Thus, in the new SI, we must resolve the

logical gap between the definition of ampere and its Ohm's law-based practical realization. As

a resolution, so-called the quantum metrology triangle (QMT) consisting of the three arms of

the QHR, JVS and the single electron tunneling (SET)-based quantized charge current must be

closed within 10-8 uncertainty to confirm the Ohm's law among them. In my talk, I will present

the progress on the QMT experiment in our institute.

25

Investigation of radiation properties of THz-wave

oscillators using Bi-2212 intrinsic Josephson

junctions for oscillator-array design

T. Tachiki and T. Uchida

Department of Electrical and Electronic Engineering, National Defense Academy, Yokosuka.

[email protected]

Electromagnetic (EM)-wave oscillators using intrinsic Josephson junctions (IJJs) in

Bi2Sr2CaCu2O8+ (Bi-2212) cuprate superconductors are promising solid-state devices to

generate continuous-waves in the terahertz (THz) range [1, 2]. The oscillators using IJJs are

expected to be used as a local oscillator in a superconducting mixer, a THz source in an active

imaging system for nondestructive testing or medical diagnosis and so on.

Recently, wide frequency range (0.3 – 2.4 THz) of EM radiation from a cylindrical Bi-2212

mesa [3], high output power (610 W @ 0.51 THz) of a 3-mesa-array [4] and a narrow

linewidth (7 MHz @ 0.75 THz) of a highly-biased mesa locked with a superconducting

integrated receiver [5] have been reported.

We performed numerical simulations by using the coupled sine-Gordon equations that can

describe EM fields in an IJJ system, and investigated radiation properties such as a bias voltage

vs. output power, linewidths and radiation patterns when cavity resonances occurred in a Bi-

2212 mesa [6, 7]. In order to compare with the simulation results, rectangular mesas with 80

m × (120 – 300) m × (1 – 2) m were fabricated on Bi-2212 single crystals grown by a self-

flux method, and bias dependencies of radiation power and frequency of these mesas were

measured. From these results, the cavity modes, e.g. 111-, 121- and 112-modes, were evaluated

[8]. The evaluated modes are useful for designing a mesa-array that can generate THz-waves

with output power more than 1 mW, since the radiation patterns of individual mesas depend on

the cavity modes, and the output of the array is obtained from the radiation pattern synthesis of

the mesas. [1] L. Ozyuzer et al., Science, 318, pp.1291–1293 (2007).

[2] Kakeya and H. B. Wang, Superconduct. Sci. Technol., 29 (7), 073001 (2016).

[3] T. Kashiwagi et al., Appl. Phys. Lett., 107 (8), 082601 (2015).

[4] T. M. Benseman et al., Appl. Phys. Lett., 103 (2), 022602 (2013).

[5] V. P. Koshelets et al., IEEE Trans. Terahz. Sci. Technol. 5 (4) pp.687–694 (2015).

[6] T. Tachiki and T. Uchida, J. Appl. Phys., 107, 103920 (2010).

[7] T. Tachiki and T. Uchida, Physica C, 471, pp.1206–1209 (2011).

[8] T. Tachiki et al., J. Infrared Milli. Terahz. Waves, 35 (6–7), pp.509–516 (2014).

26

2 THz Hot Electron Bolometer Mixer

using a Magnetic Thin Film

Akira Kawakami*, Yoshihisa Irimajiri

National Institute of Information and Communications Technology,

Kobe, Hyogo, 651-2492, Japan

* [email protected]

To expand the intermediate frequency (IF) band and improve the sensitivity of a hot electron

bolometer mixer (HEBM), we have proposed and examined a new HEBM structure using a

nickel (Ni) magnetic thin film (Ni-HEBM). We found that it was possible to suppress the

superconductivity under the electrodes of the HEBM caused by the niobium nitride (NbN) thin

film for construction of the superconducting strip by the addition of a Ni thin film. By using

Ni-HEBM structure, superconductivity exists only in the region between both electrodes and

we think that it is possible to further miniaturize the HEBM. The miniaturization acts to expand

the IF band, improve the sensitivity and is expected to reduce the required LO power. By using

the Au (100nm) / Ni (0.6 nm) bilayer for the electrodes, we fabricated Ni-HEBM with a NbN

strip of 0.1 μm-length. The IF bandwidth of the fabricated Ni-HEBMs was evaluated at 1.9

THz. We confirmed that the IF

bandwidth expands. Fig. 1 shows the

evaluation of the IF gain bandwidth of

the Ni-HEBM with strip length of 0.1

μm. Here, ±2 times the standard error

(SE) is written as fC error bars in the

figure. The IF bandwidth was evaluated

about 6.9 GHz at 4 K., and the evaluated

bandwidths was about 6.9 GHz at 4 K. The uncorrected receiver noise

temperature of same Ni-HEBM was also

evaluated at 4 K, and it was about 1220

K(DSB) at 2 THz.

[1] Kawakami, Y. Irimajiri, T. Yamashita, S.

Ochiai, Y. Uzawa, “Broadening the IF band

of a THz hot-electron bolometer mixer by

using a magnetic thin film,” IEEE Trans.

THz Sci. Technol., vol. 8, no. 6, pp. 647–653, Nov. 2018.

Fig. 1. The IF gain bandwidth of the Ni-HEBM. The

superconducting strip length and width were 0.1 μm

and 0.5 μm, respectively. The LO frequency and the

measurement temperature were 1.9 THz and 4 K,

respectively.

-3dB

fC=6.9±1.2 GHz

1 2 3 4 5 6 7 8 925

30

35

40

35.9

IF p

ow

er

(dB

)

Frequency (GHz)

fLO=1.9 THz

TMEAS.=4 KVBIAS=0.8mV

±2SE

27

Development of NbN Hot Electron Bolometer Mixer

Operating at 1.5 THz

Hsiao-Wen Chang1, Yen-Ru Huang1, Chun-Lun Wang1, and Ming-Jye Wang1

1 Institute of Astronomy and Astrophysics, Academia Sinica, Taipei

[email protected]

The ASIAA and SAO team proposed to deploy the ALMA prototype antenna with

12m dish on the summit of Greenland, the Greenland Telescope, which is one of

possible locations for terahertz (THz) astronomical observation. The Greenland

Telescope (GLT) has better angular resolutions (∼ 4 arcsec) compared with space or

airborne THz telescopes [1]. By targeting atmospheric windows around 1–1.5 THz for

GLT, we are developing the hot electron bolometer (HEB) mixers based on epitaxial

NbN thin films.

We had fabricated 1.5 THz HEB mixers using high quality superconducting NbN

ultrathin films on (001) 3C-SiC. However, the superconducting transition of few

nanometer NbN films with nano-bridge becomes seriously broadened due to the

proximity effect of the Au contact, especially in the case with thickness less than 4 nm.

The proximity effect of contact pads pattern can be significantly reduced by the adding

a ultrathin Ni layer [2]. HEB mixer with Ni (1 ~nm)/NbN (4 nm) bilayer on 3C-SiC

substrate operating at 1.5 THz LO frequency has been fabricated. The receiver

demonstrates a noise temperature of 1100 K with intermediate frequency (IF) bandwidth

of 4 GHz.

In addition, the IF bandwidth of HEB mixer can be improved by using NbN films

deposited on hexagonal GaN due to the close acoustic match to NbN and a low defect

interface [3,4]. Here, we will also present the high quality ultrathin epitaxial NbN films

deposited on (0001) hexagonal 4H-SiC substrates. The superconducting transition

temperature remains around 10K even the thickness of film is less than 3 nm.

[1] H. Hirashita, P. M. Koch, S. Matsushita, S. Takakuwa, M. Nakamura, et al. (2016), “First-generation science

cases for ground-based terahertz telescopes,” Publ. Astron. Soc. Jpn., vol. 68, R1.

[2] Kawakami, et al. (2018), “Broadening the IF Band of a THz Hot-Electron Bolometer Mixer by Using a

Magnetic Thin Film”, IEEE Transactions on Terahertz Science and Technology, 8(6), 647-653.

[3] S. Krause et al. (2016), "Reduction of phonon escape time for NbN hot electron bolometers by using GaN

buffer-layers," IEEE T. Thz. Sci. Techn., Vol 7, Issue 1, p53 - 59.

[4] S. Krause et al. (2018), "Noise and IF Gain Bandwidth of a Balanced Waveguide NbN/GaN Hot Electron

Bolometer Mixer Operating at 1.3 THz," IEEE T. Thz. Sci. Techn., Vol. 8, 3, p365-371.

28

Applications of superconducting thin films for

extensive use in terahertz functional devices.

K. Nakajima, K. Suzuki, A. Saito and H. Yamada

Graduate School of Science and Engineering, Yamagata University, Yonezawa, Japan

[email protected]

Superconducting thin films manifest a significant diversity in terms of possible terahertz (THz)

wave application. From oscillator point of view, it has been proved that the intrinsic Josephson

effect of Bi2Sr2CaCu2O8+ (Bi-2212) high-TC superconductor crystal[1] can generate monotonic

THz wave[2]. For the THz oscillation, we have succeeded to produce powerful THz emission

from intrinsic Josephson junction made of solid Bi-2212 thin film grown on MgO substrates at

operating temperatures higher than that reported earlier using “Mesa” devices made of bulky

single crystal[3]. In contrary to oscillation, superconducting thin films are also applied for

various high sensitive THz detection devices such as Superconducting Tunnel Junction(STJ),

Het Electron Bolometer(HEB) and Microwave Kinetic Inductance Detector(MKID) [4]. Among

them we has been developing NbN MKIDs array operating with a conventional GM refrigerator

for terahertz imaging.[5]

Other than these usual application, we study a possible application of Bi-2212 thin film for THz

metamaterials. For this purpose, we fabricate ultra-thin Bi-02212 films on dielectric substrates

suitable. At first, we have succeeded epitaxial growth of few nm thick Bi-2212 film by Metal

Organic Decomposition (MOD) method on SrTiO3 (STO) 100 substrates with good crystallinity

and superconductivity. However, we measured poor THz optical properties of STO then we

found NdGaO3(NGO) as a candidate for the substrate alternative of STO for THz metamaterials.

In this presentation, I overview above mentioned THz applications of superconducting thin

films and introduce recent progress of our research projects in Yamagata University.

[1] R. Kleiner and P. Müller, Phys. Rev. B 49, 1327 (1994).

[2] L. Ozyuzer et al, Science 318, 1291 (2007).

[3] T. Uchida, K. Nakajima et al, IEEE Trans Appl. Supercond, 28, 1800304(2018).

[4] P. Day, H. Leduc, B. Mazin, A. Vayonakis, and J. Zmuidzinas, Nature, 425, 817 (2003).

[5] S Ariyoshi, K Nakajima, A Saito et al, Supercond. Sci. and Technol. 29, 035012(2016).

29

Extremely Energy-Efficient Circuit Technology

based on Adiabatic Quantum Flux Parametron

N. Yoshikawa1,2, N. Takeuchi2, C. Ayala2, O. Chen2, Y. He2 and Y. Yamanashi1,2

1 Graduate School of Engineering, Yokohama National University, Yokohama.

2 Institute of Advanced Science, Yokohama National University, Yokohama.

[email protected]

Adiabatic quantum flux parametron (AQFP) is extremely energy-efficient logic whose energy-

delay product is six orders of magnitude smaller than that of the state-of-the-art semiconductor

logic [1]. Our group is developing low-power microprocessors based on the AQFP logic. In this

talk, we will present our latest research activities for realizing the AQFP microprocessor. After

showing the advantage of AQFP as a logic circuit element, we will introduce the methodology

for designing AQFP integrated circuits based on our AQFP standard cell library. Automated

top-down design environment, which consists of logic synthesis, logic simulation, and

automated routing tools, was developed for designing large-scale AQFP integrated circuits. We

will show recent circuit demonstrations of large-scale AQFP integrated circuits, including an

ALU and a register file for the microprocessor components. Recent developments of Josephson-

CMOS hybrid memories, where cryo CMOS memory cells constitute memory elements, are

also shown. We will discuss the energy efficiency of the AQFP integrated circuits by comparing

them with those using future semiconductor processes [2].

[1] N. Takeuchi, D. Ozawa, Y. Yamanashi and N. Yoshikawa, “An adiabatic quantum flux parametron as an

ultra-low-power logic device,” Supercond. Sci. Tech. 26, 035010 (2013).

[2] O. Chen, R. Cai, Y. Wang, F. Ke, T. Yamae, R. Saito, N. Takeuchi, N. Yoshikawa, “Adiabatic Quantum-

Flux-parametron: towards Building Extremely Energy-Efficient Circuits and systems,” Scientific Reports, 9,

10514 (2019).

30

Agenda for IEC/TC90 WG8 and WG14 Joint

Meeting

Title of WG8: Electronic characteristic measurements

Title of WG14: Superconductor electronic devices

Subject for discussion:

1. Confirmation of minutes of last IEC/TC90/WG8 Meeting at Busan

2. Report of IEC 61788-7 Ed. 3 FDIS and future plan

3. Report of IEC 61788-17 Ed.2 CDV

4. Report of modifications of IEC 61788-15 Ed. 2

5. Report of EUCAS2019 IEC-IEEEWG14 Meeting, new plan on LTS-SQUID transport

property and future schedule

6. Report of the measurement of dark current in superconducting junctions

Documents attached:

1. Agenda

2. Minutes of IEC/TC90/WG8 Meeting at Busan ( S.Y. Lee)

3. Report of FDIS of IEC 61788-7 Ed.3 and future schedule of WG8 (S. Ohshima)

4. Report of CDV of IEC 61788-16 Ed. 2 (H. Yamasaki)

5. Report of modifications of IEC 61788-15 Ed. 1 (S.Y. Lee)

6. Report of EUCAS2019 IEC-IEEEWG14 Meeting, new plan on LTS-SQUID transport

property and future schedule (M. Ohkubo)

7. Report on the measurement of dark current in superconducting junctions (L. You)

31

Discovery of new superconductors under high

pressure using materials informatics

Yoshihiko TAKANO1,2

1 National Institute for Materials Science (NIMS), Tsukuba City, Japan

2 Tsukuba Univ., Tsukuba City, Japan

[email protected]

High pressure is a promising tool to find new functional materials which cannot

appear under ambient pressure. For example, the discoveries of new high-Tc

superconductivity in H3S at ~200 K and LaHx at ~260K under high pressure were

recently reported. Diamond anvil cell (DAC) is most useful apparatus to generate high

pressure over 10GPa. However, the resistivity measurement using DAC is quite difficult

because it requires 4-terminal electrodes wiring to a very small sample. To make the

resistivity measurement under pressure easy, we develop the new DAC using

superconducting diamond electrodes which is fabricated on the bottom anvil. We have

explored new pressure induced superconductors using this new DAC.

Data-driven material science (materials informatics, materials genome initiative,

chemometrics) recently brings remarkable results in the field of medicine and

macromolecule and so on. On the other hand, a search for new superconducting

materials has been still conducted through a carpet-bombing type experiment depending

on the experience and inspiration of researchers.

We have exhaustively searched the candidates of new superconducting materials

using the data-driven method with first-principle calculation as a guideline which is a

specific band structure of “flat band” near fermi energy with small band gap. If the flat

band crosses the fermi energy by high pressure, superconductivity would be appeared

due to high density of state (DOS) near the fermi energy. In my presentation, I will talk

about successful demonstration of the discovery of new superconductors under high

pressure by data-driven materials research [1-2].

[1] R. Matsumoto et al., Applied Physics Express 11, 093101 (2018).

[2] R. Matsumoto et al., Science and Technology of Advanced Materials, Vol.19, 909, 2018. arXiv:1808.07973.

32

Specimen Thinning for HRTEM via Photon

illumination

H. Ichinose1 and N. Sakaguchi2

2Center for Advanced Research of Energy and Materials,

Faculty of Engineering, Hokkaido University

[email protected], [email protected]

Modern high-resolution transmission electron microscope (HRTEM) has been

prevailed as one of most powerful tools for structural analysis of complicated solid

material including high Tc superconductors; HRTEM is able to directly observe

atomic structure of materials, even a single atom. This ability is attributed to strong

interaction between electron wave and atomic potential. In order to enjoy such

excellent power, an object specimen has to be thin enough; being around a few ten

atomic layers and at the same time does not contain any additional defects in atomic

dimension in it so that original structure’s image is not disturbed by irregular

additional images due to defects. Currently we actually can prepare a thin enough

specimen but unfortunately it usually contains additional lattice defects produced

during the thinning.

In practice, an object specimen is thinned employing so called ion milling; surface

atoms are flicked off with accelerated ions one by one simply following mechanical

momentum transfer principle of point mass. Ions in gas state are accelerated in electric

field of several kV in strength. High voltage acceleration is aimed to cover poor

accuracy rate of the ion shooting by increasing of velocity; equivalent number of ions

with that of surface atomic density are enabled arrive onto the specimen in a unit time,

so that we can finish the thinning within finite time. Trouble is that this effort is

nothing but to give extremely higher energy than atomic bonding energy to the ion too.

Surplus energy of the ion is consumed to produce lattice defects and to destroy sound

crystal lattice. As far as we employ the flick off process with accelerated ion, we can’t

be free from lattice defect production in a specimen.

One possible way to escape from the situation is to employ any “quantum bullet”

instead of a “mechanical point mass bullet”. Conditions required for a new quantum

bullet to be employed is that an energy carried by it is not much excess than atomic

bonding energy and large number of bullets can carry same amount of energy at the

same time. A candidate quantum which fulfil the condition would be found among not

Fermion but Boson; photon should be most probable one. In practice, after many trials,

LASER was found to work well. A specimen thinned by our method was thin enough

with smooth surface and without any additional lattice defects.1)

[1] N. Sakaguchi, M. Kozuka, H. Ichinose Laser-assisted sample preparation of silicon for high-resolution

transmission electron microscopy Microscopy, Vol. 64, pp. 111-119 (2015).

33

Electrical signal transmission in Neural Functions

C. K. Ong1, *, Kelvin J. A. Ooi2,^, Qingwei Zhai2,* Xiaoqing Sun2, Xiaoqi Yang2 ,Chunze Li2

and Shengyong Xu3,#

1Department of Mathematics, Xiamen University Malaysia, Jalan Sunsuria, Bandar

Sunsuria, 43900 Sepang, Selangor 2School of Electrical and Computer Engineering, Xiamen University Malaysia, Jalan

Sunsuria, Bandar Sunsuria, 43900 Sepang, Selangor 3Department of Electronics, and Key Laboratory for the Physics & Chemistry of

Nanodevices, School of Electronics Engineering and Computer Science, Peking University,

Beijing *Email: [email protected]

^Email: [email protected] #Email: [email protected]

The neural system and the brain of creatures are developed and perfected gradually through

evolutionary means. The evolution process of the neural system has grounding in physics in

order to effect improvement in the nerve conduction process and system. The celebrated Nobel

prize-winning(1963) Hodgkin-Huxley model is based on the physics of electrostatics and

electrodynamics, and could thus far explain some of the nerve conduction phenomena in simple

creatures, like squids, shrimps and earthworms. Yet, the model still has its disputed

inadequacies to explain nerve conduction phenomena in complex mammalian nerve fibers,

especially the myelinated nerve fibers. Only through the continual study and refinement of the

electrical signal transmission model in neural functions of lifeforms, we could enhance our

understanding of the complexity of nerve conduction, in various aspects of neurology such as

nerve diseases, mental diseases, and how memories are stored and retrieved. In this talk, I shall

present results from our joint project with the Peking University in exploring action potential

in the form of electromagnetic soliton pulse as generated by the transmembrane ion flow and

soft-material waveguides as electromagnetic propagation conduits in order to explain nerve

conduction in myelinated nerve fibers.

34

Superconducting nanowire single photon detectors

for quantum information

Lixing You, Weijun Zhang, Hao Li, Zhen Wang, Xiaoming Xie

1 State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of

Microsystem and Information Technology (SIMIT), Chinese Academy of Sciences, 865

Changning Rd., Shanghai 200050, China

[email protected]

Quantum information technology has turned to be a bullet train supported by many countries

(EU, USA, UK, JP and CN). The quantum information process (QIP) involves quantum sources,

quantum manipulation tools as well as quantum detectors. Since the photon (of visible and near

infrared wavelengths) is one of the most popular quanta to play, single photon detectors (SPDs)

play an irreplaceable role in QIP. As a novel SPD, superconducting nanowire single photon

detector (SNSPD) surpasses the semiconducting SPDs with many merits, such as high detection

efficiency, low dark count rate, low timing jitter, higher counting rate etc. SNSPDs have

advanced various QIP experiments in the past decade. Now you may buy the commercial

SNSPD systems including the cryogenics from several start-up companies. In this talk, we will

present the latest results of SNSPDs developed by SIMIT and the applications in QIP (quantum

information, QKD, quantum computation etc.).

[1] W. Zhang et al. NbN superconducting nanowire single photon detector with efficiency over 90% at 1550 nm

wavelength operational at compact cryocooler temperature. Science China Physics, Mechanics & Astronomy

60(12): 120314. (2017)

[2] H.-L. Yin et al, Measurement-Device-Independent Quantum Key Distribution Over a 404 km Optical Fiber.

Physical Review Letters 117(19): 190501. (2016)

[3] Y. Liu et al. Device-independent quantum random-number generation. Nature 562(7728): 548-551. (2018)

35

Recent progress in research and development of

superconducting nanowire single-photon detectors

H. Terai1, M. Yabuno1, S. Miyajima1, S. Miki1, F. China1, N. Takeuchi2, and N. Yoshikawa3

1Advanced ICT Research Institute, National Institute of Information and Communications

Technology, 588-2 Iwaoka, Nishi-ku, Kobe 651-2492.

2Institute of Advanced Sciences, Yokohama National University, 79-5 Tokiwadai, Hodogaya,

Yokohama 240-8501.

3Department of Electrical and Computer Engineering, Yokohama National University, 79-5

Tokiwadai, Hodogaya, Yokohama 240-8501.

[email protected]

Superconducting nanowire single-photon detectors (SSPDs or SNSPDs) have high sensitivity in a wide wavelength range between ultraviolet and mid-infrared, which is not available in other detectors such as avalanche photo diode and photo multiplier tube. We have developed multi-channel SSPD systems with a detection efficiency over 80% for near-infrared wavelength, a low dark count rate (typically below 40 Hz), a low timing jitter (typically below 70 ps), and a high counting rate (typically 20-30 MHz) [1]. If we can make a large-format SSPD array, it will be the ultimate camera with ultra-low noise, high dynamic range, and photon-countable sensitivity for a broad spectral range, which will become powerful tools in a wide range of fields. Since SSPDs are operated at a temperature of several Kelvin, the reduction of wiring count is crucial to realize a large-format SSPD array. We proposed a cryogenic digital signal processing based on single-flux-quantum (SFQ) circuits and successfully demonstrated the operation of a 64-pixel SSPD array system combined with a 64-bit SFQ encoder circuit [2,3]. To realize larger-scale SSPD array, we recently adopted a row-column readout architecture proposed by Allman et al. in our SSPD array system [4]. This architecture allows signal readout from a N×N-pixel SSPD array using 2×N readout wirings. By combining this architecture with our SFQ cryogenic signal processor, the number of readout wirings can be reduced to two for the N×N-pixel SSPD array. Our 64-bit SFQ encoder circuit can be applied to 32×32-pixel SSPD arrays by minor circuit modifications. Also, a part of the signal processing circuit can be replaced with adiabatic quantum flux parametron (AQFP) circuits (which can be driven by an AC current of 2-3 mA), allowing further reduction of the power dissipation and bias current [5]. By adopting the SFQ/AQFP hybrid signal processor, we are aiming to realize a superconducting nanowire-based single-photon camera with over 10,000 pixels.

[1] S. Miki, T. Yamashita, H. Terai, and Z. Wang, Opt. Exp. 21(8), 10208 (2013).

[2] H. Terai, S. Miki, and Z. Wang, IEEE Trans. on Appl. Supercond., 19(3), 350 (2009).

[3] S. Miyajima, M. Yabuno, S. Miki, T. Yamashita, and H. Terai, Opt. Exp. 26(22), 29045 (2018).

36

The original seeds of dark counts of SNSPD

Labao Zhang, Qi Chen, Biao Zhang, Rui Ge, Shuya Guo, Jingrou Tan, Jiayu Lv, uecou Tu,

Qingyuan Zhao, Xiaoqin Jia, Lin Kang, Jian Chen, and Peiheng Wu

Research Institute of Superconductor Electronics of Nanjing University, Nanjing, China,

210023

Email: [email protected]

There are several phenomenological model models[1-3], such as hot-spot model and

vortex model. However, the initial seeds of superconducting phase transition triggered by

photons is still unclear. The phase slips in superconductor nanowires has been widely

investigated through the distributions of switching current[4, 5], and was released in an

impedance readout in our previous work[6], which produced voltage pulses similar to the

response pulses of SNSPDs.

In this talk, firstly we will give a brief introduction on the new applications of SNSPD at

NJU, such as lunar laser ranging, intravital fluorescence lifetime imaging and quantum-

enhanced measurement. Then, I will focus on the explorations of the original seeds of dark

counts through interleaved superconductor nanowires.

[1] J. K. W. Yang, A. J. Kerman, E. A. Dauler, V. Anant, K. M. Rosfjord, and K. K. Berggren, "Modeling the

electrical and thermal response of superconducting nanowire single-photon detectors," (in English), Ieee

Transactions on Applied Superconductivity, vol. 17, no. 2, pp. 581-585, Jun 2007.

[2] J. J. Renema et al., "Experimental Test of Theories of the Detection Mechanism in a Nanowire

Superconducting Single Photon Detector," Physical Review Letters, vol. 112, no. 11, Mar 21 2014, Art. no.

117604.

[3] H. Bartolf et al., "Current-assisted thermally activated flux liberation in ultrathin nanopatterned NbN

superconducting meander structures," (in English), Physical Review B, vol. 81, no. 2, Jan 2010.

[4] M. Lu-Dac and V. V. Kabanov, "Phase slip phenomena in superconductors: from ordered to chaotic

dynamics," Phys Rev Lett, vol. 105, no. 15, p. 157005, Oct 8 2010.

[5] W. W. Zhao, X. Liu, and M. H. W. Chan, "Quantum Phase Slips in 6 mm Long Niobium Nanowire," (in

English), Nano Letters, Article vol. 16, no. 2, pp. 1173-1178, Feb 2016.

[6] L. Zhang, X. Yan, X. Jia, J. Chen, L. Kang, and P. Wu, "Maximizing switching current of superconductor

nanowires via improved impedance matching," Applied Physics Letters, vol. 110, no. 8, p. 072602, 2017.

Superconducting Detectors and Electronics for

Astronomical Applications

W. Cui1,2

37

1Tsinghua Center for Astrophysics, Tsinghua University

2Department of Astronomy, Tsinghua University

[email protected]

Superconducting detectors and electronics have found a wide range of applications in

astronomical observations, from microwave to gamma-ray wavelengths. Of particular

relevance are transition-edge sensor (TES), microwave kinetic inductance detector (MKID),

superconducting quantum interference device (SQUID) and SQUID-based multiplexing

readout technologies. I will review the applications, highlighting the needs for detection of

weak signals at long wavelengths and for high-resolution spectroscopy at short wavelengths in

the field of astronomy.

38

Metallic magnetic calorimeters for astroparticle

physics applications

Yong-Hamb Kim1

1Center for Underground Physics, Institute for Basic Science (IBS), Daejeon Korea

[email protected]

Metallic magnetic calorimeters (MMCs) are a type of low-temperature micro-calorimeters that

demonstrated their extreme energy sensitivities. MMCs employ noble properties and

technology development of superconducting sensors and electronics. The working principle is

based on the accurate measurement of magnetic signals caused by an energy absorption in a

detector using superconducting circuits. MMCs provide not just high energy resolution in their

applications, but also their physical properties that can be adjusted for a given experimental

condition. The sensitive detectors are operable in a wide range of temperatures following the

temperature dependence of the paramagnetic sensor material. In the presentation, the principle

of MMCs are introduced with some applications in astroparticle physics such as experimental

search for neutrinoless double beta decay, direction detection of dark matter particles, direct

detection of neutrino mass. Moreover, the talk covers how the superconducting sensor

technologies play rolls in cryogenic particle detection with MMC sensors.

39

Introduction to cryogenic particle detectors for

Shanghai Light source Facility

Shuo.Zhang1

1School of Physical Science and Technology, ShanghaiTech University, Shanghai.

[email protected]

ShanghaiTech University is hosting Shanghai soft X-ray Beamline Project (SBP) and Shanghai

HIgh repetitioN rate XFEL and Extreme light facility(SHINE) project which are aimed for

applications in material science, energy, environment, physics, chemistry and bioscience etc.

In these projects, cryogenic particle detectors include Transition Edge Sensor (TES) and

Metallic Magnetic Calorimeters (MMC) based spectrometers will be deployed. Our goal is to

develop TES and MMC based spectrometers for both soft X-ray and hard X-ray wavelengths.

Up to now, our TES system is ready for data measurement, the preliminary data shows an

energy resolution of 14 eV@ 5.9keV.

40

Neutron imaging using a superconducting detector

Takekazu Ishida1,2,† , The Dang Vu 3, Hiroaki Shishido 2,4, Kazuma Nishimura 4,

Kenji M Kojima 1,5, Kenichi Oikawa 3, Masahide Harada 3, Shigeyuki Miyajima 6,

Mutsuo Hidaka 7, Takayuki Oku 3, Kazuhiko Soyama 3, Kazuya Aizawa 3,

Tomio Koyama 1, Alex Malins 8, Masahiko Machida 8, Manobu M. Tanaka 9

1 Division of Quantum and Radiation Engineering, Osaka Prefecture University, Sakai, Osaka 599-8570, Japan

2 NanoSquare Research Institute, Osaka Prefecture University, Sakai, Osaka 599-8531, Japan

3 Materials and Life Science Division, J-PARC Center, Japan Atomic Energy Agency, Tokai, Ibaraki 319-1195,

Japan

4 Department of Physics and Electronics, Osaka Prefecture University, Sakai, Osaka 599-8531, Japan

5 Centre for Molecular and Materials Science, TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3,

Canada

6 Advanced ICT Research Institute, National Institute of Information and Communications Technology, Kobe,

Hyogo 651-2492, Japan

7 National Institute of Advanced Industrial Science and Technology, Tsukuba, Ibaraki 305-8568, Japan

8 Center for Computational Science & e-Systems, Japan Atomic Energy Agency, 178-4-4 Wakashiba,

Kashiwa-shi, Chiba-ken, 277-0871, Japan

9 Institute of Particle and Nuclear Studies, KEK, Tsukuba, Ibaraki 305-0801, Japan

[email protected]

After our successful observation of neutrons using a superconducting MgB2 detector in 2008

[1], we proposed a novel transmission neutron imaging system based on a superconducting

current-biased kinetic inductance detector (CB-KID). CB-KID consists of an X stripline, a Y

stripline, and a 10B neutron conversion layer. A 4He particle or a 7Li particle released from a

10B(n, α)7Li reaction creates two hot spots in both the X and Y striplines. CB-KID utilizes a

local change in the kinetic inductance to produce a signal, leading to electromagnetic-wave

pulses of opposite polarities propagating towards the ends of each stripline [2]. Using a delay-

line method for the X and Y striplines, we obtain the position of the nuclear reaction from the

differences in arrival timestamps of the pulses at the ends of the striplines. We used a set of

analog signal discriminators with fixed thresholds and a time-to-digital converter (TDC) with

1 ns time resolution to recover the signals from 25 Hz pulsed neutrons at J-PARC. We

succeeded in achieving an energy-integrated spatial resolution of 22 μm [3]. Further

improvements in spatial resolution can be achieved by using a high-speed TDC circuit. We

performed Monte Carlo simulations of CB-KID using PHITS (Particle and Heavy Ion Transport

code System) nuclear reaction models and nuclear data libraries to model the transport of

neutrons, 7Li, 4He, electrons, gamma-rays over wide energy ranges [4]. The PHITS simulations

helped us understand the operation of CB-KID and optimize the detector design.

This work is supported by Grant-in-Aid for Scientific Research (A) No.JP16H02450 from JSPS.

The devices were fabricated in the clean room for analog-digital superconductivity (CRAVITY).

This work is supported of MLF program of J-PARC (Proposal No. 2016B0012, 2017A0011,

2017B0014, 2018A0109, No. 2018P0201, No. 2019A0004).

41

[1] T. Ishida, M. Nishikawa, Y. Fujita, S. Okayasu, M. Katagiri, K. Satoh, T. Yotsuya, H. Shimakage, S. Miki,

Z. Wang, M. Machida, T. Kano, and M. Kato., J. Low Temp. Phys. 151, 1074-1079 (2008).

[2] T. Koyama and T. Ishida, J. Phys. Conf. Ser. 1054, 012055 (2018).

[3] H. Shishido, Y. Miki, H. Yamaguchi, Y. Iizawa, Vu T. Dang, K. M. Kojima, T. Koyama, K. Oikawa, M.

Harada, S. Miyajima, M. Hidaka, T. Oku, K. Soyama, S. Y. Suzuki, and T. Ishida, Phys. Rev. Appl. 10,

044044 (2018).

[4] T. Sato, Y. Iwamoto, S. Hashimoto, T. Ogawa, T. Furuta, S. Abe, T. Kai, P.E. Tsai, N. Matsuda, H. Iwase,

N. Shigyo, L. Sihver, and K. Niita, J. Nucl. Sci. Tech. 55, 684-690 (2018).

42

A challenge to chemical-state nanoscale-imaging

with superconductor-tunnel-junction X-ray detector

for aviation industry

M. Ohkubo1, G. Fujii1, S. Shiki1, W. Peng1, M. Ukibe1, N. Yamazaki2, K. Hasegawa2 and K.

Takagi2

1National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba

2Mitsubishi Heavy Industries, Ltd., Nagoya

[email protected]

Aviation industry has been eagerly introducing light-weight structural materials with a high

strength‐to‐weight ratio: e.g. main wings with carbon-fiber reinforced plastics (CFRP).

However, the aviation industry is forced to add drilling and bolting to adhesive bonding of

CFRP parts to avoid catastrophic loss of airplanes in case of bonding failure [1]. The additional

drilling and bolting cause a mechanical strength degradation and also is time and manpower

consuming. This may come from a lack of knowledge on chemical bond structure as well as

physical boundary structure. In order to understand the adhesion mechanism, our project

consists of adhesive strength tests including micron-sized test pieces, first-principle and

molecular dynamics calculations, weak-bond imaging, and spectroscopic imaging.

One of the spectroscopic imaging techniques is a combination of X-ray emission

spectroscopy (XES) [2] using a superconductor-tunnel-junction (STJ) X-ray detector [3] with

an energy resolution better than natural line widths of characteristic X-rays from elements and

a nanoscale electron beam produced by SEM [4]. This combination is a challenge to realize

simultaneous chemical imaging of such light elements as carbon, nitrogen, and oxygen at a

special resolution better than 10 nm, which is necessary to reveal the chemical and physical

structure of CFRP/CFRP adhesive boundaries.

Our latest version of the STJ detector has an energy resolution (E) of 4 eV for 260 eV soft

X-rays, which is equivalent to 277 eV of the carbon K characteristic X-rays. In addition to E,

low energy tail usually observed in the STJ response function to X-rays was eliminated by

attaching an X-ray mask layer directly on the detector chip. Since the light elements in matrices

usually exhibit a line width range of 15-20 eV, the STJ detector can be used not only for

elemental analysis but also chemical state analysis by measuring characteristic X-ray line shape.

Conventionally, wave-dispersive spectroscopy by scanning an analyzing crystal or a grating

enables XES, but a long measurement time leads to a damage of polymer materials such as

TGDDM and DGEBA cured with 4,4’ DDS. A 100-pixel STJ detector with a photon counting

rate of 100 kcps is suitable for a quick scanning of CFRP/CFRP adhesion cross-sections without

a serious electron beam irradiation damage.

This work was supported by Innovative Science and Technology Initiative for Security, ATLA,

Japan.

[1] FAA 14CFR § 23.573 Damage tolerance and fatigue evaluation of structure (a)(5).

[2] M. Ohkubo et al., IEEE/CSC & EASAS Superconductivity News Forum, July 2017.

https://snf.ieeecsc.org/sites/ieeecsc.org/files/documents/snf/abstracts/Ohkubo_STP582_Pres.pdf.

43

[3] G. Fujii et al. (2015), Improvement of soft x-ray detection performance in superconducting-tunnel-junction

array detectors with close-packed arrangement by three-dimensional structure, Supercond. Sci. Technol. 28,

104005.

[4] G. Fujii et al. (2017), Development of an energy-dispersive X-ray spectroscopy analyzer employing

superconducting tunnel junction array detectors toward nanometer-scale elemental mapping, X-ray Spectrom.

46, 325-329.

44

High Tc Scanning SQUID Microscope

Hideo Itozaki

Osaka University, Osaka, Japan

[email protected]

A high Tc SQUID has a big potential to be applied to many fields. Since the high Tc

SQUID was developed, a Scanning SQUID Microscope has been developed by some

groups. Here, an STM-SQUID Microscope and a Laser-SQUID Microscope are

introduced.

STM-SQUID Microscope

A schematic figure of the STM-SQUID microscope around a SQUID, a needle, and a

sample is shown in figure 1. This microscope can obtain an STM image of surface

morphology simultaneously. Figure 2 shows a magnetic image of a thin nickel film. It

is a deposited film with thickness of 0.3 micrometer. Submicron magnetic domains are

observed clearly. The less than 100 nm structure can be recognized.

Laser –SQUID Microscope

A fine focused laser is used to be a probe which stimulate semiconductor to generate

current. The SQUID Microscope observes magnetic field that is introduced by the

current. This technique makes high resolution, because it depends on the size of the

laser beam. A schematic figure of this Laser-SQUID Microscope is shown in figure 3.

A laser-SQUID image of a solar cell is shown in figure 4. It indicates sub grain

boundaries in a polycrystalline silicon solar cell.

needle

sapphire rod

cooled by LN2

sample[Air]

rf-SQUID

3-axis piezo stage

[Vacuum]

tunneling currentdetection (STM)

2 µmFigure 1 Schematic figure of STM-SQUID

Microscope.

Figure2 Magnetic domain observed by

STM-SQUID Microscope.

Figure 3 Schematic figure of Laser-SQUID

Microscope.

Figure 4 Sub grain image of solar cell

observed by Laser-SQUID Microscope.

45

Optimization of constriction based Nb µ-SQUIDs for

probing nano-magnetism

Anjan K. Gupta1, Sourav Biswas1, Sagar Paul1, H. Courtois2 and Clemens Winkelmann2

1Department of Physics, Indian Institute of Technology Kanpur, Kanpur 208016, India.

2Univ. Grenoble Alpes, CNRS, Grenoble INP, Institut Nèel, 38000 Grenoble, France

[email protected]

Magnetometry using micron-size superconducting quantum interference devices (µ-SQUIDs)

has been remarkably successful [1] in probing classical as well as quantum regimes of

magnetism in single nano-particles. This technique can be further improved for higher speed

and sensitivity with hysteresis-free µ-SQUIDs. The hysteresis in these devices arises from

thermal instabilities in superconducting weak-links and neighboring region. The heat generated

in resistive normal region gives rise to a self-sustained hot-spot. This leads to two possible

states, hot (normal) and cold (superconducting), and hence bistability. Such hot-spot and

hysteresis has been modeled [2] in the past by using steady state thermal heat balance equations.

However, as we approach the hysteresis-free regime by optimizing the relative heat

evacuation, another regime of hysteresis is found in which the bistability results due to a phase

dynamic steady state. This dynamic regime is understood using a thermal model [3] that helps

us quantitatively capture the observed behavior in both hysteretic and non-hysteretic regimes

[4]. We also solve the thermal model for different shunting conditions to find that an optimal

shunt having resistance and inductance both can eliminate hysteresis and with a good sensitivity

[5]. This new model also reveals an interesting non-linear dynamical system with various

regimes. We successfully test this idea of inductive shunt eliminating hysteresis with good

sensitivity. Finally, we present preliminary results on magnetization reversal in permalloy nano-

needles and Fe3O4 nano-particles by using these optimized µ-SQUIDs as direct voltage readout

of magnetic flux. [1] W. Wernsdorfer, From micro- to nano-SQUIDs: applications to nanomagnetism, Supercond. Sci. Technol.,

22, 064013 (2009).

[2] W. J. Skocpol, M. R. Beasley, and M. Tinkham, Self-heating hotspots in superconducting thin-film

microbridges, J. Appl. Phys. 45, 4054 (1974).

[3] K. Gupta, N. Kumar, and S. Biswas, Temperature and phase dynamics in superconducting weak-link, J. Appl.

Phys. 116, 173901 (2014).

[4] S. Biswas, C. B. Winkelmann, H. Courtois, and Anjan K. Gupta, Josephson Coupling in the Dissipative State

of a Thermally Hysteretic μ-SQUID, Phys. Rev. B, 98, 174514 (2018).

[5] S. Biswas, C. B. Winkelmann, H. Courtois, and A. K. Gupta, Elimination of thermal hysteresis with large V-

Φ transduction in μ-SQUIDs by inductive shunt, arXiv:1807.07720.

46

Correlation between the critical current density and

surface resistance in YBCO thin films—reexamined

H. Yamasaki1 and S. Ohshima2

1National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba.

2Faculty of Engineering, Yamagata University, Yonezawa.

[email protected]

More than 15 years ago, S. Ohshima and co-workers examined the correlation between the

critical current density (Jc) and the surface resistance (Rs) in YBa2Cu3O7– (YBCO) thin films

[1]. They found that there was a strong correlation between Rs and Jc. The relationship

between Jc and Rs (at 22 GHz) was expressed by the equation, Rs = 2.0 107 Jc–1 (1), where

the unit of Rs is the ohm, and the unit of Jc is A/m2 [1].

Recently, Yamasaki and coworkers investigated the magnetic-field-angle and temperature

dependent Jc(H, , T), and microstructures of YBCO thin films containing a high density of

nanoprecipitates, where Jc is the critical current density flowing in the ab-plane and is the

angle between the applied magnetic field and the c-axis of YBCO [2–4]. The Jc() curves have

been reasonably explained by a simple theoretical model that considers the linear summation

of core pinning interactions and the angular dependence of the coherence length, () = ab()

= ab{cos2 + (1/2)sin2}1/2, where is the anisotropy of YBCO. If the Jc is determined by the

flux pinning of nanoprecipitates whose diameter a is larger than 2ab, Jc can be expressed as Jc

= πNpHc2ab

2()/H (2), where is the pinning efficiency factor, Np is the density of nanoprecipitates

and Hc is the thermodynamic critical field [2, 3]. When the magnetic field is parallel to the c-axis and

the flux bending occurs because of strong nanoparticle pins, the situation is slightly changed and the

equation (2) becomes Jc = (π/4)NpaHc2ab/H (3) [4]. The equation (3) can be rewritten as Jc =

(1/32πµ02)Npa0

2/ab3H (4), because Hc = 0/22πµ0ab

2. We have investigated the temperature dependence of Jc in YBCO thin films for which Rs were also

measured, and found that the self-field Jc(T) can be explained by a slight modification based on the

equation (4). Since Rs is proportional to ab3, the equation (4) can well explain the correlation between

Rs and Jc (equation (1)).

[1] Ohshima, S., Oikawa, S., Noguchi, T., Inadomaru, M., Kusunoki, M., Mukaida, M., Yamasaki, H., and

Nakagawa, Y. (2002). The correlation of the critical current density and surface resistance of YBa2Cu3O7–

thin films. Physica C, 372–376, 671–674.

[2] Yamasaki, H., Ohki, K., Yamada, H., Nakagawa, Y., and Mawatari, Y. (2008). Strong flux pinning in

YBa2Cu3O7– thin films due to nanometer-sized precipitates. Supercond. Sci. Technol., 21(12), 125011. [3] Yamasaki, H. and Yamada, H (2017). Flux pinning properties of YBa2Cu3O7–δ thin films containing a high

density of nanoprecipitates: A comparative study to reveal size effects. Physica C, 542, 46–54. [4] Yamasaki, H. (2019). Field-angular dependence study of the critical current density in (RE)Ba2Cu3O7 films

with nanoprecipitates larger than normal-core diameter of a quantized flux line. Physica C, 563, 48–58.

47

Vortex manipulation with dots and antidots on

superconductivity of REBa2Cu3O7−δ films growth by

trifluoroacetate metal organic deposition method

Fang Li1, Sansheng Wang1*, Suleman Muhammad1

1Key Laboratory of Micro-nano Measurement, Manipulation and Physics, Beihang

University, Beijing 100191, China

E-mail address: [email protected]

Vortex manipulation with pinning structures is a promoting technique for preparing high quality

two-dimension and three-dimension epitaxial films. Through introducing dots and antidots on

substrates, a valied method for enhancing superconductor property of REBa2Cu3O7−δ (RE,

rare earth) thin films with a trifluoroacetate metal organic deposition (TFA-MOD) method is

introduced. Dots and antidots in sub-micron size can provide controlled vortex motion. By this

vortex manipulation technique, the critical current density Jc and onset transition temperature

Tc(onset) of the traditional superconducting REBa2Cu3O7−δ thin film can be effective

improved. This paper provides a competitive method and theoretical guidance for the effective

improvement of superconductivity in REBa2Cu3O7−δ thin films.

48

Effects of Ionic Accumulation in Nerve Conduction

Xiaoqing Sun1,*, Kelvin J.A. Ooi1,^, C.K. Ong2,#, Shengyong Xu3, †

1School of Electrical and Computer Engineering, Xiamen University Malaysia, Selangor.

2Department of Mathematics, Xiamen University Malaysia, Selangor.

3Department of Electronics, and Key Laboratory for the Physics & Chemistry of

Nanodevices, School of Electronics Engineering and Computer Science, Peking University,

Beijing.

*Email: [email protected]

^Email: [email protected]

#Email: [email protected]

†Email: [email protected]

Voltage-gated ion channels function to establish a voltage difference across the axonal

membrane, which contributes to the generation and propagation of the action potential.

However, the behavior of the action potential propagation in relation to the physical parameters

of the axon, such as axonal diameter and length, is not very well understood. In this respect, the

study of the ionic flows at the ion channels is essential to understand the conduction behavior

of the action potential. Accumulated sodium ions that appear at the ion channel due to the rapid

inflow of the ions would have an impact on the ionic flow rate at adjacent ion channels, hence

affecting the velocity of propagation of the action potential. In this presentation, I’ll talk about

how the accumulative ions influences propagation of the action potential.

[1] Brown, A. Smith and A. Chemist, The Art of Writing Convincing Abstracts (Pergamon Press, 2000) p 868.

[2] Sagi, I., &Yechiam, E. (2008). Amusing titles in scientific journals and article citation. Journal of Information

Science, 34(5), 680-687. [3] Akaishi T, (2017). New Theoretical Model of Nerve Conduction in Unmyelinated Nerves. Front. Physiol.

8:798. Doi: 10.3389/fphys.2017.00798. [4] G. Hales, (2014). The origins of the brain’s endogenous electromagnetic field and its relationship to provision

of consciousness. Journal of Integrative Neuroscience, Vol. 13, No. 2 (2014) 313-361. Imperial College Press.

Doi: 10.1142/S0219635214400056. [5] Chawla, Aman, On Axon-Axon Interaction via Currents and Fields. (2017).Graduate Theses and

Dissertations. http://scholarcommons.usf.edu/etd/6812

[6] J H Caldwell, (2009). Action Potential Initiation and Conduction in Axons. Encyclopedia of Neuroscience,

Volume 1 (2009) 23-29.

[7] Debanne D, Campanac E, Bialowas A, Carlier E, Alcaraz G. Axon Physiology. Physiol Rev 91: 555–602,

2011; doi:10.1152/physrev.00048.2009

[8] Waxman SG,(1980). Determinants of Conduction Velocity in Myelinated Nerve Fibers. Muscle Nerve. 1980

Mar-Apr;3(2):141-50. Doi:10.1002/mus.880030207.

49

Property of HTS Josephson Junction irradiated by

Ga Focused Ion Beam

T. Ueda, K. Hayashi, R. Ohtani, S. Ariyoshi and S. Tanaka

Toyohashi University of Technology, Toyohashi

[email protected]

HTS SQUIDs (High TC Superconducting Quantum Interference Devices) mainly utilize grain

boundary Josephson junctions (JJ), e.g. a bi-crystal JJ. But bi-crystal JJs have some problems,

as the layout and number of JJs are restricted because they must be located along the grain

boundary on the substrate. Therefore, the use of Ga Focused Ion Beam (Ga-FIB) irradiation to

make HTS JJs was tested, as it introduced an atomic disorder in the superconducting region. A 100 nm thick YBa2Cu3O7-δ thin film was sputtered on an MgO substrate by Pulsed Laser

Deposition (PLD), followed by deposition of a 20 nm thick Au protection layer. Subsequently,

a 4 μm wide micro-channel was fabricated by photolithography and Ar ion milling process.

Finally, the micro-channel superconducting area was narrowed down to nano-scale by line-

scanning the Ga-FIB irradiation, which introduces an atomic disorder in the superconducting

region and turns its property into a normal conducting state. Fig.1 shows the dependence of the

critical current IC of the bridges on the FIB fluence. IC were decreased with the fluence; IC of

Wn =500 nm disappeared at 1016 ions/cm2 and Wn =1000 nm disappeared at 1017 ions/cm2. Fig.2

shows the IV-characteristic of a 500 nm wide nano-bridge irradiated by the fluence of 2.0 ×1015

ions/cm2. Under microwave irradiation of 2 GHz, several Shapiro steps were observed, the

step voltage corresponding to the theoretical value. This suggested that the nano-bridge

fabricated by Ga-FIB irradiation acted as a Josephson junction.

Fig.1 Dependence of nano-bridge’s Fig.2 I-V characteristic under microwave

IC on fluence. irradiation.

[1] K. Hayashi, T. Ueda and S. Tanaka, “Study on Change of properties of HTS Josephson Junction by Ion beam

irradiation”, Extended Abstracts of 14th International Symposium on High Temperature Superconductors in

High Frequency Fields (HTSFF2018), 56-57, 2018.

50

LTS SQUID magnetometers and gradiometers

G. Zhang1,2, Y. Wang1,2, S. Zhang1,2, X. Zhang1,2, L. Rong1,2, H. Dong1,2, L. Qiu1,2, J. Wu1,2,

Y. Pei1,2, Q. Tao1,2, L. You1,2 and X. Xie1,2

1State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of

Microsystem and Information Technology (SIMIT), Chinese Academy of Sciences (CAS),

Shanghai

2Chinese Academy of Science, Center for Excellence in Superconducting Electronics,

Shanghai

[email protected]

In this work, we report the progress of LTS SQUID at SIMIT in China. As an ultra-

sensitive magnetic flux sensor, SQUIDs are widely used in many applications such as

biomagnetism, low-field magnetic resonance imaging, geophysics and so on. State-of-the-art

SQUIDs are mostly fabricated in Nb/Al-AlOx/Nb or NbN/AlN/NbN technology [1]. At SIMIT,

superconducting electronics facilities (SELF) have been built for superconducting integrated

circuits (SIC). SQUID fabrication benefits from the advance of superconducting process

technology. We present the fabrication of SQUID magnetometers and gradiometers designed

for some practical applications.

SQUID magnetometer consists of a washer-type SQUID and a flux transformer which

includes a pickup coil and an input coil to form a superconducting loop. The input coil is usually

integrated on the SQUID washer and thus inductively coupled to the SQUID by a mutual

inductance Min. In addition, some extra coils are integrated on chip to realize SQUID bootstrap

circuit [2]. To avoid the parasitic capacitance between SQUID and input coil, multi-loop

SQUID magnetometer is also presented. The noise performance of the SQUID magnetometer

is measured by using homemade readout electronics inside magnetically shielded room (MSR).

The magnetic field noise of <3fT/√Hz in white noise region has been obtained.

A gradient pickup coil is adopted in SQUID gradiometer. We present a planar first-order

gradiometer which is fabricated on 4-inch silicon wafer. Therefore, the baseline of the

gradiometer is limited to 3.5cm considering the integrated chip numbers. In MSR, the white

gradient field noise is measured to be better than 1fT/(cm*√Hz) [3].

Both magnetometer and gradiometer have been used in our practical systems, e.g.,

biomagnetism, transient electromagnetic detection and aeromagnetic survey. [1] Q. Liu, H. Wang, Q. Zhang, H. Wang, W. Peng and Z. Wang, Temperature-dependent performance of all-

NbN DC-SQUID magnetometers. (2016). Appl. Phys. Lett., 110 222604.

[2] X. Xie, Y. Zhang, H. Wang, Y. Wang, M. Mueck, H. Dong, H.-J. Krause, A. I. Braginski, A. Offenhaesser

and M. Jiang, A voltage biased superconducting quantum interference device bootstrap circuit. (2010).

Supercond. Sci. Technol. 23 065016. [3] X. Zhang, G. Zhang, Y. Wang, L. Rong, S. Zhang, J. Wu, L. Qiu, X. Xie and Z. Wang, A High-Balance

Planar SQUID Gradiometer. (2019). IEEE Transactions on Applied Superconductivity, 29 1600503.

51

LTS SQUID Based Transient Electromagnetic

System for Geophysical Prospecting

Y. Pei1,2, L. Rong1,2 , H. Dong1,2,Q. Tao1,2, J. Wu1,2, S. Zhang1,2, G. Zhang1,2, Y. Wang1,2, L.

Qiu1,2, L. You1,2 and X. Xie1,2

1State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of

Microsystem and Information Technology (SIMIT), Chinese Academy of Sciences (CAS),

Shanghai

2Chinese Academy of Science, Center for Excellence in Superconducting Electronics,

Shanghai

[email protected]

Transient ElectroMagnetic (TEM) prospecting is widely used in mineral, groundwater, and

geothermal exploration. Compared with commonly used induction coils, Low-temperature

Superconducting Quantum Interference Devices (LTS SQUIDs) can act as a magnetic field

receiver with better performance, e.g. wider bandwidth, lower noise level(7 fT/Hz) and less

distortion, thus leading to higher shallow ground surveying accuracy and deeper exploration

depth.

In this work, we will first introduce the development of the LTS SQUID based TEM system

developed at SIMIT in China. The system bandwidth is greater than 500 kHz and its slow rate

achieves approximately 28mT/s(Dual-Channel Squid-Based TEM System). A home-made

TEM transmitter can generate strong current pulses with different pulse widths according to

different ground resistivity. With this TEM system, we successfully observed the sign-reversal

signals, which implies the induced-polarization effect. However the negative amplitude is

always bigger than modeling, we revealed the reason for the sign-reversal signals is the primary

field switch-off procedure .

We then carried out field tests in different provinces in China, such as Shanghai, Jilin,

Inner Mongolia, Henan, Yunnan, as well as in Tajikistan. Some latest results of TEM survey

in these area will be presented.

[1] Shangyu Du, Yi Zhang, Yifeng Pei, Kun Jiang, Liangliang Rong, Changchun Yin, Yanju, Ji, and Xiaoming

Xie. Study of transient electromagnetic method measurements using a superconducting quantum interference

device as B sensor receiver in polarizable survey area, Geophysics, 83(2), E111-116. 2018,

doi.org/10.1190/geo2017-0197.1

[2] Liangliang Rong, Suxin Bao, Jun Wu, Guofeng Zhang, Longqing Qiu, Shunlin Zhang, Yongliang Wang,

Hui Dong, Yifeng Pei, and Xiaoming Xie. High-Performance Dual-Channel Squid-Based TEM System

and Its Application. IEEE Transactions on Applied Superconductivity VOL. 29, NO. 8, DECEMBER 2019

52

Control of roughness and stress of Nb films for

Nb/Al‐AlOx/Nb Josephson junctions

Yu Wu1,3,4, Liliang Ying1,4, Jie Ren1,2,4, Wanning Xu1,2,4, Yingyi Shao1,2,4, Liyun Chen1,2,4,

Xue Zhang1,2,4, Xiaoping Gao1,4, Wei Peng1,2,4, Masaaki Maezawa1,4, Zhen Wang1,2,3,4

1Key laboratory of functional materials for informatics, Shanghai Institute of Microsystem

and Information Technology (SIMIT), Chinese Academy of Science (CAS), Shanghai.

2Univerisity of Chinese Academy of Science, Beijing.

3ShanghaiTech University, Shanghai.

4CAS Center for Excellence in Superconducting Electronics (CENSE), Shanghai.

[email protected]

Abstract—Nb/Al-AlOx/Nb Josephson junctions are the most fundamental components in

Rapid Single Flux Quantum (RSFQ) circuits. Very large-scale RSFQ integration often has a

strict requirement on wafer-scale junction qualities. In particular, Nb film stress and roughness

in Nb/Al-AlOx/Nb trilayer-based Josephson junctions are two important factors affecting their

qualities. In our previous work, a two-step sputtering technique was developed to prepare Nb

films with different combinations of stress and roughness conditions to study the influence of

stress and roughness on junction qualities separately, in which the film consisting of two

sublayers deposited in-situ at different sputtering Ar pressures. In this paper, we found that a

cooling procedure between the sublayer depositions improves the reproducibility of the total

stress and roughness. Besides, changing the sputtering rate and thickness of the two sublayers

has been studied to investigate the impact of the different total stress and surface roughness

conditions.

53

Tunable Josephson junction based on black

phosphorus

Zuyu Xu, Wei Chen, Wanghao Tian, Yangyang Lv, Shixian Chen, Xianjing Zhou,

Sining Dong, Jun Li, Yonglei Wang, Huabing Wang*, and Peiheng Wu

Research Institute of Superconductor Electronics (RISE), Nanjing University, Nanjing.

*[email protected]

In Josephson junctions, the physical properties of barrier layers play a key role in the tunneling

behavior of the junctions [1, 2]. Black phosphorus (BP), a two-dimensional layered material

with semiconductor properties, has been expected to be used for tuning the characteristics of

Josephson junctions as a barrier layer. Here, we applied an in-situ technique to fabricate a

Josephson junction with few-layer BP sandwiched by two niobium electrodes. It is shown that

the oxidization and interfacial degradation of BP can be well reduced, and the sputtered Nb

films can make ohmic contacts to the BP thin flakes. According to strong anisotropy of BP, we

show that the nonuniform tunneling current distribution in the junctions where supercurrent

density distribution peaked at the edges of the junctions since these are reflected in unique

features of the dependence of critical current on applied magnetic fields. Our results

demonstrate that the nonuniform supercurrent distribution dominates the Josephson tunneling

owing to the superior in-plane transport properties of BP, and the supercurrent can be well

modified by applying the ionic gel electrolyte gate. These observations could open a new

pathway for the applications of superconductor quantum circuits.

We gratefully acknowledge financial support by the National Natural Foundation of China

(Grants No.61727805, 11234006).

[1] Heersche, H.B., Jarillo-Herrero, P., Oostinga, J.B., Vandersypen, L.M. & Morpurgo, A.F. (2007). Bipolar

supercurrent in graphene. Nature 446, 56-59.

[2] Lee, G.H., Kim, S., Jhi, S.H. & Lee, H.J. (2015). Ultimately short ballistic vertical graphene Josephson

junctions. Nat Commun 6, 6181.

[3] Zhu, Y.Y. at el. (2019). Isotropic Josephson tunneling in c-axis twist bicrystals of Br2Sr2CaCu2O8+ᵹ.

Preprint at https://arxiv.org/abs/1903.07965

54

Novel Nb-based Josephson junctions using

Bi2Sr2CaCu2O8+δ as barriers

Shixian Chen, Wanghao Tian, Zuyu Xu, Tong Qing, Wenchen Yue,Sining Dong, Yonglei

Wang, Huabing Wang*, and Peiheng Wu

Research Institute of Superconductor Electronics, Nanjing University, Nanjing.

*[email protected]

High quality Nb-based Josephson junctions with various types of barriers have been employed

in voltage standards, terahertz receivers, SQUIDs, and many other applications. Tunable

junction parameters are required for novel applications, e.g. in superconducting quantum

circuits. On the other hand, Bi2Sr2CaCu2O8+δ (B2212) single crystals, typically used as

superconducting material, may have more applications due to their atomically smooth surface,

phase transition, etc [1, 2, 3]. In our experiment, B2212 flakes with large area can be obtained

by a new nano-fabrication technique. A novel Josephson junction device with a non-

superconducting B2212 flake as its barrier was fabricated by an in-situ transferring technique.

Observed have been typical current-voltage characteristics satisfying the resistively-shunted-

junction model, and clear Shapiro steps under 10-40 GHz microwave irradiation. The vertical

structure of Nb-B2212-Nb was inspected by SEM and Raman spectrum. A tunable Josephson

junction device is expected by controlling the phase transition of the B2212 barrier in the near

future.

We gratefully acknowledge financial support by the National Natural Science Foundation of

China (No. 61727805), the National Key R&D Program of China (2018YFA0209002).

[1] Y. Koval, X. Jin, C. Bergmann, Y. Simsek, L. Özyüzer, P. Müller, H. B. Wang, G. Behr, and B. Büchner.

(2010). Tuning superconductivity by carrier injection. Appl. Phys. Lett., 96, 082507.

[2] M. H. Liao, Y. Y. Zhu, J. Zhang, R. Zhong, J. Schneeloch, G. Gu, K. Jiang, D. Zhang, X. C. Ma, and Q. K.

Xue. (2018). Superconductor-Insulator Transitions in Exfoliated Bi2Sr2CaCu2O8+δ Flakes. Nano Lett., 18,

5660-5665.

[3] Zhu, Y. Y. at el. (2019). Isotropic Josephson tunneling in c-axis twist bicrystals of Br2Sr2CaCu2O8+ᵹ.

Preprint at https://arxiv.org/abs/1903.07965.

55

Proximity Effects on Mo/Cu Bilayers

F.J. Li, W. Cui, J. Ding, R. Huang, X.Y. Hua, H. Jin, Y.J. Liang, G.L. Wang, S.F. Wang, Y.R.

Wang, Y. Zhou and Y.N. Zhang

Department of Astronomy and Tsinghua Center for Astrophysics, Tsinghua University,

Beijing.

[email protected]

Hot Universe Baryon Surveyor (HUBS) space project has been proposed in China to implement

the science theme “the missing baryons”. One of the core parts of HUBS is the X-ray

spectrometer with a designed energy resolution of 2 eV@ 0.6. keV, as a high resolution

microcalorimeter made of a large array of Transition Edge Sensors. Superconducting transition-

edge sensors (TESs) as highly sensitive thermometer and/or photodetectors, have been widely

developed for potential applications of measurement across the electromagnetic spectrum from

millimeter through gamma rays as well as with weakly interacting particles in variety of

astronomical instruments. Due to their capabilities of achieving high energy resolution, tunable

transition temperature, and excellent noise limitation, proximity bilayers superconductors are

attractive for use in TES detectors. Particularly for cryogenic microcalorimeters in detecting x-

rays and gamma-rays, Molybdenum/copper (Mo/Cu) bilayers are among the most suitable

materials, which exhibit good environmental stability and provide low resistivity films to attain

adequate thermal conductivity. Here, we report a number of Mo/Cu bilayers fabricated on

silicon nitride-on-silicon (Si3N4-on-Si) by using sputtering with ultra-high vacuum, and the

low-temperature electrical characterization of these bilayers. Experimental data are analyzed

on the base of Usadel equations, in which the proximity effect in the bilayer is mainly governed

by the interface transparency between the superconductor and the normal metal, and the

superconducting critical temperature (Tc) of the superconductor. Figure 1(b) indicates that the

proximity effect model with well described behavior of Tc shows much less Tc with increased

the thickness of the normal metal. And figure 1(a) shows very narrow superconducting

transitions in R(T) curves, which could evidence the high quality of the interface. We also found

that the fabricated bare rectangle Mo/Cu bilayers have achieved Tc<100 mK, with typical Mo

single film Tc around 1.05 K. It should be noted that the variation of Tc with similar Cu thickness

of samples is mainly due to the pre-grown condition being different.

0.1 0.2 0.3 0.4

0.0

0.2

0.4

0.6

0.8

1.0

R/R

n

T (K)

75 nm

100 nm

150 nm

(a)

50 100 150 200 250

0.0

0.1

0.2

0.3

0.4

Measured

Fit

Tc

(K)

Thickness of Cu film (nm)

(b)

Fig. 1 (a) Normalized R(T) curve of Mo/Cu bilayers; (b) Tc as a function of Cu thickness for Mo/Cu bilayers

(Line is fit to proximity effect based on Usadel equations).

56

Development of Mo/Cu TES Devices

S.F. Wang, W. Cui, J. Ding, R. Huang, X.Y. Hua, H. Jin, F.J. Li, Y.J. Liang, G.L. Wang, Y.R.

Wang, Y.N. Zhang and Y. Zhou

Department of Astrophysics and Tsinghua Center for Astrophysics, Tsinghua University,

Beijing.

[email protected]

The Hot Universe Baryon Surveyor (HUBS) mission, aiming at addressing the issue of

“missing baryons” in the local universe, requires a superconducting transition-edge sensor (TES)

array with high energy resolution. Here we report the recent progress on developing the Mo/Cu

TES for HUBS.

57

Characterization of Sputtered Molybdenum Thin

Films

Y.R. Wang, W. Cui, J. Ding, R. Huang, X.Y. Hua, H. Jin, F.J. Li, Y.J. Liang, G.L. Wang, S.F.

Wang, Y.N. Zhang and Y. Zhou

Department of Astronomy and Tsinghua Center for Astrophysics, Tsinghua University,

Beijing

[email protected]

Molybdenum thin films have shown great potential in the development of high-performance

superconducting transition-edge sensors (TESs). Used in combination with a normal metal (e.g.,

copper or gold) in a bilayer film, the stress and crystalline structure of the Mo layer can affect

the residual resistivity ratio (RRR) of the bilayer, as well as the interface between the

superconducting and normal layers, and thus also the superconducting transition temperature

(Tc) of the bilayer. In this work, molybdenum is deposited on a Si3N4 film over a silicon

substrate with radiofrequency magnetron sputtering. A set of Mo films are produced with

different sputtering power and argon pressure; growth time is adjusted to keep all of the films

a roughly the same thickness. Stress is measured by calculating the curvature variation before

and after the deposition of a Mo film. The morphology and crystalline structure of the films are

characterized with a variety of techniques, including atomic force microscopy, scanning

electron microscopy, and transmission electron microscopy. It is found that the film crystalline

structure and surface roughness are strongly dependent on the sputtering power and deposition

pressure. X-ray reflectivity and X-ray diffraction measurements are also performed to measure

the density, thickness, surface roughness, grain size and residual stress of the films; the results

exhibit good consistency with those obtained with other methods. The resistivity, RRR and Tc

of the films are also measured. We present correlations (or lack thereof) between the Tc of the

Mo films and their measured morphological, mechanical, or electrical properties.

This research is conducted as a part of the development of Mo-Cu TES devices for a proposed

X-ray astronomical mission, HUBS.

58

Bi-2212 mesas made of Bi-2212 thin film for THz

emission with superior heat dissipation.

Takahiro Murakami and Kensuke Nakajima

Graduate School of Science and Engineering, Yamagata University, Yonezawa.

[email protected]

SIS layered structure included in the crystal structure of the high temperature superconductor

Bi2Sr2CaCu2O8 (Bi-2212) functions as an intrinsic Josephson junction (IJJ). Since the

superconducting energy gap frequency is high enough for terahertz regime, Bi-2212 crystals

faceted to be a THz cavity shape, that is IJJ as well, emits THz wave when the ac Josephson

frequency proportional to junction voltage across the interior SIS junctions matches the cavity

resonance frequencies. The first strongly monochromatic terahertz wave emission from Bi-

2212 IJJ was reported from mesa IJJ formed on ab-plane of bulk single crystal[1]. The organic

adhesive layer between the thick basal crystal of the mesa and the dielectric substrate prevents

heat dissipation from the voltage biased IJJ. In order to improve heat dissipation, a structure

called a stand-alone mesa which removed the basal crystal of mesa IJJ have been proposed.

However, either mesa or stand-alone mesa, these devices produced from fine bulk crystals are

artisanal product and are not suitable for industrial production. We have been developing of IJJ

made of Bi-2212 thin films grown on MgO substrates suitable for industrial production, and

succeeded in emitting terahertz wave of about 6 μW at frequency of 0.6 THz in a wide

temperature range from 60 K to 75 K, so far. This result suggested high heat dissipation of the

thin film type Bi-2212 IJJ without organic adhesive layer. On the other hand, the strongest

terahertz wave emission (30 µW, 0.438 THz, 55 K) from Bi-2212 IJJ has been reported from

the mesa IJJ with a thin basal crystal and a junction height of 2.8 µm[2]. This result indicates

the high performance of the mesa junction which overcomes the heat dissipation. Theoretically,

considering that the THz radiation intensity is proportional to the square of the number of

coherently oscillating junctions. It is considered that the key issue of strong terahertz wave

radiation is how many junctions can be kept at the optimum operating temperature to be

synchronized.

In this study, we fabricated Bi-2212 thin film mesa-type IJJ junctions using Bi-2212 thin film

to clarify its heat dissipation and terahertz wave radiation performance. We propose a metal

mask process to form a mesa IJJ as high as possible on Au/Bi-2212 thin films. A rectangular

shape 500 nm thick Nb thin film as shown in figure 1

formed on Au/Bi2212 film by reactive ion etching to be a

junction defining metal mask to withstand long time Ar ion

milling. We have fabricated IJJ with sufficient junction

height and thin basal crystal on Bi-2212 thin film by the Nb

metal mask process. We will report the voltage-current

characteristics and THz radiation characteristics of

junctions with excellent heat dissipation. [1] L. Ozyuzer et al., Science, 318 1291 (2007).

[2] S. Sekimoto et al., APPLIED PHYSICS LETTERS 103, 182601

(2013).

Fig 1. Photomicrograph of the Nb

mask formed on Au/Bi-2212 film.

59

High-power terahertz emission from Bi2Sr2CaCu2O8

intrinsic Josephson junction stacks

Z. D. Qi, H. C. Sun, H. L. Zhang, T. Qing, J. Shi, X. J. Zhou,H. B. Wang*, and P. H. Wu

Research Institute of Superconductor Electronics (RISE), Nanjing University, Nanjing.

*[email protected]

The terahertz (THz) wave is at a special position in the electromagnetic spectrum, which has

attracted much attention owing to its extensive potential applications, such as imaging, medical

diagnostics, public security, macromolecule detection, and environmental monitoring. These

practical applications need the developing of powerful continuous-wave emitters. The terahertz

generators made with stacks of intrinsic Josephson junctions (IJJs) in high critical temperature

(high-Tc) superconductor Bi2Sr2CaCu2O8 (BSCCO) are promising candidates [1, 2].

BSCCO can be regarded as a lot of Josephson junctions in series, and a 1μm thick BSCCO

stack contains about 667 junctions. Known by the ac Josephson effects, when the current

flowing through Josephson junctions is larger than the critical current (Ic), the junctions oscillate

at a frequency f = V/NΦ0, where V, N, and Φ0 are the voltage across the stack, the number of

Josephson junctions, and the flux quantum respectively. However, the relatively low output

power has always been an important factor limiting the practical applications.

In order to get higher emission power, a new “in-line” fabrication method is used to make the

sample containing more than 1000 Josephson junctions easily, and diamond substrates are used

for higher thermal conductivity. Thanks to the above-mentioned efforts, a round shape BSCCO

stack with a diameter of 200 μm, thickness of 1.65 μm is fabricated, with a record high emission

power of 258 μW at 54 K by direct detection, a frequency range of 200 to 950 GHz, and an

operating temperature up to 83 K.

Taking into account the optical path of the terahertz interferometer, we think that most of the

electromagnetic waves released by Josephson oscillation dissipate in the optical path. Inferring

from previous experimental results [3], the actual output power of this sample is about 846 μW.

Considering the radiation directionality, the output power may exceed 1 mW. This work greatly

increases the power of a single BSCCO terahertz source and improves its potential practice

value.

We gratefully acknowledge financial support by the National Natural Foundation of China

(Grants No.61727805, 11234006).

[1] L. Ozyuzer and et al, Emission of coherent THz radiation from superconductors, Science 318, 1291 (2007).

[2] H. B. Wang and et al, Coherent THz emission of intrinsic Josephson junction stacks in the hot spot regime,

Phys. Rev. Lett. 105, 057002 (2010).

[3] D. Y. An and et al, Terahertz emission and detection both based on high-Tc superconductors: Towards an

integrated receiver, Appl. Phys. Lett. 102, 092601 (2013).

60

Characterization of superconducting NbN hot-

electron bolometers as THz direct detectors

R. F. Su, X. C. Tu, J. B. Wu, X. Q. Jia, C. H. Zhang, L. Kang, B. B. Jin, W. W. Xu, H. B. Wang,

J. Chen and P. H. Wu

Research Institute of Superconductor Electronics (RISE), School of Electronic Science and

Engineering, Nanjing University, Nanjing.

[email protected]

During the past decades, superconducting hot electron bolometers (HEBs) based on the niobium

nitride (NbN) films have been widely used as heterodyne detectors (mixers) near liquid-helium

temperatures at frequencies above 1.2 THz in astronomy [1]. Due to their short response time

and high sensitivity, superconducting HEBs are also been used as THz direct detectors for the

applications in biology, medicine and security systems recently [2].

We compared the performance of an HEB direct detector at 0.65 THz with thermal, microwave

(MW) and THz biasing methods based on DC readout scheme. The current responsivity of the

NbN HEB detector with appropriate MW and THz biasing is significantly higher (about one

order) than that with thermal biasing. An optical NEP at the order of pW/√Hz is obtained by

choosing the MW frequency and power appropriately. The MW frequencies are usually around

1 GHz within the IF bandwidth of the mixer. With appropriate MW biasing, the NEP shows no

deterioration and achieves a slight improvement compared with thermal biasing. It is feasible

to replace the method of thermal biasing with MW biasing especially for a multi-pixel HEB

detector array. Furthermore, relaxation oscillations in the bi-stable region of the HEB detectors

have been studied using a microwave probe as a tool. The frequency of relaxation oscillations

switching between the superconducting and resistive states increases linearly with incident THz

power but nonlinearly with bias voltage or bath temperature. The strong periodic pulse trains

of relaxation oscillations have a maximum duty cycle of ~50%. In addition to relaxation

oscillations, we also see weaker oscillations when the HEB is in the resistive state, which we

call intrinsic oscillations. These have a constant frequency at the order of 10 kHz. Based on the

linear dependence of the relaxation oscillation frequency on the incident THz power, one can

make a digital THz power measurement from a few nW to about 1 μW. [1] J. Chen, Y. Jiang, M. Liang, L. Kang, B. B. Jin, W. W. Xu and P. H. Wu, (2011). Stability of superconducting

hot electron bolometer receivers. IEEE Trans. Appl. Supercond., 21(3), 667-670.

[2] R. F. Su, Y. D. Zhang, X. C. Tu X C, X. Q. Jia, L. Kang, B. B. Jin, W. W. Xu, J. Chen and P. H. Wu, (2019).

Terahertz direct detectors based on superconducting hot electron bolometers with different biasing methods.

IEEE Trans. Appl. Supercond, 29(5), 2300104.

[3] R. F. Su, Y. D. Zhang, X. C. Tu, X. Q. Jia, C. H. Zhang, L. Kang, B. B. Jin, W. W. Xu, H. B. Wang, J. Chen,

and P. H. Wu, (2019). Microwave probing of relaxation oscillations related to terahertz power detection in

superconducting hot electron bolometers. Supercond. Sci. Technol., 32, 105002.

61

The application of high-Tc SQUID-based low-field

NMR in human liver tumor discrimination

Shu-Hsien Liao1, Hao-Wei Huang1, Yu-Ting Liao1, Jhih-Hao Chen1, Kai-Wen Huang2,

Herng-Er Horng1

1Institute of Electro-Optical Engineering, National Taiwan Normal University, Taipei

116, Taiwan

2Department of Surgery and Hepatitis Research Center, National Taiwan University

Hospital, Taipei 100, Taiwan

[email protected]

Superconducting quantum interference device is the most sensitive sensor for magnetic field

detection. Therefore SQUID-based nuclear magnetic resonance spectrometer promises the

advantages of low cost and high sensitivity. In this study, a home-made high-Tc SQUID NMR

spectrometer was set up for tumor tissue discrimination. The T1 relaxation time of normal liver

tissues and cancerous tissues in Low Field nuclear magnetic resonance were obtained. After

detecting 30 pairs of human liver specimens, the significant difference of T1 relaxation times

was found to reveals the feasibility for liver cancer tissue discrimination by using low-field

NMR.